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Characterizing molecular fingerprint of dissolved organic matter shaped by natural and anthropogenic factors in a large macrophytic shallow lake wetland

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Frontiers of Environmental Science & Engineering 2025年第3期19卷 73-86页

作者： Shengwu Yuan Yiping Xu Pengfei Wang Ruili Xie Jiangbo Hu Zhenghui Fu Kun Wang Shuhang Wang Xia Jiang Kaifeng Rao Mei Ma Zijian Wang State Key Laboratory of Environmental Criteria and Risk Assessment National Engineering Laboratory for Lake Pollution Control and Ecological RestorationState Environment Protection Key Laboratory for Lake Pollution ControlState Environmental Protection Key Laboratory of Drinking Water Source ProtectionChinese Research Academy of Environmental ScienceBeijing 100012China Research Center for Eco-Environmental Sciences Chinese Academy of SciencesBeijing 100085China College of Resources and Environment University of Chinese Academy of SciencesBeijing 100049China

Dissolved organic matter(DOM)participates in and affects many biological processes in aquatic ecosystems,altering nutrient cycling,bioavailability and toxicity of *** water contains thousands of DOM molecules,which largely originate from natural sources and are greatly influenced by external inputs through anthropogenic *** elucidate the shaping mechanism of the DOM composition under complex habitat conditions and anthropogenic disturbances,the characteristic molecular fingerprint of DOM was determined based on chemodiversity information obtained via ultrahigh-resolution mass spectrometry for the Baiyangdian wetland(a typical large macrophytic shallow lake in North China).In the Baiyangdian wetland,the DOM composition exhibited high complexity and spatial heterogeneity,and more recalcitrant DOM molecules were identified in summer than in *** multiple natural factors(nutrient concentration,depth of water and quality of submerged macrophytes)and anthropogenic factors(different land uses and discharge of pollutants)were associated with the relative abundance of various DOM molecules,only the influences from the anthropogenic factors were statistically *** alpha diversity index of DOM could reflect variations in both the natural factors(total dissolved phosphorus)and the anthropogenic factors(discharge of nitrogen and phosphorus).Furthermore,the DOM composition in each group were clustered according to the ecological functions(natural reserves,tourism,breeding,and domestic supply functions),and exhibited molecular fingerprint *** study provides an effective approach to characterize the molecular fingerprint features of DOM and critical information to better understand the shaping mechanism of the DOM composition under complex habitat conditions and anthropogenic disturbances.

关键词： DOM FT-ICR-MS Chemodiversity Habitat Ecological function Baiyangdian wetland

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Distributed asynchronous double accelerated optimization for ethylene plant considering delays

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Chinese Journal of Chemical Engineering 2025年第2期78卷 245-250页

作者： Ting Wang Zhongmei Li Wenli Du State Key Laboratory of Industrial Control Technology East China University of Science and Technology Key Laboratory of Smart Manufacturing in Energy Chemical Process Ministry of Education East China University of Science and Technology

Considering the complexity of plant-wide optimization for large-scale industries, a distributed optimization framework to solve the profit optimization problem in ethylene whole process is proposed. To tackle the delays arising from the residence time for materials passing through production units during the process with guaranteed constraint satisfaction, an asynchronous distributed parameter projection algorithm with gradient tracking method is introduced. Besides, the heavy ball momentum and Nesterov momentum are incorporated into the proposed algorithm in order to achieve double acceleration properties. The experimental results show that the proposed asynchronous algorithm can achieve a faster convergence compared with the synchronous algorithm.

关键词： Asynchronous distributed optimization Heavy ball Inequality constraints Nesterov Plant-wide optimization

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Differential effects of microplastics on soil organic carbon via lignin phenols and amino sugars in soil aggregates

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Frontiers of Environmental Science and Engineering 2025年第7期19卷 1-14页

作者： Yu, Hong Huang, Xiang Yang, Ke Xi, Beidou Tan, Wenbing State Key Laboratory of Environmental Criteria and Risk Assessment and State Environmental Protection Key Laboratory of Simulation and Control of Groundwater Pollution Chinese Research Academy of Environmental Sciences Beijing100012 China

Accumulation of plant- and microbial-derived carbon together determines the stability of soil organic carbon (SOC) pools. To explore the accumulation characteristics and comparative contributions of organic carbon from diverse origins within soil aggregates exposed to microplastic pollution, we conducted corn pot experiments using biodegradable (polylactic acid;PLA) and conventional microplastics (polyethylene;PE) to examine the effects of microplastic pollution on microbial and plant derived carbon in macroaggregates (0.25–2 mm) and microaggregates ( © Higher Education Press 2025.

