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Environmental Chemistry and Ecotoxicology 2025年 7卷 1142-1157页

作者： Zhang, Jia Li, Dan Yuan, Ying Hui, Kunlong Tan, Wenbing State Key Laboratory of Environmental Criteria and Risk Assessment State Environmental Protection Key Laboratory of Simulation and Control of Groundwater Pollution Chinese Research Academy of Environmental Sciences Beijing100012 China

Brominated flame retardants (BFRs) have become significant contaminants of emerging concern (CECs), resulting in detrimental effects on soil health, human health, and ecosystem sustainability. Their environmental impacts have spurred extensive research into environmental chemistry and ecotoxicology. Despite the widespread detection of both BFRs and Novel Brominated Flame Retardants (NBFRs) in soils, there are few assessments of the environmental behavior and fate of the BFRs. Therefore, this review comprehensively identifies the sources, distribution, transport, transformation, ecotoxicological effects, and remediation strategies of BFRs in soils. Principal findings indicate that adsorption-desorption, mostly influenced by soil organic matter, controls the mobility and transformation of BFRs. Photolysis dominates surface soils, while aerobic and anaerobic biodegradation predominate in subsurface layers. The main factors influencing the bioavailability of BFRs are shed light on in this review. These factors such as the physicochemical properties of BFRs, soil characteristics, and combined pollution are specifically discussed. Moreover, the development, physiological, and biochemical responses of soil organisms to exposure to the BFRs are summarized. Single strategies for addressing BFRs have certain limitations. Urgent actions are needed to focus on environmental behavior and remediation strategies under the "One Health" framework to enrich research gap areas of BFRs, NBFRs, and transformation products. © 2024

关键词： Soil pollution

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state Estimation of Drive-by-Wire Chassis Vehicle Based on Dual Unscented Particle Filter Algorithm

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Chinese Journal of Mechanical Engineering 2024年第1期37卷 99-113页

作者： Zixu Wang Chaoning Chen Quan Jiang Hongyu Zheng Chuyo Kaku State Key Laboratory of Automotive Simulation and Control Jilin UniversityChangchun 130022China Jiangsu Chaoli Electric Co.Ltd. Zhenjiang 212321China

Accurate vehicle dynamic information plays an important role in vehicle driving ***,due to the characteristics of high mobility and multiple controllable degrees of freedom of drive-by-wire chassis vehicles,the current mature application of traditional vehicle state estimation algorithms can not meet the requirements of drive-by-wire chassis vehicle state *** paper proposes a state estimation method for drive-by-wire chassis vehicle based on the dual unscented particle filter algorithm,which make full use of the known advantages of the four-wheel drive torque and steer angle parameters of the drive-by-wire chassis *** the dual unscented particle filter algorithm,two unscented particle filter transfer information to each other,observe the vehicle state information and the tire force parameter information of the four wheels respectively,which reduce the influence of parameter uncertainty and model parameter changes on the estimation accuracy during *** performance with the dual unscented particle filter algorithm,which is analyzed in terms of the time-average square error,is superior of the unscented Kalman filter *** effectiveness of the algorithm is further verified by driving simulator *** this paper,a vehicle state estimator based on dual unscented particle filter algorithm was proposed for the first time to improve the estimation accuracy of vehicle parameters and states.

关键词： Drive-by-wire chassis vehicle Vehicle state estimation Dual unscented particle filter Tire force estimation Unscented particle filter

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Chemodiversity of soil dissolved organic matter affected by contrasting microplastics from different types of polymers

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Frontiers of Environmental Science & Engineering 2023年第12期17卷 149-162页

作者： Hong Yu Beidou Xi Lingling Shi Wenbing Tan State Key Laboratory of Environmental Criteria and Risk Assessment and State Environmental Protection Key Laboratory of Simulation and Control of Groundwater PollutionChinese Research Academy of Environmental SciencesBeijing 100012China

