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Disinfection byproducts in indoor swimming pool water: Detection and human lifetime health risk assessment

Journal of Environmental Sciences 2023年第4期126卷 378-386页

作者： Di Zhang Shengkun Dong Li Chen Rong Xiao Wenhai Chu State Key Laboratory of Pollution Control and Resources Reuse College of Environmental Science and EngineeringTongji UniversityShanghai 200092China Shanghai Institute of Pollution Control and Ecological Security Shanghai 200092China Southern Laboratory of Ocean Science and Engineering Key Laboratory of Water Cycle and Water Security in Southern China of Guangdong Higher Education InstituteSun Yat-sen UniversityGuangzhou 510275China

Quantification of regulated and emerging disinfection byproducts (DBPs) in swimming pool water,as well as the assessment of their lifetime health risk are limited in *** this study,the occurrence of regulated DBPs (e.g.,trihalomethanes,haloacetic acids) and emerging DBPs (e.g.,haloacetonitriles,haloacetaldehydes) in indoor swimming pool water and the corresponding source water at a city in Eastern China were *** concentrations of DBPs in swimming pool water were 1-2 orders of magnitude higher than that in source *** cancer and non-cancer risks of DBPs stemming from swimming pool water were also *** and dermal exposure were the most significant exposure routes related to swimming pool DBP cancer and non-cancer *** the first time,buccal and aural exposure were considered,and were proven to be important routes of DBP exposure (accounting for 17.9%-38.9%of total risk).The cancer risks of DBPs for all swimmers were higher than 10^(-6)of lifetime exposure risk recommended by United states Environmental Protection Agency,and the competitive adult swimmers experienced the highest cancer risk (7.82×10^(-5)).These findings provide important information and perspectives for future efforts to lower the health risks associated with exposure to DBPs in swimming pool water.

关键词： Health risk assessment Swimming pool water Disinfection byproducts Multiple exposure pathway

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Establishing an Assessment Index System for Sewage Treatment Works in China

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Engineering 2023年第8期27卷 18-22页

作者： Zuxin Xu Jin Xu State Key Laboratory of Pollution Control and Resource Reuse College of Environmental Science and EngineeringTongji UniversityShanghai 200092China Key Laboratory of Yangtze River Water Environment Ministry of EducationTongji UniversityShanghai 200092China Shanghai Institute of Pollution Control and Ecological Security Shanghai 200092China

*** The urban sewage treatment system,including sewage pipe networks and sewage treatment plants,is an important infrastructure to ensure urban social and economic *** the past few decades,due to the unremitting efforts of the Chinese government,the construction of China’s urban sewage treatment infrastructure has developed rapidly[1].

关键词： treatment Sewage sewage

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Identification of high oxygen-consuming substances in stormwater drainage systems illicitly connected with sewage system

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Journal of Environmental Sciences 2024年第4期138卷 132-140页

作者： Chen Xu Zuxin Xu Wenhai Chu Shanshan Wu Rong Xiao Lei Su State Key Laboratory of Pollution Control and Resource Reuse College of Environmental Science and EngineeringTongji UniversityShanghai 200092China Ministry of Education Key Laboratory of Yangtze River Water Environment Tongji UniversityShanghai 200092China Guangzhou Resource Environmental Protection Technology Co. Ltd.Guangzhou 510030China

The dissolved oxygen content in water is an important indicator for assessing the quality of the water environment,and maintaining a certain amount of dissolved oxygen is essential for the healthy development of the ecological *** a water body is anoxic,the activity of anaerobic microorganisms increases and organic matter is decomposed to produce a large number of blackening and odorizing substances,resulting in black and odorous water bodies,which is a very common and typical phenomenon in ***,there is still a relatively universal occurrence of illicitly connected stormwater and sewage pipes in the urban drainage pipe network in China,which makes oxygen-consuming substances be directly discharged into rivers through stormwater pipes and consume the dissolved oxygen in the water bodies,resulting in an oxygen deficiency of the *** induces seasonal or year-round black and stink phenomena in urban ***,identifying high oxygen-consuming substances,which lays the foundation for the subsequent removal of oxygen-consuming substances,is *** a series of comparisons of water quality indicators and analysis of organic characteristics,it was found that the oxygen consumption capacity of domestic sewage was higher than that of industrial wastewater in the selected area of this study,and the oxygen-consuming substances of domestic sewage were small molecular amino *** comparing 20 conventional free amino acids,it was found that seven of them consumed oxygen easily,and compared with chemical oxygen consumption,biological oxygen consumption was in a leading position.

