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Eutrophication in cold-arid lakes: molecular characteristics and transformation mechanism of DOM under microbial action at the ice-water interface

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Carbon Research 2024年第1期3卷 1-17页

作者： Wang, Tengke Feng, Weiying Liu, Jing Fan, Wenhong Li, Tingting Song, Fanhao Yang, Fang Liao, Haiqing Leppäranta, Matti School of Materials Science and Engineering Beihang University Beijing100191 China Environment Research Institute Shandong University Qingdao266273 China State Key Laboratory of Environmental Criteria and Risk Assessment Chinese Research Academy of Environmental Sciences Beijing100012 China State Key Joint Laboratory of Environment Simulation and Pollution Control School of Environment Tsinghua University Beijing100084 China Institute for Atmospheric and Earth System Research University of Helsinki Helsinki00014 Finland

During freezing periods, nutrients (carbon and organic matter, etc.) are enriched in the water and sediment of lakes in cold-arid regions, leading to potential algal bloom outbreaks and other health risks to the ecosystem. Particularly, dissolved organic matter (DOM) is a critical component of the nutrients and plays an important role in the global carbon cycle. However, the mechanisms of DOM transfer between ice and water remain unclear. This study analyzed the influence of microbial community on DOM composition using 16 s RNA, 3DEEM, and FT-ICR MS in Daihai Lake and Wuliangsuhai Lake in the Yellow River Basin, China. According to the spectral analysis, the content of endogenous organic matter, such as humus, accounted for 40% of the total DOM in water, while the content of tryptophan and tyrosine accounted for 80% of the total DOM in ice. The results of mass spectrometry showed that lignin was the main component, and the content of organic matter in the ice was less than that in the water. Molecular structures of seven DOM coexisting in the lake ice and water were elucidated with adapted Kendrick-analogous network visualization, which clearly illustrates that long-chain DOM molecules are derived from small molecules, while other heteroatoms are complexed with the side groups. The positive correlations between CHO, CHNO, CHOS, CHOS and Actinomyces indicate that DOM actively interacted with the microbial community. 44% of CHO compounds have the same molecular formula in water, the content of CHOS in the water of the two lakes was closed to 7% higher than that in the ice. Meanwhile, DOM dynamically migrate between ice and water via interstitial water because of the solubility changes under microbial transformation, which has been proved by the decrease in the contents of the humus and tryptophan-like substances in the ice from the bottom to the surface and lower contents of carbohydrate and unsaturated aromatic hydrocarbon in the water than the ice. This study helps

关键词： Aromatization

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Weak Magnetic Field Enhances Waste Molasses-Driven Denitrification During Wastewater Treatment

SSRN

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SSRN 2023年

作者： Wang, Qingxin Lin, Yuan Peng, Ling Wang, Yanru Ma, Sijia Ren, Hongqiang Xu, Ke State Key Laboratory of Pollution Control and Resource Reuse School of the Environment Nanjing University Jiangsu Nanjing210023 China

Waste molasses, the abundant byproducts of the sugar industry, is a cost-efficient carbon source for advanced denitrification. However, the efficiency of waste molasses-driven denitrification is limited by its complex carbon content, hindering its practical application. Weak magnetic field (WMF) is reported to enhance biological nitrogen removal, but its effects on molasses-driven denitrification remains unknown. In this study, we investigated whether the WMF can enhance waste molasses-driven nitrogen removal and explore the underlying mechanisms. We found WMF significantly facilitated waste molasses-driven denitrification, with total nitrogen removal efficiency increased by up to 25% (from 77% to 96%). WMF stimulated the nitrate reductase’s activity by 7-18%, and the enhancement was improved as WMF intensified. Quantitative qPCR analysis indicated that the abundances of denitrifying enzymes increased under WMF, which was consistent with the proliferation of denitrifying bacteria Denitratisoma and Devosia. Our study has demonstrated that WMF is promising for enhancing complex carbon-driven denitrification processes. © 2023, The Authors. All rights reserved.

