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Screening of indicator pharmaceuticals and personal care products in landfill leachates: a case study in Shanghai, China

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Frontiers of Environmental Science & Engineering 2023年第9期17卷 245-256页

作者： Xiping Kan Xia Yu Wentao Zhao Shuguang Lyu Shuying Sun Gang Yu Qian Sui State Environmental Protection Key Laboratory of Environmental Risk Assessment and Control on Chemical Process School of Resources and Environmental EngineeringEast China University of Science and TechnologyShanghai 200237China State Key Laboratory of Pollution Control and Resource Reuse College of Environmental Science and EngineeringTongji UniversityShanghai 200092China Advanced Interdisciplinary Institute of Environment and Ecology Beijing Normal University at ZhuhaiZhuhai 519087China Shanghai Institute of Pollution Control and Ecological Security Shanghai 200092China

Identifying potential sources of pharmaceuticals and personal care products(PPCPs)in the environment is critical for the effective control of PPCP *** leachate is an important source of PPCPs in water;however,it has barely been involved in source apportionment due to the lack of indicator-PPCPs(i-PPCPs)in landfill *** study provides the first systematic framework for identifying i-PPCPs for landfill leachates based on the wide-scope target monitoring of *** number of target PPCPs increased from<20 in previous studies to 68 in the present ***-nine PPCPs were detected,with median concentrations in leachate samples ranging from below the method quantification limit(MQL)to 41μg/L,and 19 of them were rarely reported previously.A total of 29 target compounds were determined to be PPCPs of high concern by principal component analysis according to multiple criteria,including occurrence,exposure potential,and ecological *** with source-specificity and representativeness analysis,erythromycin,gemfibrozil,and albendazole showed a significant difference in their occurrence in leachate compared to other potential sources(untreated and treated municipal wastewater and livestock wastewater)and correlated with total PPCP concentrations;these were recommended as i-PPCPs for *** screening procedure can be used to develop a sophisticated source apportionment method to identify sources of PPCPs from adjacent landfills.

关键词： Landfill leachates PPCPs Indicator Screening criteria Source-specificity

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Cobalt single-atom catalyst tailored ceramic membrane for selective removal of emerging organic contaminants

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Environmental Science and Ecotechnology 2024年第5期21卷 219-229页

作者： Jiaxuan Yang Jing Zhao Hesong Wang Yatao Liu Junwen Ding Tianyi Wang Jinlong Wang Han Zhang Langming Bai Heng Liang State Key Laboratory of Urban Water Resource and Environment School of EnvironmentHarbin Institute of TechnologyHarbin150090PR China Beijing Key Laboratory for Source Control Technology of Water Pollution College of Environmental Science and EngineeringBeijing Forestry UniversityBeijing100083PR China

Water reuse is an effective way to solve the issues of current wastewater increments and water resource ***,a promising method for water reuse,has the characteristics of low energy consumption,easy operation,and high adaptability to coupling with other water treatment ***,emerging organic contaminants(EOCs)in municipal wastewater cannot be effectively intercepted by ultrafiltration,which poses significant challenges to the effluent quality and sustainability of ultrafiltration ***,we develop a cobalt single-atom catalyst-tailored ceramic membrane(Co1-NCNT-CM)in conjunction with an activated peroxymonosulfate(PMS)system,achieving excellent EOCs degradation and anti-fouling *** interfacial reaction mechanism effectively mitigates membrane fouling through a repulsive interaction with natural organic *** generation of singlet oxygen at the Co-N3-C active sites through a catalytic pathway(PMS/PMS*/OH*/O*/OO*/1 O_(2))exhibits selective oxidation of phenols and sulfonamides,achieving>90%removal *** findings elucidate a multi-layered functional architecture within the Co1-NCNT-CM/PMS system,responsible for its superior performance in organic decontamination and membrane maintenance during secondary effluent *** highlights the power of integrating Co1-NCNT-CM/PMS systems in advanced wastewater treatment frameworks,specifically for targeted EOCs removal,heralding a new direction for sustainable water management.

