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Linking the environmental loads to the fate of PPCPs in Beijing: Considering both the treated and untreated wastewater sources

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environmental pollution (Barking, Essex : 1987) 2015年 202卷 153-9页

作者： Bin Wang Guohua Dai Shubo Deng Jun Huang Yujue Wang Gang Yu State Key Joint Laboratory of Environmental Simulation and Pollution Control School of Environment Tsinghua University Beijing 100084 China Collaborative Innovation Center for Regional Environmental Quality Tsinghua University Beijing 100084 China Tsinghua-Veolia Joint Research Center for Advanced Environmental Technology Tsinghua University Beijing 100084 China. Electronic address: thuwb@***. Tsinghua-Veolia Joint Research Center for Advanced Environmental Technology Tsinghua University Beijing 100084 China. Collaborative Innovation Center for Regional Environmental Quality Tsinghua University Beijing 100084 China. Beijing Key Laboratory of Emerging Organic Contaminants Tsinghua University Beijing 100084 China.

The environmental loads of pharmaceutical and personal care products (PPCPs) in Beijing were estimated from direct discharge of untreated wastewater and WWTP treated effluent. The annual environmental loads of 15 PPCP components ranged from 16.3 kg (propranolol) to 9.85 tons (caffeine). A fugacity model was developed to successfully estimate the PPCP pollution based on the estimated environmental load. The modeled results approximated the observed PPCP concentrations in Beijing. The untreated wastewater contributed significantly to PPCP pollution in Beijing, ranging from 46% (propranolol) to 99% (caffeine). The total environmental burden of target PPCPs ranged from 0.90 kg (propranolol) to 536 kg (caffeine). water is the most important media for the fate of PPCPs. Monte Carlo-based concentration distributions of PPCPs are consistent with the observed results. The most important way to reduce the PPCP pollution is to both improve wastewater collection rate and adopt deep treatment technologies.

关键词： environmental load Fugacity model Personal care product Pharmaceutical Sensitivity analysis Uncertainty analysis

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The climate opportunities and risks of improving building envelopes across 1,677 Chinese cities

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Cell Reports Sustainability 2024年第12期1卷

作者： Zhang, Yufei Dang, Mengyuan Chu, Chunli Behrens, Paul Berrill, Peter Zhong, Xiaoyang Jing, Rui Lei, Nuoa Jia, Hongyuan Zhang, Lixiao Shao, Chaofeng Masanet, Eric Ju, Meiting Liu, Lirong Chen, Weiqiang Cao, Zhi College of Environmental Science and Engineering Nankai University 38 Tongyan Road Jinnan District Tianjin 300350 China Institute of Environmental Sciences (CML) Leiden University RA Leiden Leiden 2300 Netherlands Oxford Martin School University of Oxford 34 Broad Street Oxford OX1 3BD United Kingdom Sustainability Economics of Human Settlements Technische Universität Berlin Fasanenstr. 88 Berlin 10623 Germany Mercator Research Institute on Global Commons and Climate Change Berlin 10829 Germany International Institute of Applied Systems Analysis (IIASA) Schlossplatz 1 Laxenburg 2361 Austria College of Energy Xiamen University Xiamen 361005 China Energy Technologies Area Lawrence Berkeley National Laboratory Berkeley 94720 CA United States School of Civil Engineering and Architecture Chongqing University of Science and Technology Chongqing 401331 China SinBerBEST Berkeley Education Alliance for Research in Singapore Singapore 138602 Singapore State Key Joint Laboratory of Environmental Simulation and Pollution Control School of Environment Beijing Normal University Beijing 100875 China Bren School of Environmental Science and Management University of California Santa Barbara 93106 CA United States Department of Mechanical Engineering University of California Santa Barbara 93106 CA United States Centre for Environment and Sustainability University of Surrey Guildford GU2 7XH United Kingdom Institute of Urban Environment Chinese Academy of Sciences Xiamen 361021 China

The global building sector consumes approximately 30% of final energy, making it crucial for climate change mitigation and adaptation. International calls for enhancing building energy efficiencies are growing, focusing on strategies such as energy-efficient building envelopes through renovation and replacement of older structures, along with electrification and fuel switching. However, the energy-saving potential of these improvements remains uncertain due to the complex interplay of building stock characteristics and climatic conditions. Here, we diagnose the compound effects of envelope improvements and climate change on China's housing energy demand using a physics-based building energy model with fine spatial and temporal granularity, covering 1,677 sub-province-level cities. Our model shows that envelope improvements play very different roles in ameliorating climate change impacts on housing energy use across the country, highlighting the need for building climate-resilient energy supply and pursuing alternative energy efficiency strategies in less climate-resilient regions. © 2024 The Authors