关键词： Efficiency

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Selective capture of Tl2O from flue gas with formation of p-n junction on V_(2)O_(5)-WO_(3)/TiO_(2)catalyst under working conditions

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Green Energy & environment 2023年第1期8卷 4-9页

作者： Jianjun Chen Rongqiang Yin Gongda Chen Junyu Lang Xiaoping Chen Xuefeng Chu Junhua Li State Key Joint Laboratory of Environment Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijingChina School of Physical Science and Technology Shanghai Tech UniversityShanghaiChina Key Laboratory of Architectural Cold Climate Energy Management Ministry of EducationJilin Jianzhu UniversityChangchunChina Guangdong Energy Group Science and Technology Research Institute Co. Ltd.GuangdongChina

Thallium(Tl)compounds,highly toxic to biology,are usually released into flue gas during fossil/minerals combustion,and further distributed in water and *** this work,we fundamentally investigated the capture of gaseous Tl_(2)O by industrial V2O5-WO3/TiO_(2)catalyst under working condition in Tl-containing flue *** and theoretical results indicated that the Tl_(2)O has significant electron-feeding capacity and easily donate electron to unoccupied orbitals of TiO_(2),leading to dismutation of Ti 2p and inartificial formation of p-n junction on TiO_(2)surface,which prompted Tl_(2)O selectively interacted with TiO_(2)in flue ***,we proposed and verified an effective way to capture gaseous Tl_(2)O,which offered almost the best choice to eliminate Tl emission from flue gas and expanded the function of the TiO_(2)-based *** formation of p-n junction on commercial V2O5-WO3/TiO_(2)catalyst under working condition was revealed for the first time,which can be a valuable reference for both heterocatalysis and electro/photocatalysis.

关键词： Tl Catalyst SCR Capture p-n junction

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Achieving robust nitritation in a modified continuous-flow reactor: From micro-granule cultivation to nitrite-oxidizing bacteria elimination

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Journal of environmental Sciences 2023年第2期35卷 117-129页

作者： Wenru Liu Jiajun Song Jianfang Wang Xiaoming Ji Yaoliang Shen Dianhai Yang National&Local Joint Engineering Laboratory for Municipal Sewage Resource Utilization Technology Suzhou University of Science and TechnologySuzhou 215009China School of Environmental Science and Engineering Suzhou University of Science and TechnologySuzhou 215009China College of Resources and Environmental Sciences Nanjing Agricultural UniversityNanjing 210095China State Key Laboratory of Pollution Control and Resources Reuse Tongji UniversityShanghai 200092China

In this study,a modified continuous-flow nitrifying reactor was successfully operated for rapid cultivation of micro-granules and achieving robust *** showed that sludge granulation with mean size of ca.100μm was achieved within three weeks by gradually increasing settling velocity-based selection pressure from 0.48 to 0.9 m/*** Nitrospira like nitrite-oxidizing bacteria(NOB)were enriched in the micro-granules with a ratio between ammonia-oxidizing bacteria(AOB)and NOB of 5.7%/6.5% on day 21,fast nitritation was achieved within one-week by gradually increasing of influent ammonium concentration(from 50 to 200 mg/L).Maintaining ammonium in-excess was the key for repressing NOB in the ***,when the influent ammonium concentration switched back to 50 mg/L still with the residual ammonium of 15–25 mg/L,the nitrite accumulation efficiency increased from 90%to 98%.Experimental results suggested that the NOB repression was intensified by both oxygen and nitrite unavailability in the inner layers of ***,continuous operation with ammonium in excess resulted in overproduction of extracellular polysaccharides and overgrowth of some bacteria(e.g.,Nitrosomonas,Arenimonas,and Flavobacterium),which deteriorated the micro-granule stability and drove the micro-granules aggregation into larger ones with irregular ***,efficient nitritation was stably maintained with extremely high ammonium oxidation potential(>50 mg/g VSS/hr)and nearly complete washout of NOB was *** suggested that smooth and spherical granule was not a prerequisite for achieving NOB wash-out and maintaining effective nitritation in the granular ***,the microgranules exhibited a great practical potential for high-rate nitritation.

