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Role of Nano-Fe3O4 for enhancing nitrate removal in microbial electrolytic cells: Characterizations and microbial patterns of cathodic biofilm

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Chemosphere 2023年第1期339卷

作者： Chen, Yuchen Yang, Jiayi Xiao, Lin Jiang, Lijuan Wang, Xiaolin Tang, Yuqiong School of the Environment Nanjing University Nanjing210023 China State Key Laboratory for Pollution Control and Resource Reuse Nanjing University Xianlin Campus Nanjing210023 China

Conductive magnetite nanoparticle (Nano-Fe3O4) can facilitate numerous biological reduction reactions as an outstanding electron mediator for electron transfer. The positive role of Nano-Fe3O4 for nitrate removal has gradually gained attention recent years, however, it has not been clarified for the persistence of the promoting effect under different concentrations addition. Performance of nitrogen removal and characteristics of cathodic biofilm were evaluated in this study after Nano-Fe3O4 addition with gradient concentration of 100∼500 mg L−1 in microbial electrolytic cells (MEC). Our study illustrated that the optimal concentration was 200 mg L−1 as the removal rate of nitrate increased by 24.76% and the removal rate of total dissolved nitrogen by 29.72%. At the optimal concentration, Nano-Fe3O4 increased cathodic biofilm DNA concentration by 61.04%, enhanced electron transport system activity, enriched iron redox bacteria, denitrifying bacteria and genes, as well as increased extracellular polymeric substances (EPS) amount, especially the protein content of soluble-EPS. However, promoting effect on nitrate removal was not visible in high concentration (500 mg L−1) addition, its electron transport system activity and EPS content were even declined. XPS results indicated that high concentration of Nano-Fe3O4 may reduce the availability of electrons to cathodic biofilm by competing for electrons, which inhibit nitrate removal. © 2023 Elsevier Ltd

关键词： Magnetite

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Evaluating coarse PM composition and sources based on bulk and molecular speciation of PM2.5 and PM10 in Nanjing, East China

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Journal of environmental Sciences 2025年第6期152卷 155-166页

作者： Wangnan Cui Zishu Wang Wei Feng Chao Qin Hong Liao Yuhang Wang Mingjie Xie Collaborative Innovation Center of Atmospheric Environment and Equipment Technology Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution ControlSchool of Environmental Science and EngineeringNanjing University of Information Science&TechnologyNanjing 210044China Nuist Reading Academy Nanjing University of Information Science&TechnologyNanjing 210044China State Environmental Protection Key Laboratory of Monitoring and Analysis for Organic Pollutants in Surface Water Jiangsu Environmental Monitoring CenterNanjing 210036China School of Earth and Atmospheric Sciences Georgia Institute of TechnologyAtlanta GA 30332United States

To understand the differences in the composition and sources of PM_(2.5) and PM_(10) caused by coarse particles,integrated PM_(2.5) and PM_(10) samples were synchronously collected in Nanjing,East China,in summer 2020 and winter 2020/*** and molecular speciation and light absorption measurements of aerosol extractswere performed,followed by positivematrix factorization(PMF)based on the PM_(2.5) and PM_(10) data sets,*** difference in average concentrations of total bulk species between PM_(2.5) and PM_(10) was mainly caused by the distribution of considerable NO_(3)^(–),SO42–,Ca^(2+),and organic carbon(OC)in coarse *** PMinfluenced by abrasion products from tirewear and leaves contributed about half of the low-volatility n-alkanes in *** contribution of coarse PM to biomass burning tracers and water-soluble OC increased in winter when biomass combustion was excessively *** than 70%of sugar polyols were attributable to coarse PM in summer,and biomass burning could be an important source in *** light-absorbing organic chromophores were almost entirely associated with PM_(2.5),but water-soluble organic carbon(WSOC)exhibited stronger light absorption in PM_(10) extracts than in PM_(2.5) extracts possibly due to the influence of coarse PMon *** analysis indicated that biomass burning,aqueous-phase reactions,and processed dust were the main contributors of organic matter and its light absorption in *** primary and secondary sources made discernable contributions only in *** differences between PM_(2.5) and PM_(10) were likely attributed to mixing of crustal dust,combustion particles,and surface reactions.

关键词： Coarse particle Bulk species Organic molecular marker Light absorption Source apportionment

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Optimization of Regional Energy-Water Nexus System Under Multiple Uncertainties 15th

Optimization of Regional Energy-Water Nexus System Under Mul...

