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Vacuum ammonia stripping from liquid digestate:Effects of pH,alkalinity,temperature,negative pressure and process optimization

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Journal of environmental Sciences 2025年第3期149卷 638-650页

作者： Qiuhong Chen Donghai Yang Xiang Chen Xiankai Wang Bin Dong Xiaohu Dai State Key Laboratory of Pollution Control and Resource Reuse College of Environmental Science and EngineeringTongji UniversityShanghai 200092China YANGTZE Eco-Environment Engineering Research Center National Engineering Research Center of Eco-environment Protection for Yangtze River Economic BeltChina Three Gorges CorporationWuhan 430010China

High ammonia-nitrogen digestate has become a key bottleneck limiting the anaerobic digestion of organic solid *** ammonia stripping can simultaneously remove and recover ammonia nitrogen,which has attracted a lot of attention in recent *** investigate the parameter effects on the efficiency and mass transfer,five combination conditions(53℃ 15 kPa,60°C 20 kPa,65°C 25 kPa,72°C 35 kPa,and 81°C 50 kPa)were conducted for ammonia stripping of sludge *** results showed that 80%of ammonia nitrogen was stripped in 45 min for all experimental groups,but the ammonia transfer coefficient varied under different conditions,which increased with the rising of boiling point temperature,and reached the maximum value(39.0 mm/hr)at 81°C 50 *** ammonia nitrogen removal efficiency was more than 80%for 30 min vacuum stripping after adjusting the initial pH to above 9.5,and adjustment of the initial alkalinity also affects the pH value of liquid *** was found that pH and alkalinity are the key factors influencing the ammonia nitrogen dissociation and removal efficiency,while temperature and vacuum mainly affect the ammonia nitrogen mass transfer and removal *** terms of the mechanism of vacuum ammonia stripping,it underwent alkalinity destruction,pH enhancement,ammonia nitrogen dissociation,and free ammonia *** this study,two-stage experiments of alkalinity destruction and ammonia removal were also carried out,which showed that the two-stage configuration was beneficial for ammonia *** provides a theoretical basis and practical technology for the vacuum ammonia stripping from liquid digestate of organic solid waste.

关键词： Liquid digestate Vacuum ammonia stripping Alkalinity Mass transfer Process optimization

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Design and fabrication of self-suspending aluminum-plastic/semiconductor photocatalyst devices for solar energy conversion

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Journal of environmental Sciences 2024年第2期136卷 615-625页

作者： Zhi-Ang Zhao Jingyun Mao Chengjing Lu Shuangqiao Yang Qingrong Qian Qinghua Chen Hun Xue Xiaoli Sun Min-Quan Yang College of Environmental and Resource Sciences College of Carbon Neutral Modern IndustryFujian Key Laboratory of Pollution Control and Resource ReuseFujian Normal UniversityFuzhou 350007China State Key Laboratory of Polymer Materials Engineering Polymer Research Institute of Sichuan UniversityChengdu 610065China

The design and synthesis of self-suspending photocatalyst device with easy recyclability is important for practical ***,this work utilizes aluminum-plastic package waste as raw material to prepare an aluminum-plastic supported TiO_(2)(AP-TiO_(2))photocatalyst device through 3D printing design and surface deposition method.A series of characterizations were carried out to explore the structure,morphology and performance of the AP-TiO_(2)*** UV light illumination,the AP-TiO_(2)-50 efficiently degrade 93.6%tetracycline hydrochloride(THC)after 4 hr,which increases by 8.3%compared with that of TiO_(2)powder suspension system with the same catalyst *** on it,AP-ZnO,AP-CdS,AP-g-C_3N_4and AP-Pt-TiO_(2)are also fabricated,and applied in photocatalytic degradation and hydrogen evolution,which all exhibit higher photoactivities than powder suspension *** work provides a new avenue for the fabrication of advanced recyclable photocatalyst ***,the work offers a novel sight for the high-value utilization of aluminum-plastic package waste,which has positive implications for environmental protection.

