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Accurate prediction of air quality response to emissions for effective control policy design

Journal of environmental Sciences 2023年第1期123卷 116-126页

作者： Min Cao Jia Xing Shovan Kumar Sahu Lei Duan Junhua Li State Key Joint Laboratory of Environmental Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing 100084China State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex Beijing 100084China

Designing effective control policy requires accurate quantification of the relationship between the ambient concentrations of O3and PM2.5and the emissions of their ***,the challenge is that precursor reduction does not necessarily lead to decreases in the concentrations of O3and PM2.5,which are formed by multiple precursors under complex physical and chemical processes;this calls for the development of advanced model technologies to provide accurate predictions of the nonlinear responses of air quality to *** from the traditional sensitivity analysis and source apportionment methods,the reduced form models(RFMs)based on chemical transport models(CTMs)are able to quantify air quality responses to emissions more accurately and efficiently with lower computational *** we review recent approaches used in RFMs and compare their structures,advantages and disadvantages,performance and *** general,RFMs are classified into three types including(1)sensitivity-based models,(2)models with simplified chemistry and physical processes,and(3)statistical models,with considerable differences in principles,characteristics and application *** prediction of nonlinear responses by RFMs enables more in-depth analysis,not only in terms of real-time prediction of concentrations and quantification of human exposure,health impacts and economic damage,but also in optimizing control ***,data assimilation and emission inventory inversion based on the nonlinear response of concentrations to emissions can also be greatly beneficial to air pollution control *** future studies,improvement in the performance of CTMs is exceedingly crucial to obtain a more reliable baseline for the prediction of air quality *** of models to determine the air quality response to emissions under varying meteorological conditions is also necessary in the context of future climate changes,which pose great challenges to the qua

关键词： Air pollution Nonlinear response Air quality management Reduced form models(RFMs) Precursor emissions

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Advanced Purification of Per-and Polyfluoroalkyl Substances in Drinking Water: Status and Challenges

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Huanjing Kexue/environmental Science 2025年第6期46卷 3440-3449页

作者： Fang, Xiao-Ya Wu, Ying-Peng Li, Tang-Rui Wu, Jia-Yang Huang, Hui Reng, Hong-Qiang State Key Laboratory of Pollution Control and Resource Reuse Schoolofthe Environment Nanjing University Nanjing210023 China

Per-and polyfluoroalkyl substances (PFASs) are a dass of emerging contaminants frequently detected in source water and drinking water. They are characterized by persistence, resistance to degradation, and various biologieal toxieities, posing serious risks to the environraent and human health. In recent years, researchers have hegun to explore ways to remove PFASs from drinking water. It is of great significance to clarify the eurrent Status and ehallenges of advanced purifieation technologies of PFASs for further researeh and teehnologieal innovation in this field. Based on the data-driven quantitative analysis of relevant papers, typical types, physicochemical properties, and environmental risks of PFASs were systematically eategorized, and their control requireraents and distrihution Status in surface water, groundwater, and drinking water were comprehensively reviewed. The researeh Status and mechanism of PFASs removal technologies were analyzed, further revealing researeh hotspots and development trends in this field. The potential ehallenges were further analyzed, and the opportunities for future innovation in advaneed purifieation technologies of PFASs were forecasted, such as the application of materials genomics, membrane Separation materials based on the physical properties of water moleeules, and micro/nano reaetors, aiming to provide referenees for the efficient removal and risk reduetion of PFASs in drinking water. © 2025 Science Press. All rights reserved.

关键词： Groundwater pollution

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Disinfection Byproducts and Their Precursors in Drinking Water Sources:Origins,Influencing Factors,and environmental Insights

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Engineering 2024年第5期36卷 36-50页

作者： Rong Xiao Yang Deng Zuxin Xu Wenhai Chu State Key Laboratory of Pollution Control and Resource Reuse College of Environmental Science and EngineeringTongji UniversityShanghai 200092China Ministry of Education Key Laboratory of the Yangtze River Water Environment Tongji UniversityShanghai 200092China Department of Earth and Environmental Studies Montclair State UniversityMontclairNJ 07043USA

