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environmental Functional Materials 2022年第3期1卷 325-337页

作者： Zhanghao Chen Xinhao Wang Ruochen Dong Yutong Zhang Xin Jin Cheng Gu State Key Laboratory of Pollution Control and Resource Reuse School of the Environment Nanjing University Nanjing 210023 PR China

Nowadays, the increasing discharge of persistent per- and polyfluoroalkyl substances (PFASs) caused serious environmental issues. In addition to advanced oxidation processes (AOPs), advanced reduction processes (ARPs) based on reducing radicals, e.g., hydrated electron and superoxide anions have attracted great attentions as promising methods for remediation of PFASs pollution. This review, based on 128 cited references, provides a critical overview on the performance of different AOPs and ARPs. The unique properties of reactive species, e.g., SO 4 •- and e aq − and their generation mechanisms in different systems were discussed. Moreover, the efficiencies of different systems were further compared from several aspects, e.g., PFASs decomposition rate, reaction time and energy consumption. More specially, for some model compounds of PFASs, such as perfluorooctanoic acid, perfluorooctane sulfonate and perfluoroalkyl ether carboxylic acids, we systematically discussed their degradation and defluorination pathways in both AOPs and ARPs. The reported literatures showed that the degradation pathways of these PFASs are closely related to their head groups in either AOPs or ARPs. Finally, some key conclusions were summarized, and the implications of the state-of-the-art knowledge on practical PFASs remediation in water treatments were summarized and the future priority research directions were proposed.

关键词： Advanced oxidation processes Advanced reduction processes Polyfluoroalkyl substances Degradation mechanism

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Characterization and source apportionment of pharmaceuticals in surface water of the Yangtze Estuary and adjacent sea

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environmental Science and pollution Research 2024年第39期31卷 52171-52180页

作者： Chen, Chunzhao Tang, Jian Li, Fei Xue, Rui Xiao, Yihua Chen, Ling Yu, Gang Advanced Interdisciplinary Institute of Environment and Ecology Beijing Normal University Zhuhai519087 China Department of Chemistry and Environmental Science New Jersey Institute of Technology NJ United States Institute of Science and Technology Information Beijing Academy of Science and Technology Beijing100089 China School of Environmental and Municipal Engineering Qingdao University of Technology Qingdao266520 China State Key Laboratory of Pollution Control and Resource Reuse College of Environmental Science and Engineering Tongji University Shanghai200092 China

Pharmaceuticals, which are closely linked to human activities, have attracted global attention. This study investigated the occurrence characteristics of 20 pharmaceuticals in surface water of the Yangtze Estuary and adjacent sea. A total of 14 targeted pharmaceuticals were detected in both spring and summer sampling campaigns. The mean concentrations of sulfonamides and non-sulfonamides were 36.60 ± 19.43 ng·L−1 and 50.02 ± 41.07 ng·L−1, respectively. As for non-antibiotics, their concentrations were in the range of 24.34 ± 916.8 ng·L−1 with caffeine accounting for 6.17 ~ 86.70% (average percentage of 42.22%). Meanwhile, spatial distribution patterns showed similarities between antibiotics and non-antibiotics, with high levels occurring near the upper estuary, aquaculture areas, wastewater treatment plants, and the maximum turbidity zone. This phenomenon could be related to the sources of pharmaceuticals and the physicochemical properties of water bodies. Obviously, the first three areas are highly impacted by human activities or serve as important sources of terrestrial contaminants entering the East China Sea. The last area retains high amounts of suspended particles which may exert strong trapping effects on hydrophobic chemicals. Principal component analysis revealed the presence of three potential sources for pharmaceuticals in the Yangtze Estuary, with a relatively high percentage originating from incompletely treated municipal sewage. As for the temporal trend, pharmaceutical contamination was found to be higher in spring compared to summer, potentially due to variations in pharmaceutical consumption patterns, local rainfalls, and water temperatures. These findings provide fundamental data support for implementing appropriate local management strategies for pharmaceutical usages. © The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2024.