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15th International Conference on environmental Science and Development, ICESD 2024

作者： Liu, Ruoyan Li, Yongping Huang, Guohe Zhou, Yanxiao Li, Yanfeng State Key Joint Laboratory of Environmental Simulation and Pollution Control School of Environment Beijing Normal University Beijing China Institute for Energy Environment and Sustainable Communities University of Regina ReginaSask Canada

ISBN: (纸本)9783031886829

In this paper, an interval chance-constrained programming (ICCP) method is proposed for collaborative energy-water nexus (EWN) system under multiple uncertainties. This method can solve the uncertainties expressed as probability distribution and interval. An ICCP-based energy-water nexus (ICCP-EWN) model is established, where 15 scenarios are designed for assessing the effect of water cycle coefficients and constraint violation risk. The results show that: (i) coal would remain the main energy sources for future energy supply, but the proportion of clean energy (e.g., natural gas, biomass) in the future power generation structure would significantly increase (about 15.6%);(ii) the water withdrawal of power generation in the energy system would be largest, where thermal power generation would have the largest proportion of water withdrawal, accounting for 85.0%;(iii) the decreasing α level and increasing p level will bring higher system benefits, and the reliability of the system would be reduced. These results can help determine the energy mix of a planned area, improve security of energy supply, and make trade-off between system benefits and the risk of violating constraints. © The Author(s), under exclusive license to Springer Nature Switzerland AG 2025.

关键词： Normal distribution

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Heteroatomic Modification of Solid-Waste-Based Mesoporous Carbon for Volatile Organic Compound Adsorption

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China Petroleum Processing & Petrochemical Technology 2023年第1期25卷 66-78页

作者： Liu Jun Li Zhi Xu Ke Zhang Xinyang Li Yunpeng Wang Ya Zhang Yongfa Yang Song Liu Shoujun Li Junhua College of Chemistry Taiyuan University of TechnologyTaiyuan 030024 State Key Joint Laboratory of Environment Simulation and Pollution Control National Engineering Laboratory for Multi Flue Gas Pollution Control Technology and EquipmentSchool of EnvironmentTsinghua UniversityBeijing 100084 State Key Laboratory of Clean and Efficient Coal Utilization College of Chemical Engineering and TechnologyTaiyuan University of TechnologyTaiyuan 030024 Shandong Pengda Ecological Technology Co. Ltd.ZiboShandong 255420 Taiyuan Green Coke Energy Co. Ltd.Taiyuan 030006

Solid-waste-based activated carbon(AC)was utilized as a carbon source to synthesize a series of carbon-based functional material RAC-X(X=P and S,where P and S denote phosphoric and sulfuric acids,respectively).The toluene adsorption capacities of the regeneration AC(RAC)samples can be significantly improved by adopting the heteroatomic modification ***-P and RAC-S have the same specific surface area(1156 m^(2)/g)and similar porous ***,they have different toluene adsorption capacities,with 316.22 mg/g for RAC-P and 460.12 mg/g for RAC-S,which are 1.6 and 2.4 times greater than that for *** X-ray photoelectron spectroscopy measurements showed that the increase in the amount ofπ–π^(2)chemical bond over the AC surface results in the improvement of the toluene adsorption *** density functional theory results showed that the S-containing functional groups loaded near the defect sites of RAC-S promote toluene ***,reusability tests showed that RAC-S still retains 86%of its adsorption activity after four consecutive adsorption–desorption *** indicates that the heteroatomic modification method affords excellent toluene adsorption performance and recycling practicability,which not only is beneficial for achieving the rational utilization of solid waste resources but also provides a practical method for the efficient elimination of volatile organic compounds.