关键词： Continuous flow Granulation Nitritation Nitrate-oxidizing bacteria repression

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Modification strategies on 2D Ni-Fe MOF-based catalysts in peroxydisulfate activation for efficient organic pollutant removal

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Chinese Chemical Letters 2023年第4期34卷 406-409页

作者： Minjun Liu Ying Liu Xinru Liu Chengcheng Chu Ducheng Yao Shun Mao College of Environmental and Chemical Engineering Shanghai University of Electric PowerShanghai 200090China College of Environmental Science and Engineering Biomedical Multidisciplinary Innovation Research InstituteShanghai East HospitalState Key Laboratory of Pollution Control and Resource ReuseTongji UniversityShanghai 200092China

This study reports several modification strategies to optimize and enhance the performance of twodimensional(2D) metal organic frameworks(MOFs)-derived catalysts in peroxydisulfate(PDS) *** raw 2D Ni-MOF and 2D Ni-Fe-MOF without modification show poor catalytic activities for PDS activation and high metal ion leaching. The carbonization of 2D MOF can increase the activity of the catalyst but cannot solve the metal leaching problem. The further acid treatment of carbonization products can further improve the catalytic activity and decrease the metal ion leaching. The in-situ growth of2D MOF on graphene oxide(GO) support with subsequent carbonization and acid treatment offers the best performance in PDS activation for organic pollutant removal with low metal ion leaching. Compared with other PDS systems, the Ni-Fe-C-acid/GO system displays much lower catalyst and PDS dosages for p-chloroaniline degradation. This study presents new insights in the modification strategies of 2D MOFbased catalysts in PDS activation.

关键词： Peroxydisulfate oxidation 2D MOF Modification strategy Synergistic effect Organic pollutant removal

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Modeling the dynamic impacts of maritime network blockage on global supply chains

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The Innovation 2024年第4期5卷 103-109,102页

作者： Shen Qu Yunlei She Qi Zhou Jasper Verschuur Lu-Tao Zhao Huan Liu Ming Xu Yi-Ming Wei Center for Energy and Environmental Policy Research Beijing Institute of TechnologyBeijing 100081China School of Management Beijing Institute of TechnologyBeijing 100081China Beijing Key Lab of Energy Economics and Environmental Management Beijing 100081China Oxford Programme for Sustainable Infrastructure Systems(OPSIS) Environmental Change InstituteUniversity of OxfordOX12JD OxfordUK State Key Joint Laboratory of Environment Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing 100084China State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex Beijing 100084China School of Environment Tsinghua UniversityBeijing 100084China

Recent phenomena such as pandemics,geopolitical tensions,and climate change-induced extreme weather events have caused transportation network interruptions,revealing vulnerabilities in the global supply chain.A salient example is the March 2021 Suez Canal blockage,which delayed 432 vessels carrying cargo valued at$92.7 billion,triggering widespread supply chain *** ability to model the spatiotemporal ramifications of such incidents remains *** fill this gap,we develop an agent-based complex network model integrated with frequently updated maritime *** Suez Canal blockage is taken as a case *** results indicate that the effects of such blockages go beyond the directly affected countries and *** Suez Canal blockage led to global losses of about$136.9($127.5–$147.3)billion,with India suffering 75%of these *** losses show a nonlinear relationship with the duration of blockage and exhibit intricate trends post *** proposed model can be applied to diverse blockage scenarios,potentially acting as an earlyalert system for the ensuing supply chain ***,high-resolution daily data post blockage offer valuable insights that can help nations and industries enhance their resilience against similar future events.

关键词： chains valued extreme

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Climate change projections for Diamer Division in lesser Himalayas using multi-global climate model ensemble

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environmental Science and pollution Research 2025年第3期32卷 1668-1680页

作者： Ahmad, Didar Faridullah, Faridullah Irshad, Muhammad Bacha, Aziz Ur Rahim Hafeez, Farhan Iqbal, Akhtar Ullah, Zahid Afridi, Muhammad Naveed Alrefaei, Abdulwahed Fahad Nazir, Rashid Department of Environmental Sciences COMSATS University Islamabad Abbottabad Campus Abbottabad22060 Pakistan State Key Laboratory of Urban Water Resource and Environment Shenzhen Key Laboratory of Organic Pollution Prevention and Control School of Eco-Environment Harbin Institute of Technology Shenzhen Shenzhen518055 China Department of Environmental Science and Engineering Fudan University Shanghai200433 China State Key Laboratory of Biogeology and Environmental Geology School of Environmental Studies China University of Geosciences Wuhan430074 China Department of Zoology College of Science King Saud University P.O. Box 2455 Riyadh11451 Saudi Arabia