关键词： building energy building envelopes climate change cooling demand heating demand stock dynamics surrogate modeling

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Effect of adoption of electric vehicles on public health and air pollution in China: a modelling study

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The Lancet Planetary Health 2021年 5卷 S8-S8页

作者： Daniel E Horton Jordan L Schnell Daniel R Peters David C Wong Xi Lu Hao Gao Hongliang Zhang Patrick L Kinney Department of Earth and Planetary Sciences and Institute for Sustainability and Energy Northwestern University Evanston IL USA Cooperative Institute for Research in Environmental Sciences at the University of Colorado Boulder National Oceanic and Atmospheric Administration Global Systems Laboratory Boulder CO USA Program in Environmental Sciences Northwestern University Evanston IL USA Environmental Defense Fund Austin TX USA US Environmental Protection Agency Research Triangle Park NC USA School of Environment State Key Joint Laboratory of Environment Simulation and Pollution Control Tsinghua University Beijing China Beijing China Department of Earth System Science University of California Irvine Irvine CA USA Department of Environmental Science and Engineering Fudan University Shanghai China Department of Environmental Health Boston University School of Public Health Boston MA USA

Background Adoption of electric vehicles has the potential to reduce air pollutant and greenhouse gas emissions, hence China has implemented policies incentivising use of electric vehicles. However, much is unknown about the potential air quality and public health benefits of electric vehicles, including optimal vehicle type prioritisation and the vehicles' ability to reduce acute health impacts due to extreme air quality events. We aimed to assess the potential climate and acute public health benefits of use of electric vehicles during an extreme winter air pollution event. Methods In this modelling study, we used the Weather Research Forecast and Community Multiscale Air Quality Modeling System air quality model to simulate the interplay between weather and atmospheric chemistry. We used this model to examine potential co-benefits of electric vehicle adoption during an extreme pollution episode in China. We simulated heavy-duty and light-duty electric vehicle adoption scenarios, in which 40% of the population adopted a heavy-duty or light-duty passenger electric vehicle, re-mapped battery power needs to energy generation facilities, and characterised differences in public health outcomes using China-specific concentration-response functions. Findings We found that widespread adoption of heavy-duty electric vehicles would reduces nitric oxide and fine particulate matter resulting in 562 (95% CI 410–723) fewer premature acute deaths than the non-electrified baseline scenario. However, widespread adoption of heavy-duty electric vehicles does not reduce carbon dioxide emissions without the addition of emission-free electricity generation. By contrast, widespread adoption of light-duty electric vehicles robustly reduces greenhouse gas emissions, but results in lesser air quality improvements and fewer premature deaths avoided (145 [95% CI 38–333]) than the heavy-duty scenario. Economic effects of human health endpoints and carbon dioxide reductions for adoption of ligh

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Corrigendum to “How urban land-use intensity affected CO 2 emissions at the county level: Influence and prediction” [Ecol. Indic. 145 (2022) 109601]

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Ecological Indicators 2023年 146卷

作者： Chuyu Xia Zhaoyingzi Dong Peng Wu Feng Dong Kai Fang Qiang Li Xiaoshun Li Zhuang Shao Zhenning Yu Faculty of Architecture Civil and Transportation Engineering Beijing University of Technology Beijing 100124 China Key Laboratory of Ocean Space Resource Management Technology MNR Hangzhou Zhejiang 310007 China State Key Joint Laboratory of Environmental Simulation and Pollution Control School of Environment Beijing Normal University Beijing 100875 China School of Public Affairs Zhejiang University Zhejiang 310058 China School of Economics Zhejiang University Hangzhou Zhejiang 310058 China School of Economics and Management China University of Mining and Technology Xuzhou 221116 China Research Center for Transition Development and Rural Revitalization of Resource-based Cities in China China University of Mining and Technology Xuzhou 221116 China School of Landscape Architecture Beijing Forestry University Beijing 100083 China School of Social and Public Administration East China University of Science and Technology Shanghai 200237 China

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Correspondence: Reply to 'Analytical flaws in a continental-scale forest soil microbial diversity study'

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Nature communications 2017年第1期8卷 15583页