关键词： waste activated carbon toluene adsorption heteroatomic modification functional groups DFT analysis

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Nitrous oxide emissions and microbial communities variation in low dissolved oxygen and low carbon-to-nitrogen ratio anoxic–oxic wastewater treatment plant

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environmental Science and pollution Research 2024年第30期31卷 42779-42791页

作者： Yan, Wanli Li, Jianguo Gu, Lide Ye, Chengsong Liang, Jieping Fu, Jinjin Zheng, Shikan Yu, Xin College of the Environment and Ecology Xiamen University Xiamen361005 China Fujian Key Laboratory of Coastal Pollution Prevention and Control Xiamen University Xiamen361005 China State Key Laboratory of Marine Environmental Science and College of Ocean and Earth Sciences Xiamen University Xiamen361005 China School of Life Sciences Xiamen University Xiamen361005 China

Dissolved oxygen (DO) levels and carbon-to-nitrogen (C/N) ratio affect nitrous oxide (N2O) emissions by influencing the physiological and ecological dynamics of nitrifying and denitrifying microbial communities in activated sludge systems. For example, Nitrosomonas is a common N2O producing nitrifying bacteria in wastewater treatment plants (WWTPs), and DO conditions can affect the N2O production capacity. Previous studies have reported N2O emission characteristics under adequate DO and C/N conditions in A/O WWTPs. However, in actual operation, owing to economic and managerial factors, some WWTPs have a long-term state of low DO levels in oxic tanks and low influent C/N. Research on N2O emission characteristics in low DO-limited and low C/N ratio WWTPs is limited. This study investigated N2O emissions and the corresponding shifts in microorganisms within an anoxic–oxic (A/O) WWTP over 9-month. Quantitative PCR was used to assess the abundance of ten functional genes related to nitrification and denitrification processes, and high-throughput sequencing of the 16S rRNA gene was employed to determine the composition change of microorganisms. The findings revealed that 1) the average N2O emission factor was 1.07% in the studied WWTP;2) the DO-limited oxic tank primarily contributed to N2O;3) NO2–, TOC, and C/N ratios were key factors for dissolved N2O in the aerobic tank;and 4) Nitrosomonas and Terrimonas exhibited a robust correlation with N2O emissions. This research provides data references for estimating N2O emission factors and developing N2O reduction policies in WWTPs with DO-limited and low C/N ratios. © The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2024.

关键词： Wastewater treatment

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Differences in distributions, assembly mechanisms, and putative interactions of AOB and NOB at a large spatial scale

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Frontiers of environmental Science & Engineering 2023年第10期17卷 55-64页

作者： Bing Zhang Chenxiang Sun Huimin Lin Wei Liu Wentao Qin Tan Chen Ting Yang Xianghua Wen College of Life and Environmental Sciences Minzu University of ChinaBeijing 100081China Environmental Simulation and Pollution Control State Key Joint Laboratory School of EnvironmentTsinghua UniversityBeijing 100084China Institute of Plant Protection Beijing Academy of Agriculture and Forestry SciencesBeijing 100097China

Ammonia-oxidizing bacteria (AOB) and nitrite-oxidizing bacteria (NOB) play crucial roles in removing nitrogen from sewage in wastewater treatment plants (WWTPs) to protect water resources. However, the differences in ecological properties and putative interactions of AOB and NOB in WWTPs at a large spatial scale remain unclear. Hence, 132 activated sludge (AS) samples collected from 11 cities across China were studied by utilizing 16S rRNA gene sequencing technology. Results indicated that Nitrosomonas and Nitrosospira accounted for similar ratios of the AOB community and might play nearly equal roles in ammonia oxidation in AS. However, Nitrospira greatly outnumbered other NOB genera, with proportions varying from 94.7% to 99.9% of the NOB community in all WWTPs. Similar compositions and, hence, a low distance–decay turnover rate of NOB (0.035) across China were observed. This scenario might have partly resulted from the high proportions of homogenizing dispersal (~13%). Additionally, drift presented dominant roles in AOB and NOB assembling mechanisms (85.2% and 81.6% for AOB and NOB, respectively). The partial Mantel test illustrated that sludge retention time and temperature were the primary environmental factors affecting AOB and NOB communities. Network results showed that NOB played a leading role in maintaining module structures and node connections in AS. Moreover, most links between NOB and other microorganisms were positive, indicating that NOB were involved in complex symbioses with bacteria in AS.