关键词： Urban drainage system Oxygen-consuming substances Domestic sewage Amino acid

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Electronic regulation to achieve efficient anaerobic digestion of organic fraction of municipal solid waste(OFMSW):strategies,challenges and potential solutions

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Frontiers of Environmental Science & Engineering 2024年第4期18卷 159-165页

作者： Yongdong Chen Hong Wang Parisa Ghofrani-Isfahani Li Gu Xiaoguang Liu Xiaohu Dai State Key Laboratory of Pollution Control and Resources Reuse College of Environmental Science and EngineeringTongji UniversityShanghai 200092China Shanghai Institute of Pollution Control and Ecological Security Tongji UniversityShanghai 200092China Department of Chemical and Biochemical Engineering Technical University of DenmarkKgs Lyngby DK-2800Denmark College of Environment and Ecology Chongqing UniversityChongqing 400045China

Anaerobic digestion(AD)of organic fraction of municipal solid waste(OFMSW)is prone to system breakdown under high organic loading rates(OLRs)condition,which subsequently reduces the efficiency of digestion process and results in substantial economic *** this perspective paper,the substances metabolisms,electrons flow,as well as microbial interaction mechanisms within AD process are comprehensively discussed,and the underlying bottleneck that causes inefficient methane production is identified,which is“electrons surplus”.Systems encountering severe electron surplus are at risk of process failure,making it crucial to proactively prevent this phenomenon through appropriate *** this basis,the present perspective proposes three potential electronic regulation strategies to prevent electrons surplus,namely,electron shunt,accelerating electron transfer and regulating methanogenic metabolism pathway,and presents specific methodologies for each ***,the potential solutions to challenges that may occur during the electronic regulation process are also presented in this *** perspective aims to provide innovative approaches to achieve the efficient and stable operation of OFMSW anaerobic digestion,especially under high OLRs condition.

关键词： Anaerobic digestion Electrons surplus Electronic regulation Electrons shunt Electron transfer Methanogenic metabolism pathway

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Destructing surfactant network in nanoemulsions by positively charged magnetic nanorods to enhance oil-water separation

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Journal of Environmental Sciences 2022年第8期34卷 112-121页

作者： Yongjiao Xiong Xiangfeng Huang Lexue Li Wanqi Liu Jialu Zhang Mengfan He Jia Liu Lijun Lu Kaiming Peng College of Environmental Science and Engineering State Key Laboratory of Pollution Control and Resource ReuseMinistry of Education Key Laboratory of Yangtze River Water EnvironmentTongji UniversityShanghai 200092China

The separation of ultrafine oil droplets from wasted nanoemulsions stabilized with high concentration of surfactants is precondition for oil reuse and the safe discharge of ***, the double barriers of the interfacial film and network structures formed by surfactants in nanoemulsions significantly impede the oil-water separation. To destroy these surfactant protective layers, we proposed a newly-developed polyethyleneimine micelle template approach to achieve simultaneous surface charge manipulation and morphology transformation of magnetic nanospheres to magnetic nanorods. The results revealed that positively charged magnetic nanospheres exhibited limited separation performance of nanoemulsions, with a maximum chemical oxygen demand(COD) removal of 50%, whereas magnetic nanorods achieved more than 95% COD removal in less than 30 s. The magnetic nanorods were also applicable to wasted nanoemulsions from different sources and exhibited excellent resistance to wide pH changes. Owing to their unique one-dimensional structure, the interfacial dispersion of magnetic nanorods was significantly promoted, leading to the efficient capture of surfactants and widespread destruction of both the interfacial film and network structure, which facilitated droplet merging into the oil phase. The easy-toprepare and easy-to-tune strategy in this study paves a feasible avenue to simultaneously tailor surface charge and morphology of magnetic nanoparticles, and reveals the huge potential of morphology manipulation for producing high-performance nanomaterials to be applied in complex interfacial interaction process. We believe that the newly-developed magnetic-nanorods significantly contribute to hazardous oily waste remediation and advances technology evolution toward problematic oil-pollution control.

