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第十四届持久性有机污染物论坛暨化学品环境安全大会

作者： Chenguang Li Jiaoqin Liu Nannan Wu Ruijuan Qu Xiaoxue Pan Jianfang Feng Zunyao Wang State Key Laboratory of Pollution Control and Resources Reuse School of the EnvironmentNanjingUniversityJiangsu Nanjing 210023P.R.China

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Corrigendum to “Dynamic scouring of multifunctional granular material enhances filtration performance in membrane bioreactor: Mechanism and modeling” [J. Membr. Sci. 663 (2022) 120979]

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Journal of Membrane Science 2024年 698卷

作者： Wenxiang Zhang Wenzhong Liang Zhien Zhang Biological and Environmental Science and Engineering Division Water Desalination and Reuse Research Center King Abdullah University of Science and Technology Thuwal Saudi Arabia State Environmental Protection Key Laboratory of Water Environmental Simulation and Pollution Control South China Institute of Environmental Sciences Ministry of Ecology and Environment of the People's Republic of China Guangzhou 510530 PR China Department of Chemical and Biomedical Engineering West Virginia University 40110 Evansdale Drive Morgantown WV 26506 USA

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Insights into the Occurrence, Elimination Efficiency and Ecological Risk of Antibiotics in Rural Domestic Wastewater Treatment Facilities Along the Yangtze River, China

SSRN

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SSRN 2022年

作者： Xing, Liqun Sun, Jie Kong, Fanjie Kong, Ming Li, Jun Zhang, Rui Li, Aimin State Key Laboratory of Pollution Control and Resource Reuse School of the Environment Nanjing University Nanjing210023 China School of Chemistry and Chemical Engineering Southeast University Nanjing210096 China Nanjing University Yancheng Academy of Environmental Protection Technology and Engineering Yancheng224000 China Suzhou Capital Greinworth Environmental Protection Technology Co. Ltd Suzhou215216 China Beijing Capital Eco-Environment Protection Group Co. Ltd Beijing100044 China Nanjing Institute of Environmental Sciences Ministry of Ecology and Environment No.8 Jiangwangmiao Street Nanjing210042 China School of Water Conservancy and Environment University of Jinan Jinan250022 China

China is embarking on the treatment of rural domestic wastewater, but little information on the characteristics of antibiotics in the rural domestic wastewater is available. Thus, the occurrence, elimination efficiency and ecological risk of antibiotics, as well as conventional wastewater quality parameters were investigated in influents and effluents from rural domestic wastewater treatment facilities (RD-WWTFs) along the Yangtze River. Elimination efficiencies of 33 out of investigated 41 RD-WWTFs (accounting for 80.5%) were effective. Higher values of conventional wastewater quality parameters in influents were found, however, more effective removal of them in the lower reaches. Of 39 target antibiotics selected, 26 ones were detected in the influents and effluents with a detection frequency (DF) between 2.4% and 100%. No significant decrease of antibiotics was observed in the effluents compared with that in the influents except chlortetracyclin (CTE) and tetracycline (TCs). The composition characteristics of antibiotics showed regional differences, but were similar between the effluents and influents. Among these antibiotics, ofloxacin (OFX), doxycycline (DOX), roxithromycin (ROX) and lincomycin (LIN) were the predominant ones with the highest DFs, totally accounted for a median percentage of more than 60% of ΣAB concentrations in both influents and effluents. The calculated ecological risk values of ΣABs showed that 11 effluents presented high risks (26.8%), 18 ones had moderate risks (43.9%), and the rest 12 ones showed low risks (29.3%). For a single antibiotic, oxytetracycline (OXY), norfloxacin (NOR), LIN and ROX contributed the most to the ecological risk values. These results indicated that the overall elimination effect of antibiotics in rural domestic wastewater was very limited, which was likely to have potential adverse impacts on aquatic ecosystems along the Yangtze River. © 2022, The Authors. All rights reserved.