关键词： Single-atom catalytic ceramic membrane Peroxymonosulfate activation Selective oxidation Interfacial response Multi-layer functional zones

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Rapid reduction of air pollution and short-term exposure risks in China

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Journal of Environmental Sciences 2025年第3期149卷 126-138页

作者： Hao Fan Chuanfeng Zhao Yikun Yang Xingchuan Yang State Key Joint Laboratory of Environmental Simulation and Pollution Control School of EnvironmentBeijing Normal UniversityBeijing 100875China Laboratory for Climate and Ocean-Atmospheric Studies Department of Atmospheric and Oceanic SciencesSchool of PhysicsPeking UniversityBeijing 100871China College of Resource Environment and Tourism Capital Normal UniversityBeijing 100048China

With the continuous control of anthropogenic emissions,China’s air quality has improved significantly in recent *** this background,research on how the short-term exposure risks caused by air pollution in China have changed is *** study utilized hourly concentration data from ground observation stations and the official air quality guidelines of the Ministry of Ecology and Environment of China and the World Health Organization as standards to systematically investigate the spatiotemporal characteristics and short-term exposure risks of air pollution in China from 2015 to *** results indicate that various atmospheric pollutants except for ozone showed a decreasing trend ***,both single pollutant air pollution days(SAPDs)and multiple pollutant air pollution days(MAPDs)showed varying degrees of reduction within 15 and 25 days,*** was dominated mainly by excessive PM_(2.5)and PM_(10)pollutants,while MAPD was dominated mainly by excessive pollutant combinations,including PM_(2.5)+PM_(10),CO+PM_(2.5)+PM_(10),and SO_(2)+PM_(2.5)+PM_(10).As the concentration of atmospheric pollutants decreased,the total excess risk(ER)decreased yearly from 2015 to 2022,but there were significant regional ***,the ER is less than 0.25%in southern China,in the range of 0.25%-0.5%in the North China Plain and some cities in the northeast,and higher than 1%in the *** matter is currently the primary pollutant posing short-term exposure risk in China,especially due to the impact of sandstorm *** study indicates that China’s atmospheric cleaning action is significantly beneficial for reducing health risks.

关键词： Air pollution Emission-reduction Total excess risk Particulate matter China

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Getting insights into gas-phase sulfation effect on catalytic performance of praseodymium oxides in NH_(3)-SCR of NO

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Journal of Rare Earths 2023年第6期41卷 952-958,I0005页

作者： Yandi Cai Peng Yang Qinglong Liu Kaili Ma Wenxin Ma Wang Song Qiuhui Qian Fei Gao Wei Tan Lin Dong State Key Laboratory of Pollution Control and Resource Reuse School of EnvironmentJiangsu Key Laboratory of Vehicle Emissions ControlCenter of Modern AnalysisKey Laboratory of Mesoscopic Chemistry of MOESchool of Chemistry and Chemical EngineeringNanjing UniversityNanjing 210023China Analysis and Testing Center Southeast UniversityNanjing 211189China National and Local Joint Engineering Laboratory of Municipal Sewage Resource Utilization Technology School of Environmental Science and EngineeringSuzhou University of Science and TechnologySuzhou 215009China

Sulfation treatment has been widely used to promote the catalytic performance of ceria(CeO_(2))based catalysts for the selective catalytic reduction of NO by NH_(3)(NH_(3)-SCR of NO).Praseodymium oxide(PrO_(x)),another commonly used rare earth material with similar structural properties as CeO_(2),also shows satistactory redox properties due to the facile redox cycle of Pr^(3+)■Pr^(4+).In this work,gas phase sulfation treatment with varied duration was performed on PrO_(x) at 200℃,and the NH_(3)-SCR activity of sulfated PrO_(x) was *** on the results of systematic characterizations(e.g.,N_(2)-physisorption,NH_(3) oxidation,NO oxidation,in situ diffuse Fourier transform infrared spectroscopy),it is revealed that the catalytic performance of sulfated PrO_(x)is highly dependent on the sulfation time(or the amount of sulfate species deposited on PrO_(x)),which has a significant impact on the competitive reaction between NH_(3) oxidation and NH_(3)-SCR of NO,thus determining the NH_(3)-SCR activity of PrO_(x).This work provides new insight into tuning the interaction between PrO_(x) surface and reactants(NO,NH_(3))via sulfation treatment,which cam guide the design and application of PrO_(x)based catalysts for NH_(3)-SCR of NO in the future.