Tracing the contamination origins in water sources and identifying the impacts of natural and human processes are essential for ecological safety and public ***,current analysis approaches are not ideal,as they tend to be laborious,time-consuming,or technically *** byproducts(DBPs)are a family of well-known secondary pollutants formed by the reactions of chemical disinfectants with DBP precursors during water disinfection *** DBP precursors have various origins(e.g.,natural,domestic,industrial,and agricultural sources),and since the formation of DBPs from different precursors in the presence of specific disinfectants is distinctive,we argue that DBPs and DBP precursors can serve as alternative indicators to assess the contamination in water sources and identify pollution *** providing a retrospective of the origins of DBPs and DBP precursors,as well as the specific formation patterns of DBPs from different precursors,this article presents an overview of the impacts of various natural and anthropogenic factors on DBPs and DBP precursors in drinking water *** practice,the DBPs(i.e.,their concentration and speciation)originally present in source water and the DBP precursors determined using DBP formation potential tests—in which water samples are dosed with a stoichiometric excess of specific disinfectants in order to maximize DBP formation under certain reaction conditions—can be considered as alternative *** jointly used with other water quality parameters(e.g.,dissolved organic carbon,dissolved organic nitrogen,fluorescence,and molecular weight distribution)and specific contaminants of emerging concern(e.g.,certain pharmaceuticals and personal care products),DBPs and DBP precursors in drinking water sources can provide a more comprehensive picture of water pollution for better managing water resources and ensuring human health.

关键词： Disinfection byproducts Disinfection byproduct precursors Drinking water sources Contamination indicator Natural factors Human factors

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"Forever chemicals":a sticky environmental problem

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Frontiers of environmental Science & Engineering 2024年第10期18卷 175-183页

作者： Junhua Fang Shaolin Li Rongliang Qiu Wei-Xian Zhang College of Environmental Science and Engineering State Key Laboratory of Pollution Control and Resource ReuseTongji UniversityShanghai 200092China Guangdong Laboratory for Lingnan Modern Agriculture Guangzhou 510642China College of Natural Resources and Environment Guangdong Provincial Key Laboratory of Agricultural&Rural Pollution Abatement and Environmental SafetySouth China Agricultural UniversityGuangzhou 510642China

The discovery and widespread use of per-and poly-fluoroalkyl substances(PFAS)have exemplified the beneficial role of chemistry in modern life,yet *** also underscored significant environmental and health *** "forever chemicals"due to their remarkable persistence,PFAS present formidable challenges in terms of contamination and *** to address these challenges have led to the development of innovative degradation technologies,such as hydrothermal alkali treatment(HALT),low-temperature mineralization,and mechanochemical degradation,offering promising solutions to PFAS ***,these advancements must be accompanied by robust investment in research,collaboration among stakeholders,and global responsibility to ensure effective management of PFAs contamination and mitigate its adverse impacts on ecosystems and humanhealth.

关键词： PFAS Degradation technologies environmental remediation Global responsibility

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PICRUSt2 functionally predicts organic compounds degradation and sulfate reduction pathways in an acidogenic bioreactor

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Frontiers of environmental Science & Engineering 2022年第4期16卷 81-93页

作者： Jun Li Aimin Li Yan Li Minhui Cai Gan Luo Yaping Wu Yechao Tian Liqun Xing Quanxing Zhang State Key Laboratory of Pollution Control and Resources Reuse School of the EnvironmentNanjing UniversityNanjing 210023China Jiangsu Key Laboratory of Chemical Pollution Control and Resources Reuse School of Environmental and Biological EngineeringNanjing University of Science and TechnologyNanjing 210094China

For comprehensive insights into the influences of sulfate on performance,microbial community and metabolic pathways in the acidification phase of a two-phase anaerobic system,a laboratory-scale acidogenic bioreactor was continuously operated to treat wastewater with elevated sulfate concentrations from 2000 to 14000 mg/*** results showed that the acidogenic bioreactor could achieve sulfate reduction efficiency of greater than 70%for influent sulfate content less than 12000 mg/*** sulfate induced the accumulation of volatile fatty acids(VPAs),especially propionate and butyrate,which was the primary negative effects to system performance under the high-sulfate ***-throughput sequencing coupled with PICRUSt2 uncovered that the accumulation of VFAs was triggered by the decreasing of genes encoding short-chain acyl-CoA dehydrogenase(EC:1.3.8.1),regulating the transformation of propanoyl-CoA to propenoyl-CoA and butanoyl-CoA to crotonyl-CoA of propionate and butyrate oxidation pathways,which made these two process hardly ***,genes encoding(EC:1.3.8.1)were mainly carried by order *** was the most abundant sulfate-reducing bacteria and identified as the primary host of dissimilatory sulfate reduction ftinctional *** analysis indicated the dissimilatory sulfate reduction process predominated under a low sulfate environment,but was not favored under the circumstance of *** the increase of sulfate,the assimilatory sulfate reduction process finally overwhelmed dissimilatory as the dominant sulfate reduction pathway in acidogenic bioreactor.