关键词： Microplastic pollution Soil organic carbon Soil aggregate Plant lignin Microbial necromass

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Emission control status and future perspectives of diesel trucks in China

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Journal of Environmental Sciences 2025年第2期148卷 702-713页

作者： Shihai Zhang Mingliang Fu Hefeng Zhang Hang Yin Yan Ding State Environmental Protection Key Laboratory of Vehicle Emission Control and Simulation Chinese Research Academy of Environmental SciencesBeijing 100012China Vehicle Emission Control Center Chinese Research Academy of Environmental SciencesBeijing 100012China

Chinese diesel trucks are the main contributors to NOx and particulate matter(PM)vehicle *** increase in diesel trucks could aggravate air pollution and damage human *** Chinese government has recently implemented a series of emission control technologies andmeasures for air quality *** paper summarizes recent control technologies and measures for diesel truck emissions in China and introduces the comprehensive application of control technologies and measures in Beijing-Tianjin-Hebei and surrounding *** onlinemonitoring technology has been adopted according to the China VI standard for heavy-duty diesel trucks,and control measures such as transportation structure adjustment and heavy pollution enterprise classification control continue to support the battle action plan for pollution *** and suggestions are provided for promoting pollution control and supervision of diesel truck emissions:adhere to the concept of overall management and control,vigorously promote the application of systematic and technological means in emission monitoring,continuously facilitate cargo transportation structure adjustment and promote new energy freight *** paper aims to accelerate the implementation of control technologies and measures throughout *** is endeavouring to control diesel truck exhaust *** is willing to cooperate with the world to protect the global ecological environment.

关键词： Air quality Diesel truck emissions Emission control technology control measures

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Monitoring fossil fuel CO_(2) emissions from co-emitted NO_(2) observed from space:progress,challenges,and future perspectives

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Frontiers of Environmental Science & Engineering 2025年第1期19卷 23-45页

作者： Hui Li Jiaxin Qiu Kexin Zhang Bo Zheng Shenzhen Key Laboratory of Ecological Remediation and Carbon Sequestration Institute of Environment and EcologyTsinghua Shenzhen International Graduate SchoolTsinghua UniversityShenzhen 518055China State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex Beijing 100084China

Developing an anthropogenic carbon dioxides(CO_(2))emissions monitoring and verification support(MVS)capacity is essential to support the Global Stocktake(GST)and ratchet up Nationally Determined Contributions(NDCs).The 2019 IPCC refinement proposes top-down inversed CO_(2)emissions,primarily from fossil fuel(FFCO_(2)),as a viable emission *** substantial progress in directly inferring FFCO_(2)emissions from CO_(2)observations,substantial challenges remain,particularly in distinguishing local CO_(2)enhancements from the high background due to the long atmospheric ***,using short-lived and co-emitted nitrogen dioxide(NO_(2))as a proxy in FFCO_(2)emission inversion has gained *** methodology is broadly categorized into plume-based and emission ratios(ERs)-based inversion *** the plume-based methods,NO_(2)observations act as locators,constraints,and validators for deciphering CO_(2)plumes downwind of sources,typically at point source and city *** ERs-based inversion approach typically consists of two steps:inferring NO_(2)-based nitrogen oxides(NO_(x))emissions and converting NO_(x)to CO_(2)emissions using CO_(2)-to-NO_(x)*** integrating NO_(2)observations into FFCO_(2)emission inversion offers advantages over the direct CO_(2)-based methods,uncertainties persist,including both structural and data-related *** these uncertainties is a primary focus for future research,which includes deploying nextgeneration satellites and developing advanced inversion ***,data caveats are necessary when releasing data to users to prevent potential *** NO_(2)-based CO_(2)emission inversion requires interdisciplinary collaboration across multiple communities of remote sensing,emission inventory,transport model improvement,and atmospheric inversion algorithm development.

关键词： Fossil fuel CO_(2) emissions CO_(2) satellites NO_(2) satellites Emission inversion methods Uncertainty management Future perspectives

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Effects of Corona Discharge from the Grounding Tip on Charge Evolution of Wall Bushing

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IEEE Transactions on Power Delivery 2025年第3期40卷 1682-1693页

作者： Bai, Zheng Zhou, Yuanxiang Zhang, Yunxiao Huang, Xin Xie, Xiongjie Liu, Taiwei Tsinghua University State Key Laboratory of Power System Operation and Control Department of Electrical Engineering Beijing100084 China Electric Power Research Institute State Key Laboratory of Power Grid Environmental Protection Wuhan430204 China

