In this work,a three-dimensional crystal-plasticity-based phase-field model considering three kinds of inelastic deformation mechanisms,i.e.,martensitic transformation,dislocation slip in austenite,and dislocation sli...
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In this work,a three-dimensional crystal-plasticity-based phase-field model considering three kinds of inelastic deformation mechanisms,i.e.,martensitic transformation,dislocation slip in austenite,and dislocation slip in martensite,is established to simulate the stress-assisted two-way shape memory effect(SATWSME)of NiTi single crystals and its cyclic *** simulation results show that the ability of the SATWSME of NiTi single crystal increases as increasing the constant stress in the range discussed in this work(10–100 MPa),which is due to the increase of reoriented martensite formed in the cooling process due to the enhanced variant-selection capability of increased constant *** martensitic transformation and its reverse in the cyclic process reflecting the SATWSME show more and more obvious localization characteristics,resulting in the accumulation of significantly heterogeneous plastic deformation(mainly caused by the dislocation slip in austenite),which leads to the cyclic degradation of *** simulation results and the conclusions drawn from this work are helpful for further understanding the mechanism of functional cyclic degradation of NiTi alloys.
Single-atom catalysts are highly effective in catalyzing a wide range of reactions owing to their capacity to have precise coordination patterns and fully leverage the potential of metal *** several techniques have be...
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Single-atom catalysts are highly effective in catalyzing a wide range of reactions owing to their capacity to have precise coordination patterns and fully leverage the potential of metal *** several techniques have been reported for the preparation of single-atom catalysts,adopting a convenient method to construct them still has a *** this work,we report a convenient method for the preparation of Zr-based single-atom catalyst that takes advantage of the nanoconfined environments between the template and silica wall in template-occupied silica *** introducing Zr-containing precursor into the nanoconfined environments of the templateoccupied silica SBA-15 using solid-phase milling,Zrbased single-atom catalysts were produced via the following calcination *** functional theory calculations and experimental findings show that Zr atoms form Zr-O-Si structure in the silica *** Zr single-atom catalyst synthesized using the nanoconfined environments exhibited notably superior catalytic performance in the synthesis of benzyl acetate from the esterification reaction between acetic acid and benzyl alcohol(63.3%yield),outperforming the counterpart that synthesized without such nanoconfined environments(19.8%yield).
Antimony selenide(Sb_(2)Se_(3))is one of the perspective candidates for potassium-ion batteries due to its advanced virtues stem including featured high capacity,fertile reserves and the relative narrow band *** the u...
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Antimony selenide(Sb_(2)Se_(3))is one of the perspective candidates for potassium-ion batteries due to its advanced virtues stem including featured high capacity,fertile reserves and the relative narrow band *** the unique advantages,it is still plagued by the unstable interface compatibility and poor wider-temperature *** optimization of microstructure and the construction of inorganic-organic hybrids with a low desolvation barrier and rapid kinetics behaviors are efficient to address these *** Sb_(2)Se_(3)nanorods enclosed by the S-doped carbon layer(SC),further crosslinked by the poly(N-isopropylacrylamide)(PM)film(PM@Sb_(2)Se_(3)@SC),were artificially fabricated,and it displays the enrichment ion aggregated model as well as contacted ion pair state,the well-tailored cooperation environment of potassium bonds,assuring a homogeneous potassium deposition and an excellent widertemperature *** complicated experimental studies and theoretical calculations authenticate the synergistic effects of geometric conformation and compositional design for the tremendously enhanced potassium ***,the full device over PM@Sb_(2)Se_(3)@SC anode and the potassium Prussian blue cathode manifests impressively durable cycling life and wider-temperature adaptability,verifying the glorious contribution from the finely manipulation in solvation structure and potassium bonds to enhancing the potassium storage behaviors.
The GFL-GFM hybrid wind farm (HWF) combines the voltage source control advantages of grid-forming (GFM) wind turbines (WTs) with the current source control advantages of grid-following (GFL) wind turbines. It becomes ...
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The GFL-GFM hybrid wind farm (HWF) combines the voltage source control advantages of grid-forming (GFM) wind turbines (WTs) with the current source control advantages of grid-following (GFL) wind turbines. It becomes a new type of large-scale grid-connected wind power generation. In this paper, we propose an HWF frequency-voltage active support based on GFL and GFM hierarchical subgroup control. It aims to realize the support of active power and reactive power under the premise of ensuring system stability. The strategy consists of the determination of the control objectives of the GFM-GFL subgroups, the distributed control (DC) of the GFM-GFL subgroups, and the adaptive control and switching of each unit of the GFM and GFL groups. The GFM-group maintains the grid-connected voltage stability and the GFL-group exhausts the active support. DC at the group level and adaptive control at the unit level are included under the hierarchy of the respective objectives. Finally, a GFL-GFM HWF model is established on the MATLAB/Simulink platform, and the simulation verifies that the proposed strategy can realize the enhancement of the frequency-voltage support capability of the HWF under the premise of grid-connected stability.
Background Chickens and ducks are vital sources of animal protein for *** pangenome studies suggest that a single genome is insufficient to represent the genetic information of a species,highlighting the need for more...