关键词： Acidogenic phase reactor High-sulfate wastewater Sulfate reduction Acidogenic fermentation PICRUSt2

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Dual-selective silver recovery strategy by simultaneous adsorption-reduction boosted by in-situ magnetic field

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Green Energy & environment 2025年第2期10卷 433-440页

作者： Jianran Ren Zhiliang Zhu Yanling Qiu Fei Yu Tao Zhou Jie Ma Jianfu Zhao Research Center for Environmental Functional Materials State Key Laboratory of Pollution Control and Resource ReuseCollege of Environmental Science and EngineeringTongji UniversityShanghai200092China School of Civil Engineering Kashi UniversityKashi844000China College of Marine Ecology and Environment Shanghai Ocean UniversityShanghai201306China

The mainstream silver recovery has problems such as resource waste,weak silver selectivity,and complicated ***,self-propelled magnetic enhanced capture hydrogel(magnetic NbFeB/MXene/GO,MNMGH)was prepared by self-crosslinking encapsulation *** achieved high selectivity(K_(d)=23.31 mL/g)in the acidic range,and exhibited ultrahigh silver recovery capacity(1604.8 mg/g),which greatly improved by 66%with the assistance of in-situ magnetic *** recovered silver crystals could be directly physically exfoliated,without acid/base *** selective sieving effect of adsorption,MNMGH preferentially adsorbed Ag(I),and then selectively reduced to Ag(0),realizing dual-selective *** in-situ magnetic field enhanced selective adsorption by enhancing mass transfer,reactivity of oxygen-containing functional ***,density function theory simulations demonstrated that the in-situ magnetic field could lower the silver reduction reaction energy barrier to enhance the selective ***-drive synergy system(reduction drive,adsorption drive and magnetic drive)achieved ultrahigh silver recovery *** study pioneered an in-situ magnetic field assisted enhancement strategy for dual-selective(adsorption/reduction)recovery of precious metal silver,which provided new idea for low-carbon recovery of noble metal from industrial waste liquids.

关键词： In-situ magnetic field Silver recovery Adsorption-reduction Selectivity Physical separation

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Release characteristics of arsenic from sediments and its source or sink competition with phosphorus:A case of a great lake with grass-algae alternation

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Journal of environmental Sciences 2025年第3期149卷 278-287页

作者： Shuhang Wang Yongsheng Chang Wei Huang Dianhai Yang Feifei Che State Key Laboratory of Pollution Control and Resource Reuse College of Environmental Science and EngineeringTongji UniversityShanghai 200092China College of Environmental Science and Engineering Donghua UniversityShanghai 201620China National Engineering Laboratory for Lake Pollution Control and Ecological Restoration Chinese Research Academy of Environmental SciencesBeijing 100012China

The arsenic(As)release from sediments in great lakes is affected by various *** this study,the characteristics of As release fromsediments was investigated,and the As sources and sinks with the strengths in sediments from different areas(grass-type,algae-type,and grass-algae alternation areas)in great shallow lakes(Taihu Lake,China)were analyzed,and the influence of P competition in the process of As release was also *** results showed that changing trend of the values of equilibrium As concentration in sediments were consistent with the regional changes(0 to 28.12μg/L),and the sediments from algaetype areas had the higher *** sediments from western lake and northwest lake bay were a strong As and a weak P source,and the north lake bay had the opposite trend of these two *** P source competition with As from the sediments occurred in algae-type *** grass-type areas had strong As and P retention capacities,indicating a sink role of sediment with high As and P sorption *** degree of As and P saturation had similar trend in sediments,and the grass-type areas had the higher values,18.3%-21.4%and 15.31%-20.34%,*** analysis results showed that most of As release contribution was from the bottom(30-50 cm)sediments,and the surface(0-10 cm)sediments from algae-type areas contributed more to the overlying water than other region.

关键词： Arsenic Phosphorus Sediment Source and sink Contribution

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Fabrication of MnO2 coating on aluminum honeycomb for fast catalytic decomposition of ozone at room temperature

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Journal of environmental Sciences 2023年第12期134卷 34-43页

作者： Yunjuan He Pengyi Zhang Jie Yang Shan Wang Jinge Li State Key Joint Laboratory of Environment Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing 100084China Beijing Key Laboratory for Indoor Air Quality Evaluation and Control Beijing 100084China

Herein, the coating of MnO2nanomaterials on the surface of aluminum honeycomb was carried out to meet the requirements of high air velocity, low pressure drop and high activity in ozone removal scenarios. A commercially readily available waterborne silica sol mixed with waterborne acrylate latex was creatively utilized as the binder. A series of coating samples were prepared by spray coating method and evaluated focusing on their adhesion strength and catalytic activity towards ozone decomposition in an air duct at room temperature, by varying MnO2/binder mass ratio and number of sprayings. It was found that the adhesion strength of the catalytic coatings on the aluminum honeycomb increased with the increase of binder mass ratio, but the increased binder made the catalyst particles closely packed,resulting in reduced exposure of active sites and decrease of ozone conversion. Accordingly,catalyst slurry with 81.8 wt.% MnO2in dry coating and spraying times of two were determined as the optimal process parameters. As-prepared aluminum honeycomb filter with MnO2layer of 50 μm thickness achieved ozone conversion of 29.3%±1.7% under conditions of air velocity 3.0 m/sec, relative humidity50%, room temperature(26°C) and initial ozone concentration of 200 ppbV. This filter can be well adaptable to indoor air purification equipment operating at high air velocity with low wind resistance.