Manufacturers consider that the grounding tip near the wall bushing flange is a potentially important factor in several sheath perforation accidents. Taking a ±100 kV true type SF6 gas-insulated bushing as a typical wall bushing, this paper tests the impact of the nearby grounding tip on the charge accumulation. Based on the experiment results, we propose the three-dimensional nonlinear conduction model to unravel the charge accumulation process and the three-dimensional corona ion migration model to clarify the corona process. It is concluded that the consumption of gas ions leads to the nonlinear charge relaxation process. When the corona of grounding tip incepts, numerous ions are generated, forming an "overcharge" phenomenon. The electric field at the insulator-sheds interface and the SF6-insulator interface increases compared to the normal condition, with non-uniform distribution along the circumferential direction. Material inhomogeneity amplifies electric field distortion and creates insulation weaknesses, making insulation aging more likely and potentially leading to a slowly developing electrical tree breakdown process. The length of the needle tip affects the duration of the corona effect;an excessively long needle tip can cause a sustained corona discharge. This research provides a foundation for bushing accidents analysis and operation reliability improvement. © 1986-2012 IEEE.

关键词： Bushings

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Molecular characteristics of dissolved organic phosphorus in watershed runoff:Coupled influences of land use and precipitation

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Journal of Environmental Sciences 2025年第2期148卷 387-398页

作者： Zhanyao Shi Yao Du Hongni Liu Yamin Deng Yiqun Gan Xianjun Xie State Environmental Protection Key Laboratory of Source Apportionment and Control of Aquatic Pollution China University of GeosciencesWuhan 430078China Hubei Key Laboratory of Yangtze Catchment Environmental Aquatic Science China University of GeosciencesWuhan 430078China School of Environmental Studies&State Key Laboratory of Biogeology and Environmental Geology China University of GeosciencesWuhan 430078China

Land use and precipitation are two major factors affecting phosphorus(P)pollution of watershed ***,molecular characterization of dissolved organic phosphorus(DOP)in runoff under the joint influences of land use and precipitation remains *** study used Fourier transform ion cyclotron resonance mass spectrometry(FT-ICR-MS)to study the molecular characteristics of DOP in a typical P-polluted watershed with spatially variable land use and *** results showed that low precipitation and intense human activity,including phosphate mining and associated industries,resulted in the accumulation of aliphatic DOP compounds in the upper reaches,characterized by low aromaticity and low biological *** precipitation and widespread agriculture in the middle and lower reaches resulted in highly unsaturated DOP compounds with high biological stability constituting a higher proportion,compared to in the upper ***,under similar precipitation,more aliphatic DOP compounds characterized by lower aromaticity and higher saturation were enriched in the lower reaches due to more influence from urban runoff relative to the middle *** and/or microbial processes did result in changes in the characteristics of DOP compounds during runoff processes due to the prevalence of low molecular weight and low O/C bioavailable aliphatic DOP molecules in the upper reaches,which were increasingly transformed into refractory compounds from the upper tomiddle *** results of this study can increase the understanding of the joint impacts of land use and precipitation on DOP compounds in watershed runoff.

关键词： Watershed runoff DOP FT-ICR MS Land use Precipitation

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Simultaneous catalytic removal of NO and chlorobenzene over Mn-Ce-Sm-Sn-O_x/P84 composite catalytic filter

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Journal of Rare Earths 2025年第3期43卷 526-533,I0004页

作者： Mutao Xu Liguo Chen Xinpei Cheng Qijie Jin Ranran Zhou Jian Yang Chengzhang Zhu Sheng Wang Haitao Xu School of Environmental Science and Engineering Nanjing Tech UniversityNanjing210009China State Key Laboratory for Clean and Efficient Coal-fired Power Generation and Pollution Control State Key Laboratory of Low-carbon Smart Coal-fired Power Generation and Ultra-clean EmissionNanjing210046China College of Materials Science and Engineering Nanjing Tech UniversityNanjing210009China State Key Laboratory of Materials-Oriented Chemical Engineering Nanjing Tech UniversityNanjing210009China Nanjing Gekof Institute of Environmental Protection Technology&Equipment Co. Nanjing210031China

The integration of surface filtration and catalytic decomposition functions in catalytic bags enables the synergistic removal of multiple pollutants(such as dust,nitrogen oxide,acid gases,and dioxins)in a single reactor,thus effectively reducing the cost and operational difficulties associated with flue gas *** this study,Mn-Ce-Sm-Sn(MCSS)catalysts were prepared and loaded onto hightemperature resistant polyimide(P84)filter through ultrasonic impregnation to create composite catalytic *** results demonstrate that the NO conversion rates of the composite catalytic filter consistently achieve above 95%within the temperature range of 160-260℃,with a chlorobenzene T_(90)value of 230℃.The ultrasonic impregnation method effectively loaded the catalyst onto the filter,ensuring high dispersion both on the surface and inside the *** increased exposure of catalyst active sites enhances the catalytic activity of the composite catalytic ***,increasing the catalyst loading leads to a gradual decrease in permeability,an increase in pressure drops and the long residence time of the flue gas,thereby improving catalytic *** to ordinary impregnation methods,ultrasonic impregnation improves the bonding strength between the catalyst and filter,as well as the permeability of the composite catalytic filter under the same loading ***,this study presents a novel approach to prepare composite catalytic filter for the simultaneous removal of NO and chlorobenzene at low temperatures.