关键词： NH_(3)-SCR Praseodymium oxides Sulfation treatment Surface acidity NH_(3)oxidation Rare earths

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Synergistic enhancement of pollutant removal from high-salt wastewater using coagulation-flotation combined process

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Green Chemical Engineering 2025年第3期6卷 410-419页

作者： Enze Li Jing Dong Yongsheng Jia Zihe Pan Hongzhou Lv Zhiping Du Guandao Gao Fangqin Cheng Institute of Resources and Environmental Engineering State Environmental Protection Key Laboratory of Efficient Utilization Technology of Coal Waste ResourcesShanxi Laboratory of Yellow RiverShanxi UniversityTaiyuan030006China School of Environmental Science&Engineering Huazhong University of Science and TechnologyWuhan430074China State Key Laboratory of Pollution Control and Resource Reuse School of EnvironmentNanjing UniversityNanjing210023China

Sufficient treatment of industrial organic wastewater with high salt and large amounts of suspended particulate matter remains a challenge *** this work,a novel coagulation-flotation combined process was developed to treat the suspended particles as well as significantly reduce organic pollutants content in the actual high-salt organic *** typical inorganic and organic flocculants(poly aluminum chloride(PAC),poly ferric sulfate(PFS),polyacrylamide(PAM),and modified cationic starch(CS))were selected for compounding to obtain an optimized flocculation system for high-salt *** results showed that the PAC-PAM with a 10:1 ratio in mass exhibited the best coagulation behaviors with the removal efficiency of turbidity and chemical oxygen demand(COD)being 95.33%and 9.21%,respectively,under the optimal operation conditions,and the sedimentation process of coagulant conformed to the quasi-second-order *** PAC-PAM flocs exhibited stronger netting,sweeping,and adsorption bridging capabilities,which were conducive to removing suspended *** the flotation was conducted after coagulation,the COD decreased significantly by 20.82%.In addition,this combined process could reduce the treatment time by 50%compared to the process with only coagulation *** the flotation process,floc particles companies with hydrophobic polycyclic aromatic hydrocarbons could collide and adhere to microbubbles and be floated to the surface,resulting in an effective reduction of *** work could provide a novel strategy and step forward to design and optimize the pretreatment process engineering for organic high-salt wastewater.

关键词： High-salt organic wastewater Coagulation-flotation combined process Sedimentation kinetics Bubble-floc aggregate

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MSWNet:A visual deep machine learning method adopting transfer learning based upon ResNet 50 for municipal solid waste sorting

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Frontiers of Environmental Science & Engineering 2023年第6期17卷 165-176页

作者： Kunsen Lin Youcai Zhao Lina Wang Wenjie Shi Feifei Cui Tao Zhou The State Key Laboratory of Pollution Control and Resource Reuse College of Environmental Science and EngineeringTongji UniversityShanghai 200092China Shanghai Institute of Pollution Control and Ecological Security Shanghai 200092China Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention(LAP3) Department of Environmental Science and EngineeringFudan UniversityShanghai 200433China Institute of Eco-Chongming(IEC) Shanghai 202150China Institute of Fundamental and Frontier Sciences University of Electronic Science and Technology of ChinaChengdu 610054China

An intelligent and efficient methodology is needed owning to the continuous increase of global municipal solid waste(MSW).This is because the common methods of manual and semi-mechanical screenings not only consume large amount of manpower and material resources but also accelerate virus community *** the categories of MSW are diverse considering their compositions,chemical reactions,and processing procedures,etc.,resulting in low efficiencies in MSW sorting using the traditional *** machine learning can help MSW sorting becoming into a smarter and more efficient *** study for the first time applied MSWNet in MSW sorting,a ResNet-50 with transfer *** method of cyclical learning rate was taken to avoid blind finding,and tests were repeated until accidentally encountering a good *** of visualization were also considered to make the MSWNet model more transparent and *** showed transfer learning enhanced the efficiency of training time(from 741 s to 598.5 s),and improved the accuracy of recognition performance(from 88.50%to 93.50%);MSWNet showed a better performance in MSW classsification in terms of sensitivity(93.50%),precision(93.40%),F1-score(93.40%),accuracy(93.50%)and AUC(92.00%).The findings of this study can be taken as a reference for building the model MSW classification by deep learning,quantifying a suitable learning rate,and changing the data from high dimensions to two dimensions.