关键词： Activated sludge Spatial distributions Microbial assembly Co-occurrence patterns Nitrifying bacteria

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Facilitating Se(VI) adsorption and electron transfer by introducing αFeOOH to sulfidated zero-valent iron

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Separation and Purification Technology 2024年 344卷

作者： Li, Ke Zhang, Yue Qu, Guanjun Xu, Chunhua Shandong Key Laboratory of Water Pollution Control and Resource Reuse School of Environmental Science and Engineering Shandong University Qingdao266237 China

Sulfidation of zerovalent iron (SZVI) enhances electron transfer ability due to the formation of FeSx, which facilitates pollutant removal. However, for pollutants that are difficult to adsorb onto SZVI, the longer electron transfer distance results in inefficient removal. The presence of iron (hydr)oxides on ZVI and SZVI is inevitable, and it can adsorb highly mobile pollutants (such as Se(VI)). Here, we regulated the composition of iron (hydr)oxides on ZVI and SZVI surfaces by aging treatment, which improves their Se(VI) removal performance. Based on this, αFeOOH which has a strong affinity for Se(VI), is introduced onto SZVI to synthesize the high-quality composite SZVI-αFeOOH. The characterization results showed that Fe-OH from αFeOOH and FeSx successfully combined and uniformly distributed on SZVI-αFeOOH, creating active sites, and the Se(VI) removal rate (kobs = 0.2211 min−1) increased ∼ 7.4 times over SZVI (kobs = 0.0297 min−1). The adsorption and reduction of Se(VI) were optimized by regulating the mass ratio of αFeOOH to SZVI. In addition, different initial Se(VI) concentrations and solution pH were designed to explore the effects on Se(VI) removal and evaluate the best removal reaction condition. The mechanism of Se(VI) removal by SZVI-αFeOOH is as follows: Se(VI) is firstly adsorbed on αFeOOH, which shortens the electron transfer distance, and then the absorbed Se(VI) is reduced to readily immobilized states by SZVI. This work proposes a targeted strategy to modify SZVI to efficiently remove pollutants with strong mobile and difficult adsorption. © 2024 Elsevier B.V.

关键词： Adsorption

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Long-Term and Multi-Scale Assessment of Enhancing Mechanisms of Methanogenesis in Magnetite Nanoparticle-Mediated Anaerobic Digestion: From Digester Performance, Biochemical Parameters to Microbial Communities

SSRN

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SSRN 2024年

作者： Li, Jibin Sun, Desheng Wu, Siqi Yang, Wenlan Xiong, Lei Zhang, Weiming Hua, Ming Pan, Bingcai State Key Laboratory of Pollution Control and Resource Reuse School of the Environment Nanjing University Nanjing210023 China School of the Environmental Science and Engineering Yangzhou University Yangzhou225000 China

Magnetite nanoparticles (Fe3O4-NPs) have been demonstrated to be involved in direct interspecies electron transfer between syntrophic bacteria, yet a comprehensive assessment of the ability of Fe3O4-NPs to cope with process instability and volatile fatty acids (VFAs) accumulation in scaled-up anaerobic reactors is still lacking. Here, we investigated the start-up characteristics of an expanded granular sludge bed (EGSB) with Fe3O4-NPs as an adjuvant at high organic loading rate (OLR). The results showed that methane production rate of R1 (with Fe3O4-NPs) was approximately 1.65 folds of R0 (control), and effluent COD removal efficiency was maintained at approximately 98.32% upon 20 kg COD/(m3·d) OLR. The components of volatile fatty acids are acetate and propionate, and the rapid scavenging of propionate accumulation was the difference between R1 and the control. The INT-ETS activity of R1 was consistently higher than that of R0 and R2, and the electron transfer efficiencies increased by 68.78% and 131.44%, respectively. Meanwhile, the CV curve analysis showed that the current of R1 was 40% higher than R3 (temporary addition of Fe3O4-NPs ), indicating that multiple electron transfer modes might coexist. High-throughput analysis further revealed that it was difficult to reverse the progressive deterioration of system performance with increasing OLR by simply reconfiguring bacterial community structure and abundance, demonstrating that the Fe3O4-NPs-mediated DIET pathway is a prerequisite for establishing multiple electron transfer systems. This study provides a long-term and multi-scale assessment of the gaining effect of Fe3O4-NPs in anaerobic digestion scale-up devices, and provides technical support for their practical engineering applications. © 2024, The Authors. All rights reserved.