关键词： Nanoemulsions Surface charge Magnetic nanorods Surfactant Interfacial film Oil-water separation

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La^(3+)@BC500-S_(2)O_(8)^(2−)system for removal of sulfonamide antibiotics in water

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Journal of Environmental Sciences 2024年第12期146卷 140-148页

作者： Bing Wang Dongsu Bi Juan Wang Hengbo Qiao Yalei Zhang Zheng Shen School of Chemical and Environmental Engineering Shanghai Institute of TechnologyShanghai 201418China State Key Laboratory of Pollution Control and Resources Reuse Key Laboratory of Yangtze River Water Environment of MOENational Engineering Research Center of Protected AgricultureShanghai Engineering Research Center of Protected AgricultureTongji UniversityShanghai 200092China

Sulfonamide antibiotics(SAs)widely used have potentially negative effects on human beings and *** and advanced oxidation methods have been exten-sively applied in SAs wastewater *** this study,compared with Al^(3+)@BC500 and Fe^(3+)@BC500,La^(3+)@BC500 for activating persulfate(S2O82−)had the best effect removal per-formance of sulfadiazine(SDZ)and sulfamethoxazole(SMX).Morphology,acidity,oxygen-containing functional groups,and loading of La^(3+)@BC500 were analyzed by techniques,in-cluding EA,BET,XRD,XPS,*** results show that with the increase of La^(3+)loading,the surface characteristics of biochar gradually changed from CaCO_(3)to LaCO_(3)*** EPR technology,it is proved that LaCO_(3)OH on the surface of La^(3+)@BC500 can not only acti-vate S2O82−to generate SO_(4)^(−)•,but also to produce•*** the optimization experiment,the optimal dosage of La^(3+)is between 0.05 and 0.2(mol/L)/*** had a good removal effect at pH(5-9),but SMX had a good removal effect only at pH=*** potential also proves that the material is more stable under acidic *** removal process of SDZ is more in accord with pseudo-first-order kinetics(R^(2)=0.9869),while SMX is more in line with pseudo-second order kinetics(R^(2)=0.9926).

关键词： Sulfadiazine Sulfamethoxazole La^(3+)@BC500 Persulfate

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Fluorescence analysis of antibiotics and antibiotic-resistance genes in the environment: A mini review

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Chinese Chemical Letters 2024年第10期35卷 82-91页

作者： Yuxin Li Chengbin Liu Qiuju Li Shun Mao College of Environmental Science and Engineering State Key Laboratory of Pollution Control and Resource ReuseTongji UniversityShanghai 200092China Institute for Agri-food Standards and Testing Technology Shanghai Academy of Agricultural SciencesShanghai 201403China

Antibiotics,as widely used antibacterial drug,exist in various environmental *** residues can affect biological metabolism and lead to bacterial resistance and the formation of antibiotic-resistance genes,posing a threat to human health and ecological *** efficient detection methods for antibiotics and antibiotic-resistance genes has great environmental *** detection methods,due to their fast response,high sensitivity and specificity,and low-cost,are widely used in chemical and biological *** review first summarizes the pre-treatment methods for different types of environmental samples,and then focuses on the recent advances of fluorescence methods for the detection of antibiotics and antibiotic-resistance ***,main challenges and future research directions of fluorescence methods for antibiotic and antibiotic-resistance genes detection are *** review highlights the promising prospect of fluorescence methods in-situ detection and monitoring of antibiotics and antibiotic-resistance genes,and provides guidance for the construction of overall risk assessment system of environmental media.

关键词： Antibiotics Antibiotic-resistancegenes Fluorescence detection Environmental samples In-situdetection

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ZnS-embedded porous carbon for peroxydisulfate activation:Enhanced electron transfer for bisphenol A degradation

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Environmental Science and Ecotechnology 2024年第3期19卷 161-169页

作者： Ying Liu Ningjie Du Xinru Liu Ducheng Yao Deli Wu Zhuo Li Shun Mao College of Environmental Science and Engineering Biomedical Multidisciplinary Innovation Research InstituteShanghai East HospitalState Key Laboratory of Pollution Control and Resource ReuseTongji University1239 Siping RoadShanghai200092China Shanghai Institute of Pollution Control and Ecological Security Shanghai200092China

Transition metal sulfides have garnered increasing attention for their role in persulfate activation,a crucial process in environmental ***,the function of metal sulfides without reversible valence changes,such as ZnS,remains largely unexplored in this *** we report ZnS-embedded porous carbon(ZnS-C),synthesized through the pyrolysis of Zn-MOF-74 and dibenzyl ***-C demonstrates remarkable activity in activating peroxydisulfate(PDS)across a wide pH range,enabling the efficient mineralization removal of bisphenol A(BPA).Through electrochemical investigation and theoretical simulations of charge density distributions,we unveil that the electron transfer from BPA to PDS mediated by the ZnS-C catalyst governs the *** study,both in theory and experiment,demonstrates metal sulfide as electron pump that enhances electron transfer efficiency in PDS *** findings redefine the role of metal sulfide catalysts,shedding new light on their potential for regulating reaction pathways in PDS activation processes.