关键词： Municipal solid waste sorting Deep residual network Transfer learning Cyclic learning rate Visualization

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Sulfur-driven methylmercury production in paddies continues following soil oxidation

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Journal of Environmental Sciences 2022年第9期34卷 166-174页

作者： Wenli Tang Chao Tang Pei Lei School of the Environment State Key Laboratory of Pollution Control and Resource ReuseNanjing UniversityNanjing 210023China School of Environment Nanjing Normal UniversityNanjing 210023China

Methylmercury(MeHg) production in paddy soils and its accumulation in rice raise global concerns since rice consumption has been identified as an important pathway of human exposure to MeHg. Sulfur(S) amendment via fertilization has been reported to facilitate Hg methylation in paddy soils under anaerobic conditions, while the dynamic of S-amendment induced MeHg production in soils with increasing redox potential remains unclear. This critical gap hinders a comprehensive understanding of Hg biogeochemistry in rice paddy system which is characterized by the fluctuation of redox potential. Here, we conducted soil incubation experiments to explore MeHg production in slow-oxidizing paddy soils amended with different species of S and doses of sulfate. Results show that the elevated redox potential(1) increased MeHg concentrations by 10.9%-35.2%, which were mainly attributed to the re-oxidation of other S species to sulfate and thus the elevated abundance of sulfatereducing bacteria, and(2) increased MeHg phytoavailability by up to 75% due to the reductions in acid volatile sulfide(AVS) that strongly binds MeHg in soils. Results obtained from this study call for attention to the increased MeHg production and phytoavailability in paddy soils under elevated redox potentials due to water management, which might aggravate the MeHg production induced by S fertilization and thus enhance MeHg accumulation in rice.

关键词： Mercury Sulfur Availability Mercury methylation Rice

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Biochar nanoparticles-mediated transport of organic contaminants in porous media: dependency on contaminant properties and effects of biochar aging

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Carbon Research 2023年第1期2卷 1-15页

作者： Ma, Pengkun Qi, Zhichong Wu, Xuan Ji, Rong Chen, Wei College of Environmental Science and Engineering Ministry of Education Key Laboratory of Pollution Processes and Environmental Criteria Tianjin Key Laboratory of Environmental Remediation and Pollution Control Nankai University Tianjin300350 China China Water Resources Beifang Investigation Design and Research Co. Ltd. Tianjin300222 China College of Chemistry and Chemical Engineering Henan Joint International Research Laboratory of Environmental Pollution Control Materials Henan University Kaifeng475004 China State Key Laboratory of Pollution Control and Resource Reuse School of the Environment Nanjing University Nanjing210023 China

Land application of biochar has been recommended as an effective soil amendment measure. Nonetheless, the applied biochar can accumulate co-existing contaminants. Meanwhile, nanoparticles formed due to biochar disintegration may facilitate contaminant transport in vadose zone and groundwater, posing a potential risk to the subsurface environment. Here, we show that the presence of pinewood- and rice straw-derived biochar nanoparticles (BCNPs) at parts per million level (~ 20 mg/L) can result in significant mobilization of hydrophobic, nonpolar contaminants (naphthalene and pyrene) and positively charged polar contaminants (trimethoprim and ciprofloxacin) in saturated sandy soil, but slightly inhibits the transport of negatively charged or neutral hydrophilic compounds (sulfamethoxazole and bisphenol A). With supplemental adsorption and desorption experiments we show that the ability of BCNPs in mediating contaminant transport (either enhancing or inhibiting) relies primarily on the extent of irreversible binding of a contaminant to the BCNPs. Sulfide reduction and leaching of organic carbon, two relatively mild (in terms of modification of physicochemical properties, e.g., surface O/C ratio) but widely occurring aging processes, facilitate co-transport of pyrene and bisphenol A with the BCNPs. However, this is mainly the result of increased mobility of the BCNPs (i.e., the carrier), rather than enhanced interactions between the BCNPs and the contaminants being carried. The findings underline the significant effects of BCNPs on the fate and transport of environmental contaminants, and further highlight the important role of aging in affecting environmental behaviors and effects of biochar materials. Graphical Abstract: [Figure not available: see fulltext.] © 2023, The Author(s).