关键词： Effluents

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Electronic-property dependent interactions between tetracycline and graphene nanomaterials in aqueous solution

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Journal of Environmental Sciences 2018年第4期30卷 286-294页

作者： Lin He Fei-fei Liu Mengyao Zhao Zhen Qi Xuefei Sun Muhammad Zaheer Afzal Xiaomin Sun Yanhui Li Jingcheng Hao Shuguang Wang Shandong Key Laboratory of Water Pollution Control and Resource Reuse School of Environmental Science and EngineeringShandong University Insistute of Marine Science and Technology Shandong University Environment Research Institute Shandong University Laboratory of Fiber Materials and Modern Textile The Growing Base for State Key Laboratory Qingdao University Key Laboratory of Colloid and Interface Chemistry Ministry of Education Shandong University

Understanding the interactions between graphene nanomaterials（GNMs） and antibiotics in aqueous solution is critical to both the engineering applications of GNMs and the assessment of their potential impact on the fate and transport of antibiotics in the aquatic environment. In this study, adsorption of one common antibiotic, tetracycline, by graphene oxide（GO） and reduced graphene oxide（RGO） was examined with multi-walled carbon nanotubes（MWCNTs） and graphite as comparison. The results showed that the tetracycline adsorption capacity by the four selected carbonaceous materials on the unit mass basis followed an order of GO ＆gt; RGO ＆gt; MWCNTs ＆gt; graphite. Upon normalization by surface area,graphite, RGO and MWCNTs had almost the same high tetracycline adsorption affinity while GO exhibited the lowest. We proposed π-electron-property dependent interaction mechanisms to explain the observed different adsorption behaviors. Density functional theory（DFT） calculations suggested that the oxygen-containing functional groups on GO surface reduced its π-electron-donating ability, and thus decreased the π-based interactions between tetracycline and GO surface. Comparison of adsorption efficiency at different p H indicated that electrostatic interaction also played an important role in tetracycline-GO interactions. Site energy analysis confirmed a highly heterogeneous distribution of the binding sites and strong tetracycline binding affinity of GO surface.

关键词： Graphene oxide Reduced graphene oxide Tetracycline Adsorption DFT calculation π-Based interaction

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Overturned Loading of Inert CeO2to Active Co3O4for Unusually Improved Catalytic Activity in Fenton-Like Reactions

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Angewandte Chemie 2022年第16期134卷

作者： Chunli Song Qing Zhan Dr. Fei Liu Chuan Wang Dr. Hongchao Li Xuan Wang Prof. Xuefeng Guo Prof. Yingchun Cheng Wei Sun Prof. Li Wang Prof. Jieshu Qian Prof. Bingcai Pan Jiangsu Key Laboratory of Chemical Pollution Control and Resources Reuse School of Environmental and Biological Engineering Nanjing University of Science and Technology 200 Xiao Ling Wei Nanjing 210094 China Key Laboratory of Flexible Electronics & Institute of Advanced Materials Jiangsu National Synergetic Innovation Center for Advanced Materials Nanjing Tech University Nanjing 211816 China Key Lab of Mesoscopic Chemistry MOE School of Chemistry & Chemical Engineering Nanjing University Nanjing 210023 China Key Laboratory of Catalysis and Energy Materials Chemistry of Ministry of Education South-Central University for Nationalities Wuhan 430074 China Research Center for Environmental Nanotechnology (ReCENT) School of Environment State Key Laboratory of Environmental Pollution and Resources Reuse Nanjing University Nanjing 210023 China

In the past decades, numerous efforts have been devoted to improving the catalytic activity of nanocomposites by either exposing more active sites or regulating the interaction between the support and nanoparticles while keeping the structure of the active sites unchanged. Here, we report the fabrication of a Co 3 O 4 −CeO 2 nanocomposite via overturning the loading direction, i.e., loading an inert CeO 2 support onto active Co 3 O 4 nanoparticles. The resultant catalyst exhibits unexpectedly higher activity and stability in peroxymonosulfate-based Fenton-like reactions than its analog prepared by the traditional impregnation method. Abundant oxygen vacancies (O v with a Co⋅⋅⋅O v ⋅⋅⋅Ce structure instead of Co⋅⋅⋅O v ) are generated as new active sites to facilitate the cleavage of the peroxide bond to produce SO 4 .− and accelerate the rate-limiting step, i.e., the desorption of SO 4 .− , affording improved activity. This strategy is a new direction for boosting the catalytic activity of nanocomposite catalysts in various scenarios, including environmental remediation and energy applications.