关键词： Peroxydisulfate activation Reaction pathway regulation Electron transfer ZnS Bisphenol A

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High potential in synergizing the reduction of dissolved organic carbon concentration and carbon dioxide emissions for submerged-vegetationcovered river networks

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Journal of Environmental Sciences 2025年第5期151卷 298-309页

作者： Qingqian Li Ruixia Liu Zhangmu Jing Yanjie Wei Shengqiang Tu Huibin Yu Hongjie Gao Peng Yuan State Key Laboratory of Environmental Criteria and Risk Assessment Chinese Research Academy of Environmental ScienceBeijing 100012China State Environmental Protection Key Laboratory of Estuarine and Coastal Environment Chinese Research Academy of Environmental ScienceBeijing 100012China State Key Laboratory of Pollution Control and Resource Reuse College of Environmental Science and EngineeringTongji UniversityShanghai 200092China College of Municipal and Environmental Engineering Shenyang Jianzhu UniversityShenyang 110168China

Various technologies and projects have been explored and developed for the synergetic control of environmental pollution and carbon emissions in aquatic *** submerged vegetation in shallow waters was also expected to achieve this ***,the magnitude and mechanism of carbon dioxide(CO_(2))emission affected by submerged vegetation is not clear enough in complex aquatic *** study investigated the influences of submerged plants on CO_(2)emission,ecosystem metabolism features,and microbial community traits based on observations in river networks on the Changjiang River *** results showed that CO_(2)emission from planted waters accounted for 73%of unplanted ***,planted waters had higher dissolved organic carbon removal capacity in overlying water and higher potential of carbon sequestration in sediment at the same *** distinctions between the two habitats were attributed to(1)improved CO_(2)and bicarbonate consumption in water columns via enhancing photosynthesis and(2)inhibited CO_(2)production by reconstructing the benthic microbial *** eco-advantages were found in planted sediments,such as a high potential of methane oxidation and xenobiotics biodegradation and a low risk of becoming black and *** brief,submerged vegetation is beneficial in promoting pollution removal and carbon retention *** study advances our understanding of the feedback between aquatic metabolism and CO_(2)emission.

关键词： Mitigated CO_(2)emission Submerged vegetation Paired O_(2)-CO_(2)departure Carbon uptake velocity Microbial metabolism pathways The Changjiang River

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Nonpolar cross-stacked super-aligned carbon nanotube membrane for efficient wastewater treatment

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Frontiers of Environmental Science & Engineering 2023年第3期17卷 37-47页

作者： Shuang Zhang Shuai Liang Yifan Gao Yang Wu Xia Huang Bejing Key Laboratory for Source Control Technology of Water Pollution College of Environmental Science and EngineeringBeijing Forestry UniversityBeijing 100083China Engineering Research Center for Water Pollution Source Control&Eco-remediation College of Environmental Science and EngineeringBeijing Forestry UniversityBeijing 100083China State Key Joint Laboratory of Environment Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing 100084China Department of Physics and Tsinghua-Foxconn Nanotechnology Research Center Tsinghua UniversityBeijing 100084China

Membrane separation technology has made great progress in various practical applications,but the unsatisfactory separation performance of prevailing membrane materials hampers its further sustainable *** study proposed a novel nonpolar super-aligned carbon nanotube(SACNT)membrane,which was prepared with a layer-by-layer cross-stacking *** controlling the number of stacked SACNT layers,three kinds of SACNT membranes(SACNT_200,SACNT 300,and SACNT_400)were *** characterizations and filtration tests were performed to investigate their physico-chemical properties,surface wetting behavior,and filtration *** with two commercial membranes(Com_0.22 and Com_0.45),all the SACNT membranes achieved smoother and more uniform *** to the hexagonal graphene structure of CNTs,the surface chemistry of the SACNT membranes is simple and inert,thereby potentially eliminating the covalent-bonding-induced membrane ***,the SACNT membranes exhibited a typical nonpolar wetting behavior,with high contact angles for polar liquids(water:~124.9°-126.5°;formamide:~80.0°-83.99)but low contact angles for nonpolar diodomethane(~18.8°-20.99).This unique nonpolar feature potentially leads to weak interactions with polar ***,compared with the commercial membranes,the SACNT membranes obtained a significantly higher selectivity while achieving a comparable or higher permeability(depending on the number of stacked layers).Moreover,the SACNT membranes exhibited superior separation performance in various application scenarios,including municipal wastewater treatment(2.3 times higher cleaning efficiency),electro-assistant fouling inhibition(or even self-cleaning),and oil/water separation(>99.2%of separation efficiency),suggesting promising application prospects in various fields.

关键词： Membranefouling Wastewater Membrane separation Antifouling Aligned carbon nanotube

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