关键词： TiO_(2) Self-suspending Photocatalyst device Aluminum plastic

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Metagenomics reveals the microbial community and functional metabolism variation in the partial nitritation-anammox process:From collapse to recovery

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Journal of environmental Sciences 2024年第1期135卷 210-221页

作者： Hong Wang Hui Gong Xiaohu Dai Min Yang State Key Laboratory of Pollution Control and Resource Reuse College of Environmental Science and EngineeringTongji UniversityShanghai 200092China BIOMATH Department of Data Analysis and Mathematical ModellingGhent UniversityGhent 9000Belgium

Mainstream partial nitritation-anammox(PNA)process easily suffers from performance instability and even reactor collapse in ***,it is of great significance to unveil the characteristic of performance recovery,understand the intrinsic mechanism and then propose operational *** this study,we combined long-term reactor operation,batch tests,and metagenomics to reveal the succession of microbial community and functional metabolism variation from system collapse to *** aeration control(0.10-0.25mg O_(2)/L)was critical for performance *** was also found that Candidatus Brocadia became the dominant flora and its abundance increased from 3.5%to 11.0%.Significant enhancements in carbon metabolism and phospholipid biosynthesis were observed during system recovery,and the genes abundance related to signal transduction was dramatically *** up-regulation of sdh and suc genes showed the processes of succinate dehydrogenation and succinyl-CoA synthesis might stimulate the production of amino acids and the synthesis of proteins,thereby possibly improving the activity and abundance of AnAOB,which was conducive to the performance ***,the increase in abundance of hzs and hdh genes suggested the enhancement of the anammox *** in the abundance of key genes involved in nitrogen metabolism indicated that nitrogen removal pathway was more diverse after system *** achievement of performance recovery was driven by anammox,nitrification and denitrification coupled with dissimilatory nitrate reduction to *** results provide deeper insights into the recovery mechanism of PNA system and also provide a potential regulation strategy for the stable operation of the mainstream PNA process.

关键词： Partial nitritation-anammox Metagenomics Microbial community Functional metabolism Recovery

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Highly active copper-intercalated weakly crystallized δ-MnO_(2) for low-temperature oxidation of CO in dry and humid air

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Frontiers of environmental Science & Engineering 2024年第5期18卷 127-136页

作者： Hao Zhang Huinan Li Pengyi Zhang Tingxia Hu Xianjie Wang State Key Joint Laboratory of Environment Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing100084China Beijing Key Laboratory for Indoor Air Quality Evaluation and Control Beijing100084China Midea Corporate Research Center Foshan528311China

Copper intercalated birnessite MnO_(2)(δ-MnO_(2))with weak crystallinity and high specific surface area(421 m^(2)/g)was synthesized by a one-pot redox method and investigated for low-temperature CO *** molar ratio of Cu/Mn was as high as 0.37,which greatly weakened the Mn-O bond and created a lot of low-temperature active oxygen *** situ DRIFTS revealed strong bonding of copper ions with ***-synthesized MnO_(2)-150Cu achieved 100%conversion of 250 ppm CO in normal air(3.1 ppm H_(2)O)even at−10°C under the weight-hourly space velocity(WHSV)of 150 L/(g·h).In addition,it showed high oxygen storage capacity to oxidize CO in inert *** the concurrent moisture in air significantly inhibited CO adsorption and its conversion at ambient temperature,MnO_(2)-150Cu could stably convert CO in 1.3%moisture air at 70°C owing to its great low-temperature activity and reduced competitive adsorption of water with increased *** study discovers the excellent low-temperature activity of weakly crystallized δ-MnO_(2) induced by high content intercalated copper ions.

关键词： CO oxidation Birnessite Interlayer copper Low-temperature Oxygen storage capacity

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Microstructure-Dependent Ion Selectivity in Graphene Oxide-Based Membranes

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ACS Applied Materials and Interfaces 2025年第22期17卷 32806-32815页

作者： Ren, Jing Chen, Xinran Tong, Xin State Key Laboratory of Pollution Control and Resource Reuse Shanghai Institute of Pollution Control and Ecological Security Tongji Advanced Membrane Technology Center School of Environmental Science and Engineering Tongji University 1239 Siping Road Shanghai200092 China

Graphene oxide (GO) membranes hold promise for precise separation due to their unique laminar structures and tunable separation properties. However, although water transport in GO membranes has been extensively investigated, the key mechanisms governing ion transport and selectivity remain poorly understood. In this work, we fabricated pristine and propylenediamine (PPD)/pentamethylenediamine (PTD)-cross-linked GO membranes via vacuum filtration and employed low-field nuclear magnetic resonance (LF-NMR) to elucidate their nanoscale pore architectures, including pinholes and structural defects. Our results show that cross-linking leads to a more ordered arrangement of the nanochannels and reduces the dimensions of structural defects. Ion diffusion experiments demonstrated that the membrane microstructure plays a crucial role in determining the tortuosity of the ion transport pathways. Notably, large structural defects dominate ion transport;when present, ions tend to bypass the interlayer nanochannels, leading to reduced ion selectivity. In contrast, intrinsic pinholes are too small to significantly contribute to ion transport. Molecular dynamics simulations showed that interlayer spacing, ion properties, and interactions with the membrane jointly govern ion diffusion within the GO-based nanochannels. More importantly, the simulation results deviated from experimental observations, further implying the pivotal role of large structural defects in ion transport. These findings provide valuable guidelines for designing next-generation GO-based membranes with improved ion selectivity and performance for precise separation. © 2025 American Chemical Society.