关键词： Manganese dioxide Waterborne binder Coating Ozone conversion Catalyst

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Steam disinfection enhances bioaccessibility of metallic nanoparticles in nano-enabled silicone-rubber baby bottle teats,pacifiers,and teethers

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Journal of environmental Sciences 2024年第2期136卷 161-171页

作者： Yu Su BinWang Xin Tong Shuchuan Peng Sijin Liu Baoshan Xing Rong Ji State Key Laboratory of Pollution Control and Resource Reuse School of the EnvironmentNanjing UniversityNanjing 210023China School of Resources and Environmental Engineering Hefei University of TechnologyHefei 230009China State Key Laboratory of Environmental Chemistry and Ecotoxicology Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China Stockbridge School of Agriculture University of MassachusettsAmherstMA 01003USA

Nano-enabled silicone-rubber articles for feeding or chewing could be a source of metallic nanoparticles(NPs)directly exposed to infants and young ***,the impact of steam disinfection on release of NPs and the related potential risks to children's health are ***,we investigated contents and form of Ag and Zn in 57 nano-enabled silicone-rubber baby bottle teats,pacifiers,and teethers of seven countries and examined the impacts of steam disinfection on in vitro bioaccessibility(IVBA)of Ag and Zn in the *** 89%articles had a mixture of Ag-and Zn-containing NPs and the teethers had relatively high Ag and Zn contents(up to 501 and 254μg/g,respectively).Steam disinfection caused rubber decomposition into micro(nano)plastics(0.54-15.7μm)and NP release from the interior of bulk rubber and micro-sized plastics,thus enhancing the IVBA of Ag and Zn by up to 5.5 *** findings provide insights into mechanisms for NP release by steam *** oral exposure risk assessment suggested low health concerns on individual metal release,our study points out the need to assess the potential health risks of child co-exposure to metallic NPs and micro(nano)plastics.

关键词： Silicone rubber Metallic nanoparticles Micro(nano)plastics Bioaccessibility Children's health

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Synergistic effects of peroxydisulfate on UV/O_(3) process for tetracycline degradation:Mechanism and pathways

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Chinese Chemical Letters 2024年第10期35卷 408-413页

作者： Fengrui Yang Debing Wang Xinying Zhang Jie Zhang Zhichao Wu Qiaoying Wang State Key Laboratory of Pollution Control and Resource Reuse Shanghai Institute of Pollution Control and Ecological SecuritySchool of Environmental Science and EngineeringTongji UniversityShanghai 200092China Fujian Provincial Engineering Research Center of Rural Waste Recycling Technology College of Environment&Safety EngineeringFuzhou University.Fuzhou 350108China

Tetracycline(TC)as a typical emerging pollutant is becoming a serious threat to the environment and human health.A combined advanced oxidation technology of UV/Ozone(O_(3))/peroxydisulfate(PDS)process was developed to explore an efficient and economic treatment process of TC in ***,the reactive sites and transformation pathways of TC were explored and the toxicity of the intermediates was quantified with a quantitative structure-activity relationship(QSAR)*** degradation performance of TC was substantially enhanced in UV/O_(3)/PDS process with a kobsof 0.0949 min-1,which was 2.3 times higher than UV/O_(3)and 3.2 times than sole *** results demonstrated that there was a superior synergistic effect of PDS on UV/O_(3)processes for the degradation of *** paramagnetic resonance(EPR)analysis and quenching experiments show that·OH,SO_(4)·-,O_(2)·-and1O_(2)all contributed to TC degradation in the UV/O_(3)/PDS process and exhibited a synergistic effect,which inhibited the generation of harmful *** addition,the UV/O_(3)/PDS system can effectively degrade TC in a wide range of substrate concentrations and pH,and also showed excellent adaptability to various concentrations of anions(Cl-and HCO_(3)-).This study proves the feasibility of UV/O_(3)/PDS process for treating TC contaminated wastewater with complicated water matrix.

关键词： UV/ozonation/peroxydisulfate Synergistic effect Tetracycline Degradation Wastewater

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