关键词： Antibiotics

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In-situ synthesis of Z-scheme CeO_(2)@WO_(3) heterojunction with aromatic rings as electron medium for efficient photocatalytic degradation of perfluorobutane sulfonate

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Journal of Rare Earths 2025年第3期43卷 470-479,I0002页

作者： Shihai Cao Haocheng Yang Cheng Cheng Jinheng Dai Shuaishuai Lu Yao Lu College of Environmental Engineering Nanjing Institute of TechnologyNanjing211167China Jiangsu Environmental Engineering Technology Co. Ltd.Nanjing210019China Key Laboratory of Jjiangsu Province for Chemical Pollution Control and Resources Reuse School of Environmental and Biological EngineeringNanjing University of Science and TechnologyNanjing210094China School of Environment and Safety Engineering School of Emergency ManagementInstitute of Environment and EcologyJiangsu UniversityZhenjiang 212013China Jiangsu Collaborative Innovation Center of Technology and Material of Water Treatment Suzhou University of Science and TechnologySuzhou215009China

Photocatalytic technology has been proven to be a simple and effective method for degrading recalcitrant organic *** this study,a series of Z-scheme heterojunction nanocomposites composed of CeO_(2)and terephthalic acid-modified WO_(3) was prepared and further used as photocatalysts for perfluorobutane sulfonate(PFBS)*** this design,terephthalic acid was used as an electron recombination center and heterojunction mediator,which effectively enhances the migration ability of electron-hole pairs and the physicochemical stability of the *** addition,in situ synthesis of CeO_(2)onto the WO_(3) surface by the coordinate bond between terephthalic acid and Ce ions can avoid CeO_(2)*** a result,the CeO_(2)@WO_(3) photocatalyst exhibits excellent PFBS degradation ability(94%for CeO_(2)@WO_(3) vs.19%for CeO_(2)).After the fifth cyclic degradation experiment,the CeO_(2)@WO_(3) photocatalyst still maintains stable degradation ***,the reaction mechanism of the PFBS in CeO_(2)@WO_(3) photocatalytic process was analyzed by free radical trapping experiment and liquid chromatography tandem mass spectrometry(LC-MS)*** study provides new insights for constructing Z-scheme heterojunction and demonstrates that CeO_(2)@WO_(3) photocatalysts possess a promising prospect for degrading PFBS pollutants.

关键词： CeO_(2) WO_(3) Photocatalytic Z-Scheme heterojunction Perfluorobutane sulfonate(PFBS) Rare earths

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Efficient Adsorption of Hydroxychloroquine by Carboxylated Lignin-Based Sponge: Quantification of the Adsorption Contribution of Interactions

SSRN

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SSRN 2024年

作者： Gao, Boqiang Ma, Shuanglong Liang, Haoge Wang, Jie Huang, Yan Wang, Jingzhen Song, Jia Hu, Pan Yang, Hu College of Resources and Environment Henan Agricultural University Zhengzhou450002 China State Key Laboratory of Pollution Control and Resource Reuse School of the Environment Nanjing University Nanjing210023 China

Hydroxychloroquine (HCQ) as an antiviral pharmaceutical has been widely detected in the aquatic environment. Adsorption is an effective method for removal of HCQ, but the quantitative study of the adsorption interactions is unclear. In this study, a carboxylated lignin-based sponge (PLC) was fabricated, and the adsorption contributions of electrostatic attraction (EA), hydrogen bond (HB), and π-π electron donor-acceptor (π-π EDA) interactions were quantitatively investigated. The results showed that PLC exhibited excellent adsorption performance under wide pH range (4.0 0.822) and three molecular probes (R2 > 0.749) was established, respectively. The optimal adsorption capacity was achieved by the synergistic combination of the deprotonated carboxyl of PLC with the HB of Ka1 amino, EA of Ka2 amino, and the π-π EDA of the quinoline ring. This study provided a new strategy for the quantitative construction of structure-activity relationships of adsorbents. © 2024, The Authors. All rights reserved.