关键词： Magnetite

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Mechanistic investigation on Ag-Cu_(2)O in electrocatalytic CO_(2) to CH_(4) by in situ/operando spectroscopic and theoretical analysis

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Journal of Energy Chemistry 2024年第1期88卷 521-531,I0012页

作者： Min Sun Luxiao Zhang Fuli Tian Jiaxin Li Yanqiu Lei Heng Zhang Lifeng Han Zhihua Guo Yonghui Gao Fenrong Liu Yan Wang Luhui Wang Shanghong Zeng School of Chemistry and Chemical Engineering Inner Mongolia UniversityHohhot 010021Inner MongoliaChina Key Laboratory of Medicinal and Edible Plants Resources of Hainan Province Hainan Vocational University of Science and TechnologyHaikou 571126HainanChina State Key Laboratory of Baiyunobo Rare Earth Resource Research and Comprehensive Utilization Baotou Research Institute of Rare EarthsBaotou 014030Inner MongoliaChina Zhejiang Key Laboratory of Petrochemical Environmental Pollution Control Zhejiang Ocean UniversityZhoushan 316022ZhejiangChina

Silver-copper electrocatalysts have demonstrated effectively catalytic performance in electroreduction CO_(2) toward CH_(4),yet a revealing insight into the reaction pathway and mechanism has remained ***,we construct chemically bonded Ag-Cu_(2)O boundaries,in which the complete reduction of Cu_(2)O to Cu has been strongly impeded owing to the presence of surface Ag *** interfacial confinement effect helps to maintain Cu^(+)sites at the Ag-Cu_(2)O *** in situ/operando spectroscopy and theoretical simulations,it is revealed that CO_(2) is enriched at the Ag-Cu_(2)O boundaries due to the enhanced physisorption and chemisorption to CO_(2),activating CO_(2) to form the stable intermediate^(*)*** boundaries between Ag shell and the Cu_(2)O mediate local^(*)CO coverage and promote^(*)CHO intermediate formation,consequently facilitating CO_(2)-to-CH_(4) *** work not only reveals the structure-activity relationships but also offers insights into the reaction mechanism on Ag-Cu catalysts for efficient electrocatalytic CO_(2) reduction.

关键词： Ag shell Interfacial confinement effect Cu~+ Local*CO coverage CO_(2)reduction

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Improving Fugitive Dust Emission Inventory from Construction Sector Using UAV Images Recognition

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Aerosol and Air Quality Research 2024年第8期24卷 1-18页

作者： He, Yuyao Jang, Jicheng Zhu, Yun Chiang, Pen-Chi Xing, Jia Wang, Shuxiao Zhao, Bin Long, Shicheng Yuan, Yingzhi Guangdong Provincial Key Laboratory of Atmospheric Environment and Pollution Control College of Environment and Energy South China University of Technology Guangzhou Higher Education Mega Center Guangzhou510006 China Graduate Institute of Environmental Engineering Taiwan University Taipei10673 Taiwan Carbon Cycle Research Center National Taiwan University Taipei10672 Taiwan Department of Civil and Environmental Engineering University of Tennessee KnoxvilleTN37996 United States State Key Joint Laboratory of Environment Simulation and Pollution Control School of Environment Tsinghua University Beijing100084 China

Over rapidly developing and urbanizing countries, frequent construction activities are the primary drivers behind the substantial emissions and contributors of fugitive dust. In this study, an innovative method was developed to compile a high-resolution spatiotemporal emission inventory from construction sector, utilizing unmanned aerial vehicle (UAV) images. This methodology offered detailed activity level information by distinguishing various types of construction lands and equipment. Focusing on the Shunde District of Guangdong in China, the new emission inventory derived from this method highlighted that travel, topsoil excavation, and loading collectively contributed up to 90% of particulate matter (PM) emissions during the earthwork phase. Moreover, this new inventory rectified the tendency of traditional methods to underestimate PM10 emissions and overestimate PM2.5 emissions, while revealing the non-linear relationship between PM emissions and construction area. This improved PM emission inventory appeared to precisely identify major emission hotspots and enhanced performance of the Community Multi-scale Air Quality (CMAQ) model, and the correlation coefficient (R-value) is 0.08 ± 0.02 higher than that of the traditional emission inventory. Post integration of monitoring data through the Software for the Modeled Attainment Test-Community Edition (SMAT-CE), the contributions of construction dust to local PM10 and PM2.5 concentrations were estimated at 3.27 ± 0.8 µg m–3 and 1.11 ± 0.27 µg m–3, respectively, with more pronounced impacts observed in the central, northwestern, and south-central zones of the study region. This study provides valuable insight for improving construction dust and PM emission inventories, which should be benefiting the development of air pollution prevention and control strategies over this study area as well as other rapidly growing urban areas. © The Author(s).

关键词： Image enhancement

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