作者： Jizhong Zhou Ye Deng Lina Shen Chongqing Wen Qingyun Yan Daliang Ning Yujia Qin Kai Xue Liyou Wu Zhili He James W Voordeckers Joy D Van Nostrand Vanessa Buzzard Sean T Michaletz Brian J Enquist Michael D Weiser Michael Kaspari Robert Waide Yunfeng Yang James H Brown State Key Joint Laboratory of Environment Simulation and Pollution Control School of Environment Tsinghua University Beijing 100084 China. Institute for Environmental Genomics Department of Microbiology and Plant Biology and School of Civil Engineering and Environmental Sciences University of Oklahoma Norman Oklahoma 73019 USA. Earth Science Division Lawrence Berkeley National Laboratory Berkeley California 94270 USA. CAS Key Laboratory for Environmental Biotechnology Research Center for Eco-Environmental Science Chinese Academy of Sciences Beijing 100085 China. Department of Ecology and Evolutionary Biology University of Arizona Tucson Arizona 85721 USA. The Santa Fe Institute 1399 Hyde Park Rd Santa Fe New Mexico 87501 USA. EEB Graduate Program Department of Biology University of Oklahoma Norman Oklahoma 73019 USA. Smithsonian Tropical Research Institute Balboa 0843-03092 Republic of Panama. Department of Biology University of New Mexico Albuquerque New Mexico 87131 USA.

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"what We Breathe Impacts Our Health: Improving Understanding of the Link between Air pollution and Health"

"what We Breathe Impacts Our Health: Improving Understanding...

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作者： West, J. Jason Cohen, Aaron Dentener, Frank Brunekreef, Bert Zhu, Tong Armstrong, Ben Bell, Michelle L. Brauer, Michael Carmichael, Gregory Costa, Dan L. Dockery, Douglas W. Kleeman, Michael Krzyzanowski, Michal Künzli, Nino Liousse, Catherine Lung, Shih-Chun Candice Martin, Randall V. Pöschl, Ulrich Pope, C. Arden Roberts, James M. Russell, Armistead G. Wiedinmyer, Christine Environmental Sciences and Engineering University of North Carolina at Chapel Hill Chapel HillNC27599 United States Health Effects Institute BostonMA02110 United States European Commission Joint Research Centre Institute for Environment and Sustainability IspraI. 21027 Italy Institute for Risk Assessment Sciences Universiteit Utrecht Julius Center for Health Sciences and Primary Care University Medical Center Utrecht Utrecht3584 CJ Netherlands State Key Lab for Environmental Simulation and Pollution Control College of Environmental Science and Engineering Peking University Beijing100871 China Social and Environmental Health Research London School of Hygiene and Tropical Medicine LondonWC1E 7HT United Kingdom School of Forestry and Environmental Studies Yale University New HavenCT06511 United States School of Population and Public Health University of British Columbia VancouverBCV6T 1Z3 Canada Chemical and Biochemical Engineering University of Iowa Iowa CityIA52242 United States Air Climate and Energy Research Program Office of Research and Development Environmental Protection Agency DurhamNC27705 United States Harvard T. H. Chan School of Public Health BostonMA02115 United States Civil and Environmental Engineering University of California at Davis DavisCA95616 United States Environmental Research Group King's College London LondonSE1 9NH United Kingdom Epidemiology and Public Health Swiss Tropical and Public Health Institute Basel Switzerland University of Basel Basel Switzerland Laboratoire d' Aérologie CNRS-Université de Toulouse Toulouse31400 France Research Center for Environmental Changes Academia Sinica Taipei Taiwan Physics and Atmospheric Science Dalhousie University HalifaxNSB3H 4R2 Canada Harvard-Smithsonian Center for Astrophysics CambridgeMA02138 United States Multiphase Chemistry Department Max Planck Institute for Chemistry Mainz55128 Germany Economics Brigham Young University ProvoUT84602 United States Ea

Air pollution contributes to the premature deaths of millions of people each year around the world, and air quality problems are growing in many developing nations. While past policy efforts have succeeded in reducing particulate matter and trace gases in North America and Europe, adverse health effects are found at even these lower levels of air pollution. Future policy actions will benefit from improved understanding of the interactions and health effects of different chemical species and source categories. Achieving this new understanding requires air pollution scientists and engineers to work increasingly closely with health scientists. In particular, research is needed to better understand the chemical and physical properties of complex air pollutant mixtures, and to use new observations provided by satellites, advanced in situ measurement techniques, and distributed micro monitoring networks, coupled with models, to better characterize air pollution exposure for epidemiological and toxicological research, and to better quantify the effects of specific source sectors and mitigation strategies. © 2016 American Chemical Society.