关键词： Lignin

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Measurement of atmospheric nanoparticles:Bridging the gap between gas-phase molecules and larger particles

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Journal of environmental Sciences 2023年第1期123卷 183-202页

作者： Chao Peng Chenjuan Deng Ting Lei Jun Zheng Jun Zhao Dongbin Wang Zhijun Wu Lin Wang Yan Chen Mingyuan Liu Jingkun Jiang Anpei Ye Maofa Ge Weigang Wang State Key Laboratory for Structural Chemistry of Unstable and Stable Species Beijing National Laboratory for Molecular Sciences(BNLMS)CAS Research/Education Center for Excellence in Molecular SciencesInstitute of ChemistryChinese Academy of SciencesBeijing 100190China State Key Joint Laboratory of Environment Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing 100084China School of Environment Science and Engineering Nanjing University of Information Science&TechnologyNanjing 210044China School of Atmospheric Sciences Sun Yat-sen UniversityZhuhaiGuangdong 519082China State Key Joint Laboratory of Environmental Simulation and Pollution Control College of Environmental Sciences and EngineeringPeking UniversityBeijing 100871China Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention(LAP3) Department of Environmental Science&EngineeringFudan UniversityShanghai 200433China Key Laboratory for the Physics and Chemistry of Nanodevices Department of ElectronicsSchool of Electronics Engineering and Computer SciencePeking UniversityBeijing 100871China University of Chinese Academy of Sciences Beijing 100049China

Atmospheric nanoparticles are crucial components contributing to fine particulate matter(PM_(2.5)),and therefore have significant effects on visibility,climate,and human *** to the unique role of atmospheric nanoparticles during the evolution process from gas-phase molecules to larger particles,a number of sophisticated experimental techniques have been developed and employed for online monitoring and characterization of the physical and chemical properties of atmospheric nanoparticles,helping us to better understand the formation and growth of new *** this paper,we firstly review these state-of-the-art techniques for investigating the formation and growth of atmospheric nanoparticles(e.g.,the gas-phase precursor species,molecular clusters,physicochemical properties,and chemical composition).Secondly,we present findings from recent field studies on the formation and growth of atmospheric nanoparticles,utilizing several advanced ***-more,perspectives are proposed for technique development and improvements in measuring atmospheric nanoparticles.

关键词： Nanoparticle Measurement techniques Size distributions Physical properties Chemical composition

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Microplastics in landfill leachate:Sources,detection,occurrence,and removal

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environmental Science and Ecotechnology 2023年第4期16卷 26-37页

作者： Mosarrat Samiha Kabir Hong Wang Stephanie Luster-Teasley Lifeng Zhang Renzun Zhao Department of Nanoengineering North Carolina Agricultural and Technical State UniversityGreensboroNC27411USA State Key Laboratory of Pollution Control and Resource Reuse College of Environmental Science and EngineeringTongji UniversityShanghai200092China Shanghai Institute of Pollution Control and Ecological Security Shanghai200092China Civil Architectural and Environmental Engineering DepartmentNorth Carolina Agricultural and Technical State UniversityGreensboroNC27411USA

Due to the accumulation of an enormous amount of plastic waste from municipal and industrial sources in landfills,landfill leachate is becoming a significant reservoir of *** release of microplastics from landfill leachate into the environment can have undesirable effects on humans and *** study provides the state of the science regarding the source,detection,occurrence,and remediation of microplastics in landfill leachate based on a comprehensive review of the scientific literature,mostly in the recent *** waste and wastewater treatment residue are the primary sources of microplastics in landfill *** concentration in raw and treated landfill leachate varied between 0-382 and 0-2.7 items L^(−1).Microplastics in raw landfill leachate are largely attributable to local plastic waste production and solid waste management ***,polystyrene,and polypropylene are the most prevalent microplastic polymers in landfill *** though the colors of microplastics are primarily determined by their parent plastic waste,the predominance of light-colored microplastics in landfill leachate indicates long-term *** identified morphologies of microplastics in leachate from all published sources contain fiber and fragments the *** on the treatment method,leachate treatment processes can achieve microplastic removal rates between 3%and 100%.The review also provides unique perspectives on microplastics in landfill leachate in terms of remediation,final disposal,fate and transport among engineering systems,and source reduction,*** landfill-wastewater treatment plant loop and bioreactor landfills present unique difficulties and opportunities for managing microplastics induced by landfill leachate.