关键词： Compound catalytic filter Simultaneous catalysis Polyimide fibers Ultrasonic impregnation Rare earths

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High potential in synergizing the reduction of dissolved organic carbon concentration and carbon dioxide emissions for submerged-vegetationcovered river networks

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Journal of Environmental Sciences 2025年第5期151卷 298-309页

作者： Qingqian Li Ruixia Liu Zhangmu Jing Yanjie Wei Shengqiang Tu Huibin Yu Hongjie Gao Peng Yuan State Key Laboratory of Environmental Criteria and Risk Assessment Chinese Research Academy of Environmental ScienceBeijing 100012China State Environmental Protection Key Laboratory of Estuarine and Coastal Environment Chinese Research Academy of Environmental ScienceBeijing 100012China State Key Laboratory of Pollution Control and Resource Reuse College of Environmental Science and EngineeringTongji UniversityShanghai 200092China College of Municipal and Environmental Engineering Shenyang Jianzhu UniversityShenyang 110168China

Various technologies and projects have been explored and developed for the synergetic control of environmental pollution and carbon emissions in aquatic *** submerged vegetation in shallow waters was also expected to achieve this ***,the magnitude and mechanism of carbon dioxide(CO_(2))emission affected by submerged vegetation is not clear enough in complex aquatic *** study investigated the influences of submerged plants on CO_(2)emission,ecosystem metabolism features,and microbial community traits based on observations in river networks on the Changjiang River *** results showed that CO_(2)emission from planted waters accounted for 73%of unplanted ***,planted waters had higher dissolved organic carbon removal capacity in overlying water and higher potential of carbon sequestration in sediment at the same *** distinctions between the two habitats were attributed to(1)improved CO_(2)and bicarbonate consumption in water columns via enhancing photosynthesis and(2)inhibited CO_(2)production by reconstructing the benthic microbial *** eco-advantages were found in planted sediments,such as a high potential of methane oxidation and xenobiotics biodegradation and a low risk of becoming black and *** brief,submerged vegetation is beneficial in promoting pollution removal and carbon retention *** study advances our understanding of the feedback between aquatic metabolism and CO_(2)emission.

关键词： Mitigated CO_(2)emission Submerged vegetation Paired O_(2)-CO_(2)departure Carbon uptake velocity Microbial metabolism pathways The Changjiang River

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Degradation of chloroxylenol by CoS_x activated peroxomonosulfate:Role of cobalt-sulfur ratio

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Chinese Chemical Letters 2025年第4期36卷 379-383页

作者： Jiayi Guo Liangxiong Ling Qinwei Lu Yi Zhou Xubiao Luo Yanbo Zhou State Environmental Protection Key Laboratory of Environmental Risk Assessment and Control on Chemical Process East China University of Science and TechnologyShanghai 200237China School of Life Sciences Key Laboratory of Jiangxi Province for Functional Biology and Pollution Control in Red Soil RegionsJinggangshan UniversityJi'an 343009China State Key Laboratory of Coal Liquification Gasification and Utilization with High Efficiency and Low Carbon TechnologyShanghai 200237China

Cobalt sulfide has received widespread attention in the advanced oxidation treatment of wastewater,and its catalytic activity is infiuenced by crystal structure and exposed active *** work successfully constructed three types of cobalt sulfides,namely Co_(9)S_(8),Co_(3)S_(4)and CoS_(2),by changing the molar ratio of cobalt to *** results showed that the degradation efficiency of Co_(9)S_(8),Co_(3)S_(4)and CoS_(2) on chloroxylenol by activated peroxomonosulfate(PMS)were 100%,88.70%and 67.73%,*** with density functional theory(DFT),the structural properties and reaction energy barriers of different cobaltsulfur ratios were *** the ratio of cobalt to sulfur increases,the sulfur vacancies realized a fuller exposure of active sites(Co_(surf.)^(2+))on the surface of the catalysts,with a highly linear relationship with the reaction rate constant(R^(2)=0.945).This work explores the structure-activity relationship between cobalt sulfur ratio and degradation efficiency,which can guide new catalyst synthesis.

关键词： Peroxymonosulfate Fenton-like reaction Cobalt sulfides Chloroxylenol degradation Morphology control

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