关键词： Health

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Corrigendum to“Optical measurements of dissolved organic matter as proxies for COD_(Mn)and BOD_(5)in plateau lakes”[***.19(2024)100326]

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environmental Science and Ecotechnology 2024年第4期20卷 140-140页

作者： Xuan Yang Yongqiang Zhou Xiaoying Yang Yunlin Zhang Robert G.M.Spencer Justin D.Brookes Erik Jeppesen Hucai Zhang Qichao Zhou Institute for Ecological Research and Pollution Control of Plateau Lakes School of Ecology and Environmental SciencesYunnan UniversityKunming650500China Institute of International River and Eco-security Yunnan UniversityKunming650500China Zhejiang College of Security Technology Wenzhou325016China Taihu Laboratory for Lake Ecosystem Research State Key Laboratory of Lake Science and EnvironmentNanjing Institute of Geography and LimnologyChinese Academy of SciencesNanjing210008China Department of Earth Ocean and Atmospheric ScienceFlorida State UniversityTallahassee32306United States Water Research Centre School of Biological ScienceThe University of AdelaideAdelaide5005Australia Department of Ecoscience Aarhus UniversityAarhus8000Denmark Sino-Danish Centre for Education and Research Chinese Academy of SciencesBeijing100101China Limnology Laboratory Department of Biological Sciences and Centre for Ecosystem Research and ImplementationMiddle East Technical UniversityAnkara06800Turkey Institute of Marine Sciences Middle East Technical UniversityErdemliMersin33731Turkey Yunnan Key Laboratory of Pollution Process and Management of Plateau Lake-Watershed Yunnan Research Academy of Eco-environmental SciencesKunming650034China

The authors regret that the following statements in the original article were wrong and have been *** authors would like to apologise for any inconvenience caused.

关键词： plateau dissolved wrong

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Correction: Emerging per- and polyfluoroalkyl substances (PFAS) in human milk from Sweden and China

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environmental science. Processes & impacts 2021年第1期23卷 188页

作者： Raed Awad Yihui Zhou Elisabeth Nyberg Shahla Namazkar Wu Yongning Qianfen Xiao Yaije Sun Zhiliang Zhu Åke Bergman Jonathan P Benskin Department of Environmental Science (ACES) Stockholm University 106 91 Stockholm Sweden. Raed.Awad@ivl.se Jon.Benskin@aces.su.se and Swedish Environmental Research Institute (IVL) 114 28 Stockholm Sweden. State Key Laboratory of Pollution Control and Resource Reuse College of Environmental Science and Engineering Tongji University Shanghai 200092 China. Department of Contaminants Swedish Environmental Protection Agency Virkesvägen 2 SE-106 48 Stockholm Sweden. Department of Environmental Science (ACES) Stockholm University 106 91 Stockholm Sweden. Raed.Awad@ivl.se Jon.Benskin@aces.su.se. NHC Key Laboratory of Food Safety Risk Assessment China National Center for Food Safety Risk Assessment Beijing 100021 China. Key Laboratory of Yangtze River Water Environment (Ministry of Education) College of Environmental Science and Engineering Tongji University Shanghai 200092 China. Department of Environmental Science (ACES) Stockholm University 106 91 Stockholm Sweden. Raed.Awad@ivl.se Jon.Benskin@aces.su.se and State Key Laboratory of Pollution Control and Resource Reuse College of Environmental Science and Engineering Tongji University Shanghai 200092 China and Department of Science and Technology Örebro University 701 82 Örebro Sweden.

Correction for 'Emerging per- and polyfluoroalkyl substances (PFAS) in human milk from Sweden and China' by Raed Awad et al., Environ. Sci.: Processes Impacts, 2020, 22, 2023-2030, DOI: 10.1039/D0EM00077A.

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Author Correction: Near-real-time monitoring of global CO2 emissions reveals the effects of the COVID-19 pandemic

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Nature communications 2020年第1期11卷 6292页