关键词： CO Oxidation Fenton-Like Reaction Nanocomposite Catalyst Overturned Loading Oxygen Vacancy

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Ketyl Radical Anion Mediated Radical Polymerization and Anionic Ring-Opening Polymerization to Give Polymers with Low Molecular Weight Distribution

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Angewandte Chemie 2023年第31期135卷

作者： Yu-Jiao Chen Liang-Tao Wu Tai-An Li Meng-Qin Pu Prof. Xiao-Li Sun Prof. Hongli Bao Prof. Wen-Ming Wan College of Environment and Resources Engineering Research Center of Polymer Green Recycling of Ministry of Education Fujian Key Laboratory of Pollution Control & Resource Reuse Fujian Normal University Fuzhou 350007 P. R. China Key Laboratory of Coal to Ethylene Glycol and Its Related Technology State Key Laboratory of Structural Chemistry Center for Excellence in Molecular Synthesis Fujian Institute of Research on the Structure of Matter Chinese Academy of Sciences Fuzhou 350002 P. R. China College of Chemistry and Materials Science Fujian Normal University Fuzhou 350007 P. R. China

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Frontispiece: A Showcase of Green Chemistry: Sustainable Synthetic Approach of Zirconium-Based MOF Materials

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Chemistry – A European Journal 2021年第39期27卷

作者： Jiarui Fu Dr. Yi-nan Wu College of Environmental Science and Engineering State Key Laboratory of Pollution Control and Resource Reuse Tongji University Siping Rd 1239 200092 Shanghai P.R. China Shanghai Institute of Pollution Control and Ecological Security Siping Rd 1239 200092 Shanghai P.R. China

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Improving The Biodegradability of Rice Straw by Electrochemical Pretreatment

SSRN

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SSRN 2022年

作者： Sun, Shaohua Zhang, Yuanyuan Yang, Zhaoyang Liu, Chunmei Zuo, Xiaoyu Tang, Yang Wan, Pingyu Liu, Yanping Li, Xiujin Coulon, Frederic Hu, Qing Yang, Xiao Jin State Key Laboratory of Chemical Resource Engineering Beijing University of Chemical Technology 15 Beisanhuan East Road Chaoyang District Beijing100029 China Beijing City Environmental Pollution Control and Resource Reuse Engineering Center Beijing University of Chemical Technology 15 Beisanhuan East Road Chaoyang District Beijing100029 China National Fundamental Research Laboratory of New Hazardous Chemicals Assessment and Accident Analysis Beijing University of Chemical Technology Beijing100029 China School of Water Energy and Environment Cranfield University Cranfield MK43 0AL United Kingdom School of Environmental Science and Engineering South University of Science and Technology Guangdong Shenzhen518055 China Beijing Huanding Environmental Big Data Institute No. 1 Wangzhuang Road Beijing100083 China

In this study, the efficacy of three different pretreatments of rice straw including alkaline hydrogen peroxide (NaOH-H2O2), electrochemically produced NaOH-H2O2 (eNaOH-H2O2) and electrohydrolysis (EH) was investigated. All three pretreatments allowed to reach 80% of total biogas production within 23 and 25 days which was 3 to 5 days faster compared to conventional NaOH pretreatment. The cumulative biogas production was enhanced by 8%, 22% and 14% for NaOH-H2O2, eNaOH-H2O2 and EH, respectively compared to traditional treatment. The eNaOH-H2O2 pretreatment decreased the crystallinity of cellulose and created a porous surface vein, thus promoting microbial degradation of lignocellulose. The findings of this study demonstrate that electrochemical pretreatment provides a promising approach for efficiently utilizing rice straw biomass to produce renewable electricity. © 2022, The Authors. All rights reserved.