Pakistan, like many other regions around the world, is experiencing the impacts of climate change, particularly in its northern region. These changes have adverse impacts on ecosystems and biodiversity. Herein, we have investigated future projections of temperature and precipitation trends for three periods historical (HT = 1975–2005), near-term (NT = 2010–2029), and mid-term (MT = 2030–2050) using climate model intercomparison projects along with global climate models (GCMs) including RCP4.5 and RCP8.5. The historical records spanning from 1975 to 2005 reveal that the Chilas region has a notable rise of 8 °C in maximum temperature (Tmax), whereas the Astore district exhibited a trend of decreasing temperatures. When examining the projected temperature trends using GCMs (RCP4.5 and RCP8.5), the Chilas region is predicted to undergo a further increase of 6 °C in Tmax. In contrast, the Babusar region is projected to observe a significant decrease of 2 °C for the period between 2010 and 2050. Additionally, the precipitation results obtained from historical-based analysis for the period 1975 to 2005 indicated that the Babusar area exhibited increased precipitation patterns to 20 mm on an annual basis. Similarly, the Astore region has the most significant decline in precipitation, with a reduction of 40 mm annually. The predicted precipitation patterns for the period between 2010 and 2050 under the RCP8.5 revealed that the Babusar region has maximum precipitation (25 mm). Conversely, the Astore region exhibited reduced precipitation patterns, recording minimum precipitation (40 mm). In the results from RCP4.5, the precipitation showed a similar pattern with a maximum of 35 mm and a minimum of 15 mm in the Babusar and Astore, respectively. The region’s glaciers, snow cover, and land use systems are deteriorated by these changes in temperature and precipitation patterns. The increased winter and decreased summer precipitation under varied temperatures and precipitation cau

关键词： Miocene

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Phosphate removal by a La(OH)_(3) loaded magnetic MAPTAC-based cationic hydrogel:Enhanced surface charge density and Donnan membrane effect

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Journal of environmental Sciences 2022年第3期34卷 26-39页

作者： Yanqing Zhou Yili Wang Shuoxun Dong Haotian Hao Junyi Li Chenyang Liu Xiaolin Li Yao Tong College of Environmental Science and Engineering Beijing Key Lab for Source Control Technology of Water PollutionBeijing Forestry UniversityBeijing 100083China Center for Water and Ecology State Key Joint Laboratory of Environment Simulation and Pollution ControlSchool of EnvironmentTsinghua UniversityBeijing 100083China State Key Laboratory of Environmental Aquatic Chemistry Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China

Cationic hydrogels have received great attention to control eutrophication and recycle *** this study,a type of La(OH)_(3) loaded magnetic MAPTAC-based cationic hydrogel(La(OH)_(3)@MMCH)was developed as a potential adsorbent for enhanced phosphate removal from aqueous ***(OH)_(3)@MMCH exhibited high adsorption capacity of 105.72±5.99 mg P/g,and reached equilibrium within 2 ***(OH)_(3)@MMCH could perform effectively in a wide pH range from 3.0 to 9.0 and in the presence of coexisting ions(including SO_(4)^(2-),Cl^(-),NO_(3)^(-),HCO_(3)^(-),SiO_(4)^(4-) and HA).The adsorption-desorption experiment indicated that La(OH)_(3)@MMCH could be easily regenerated by using NaOH-NaCl as the desorption agent,and 73.3%adsorption capacity remained after five ***,La(OH)_(3)@MMCH was employed to treat surface water with phosphate concentration of 1.90 mg/L and showed great removal efficiency of 95.21%.Actually,MMCH showed high surface charge density of 34.38-59.38 meq/kg in the pH range from 3.0 to 11.0 and great swelling ratio of 3014.57%within 24 h,indicating that MMCH could produce the enhanced Donnan membrane effect to pre-permeate ***,the bifunctional structure of La(OH)_(3)@MMCH enabled it to capture phosphate through electrostatic attraction and ligand *** the results prove that La(OH)_(3)@MMCH is a promising adsorbent for eutrophication control and phosphate recovery.