关键词： Landfill leachate Microplastics Source Detection Occurrence Treatment

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Temporal patterns of algae in different urban lakes and their correlations with environmental variables in Xi’an,China

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Journal of environmental Sciences 2023年第11期133卷 138-151页

作者： Shengnan Chen Hanyan Liu Haihan Zhang Kai Li Na Wang Weimin Sun Xiang Liu Limin Niu Ben Ma Fan Yang Haiyun Li Daijuan Zhao Yan Xing Shaanxi Key Laboratory of Environmental Engineering Key Laboratory of Northwest Water ResourceEnvironment and EcologyMOEXi’an University of Architecture and TechnologyXi’an 710055China School of Environmental and Municipal Engineering Xi’an University of Architecture and TechnologyXi’an 710055China National-Regional Joint Engineering Research Center for Soil Pollution Control and Remediation in South China Guangdong Key Laboratory of Integrated Agro-environmental Pollution Control and ManagementInstitute of Eco-environmental and Soil SciencesGuangdong Academy of SciencesGuangzhou 510650China Guangdong-Hong Kong-Macao Joint Laboratory for Environmental Pollution and Control Guangzhou Institute of GeochemistryChinese Academy of SciencesGuangzhou 510640China Shaanxi Environmental Monitoring Center Xi’an 710054China

Urban lakes were critical in aquatic ecology environments,but how environmental factors affected the distribution and change characteristics of algal communities in urban lakes of Xi’an city was not ***,we investigated the algal community structure of six urban lakes in Xi’an and evaluated the effects of water quality parameters on *** results indicated that the significant differences on physicochemical parameters existed in different urban *** maximum concentration of total phosphorus in urban lakes was(0.18±0.01)mg/L and there was a phenomenon of phosphorus *** addition,51 genera of algae were identified and Chlorella *** the dominant algal species,which was affiliated with *** analysis elucidated that each lake had a unique algal community network and the positive correlation was dominant in the interaction between algae species,illustrating that mature microbial communities existed or occupied similar *** analysis illustrated that environmental factors explained 47.35% variance of algal species-water quality correlation collectively,indicating that water quality conditions had a significant influence on the temporal variations of *** equation model further verified that algal community structure was directly or indirectly regulated by different water quality *** study shows that temporal patterns of algal communities can reveal the dynamics and interactions of different urban ecosystem types,providing a theoretical basis for assessing eutrophication levels and for water quality management.

关键词： Urban lakes Algal community structure Network analysis Species interaction pattern Structural equation model

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Identify the contribution of vehicle non-exhaust emissions:a single particle aerosol mass spectrometer test case at typical road environment

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Frontiers of environmental Science & Engineering 2023年第5期17卷 117-128页

作者： Qijun Zhang Jiayuan Liu Ning Wei Congbo Song Jianfei Peng Lin Wu Hongjun Mao Tianjin Key Laboratory of Urban Transport Emission Research&State Environmental Protection Key Laboratory of Urban Ambient Air Particulate Matter Pollution Prevention and Control College of Environmental Science and EngineeringNankai UniversityTianjin 300071China School of Geography Earth and Environment Sciences University of BirminghamBirmingham B152TTUK

A single particle aerosol mass spectrometer(SPAMS)was used to accurately quantify the contribution of vehicle non-exhaust emissions to particulate matter at typical road *** PM_(2.5),black carbon,meteorological parameters and traffic flow were recorded during the test *** daily trend for traffic flow and speed on TEDA Street showed obvious“M”and“W”characteristics.6.3 million particles were captured via the SPAMS,including 1.3 million particles with positive and negative spectral map *** Metal,High molecular Organic Carbon,Organic Carbon,Mixed Carbon,Elemental Carbon,Rich Potassium,Levo-rotation Glucose,Rich Na,SiO_(3) and other categories were *** particle number concentration measured by SPAMS showed a good linear correlation with the mass concentrations of PM_(2.5) and BC,which indicates that the particulate matter captured by the SPAMS reflects the pollution level of fine particulate ***,ECOC,OC,HM and crustal dust components were found to show high values from 7:00–9:00 AM,showing that these chemical components are directly or indirectly related to vehicle *** on the PMF model,7 major factors are *** relative contributions of each factor were determined:vehicle exhaust emission(44.8%),coal-fired source(14.5%),biomass combustion(12.2%),crustal dust(9.4%),ship emission(9.0%),tires wear(6.6%)and brake pads wear(3.5%).The results show that the contribution of vehicle non-exhaust to particulate matter at roadside environment is approximately 10.1%.Vehicle non-exhaust emissions are the focus of future research in the vehicle pollutant emission control field.