关键词： Naphthalene

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Trifunctional Cu-Mesh/Cu_(2)O@FeO Nanoarrays for Highly Efficient Degradation of Antibiotic, Inactivation of Antibiotic-Resistant Bacteria, and Damage of Antibiotics Resistance Genes

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Energy & Environmental Materials 2023年第1期6卷 349-359页

作者： Long Zhao Wei Zhou Ming Wen Qingsheng Wu Weiying Li Yongqing Fu Quanjing Zhu Sheng Chen and Jiaqi Ran Shanghai Key Laboratory of Chemical Assessment and Sustainability State Key Laboratory of Pollution Control and Resource ReuseSchool of Chemical Science and EngineeringCollege of Environmental Science and EngineeringTongji UniversityShanghai 200092China Faculty of Engineering and Environment Northumbria UniversityNewcastle upon Tyne NE99UK

Trifunctional Cu-mesh/Cu_(2)O@FeO nanoarrays heterostructure is designed and fabricated by integrating CuCu_(2)O@FeO nanoarrays onto Cu-mesh(CM)via an in situ growth and phase transformation *** is successfully applied to efficiently mitigate the antibiotic pollution,including degradation of antibiotics,inactivation of antibiotic-resistant bacteria(ARB),and damage of antibiotics resistance genes(ARGs).Under visible-light irradiation,CM/CuCu_(2)O@FeO nanoarrays exhibit a superior degradation efficiency on antibiotics(e.g.,up to 99%in 25 min for tetracycline hydrochloride,TC),due to the generated reactive oxygen species(ROS),especially the dominant·O^(2−).It can fully inactivate ***(HB101)with initial number of~108 CFU mL^(−1) in 10 min,which is mainly attributed to the synergistic effects of 1D nanostructure,dissolved metal ions,and generated ***,it is able to damage ARGs after 180 min of photodegradation,including tetA(vs TC)of 3.3 log 10,aphA(vs kanamycin sulfate,KAN)of 3.4 log 10,and tnpA(vs ampicillin,AMP)of 4.4 log 10,*** work explores a green way for treating antibiotic pollution under visible light.

关键词： antibiotic antibiotic resistance genes antibiotic-resistant bacteria Cu-Mesh/Cu_(2)O@FeO nanoarrays photocatalytic degradation

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Steam disinfection enhances bioaccessibility of metallic nanoparticles in nano-enabled silicone-rubber baby bottle teats,pacifiers,and teethers

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Journal of Environmental Sciences 2024年第2期136卷 161-171页

作者： Yu Su BinWang Xin Tong Shuchuan Peng Sijin Liu Baoshan Xing Rong Ji State Key Laboratory of Pollution Control and Resource Reuse School of the EnvironmentNanjing UniversityNanjing 210023China School of Resources and Environmental Engineering Hefei University of TechnologyHefei 230009China State Key Laboratory of Environmental Chemistry and Ecotoxicology Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China Stockbridge School of Agriculture University of MassachusettsAmherstMA 01003USA

Nano-enabled silicone-rubber articles for feeding or chewing could be a source of metallic nanoparticles(NPs)directly exposed to infants and young ***,the impact of steam disinfection on release of NPs and the related potential risks to children's health are ***,we investigated contents and form of Ag and Zn in 57 nano-enabled silicone-rubber baby bottle teats,pacifiers,and teethers of seven countries and examined the impacts of steam disinfection on in vitro bioaccessibility(IVBA)of Ag and Zn in the *** 89%articles had a mixture of Ag-and Zn-containing NPs and the teethers had relatively high Ag and Zn contents(up to 501 and 254μg/g,respectively).Steam disinfection caused rubber decomposition into micro(nano)plastics(0.54-15.7μm)and NP release from the interior of bulk rubber and micro-sized plastics,thus enhancing the IVBA of Ag and Zn by up to 5.5 *** findings provide insights into mechanisms for NP release by steam *** oral exposure risk assessment suggested low health concerns on individual metal release,our study points out the need to assess the potential health risks of child co-exposure to metallic NPs and micro(nano)plastics.

关键词： Silicone rubber Metallic nanoparticles Micro(nano)plastics Bioaccessibility Children's health

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