作者： Zhu Liu Philippe Ciais Zhu Deng Ruixue Lei Steven J Davis Sha Feng Bo Zheng Duo Cui Xinyu Dou Biqing Zhu Rui Guo Piyu Ke Taochun Sun Chenxi Lu Pan He Yuan Wang Xu Yue Yilong Wang Yadong Lei Hao Zhou Zhaonan Cai Yuhui Wu Runtao Guo Tingxuan Han Jinjun Xue Olivier Boucher Eulalie Boucher Frédéric Chevallier Katsumasa Tanaka Yiming Wei Haiwang Zhong Chongqing Kang Ning Zhang Bin Chen Fengming Xi Miaomiao Liu François-Marie Bréon Yonglong Lu Qiang Zhang Dabo Guan Peng Gong Daniel M Kammen Kebin He Hans Joachim Schellnhuber Department of Earth System Science Tsinghua University Beijing China. zhuliu@***. Laboratoire des Sciences du Climat et de l'Environnement LSCE CEA CNRS UVSQ Centre d'Etudes Orme de Merisiers Gif-sur-Yvette France. Department of Earth System Science Tsinghua University Beijing China. Department of Meteorology and Atmospheric Science The Pennsylvania State University University Park PA USA. Department of Earth System Science University of California Irvine 3232Croul Hall Irvine CA USA. Division of Geological and Planetary Sciences California Institute of Technology Pasadena CA USA. Jet Propulsion Laboratory California Institute of Technology Pasadena CA USA. Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control Collaborative Innovation Center of Atmospheric Environment and Equipment Technology School of Environmental Science and Engineering Nanjing University of Information Science and Technology Nanjing China. Key Laboratory of Land Surface Pattern and Simulation Institute of Geographical Sciences and Natural Resources Research Chinese Academy of Sciences Beijing China. Climate Change Research Center Institute of Atmospheric Physics Chinese Academy of Sciences Beijing China. Key Laboratory of Middle Atmosphere and Global Environment Observation Institute of Atmospheric Physics Chinese Academy of Sciences Beijing China. School of Environment Tsinghua University Beijing China. School of Mathematical School Tsinghua University Beijing China. Department of Mathematical Sciences Tsinghua University Beijing China. Center of Hubei Cooperative Innovation for Emissions Trading System Wuhan China. Faculty of Management and Economics Kunming University of Science and Technology 13 Kunming China. Economic Research Centre of Nagoya University Furo-cho Chikusa-ku Nagoya Japan. Institut Pierre-Simon Laplace Sorbonne Université/CNRS Paris France. Université Paris Dauphine Place du Maréchal de Lattre de Tassigny 75016 Paris France.

A Correction to this paper has been published: https://***/10.1038/s41467-020-20254-5.

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Urea/Thiourea Imine Linkages Provide Accessible Holes in Flexible Covalent Organic Frameworks and Dominates Self-Adaptivity and Exciton Dissociation

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Angewandte Chemie 2024年第7期137卷

作者： Chencheng Qin Prof. Xiaodong Wu Wenyan Zhou Miao Li Prof. Shuai Bi Prof. Lin Tang Dr. Hao Huang Prof. Wenguang Tu Prof. Xingzhong Yuan Prof. Edison Huixiang Ang Prof. Weiling Sun Long Chen Zhaoli Liu Prof. Bing He Prof. Lai Lyu Prof. Yan Wu Prof. Wen Liu Prof. Hou Wang College of Environmental Science and Engineering and Key Laboratory of Environmental Biology and Pollution Control (Ministry of Education) Hunan University Changsha 410082 China These authors equally contributed this work College of Materials Science and Engineering Nanjing Tech University Nanjing 211816 China School of Chemistry Chemical Engineering and Biotechnology Nanyang Technological University 21 Nanyang Link Singapore 637371 Singapore School of Science and Engineering The Chinese University of Hong Kong Shenzhen 518172 Guangdong P. R. China Natural Sciences and Science Education National Institute of Education Nanyang Technological University Singapore 637616 Singapore The Key Laboratory of Water and Sediment Sciences Ministry of Education College of Environmental Sciences and Engineering Peking University Beijing 100871 China State Key Laboratory of New Textile Materials and Advanced Processing Technologies Wuhan Textile University 430200 Wuhan China Institute of Rural Revitalization Guangzhou University Guangzhou 510006 China College of Environment and Ecology Hunan Agricultural University Changsha 410128 P. R China National Laboratory for Molecular Sciences Peking University Beijing 100871 China

Unraveling the robust self-adaptivity and minimal energy-dissipation of soft reticular materials for environmental catalysis presents a compelling yet unexplored avenue. Herein, a top-down strategy, tailoring from the unique linkage basis, flexibility degree, skeleton electronics to trace-guest adaptability, is proposed to fill the understanding gap between micro-soft covalent organic frameworks (COFs) and photocatalytic performance. The thio(urea)-basis-dominated linkage within benzotrithiophene-based COFs induce the framework contraction/swelling (intralayer micro-flexibility) in response to tetrahydrofuran or water. Adaptability of micro-flexible thiourea-COF with pore hydrophilicity not only contributes to the favorable mass transfer, but also enhances the accessible redox active sites, culminating in nearly 100 % removal of micropollutant with low-energy dissipation in wastewater. The incorporating urea/thiourea into imine linkage facilitates polarization reduction and exciton dissociation within skeleton wall, inducing strong localization for holes. This transformation facilitates interchain charge transport and unbalanced distribution conducive to oxidative holes-mediated micropollutant decomposition.

关键词： micro-flexible COFs conformation photocatalysis self-adaptivity

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