关键词： Oxidation

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Enhanced debromination of 4-bromophenol by the UV/sulfite process：Efficiency and mechanism

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Journal of Environmental Sciences 2017年第4期29卷 231-238页

作者： Bihuang Xie Xuchun Li Xianfeng Huang Zhe Xu Weiming Zhang Bingcai Pan State Key Laboratory of Pollution Control and Resource Reuse School of the EnvironmentNanjing University

Halogenated aromatic compounds have attracted increasing concerns due to their toxicity and persistency in the environment, and dehalogenation is one of the promising treatment and detoxification methods. Herein, we systematically studied the debromination efficiency and mechanism of para-bromophenol（4-BP） by a recently developed UV/sulfite process. 4-BP underwent rapid degradation with the kinetics accelerated with the increasing sulfite concentration, pH（6.1–10） and temperature, whereas inhibited by dissolved oxygen and organic solvents. The apparent activation energy was estimated to be 27.8 kJ/mol. The degradation mechanism and pathways of 4-BP were explored by employing N2O and nitrate as the electron scavengers and liquid chromatography/mass spectrometry to identify the intermediates. 4-BP degradation proceeded via at least two pathways including direct photolysis and hydrated electron-induced debromination. The contributions of both pathways were distinguished by quantifying the quantum yields of 4-BP via direct photolysis and hydrated electron production in the system. 4-BP could be readily completely debrominated with all the substituted Br released as Br-, and the degradation pathways were also proposed. This study would shed new light on the efficient dehalogenation of brominated aromatics by using the UV/sulfite process.

关键词： Debromination Brominated aromatics UV/sulfite process Hydrated electron Mechanism

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Phytotoxicity and groundwater impacts of leaching from thermal treatment residues in roadways

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Journal of Environmental Sciences 2018年第1期30卷 58-67页

作者： Khamphe Phoungthong Li-Ming Shao Pin-Jing He Hua Zhang State Key Laboratory of Pollution Control & Resource Reuse Tongji University Institute of Waste Treatment and Reclamation Tongji University Centre for the Technology Research and Training on Household Waste in Small Towns & Rural Area Ministry of Housing and Urban-Rural Development of PR China (MOHURD)

The use of coal fly ash（CFA）, municipal solid waste incinerator bottom ash（MSWIBA） and flue gas desulfurization residue（FGDR） in road construction has become very common owing to its economical advantages. However, these residues may contain toxic constituents that pose an environmental risk if they leach out and flow through the soil, surface water and ***, it is necessary to assess the ecotoxicity and groundwater impact of these residues before decisions can be made regarding their utilization for road construction. In this study,the physico-chemical characteristics, leaching and phytotoxicity of these residues were investigated. Specifically, multivariate analyses were used to evaluate the contributions of the leaching constituents of the CFA, MSWIBA and FGDR leachates to the germination index of wheat seeds. B, Ba, Cr, Cu, Fe and Pb were found to be more toxic to the wheat seeds than the other heavy metals. Furthermore, the leached concentrations of the constituents from the CFA, MSWIBA and FGDR were below the regulatory threshold limits of the Chinese identification standard for hazardous wastes. Analyses conducted using a numerical groundwater model（Wisc LEACH） indicated that the predicted field concentrations of metals from the CFA, MSWIBA and FGDR increased with time up to about 30 years at the point of compliance, then decreased with time and distance. Overall, this study demonstrated that the risks resulting from MSWIBA, CFA and FGDR leaching could be assessed before its utilization for road construction, providing crucial information for the adoption of these alternative materials.

关键词： Thermal treatment residues Bottom ash Flue gas desulfurization residue Heavy metals Phytotoxicity Groundwater impact

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