关键词： Non-exhaust emissions SPAMS PMF Roadside environment

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Research on risk Assessment and decision support for underwater Platform in Naval Battle field environment

Research on risk Assessment and decision support for underwa...

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2022 International Conference on Information Processing in Ocean Science and Technology, ICIPOST 2022

作者： Zilong, Guo Hong, Mei Shi, Jian Yunxiang, Zhang Qiuliang, Hu Research Centre of Ocean Environment Numerical Simulation Institute of Meteorology and Oceanography PLA University of Science and Technology Nanjing China Key Laboratory of Surficial Geochemistry Ministry of EducationDepartment of Hydrosciences School of Earth Sciences and Engineering State Key Laboratory of Pollution Control and Resource Reuse Nanjing University Nanjing210093 China

Autonomous underwater unmanned platforms have become important facilities in the marine field since countries attach importance to maritime rights and interests, and play an important role in both military and civilian use. However, complex underwater marine environmental elements will have a huge impact on the performance of underwater unmanned platforms, and how to ensure the safe and stable operation of underwater unmanned platforms has become an urgent problem to be solved. Based on this practical problem, this paper studies the influence of marine environmental elements on the operation of underwater unmanned platforms with reference to the hydrological data of the South China Sea, and uses Bayesian methods to carry out risk zoning of the impact of the marine environment in the South China Sea on underwater unmanned platforms. © Published under licence by IOP Publishing Ltd.

关键词： Risk assessment

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High-gain signal-on PEDOT:PSS organic photoelectrochemical transistor biosensing modulated by a MXene/MOFs/NiO Schottky heterojunction

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Science China Chemistry 2023年第2期66卷 578-585页

作者： Zheng Li Yi-Tong Xu Jin Hu Ting Wang Fang-Qing Liu Hong Zhou Guang-Xu Chen Peng Lin Wei-Wei Zhao Jing-Juan Xu Hong-Yuan Chen State Key Laboratory of Analytical Chemistry for Life Science School of Chemistry and Chemical EngineeringNanjing UniversityNanjing210023China Shenzhen Key Laboratory of Special Functional Materials&Guangdong Research Center for Interfacial Engineering of Functional Materials College of Materials Science and EngineeringShenzhen UniversityShenzhen518060China Shandong Key Laboratory of Biochemical Analysis College of Chemistry and Molecular EngineeringQingdao University of Science and TechnologyQingdao266042China School of Environment and Energy State Key Laboratory of Luminescent Materials and DevicesGuangdong Provincial Key Laboratory of Atmospheric Environment and Pollution ControlSouth China University of TechnologyGuangzhou510006China

Herein we report a high-gain signal-on poly(3,4-ethylenedioxythiophene):poly(styrene sulfonate)(PEDOT:PSS)organic electrochemical transistor(OECT)biosensing using an accumulation-mode PEDOT:PSS OECT modulated by a light-fueled MXene/MOFs/Ni O Schottky *** such a system,the MXene/MOFs/Ni O Schottky heterojunction exhibited superior gating effect,as it not only enabled the fast-directional charge transfer but also guaranteed the maximal accessibility of the electrolyte to topped 2D MXene with large surface *** linkage with a bi-enzyme cascade system,the quinone derivatives produced by the cascade reaction of alkaline phosphatase(ALP)and tyrosinase(TYR)could serve as effective electron acceptors for the representative Ti_(3)C_(2)/PCN-224/Ni O heterojunction,underpinning an innovative method for sensitive detection of ALP activity with a low detection limit of 0.001 U L^(-1).Remarkably,the as-developed system demonstrated a remarkable current gain as high as near 10^(4),which to our knowledge is the highest one among existing OECT biosensory *** work represents a generic protocol to develop the novel signal-on PEDOT:PSS OECT platform towards biochemical detection and beyond.

关键词： signal-on PEDOT:PSS organic electrochemical transistor biosensing Schottky heterojunction

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