关键词： Crosslinking

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Year-round changes in tropospheric nitrogen dioxide caused by COVID-19 in China using satellite observation

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Journal of environmental Sciences 2023年第10期132卷 162-168页

作者： Zhenyu Luo Hailian Xu Zhining Zhang Songxin Zheng Huan Liu State Key Joint Laboratory of ESPC State Environmental Protection Key Laboratory of Sources and Control of Air Pollution ComplexSchool of EnvironmentTsinghua UniversityBeijing 100084China

The lockdown policy deals a severe blow to the economy and greatly reduces the nitrogen oxides(NOx)emission in China when the coronavirus 2019 spreads widely in early *** we use satellite observations from Tropospheric Monitoring Instrument to study the year-round variation of the nitrogen dioxide(NO_(2))tropospheric vertical column density(TVCD)in *** NO_(2)TVCD reveals a sharp drop,followed by small fluctuations and then a strong rebound when compared to *** the end of 2020,the annual average NO_(2)TVCD declines by only 3.4%in Chinamainland,much less than the reduction of 24.1%in the lockdown *** the basis of quantitative analysis,we find the rebound of NO_(2)TVCD is mainly caused by the rapid recovery of economy especially in the fourth quarter,when contribution of industry and power plant on NO_(2)TVCD continues to *** revenge bounce of NO_(2)indicates the emission reduction of NOx in lockdown period is basically offset by the recovery of economy,revealing the fact that China’s economic development and NOx emissions are still not *** efforts are still required to stimulate low-pollution development.

关键词： COVID-19 Tropospheric NO2 TROPOMI Economy recovery environment sustainability

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Sludge-based biochar adsorbent:pore tuning mechanisms,challenges,and role in carbon sequestration

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Biochar 2023年第1期5卷 1419-1441页

作者： Md Manik Mian Wenya Ao Shubo Deng State Key Joint Laboratory of Environment Simulation and Pollution Control(SKLESPC) Beijing Key Laboratory for Emerging Organic Contaminants ControlSchool of EnvironmentTsinghua UniversityBeijing 100084China

Sludge biochar,a carbonized product of raw sludge,contains porous architectures that can act as epicenters for adsorbing external molecules through physical or chemical *** biochar also immobilizes innate micropollutants,which is advantageous over conventional sludge disposal *** date,numerous strategies have been discovered to improve sludge biochar morphology,but the influential factors,pore tuning mechanisms,and process feasibility remain *** knowledge gap limits our ability to design a robust sludge-based ***,we present state-of-the-art sludge biochar synthesis methods with insight into structural and chemical transformation *** and novel concepts for improving sludge biochar porous architecture are *** the first time,sludge biochar properties,adsorption performances,and techno-economic perspectives were compared with commercial activated carbon(AC)to reveal the precise challenges in sludge biochar *** importantly,sludge biochar role in carbon sequestration is detailed to demonstrate the environmental significance of this ***,the review concludes with an overview of prospects and an outlook for developing sludge biochar-based research.

关键词： Sludge-based adsorbent Micropores Feasible methods Challenges Carbon sequestration

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A systematic review of the inequality of health burdens related to climate change

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Frontiers of environmental Science & Engineering 2024年第5期18卷 137-153页

作者： Xinke Song Shihui Zhang Hai Huang Qun Ding Fang Guo Yaxin Zhang Jin Li Mingyu Li Wenjia Cai Can Wang State Key Joint Laboratory of Environment Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing100084China Department of Earth System Science Tsinghua UniversityBeijing100084China

Climate change significantly impacts human health,exacerbating existing health inequalities and creating new *** study addresses the lack of systematic review in this area by analyzing 2440 publications,focusing on four key terms:health,disparities,environmental factors,and climate *** inclusion criteria limited the selection to English-language,peer-reviewed articles related to climate health hazards,ensuring the relevance and rigor of the synthesized *** process synthesized 65 relevant *** investigation revealed that recent research,predominantly from developed countries,has broadened its scope beyond temperature-related impacts to encompass diverse climate hazards,including droughts,extreme weather,floods,mental health issues,and the intersecting effects of Coronavirus Disease *** has highlighted exposure as the most studied element in the causal chain of climate change-related health inequalities,followed by adaptive capability and inherent *** most significant vulnerabilities were observed among populations with low socioeconomic status,ethnic minorities,and *** study further reveals research biases and methodological limitations,such as the paucity of attention to underdeveloped regions,a narrow focus on non-temperature-related hazards,challenges in attributing climate change effects,and a deficit of large-scale empirical *** findings call for more innovative research approaches and a holistic integration of physical,socio-political,and economic dimensions to enrich climate-health discourse and inform equitable policy-making.