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Background Chickens and ducks are vital sources of animal protein for *** pangenome studies suggest that a single genome is insufficient to represent the genetic information of a species,highlighting the need for more comprehensive *** bird genome has more than tens of microchromosomes,but comparative genomics,annotations,and the discovery of variations are hindered by inadequate telomere-to-telomere level *** aim to complete the chicken and duck genomes,recover missing genes,and reveal common and unique chromosomal features between *** The near telomere-to-telomere genomes of Silkie Gallus gallus and Mallard Anas platyrhynchos were successfully assembled via multiple high-coverage complementary technologies,with quality values of 36.65 and 44.17 for Silkie and Mallard,respectively;and BUSCO scores of 96.55%and 96.97%for Silkie and Mallard,respectively;the mapping rates reached over 99.52%for both assembled genomes,these evaluation results ensured high completeness and *** successfully annotated 20,253 and 19,621 protein-coding genes for Silkie and Mallard,respectively,and assembled gap-free sex chromosomes in Mallard for the first *** analysis revealed that microchromosomes differ from macrochromosomes in terms of GC content,repetitive sequence abundance,gene density,and levels of 5mC *** types of arrangements of centromeric repeat sequence centromeres exist in both Silkie and the Mallard genomes,with Mallard centromeres being invaded by *** highly heterochromatic W chromosome,which serves as a refuge for ERVs,contains disproportionately long *** Silkie and the Mallard genomes presented relatively high 5mC methylation levels on sex chromosomes and microchromosomes,and the telomeres and centromeres presented significantly higher 5mC methylation levels than the whole ***,we recovered 325 missing genes via our new genomes and annotated TNFA in Mallard for the first time,r
作者:
Si, XiaopengHuang, HeYu, JiayueMing, DongTianjin University
Academy of Medical Engineering and Translational Medicine State Key Laboratory of Advanced Medical Materials and Devices Haihe Laboratory of Brain-computer Interaction and Human-machine Integration Tianjin Key Laboratory of Brain Science and Neural Engineering Institute of Applied Psychology Tianjin300072 China Tianjin University
Academy of Medical Engineering and Translational Medicine State Key Laboratory of Advanced Medical Materials and Devices Haihe Laboratory of Brain-computer Interaction and Human-machine Integration Tianjin Key Laboratory of Brain Science and Neural Engineering Tianjin300072 China
The affective brain-computer interface (aBCI) facilitates the objective identification or regulation of human emotions. Current aBCI mainly relies on electroencephalography (EEG). However, research shows that emotions...
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A series of carbon nitride(CN)materials represented by graphitic carbon nitride(g-C_(3)N_(4))have been widely used in bioimaging,biosensing,and other fields in recent years due to their nontoxicity,low cost,and high l...
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A series of carbon nitride(CN)materials represented by graphitic carbon nitride(g-C_(3)N_(4))have been widely used in bioimaging,biosensing,and other fields in recent years due to their nontoxicity,low cost,and high luminescent quantum *** is more attractive is that the luminescent properties such as wavelength and intensity can be regulated by controlling the structure at the molecular ***,it is time to summarize the related research on CN structural evolution and make a prospect on future *** this review,we first summarize the research history and multiple structural evolution of ***,the progress of improving the luminescence performance of CN through structural evolution was ***,the relationship between CN structure evolution and energy conversion in the forms of photoluminescence,chemiluminescence,and electrochemiluminescence was ***,key challenges and opportunities such as nanoscale dispersion strategy,luminous efficiency improving methods,standardization evaluation,and macroscopic preparation of CN are highlighted.
Layered oxide is a promising cathode material for sodium-ion batteries because of its high-capacity,high operating voltage,and simple *** performance is an important criterion for evaluating the application prospects ...
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Layered oxide is a promising cathode material for sodium-ion batteries because of its high-capacity,high operating voltage,and simple *** performance is an important criterion for evaluating the application prospects of ***,facing challenges,including phase transitions,ambient stability,side reactions,and irreversible anionic oxygen activity,the cycling performance of layered oxide cathode materials still cannot meet the application ***,this review proposes several strategies to address these ***,bulk doping is introduced from three aspects:cationic single doping,anionic single doping,and multi-ion ***,homogeneous surface coating and concentration gradient modification are *** addition,methods such as mixed structure design,particle engineering,high-entropy material construction,and integrated modification are ***,a summary and outlook provide a new horizon for developing and modifying layered oxide cathode materials.
As a gateway to handle all intranet terminal traffic, SOHO router plays an important role in the network. In this paper, we introduced the security threats faced by SOHO routers, and on this basis, we propose a packet...
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The sluggish kinetics behaviors and vast volume variations of Na^(+)hosts to FeS_(2)anode involved intercalation,and conversion reactions plague its applicability of sodium-ion batteries(SIBs).Here,a significantly exp...
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The sluggish kinetics behaviors and vast volume variations of Na^(+)hosts to FeS_(2)anode involved intercalation,and conversion reactions plague its applicability of sodium-ion batteries(SIBs).Here,a significantly expedited kinetics via cation intercalation and considerably relieved stress accumulation by constructing the concave scaffold protector are approached for FeS_(2)*** Mn^(2+)intercalation into FeS_(2),a new stable Mn-FeS_(2)was generated with distorted coordination;elevated antibonding orbital occupancy and lowed d band center to the release of more free Na^(+)were achieved,which was further encapsulated by hollow bowl-like carbon spheres(BC)This cation intercalation and concave morphology strategies confer Mn-FeS_(2)@BC significantly enhanced electron ion transport kinetics via reversed electron transfer to FeS_(2)fast desolvation kinetics,and evidently depressed structural deformation during Na^(+)insertion and ***,Mn-FeS_(2)@BC delivers the longevity and stable Na^(+)storage capacity in both half and full cell ***,Mn-FeS_(2)@BC also displays excellen adaptability in a wider temperature *** work proposes new views into the deep regulation of electrochemical performance of transition metal anodes via intercalation chemistry and concave engineering.
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