关键词： Cationic hydrogel La(0H)_(3) Phosphate adsorption Enhanced Donnan membrane effect

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Vehicle emissions of primary air pollutants from 2009 to 2019 and projection for the 14th Five-Year Plan period in Beijing, China

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Journal of environmental Sciences 2023年第2期35卷 513-521页

作者： Tongran Wu Yangyang Cui Aiping Lian Ye Tian Renfei Li Xinyu Liu Jing Yan Yifeng Xue Huan Liu Bobo Wu National Engineering Research Center of Urban Environmental Pollution Control Beijing Municipal Research Institute of Environmental ProtectionBeijing 100037China Beijing Municipal Ecology and Environment Bureau Beijing 100048China State Key Joint Laboratory of ESPC School of EnvironmentTsinghua UniversityBeijing 100084China School of Ecology and Environment Beijing Technology and Business UniversityBeijing 100048China

Over the past decade,the emission standards and fuel standards in Beijing have been upgraded twice,and the vehicle structure has been improved by accelerating the elimination of 2.95 million old *** the formulation and implementation of these policies,the emissions of carbon monoxide(CO),volatile organic compounds(VOCs),nitrogen oxides(NO_(x)),and fine particulate matter(PM_(2.5))in 2019 were 147.9,25.3,43.4,and 0.91 kton in Beijing,*** emission factor method was adopted to better understand the emissions characteristics of primary air pollutants from combustion engine vehicles and to improve pollution *** combination with the air quality improvement goals and the status of social and economic development during the 14th Five-Year Plan period in Beijing,different vehicle pollution control scenarios were established,and emissions reductions were *** results show that the emissions of four air pollutants(CO,VOCs,NO_(x),and PM_(2.5))fromvehicles in Beijing decreased by an average of 68% in 2019,compared to their levels in *** contribution of NOx emissions from diesel vehicles increased from 35% in 2009 to 56% in 2019,which indicated that clean and energy-saving diesel vehicle fleets should be further *** vehicle adoption could be an important measure to reduce pollutant *** the further upgrading of vehicle structure and the adoption of electric vehicles,it is expected that the total emissions of the four vehicle pollutants can be reduced by 20%-41% by the end of the 14th Five-Year Plan period.

关键词： Emission variations Vehicle structure Electric vehicle 14th Five-Year Plan Air pollution

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Insights into effects of algae on decay and distribution of bacterial pathogens in recreational water:Implications for microbial risk management

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Journal of environmental Sciences 2022年第3期34卷 92-103页

作者： Tingting Fang Zuotao Zhang Hui Wang Matt Rogers Qijia Cui State Key Joint Laboratory on Environment Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing 100084China Department of Civil and Environmental Engineering National University of SingaporeEngineering Drive 3117576Singapore

The decay and distribution of bacterial pathogens in water is an important information for the health risk assessment to guide water safety management, and suspended algae might affect bacterial pathogens in water. This study established microcosms to investigate the effects of algae-related factors on the representative indicators and opportunistic pathogen species in water. We found that suspended algae increased the persistence of targeted species by 1-2 orders of magnitude of concentrations compared to microcosms without algae;and the effect of algae on microbial survival was affected by water nutrient levels(i.e., carbon, nitrogen and phosphorus), as the increased microbial persistence were correlated to the increased algae concentrations with more nutrient supplies. Moreover, decay and distribution profiles of representative species were determined. The three opportunistic pathogen species( Pseudomonas aeruginosa, Aeromonas hydrophila and Staphylococcus aureus) showed lower decay rates(0.82–0.98/day, 0.76–0.98/day, 0.63–0.87/day) largely affected by algae-related factors, while the enteric species( Escherichia coli and Enterococcus faecalis) had higher decay rates(0.94–1.31/day, 0.89–1.21/day) with little association with algae, indicating the propensity for attachment to algae is an important parameter in microbial fate. Together results suggest suspended algae played an evident role in the decay and distribution of bacterial pathogens, providing important implications regarding microbial safety in recreational water.

关键词： Suspended algae Bacterial pathogen decay Bacterial pathogen distribution Recreational water Microbial risk assessment

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