关键词： Climate change Health impact Human well-being Inequality Vulnerability

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Risk assessment and management of radionuclide leakage in nuclear power plants

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National Science Open 2025年第1期4卷 75-100页

作者： Boyang Huang Yuxin Liu Xiaoyan Sun Lei Huang Shipeng Dong Liang Mao State Key Laboratory of Pollution Control and Resource Reuse School of the EnvironmentChemistry and Biomedicine Innovation CenterNanjing UniversityNanjing 210023China Nanjing Qixia District Hospital Nanjing 210023China

Nuclear power plants are designed with stringent safety measures to prevent accidents and radioactive ***,major accidents like the Three Mile Island(1979),Chornobyl(1986),and Fukushima Daiichi(2011)have sig-nificantly impacted human health,the environment,and public perception of nuclear *** during normal operation,nuclear power plants release effluents that can have some impact on the *** effluents are carefully monitored and regulated to minimize their environmental *** releases have potential long-term consequences for human health and the *** mitigate the risks of accidents and the environmental impact of normal operation,continued focus on nuclear safety,rigorous regulatory oversight,and improved emergency response measures are *** behavior and impact of radionuclides in the environment,models and methods for simulating the transport and deposition of radio-nuclides in the atmosphere and ocean,toxicokinetic and toxicodynamic studies to predict the potential impacts of radionuclide releases and support risk management decisions,and environmental monitoring and control technology of nuclides,et al are *** article aims to provide an overview of the importance of environmental toxicology in radioactive risk as-sessment and management,discuss the unique challenges associated with monitoring and remediating radioactive releases,and suggest future research directions.

关键词： radionuclide leakage nuclear power plants risk assessment environmental toxicology remediation methods

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Destructing surfactant network in nanoemulsions by positively charged magnetic nanorods to enhance oil-water separation

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Journal of environmental Sciences 2022年第8期34卷 112-121页

作者： Yongjiao Xiong Xiangfeng Huang Lexue Li Wanqi Liu Jialu Zhang Mengfan He Jia Liu Lijun Lu Kaiming Peng College of Environmental Science and Engineering State Key Laboratory of Pollution Control and Resource ReuseMinistry of Education Key Laboratory of Yangtze River Water EnvironmentTongji UniversityShanghai 200092China

The separation of ultrafine oil droplets from wasted nanoemulsions stabilized with high concentration of surfactants is precondition for oil reuse and the safe discharge of ***, the double barriers of the interfacial film and network structures formed by surfactants in nanoemulsions significantly impede the oil-water separation. To destroy these surfactant protective layers, we proposed a newly-developed polyethyleneimine micelle template approach to achieve simultaneous surface charge manipulation and morphology transformation of magnetic nanospheres to magnetic nanorods. The results revealed that positively charged magnetic nanospheres exhibited limited separation performance of nanoemulsions, with a maximum chemical oxygen demand(COD) removal of 50%, whereas magnetic nanorods achieved more than 95% COD removal in less than 30 s. The magnetic nanorods were also applicable to wasted nanoemulsions from different sources and exhibited excellent resistance to wide pH changes. Owing to their unique one-dimensional structure, the interfacial dispersion of magnetic nanorods was significantly promoted, leading to the efficient capture of surfactants and widespread destruction of both the interfacial film and network structure, which facilitated droplet merging into the oil phase. The easy-toprepare and easy-to-tune strategy in this study paves a feasible avenue to simultaneously tailor surface charge and morphology of magnetic nanoparticles, and reveals the huge potential of morphology manipulation for producing high-performance nanomaterials to be applied in complex interfacial interaction process. We believe that the newly-developed magnetic-nanorods significantly contribute to hazardous oily waste remediation and advances technology evolution toward problematic oil-pollution control.

关键词： Nanoemulsions Surface charge Magnetic nanorods Surfactant Interfacial film Oil-water separation

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