Chemodiversity of dissolved organic matter(DOM)is a crucial factor controlling soil nutrient availability,greenhouse gas emissions,and pollutant ***(MPs)are widespread pollutants in terrestrial ecosystems in many ***,the effects of MPs on DOM chemodiversity are not sufficiently understood,particularly under different types of *** UV-Vis spectroscopy,3D fluorescence spectroscopy,and Fourier-transform ion cyclotron resonance mass spectrometry,the effects of three prevalent MPs[polyethylene,polystyrene,and polyvinyl chloride(PVC)]on the chemical properties and composition of soil DOM were investigated via a 310-d soil incubation *** results showed that MPs reduced the aromatic and hydrophobic soil DOM components by more than 20%,with PVC MPs having the greatest ***,as MP contents increase,the humification level of soil DOM significantly *** increased DOM molecules with no heteroatom by 8.3%-14.0%,but decreased DOM molecules with nitrogen content by 17.0%-47.8%.This may be because MPs cause positive“priming effect,”resulting in the breakdown of bioavailable components in soil *** is also related to MPs changing microbial richness and diversity and enriching microbial communities involved in lignin compositions *** the presence of MPs,soil DOM chemodiversity depended on soil pH,electrical conductivity,dissolved organic carbon,soil organic matter,bacterial Shannon,and fungal Chao ***,DOM in MP-contaminated soils featured more lipids and less condensed aromatics and proteins/amino sugars,thereby conferring a lower DOM aromaticity and higher lability.

关键词： Microplastics Dissolved organic matter FT-ICR MS Chemodiversity Molecular signature

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Fabrication of MnO2 coating on aluminum honeycomb for fast catalytic decomposition of ozone at room temperature

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Journal of Environmental Sciences 2023年第12期134卷 34-43页

作者： Yunjuan He Pengyi Zhang Jie Yang Shan Wang Jinge Li State Key Joint Laboratory of Environment Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing 100084China Beijing Key Laboratory for Indoor Air Quality Evaluation and Control Beijing 100084China

Herein, the coating of MnO2nanomaterials on the surface of aluminum honeycomb was carried out to meet the requirements of high air velocity, low pressure drop and high activity in ozone removal scenarios. A commercially readily available waterborne silica sol mixed with waterborne acrylate latex was creatively utilized as the binder. A series of coating samples were prepared by spray coating method and evaluated focusing on their adhesion strength and catalytic activity towards ozone decomposition in an air duct at room temperature, by varying MnO2/binder mass ratio and number of sprayings. It was found that the adhesion strength of the catalytic coatings on the aluminum honeycomb increased with the increase of binder mass ratio, but the increased binder made the catalyst particles closely packed,resulting in reduced exposure of active sites and decrease of ozone conversion. Accordingly,catalyst slurry with 81.8 wt.% MnO2in dry coating and spraying times of two were determined as the optimal process parameters. As-prepared aluminum honeycomb filter with MnO2layer of 50 μm thickness achieved ozone conversion of 29.3%±1.7% under conditions of air velocity 3.0 m/sec, relative humidity50%, room temperature(26°C) and initial ozone concentration of 200 ppbV. This filter can be well adaptable to indoor air purification equipment operating at high air velocity with low wind resistance.

关键词： Manganese dioxide Waterborne binder Coating Ozone conversion Catalyst

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Application of Omega vortex identification method in cavity buffeting noise

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Journal of Hydrodynamics 2021年第2期33卷 259-270页

作者： Yang-hui Zhang Xing-jun Hu Wei Lan Yi-chen Liu Mo Wang Jing-yu Wang State Key Laboratory of Automobile Simulation and Control Jilin UniversityChangchun 130025China

The cavity buffeting noise is related to the free shear layer oscillation and the periodic vortex shedding,where weak vortices coexist with strong vortices and the strong shear phenomenon also exists at the opening of the ***,it is of great significance to accurately capture vortices at the opening for the control of the cavity buffeting *** paper first compares the Omega vortex identification method with the Q andλ2criteria based on the large eddy simulation(LES)of the backward-facing step flow,and it is found that the Omega method enjoys the following advantages:it is not sensitive to a moderate threshold change andΩ=0.52 can be used as a fixed threshold,it can capture both the strong and weak vortices at the same time;and it will not be contaminated by the *** the Omega(Ω)method is applied to the LES of the cavity buffeting noise:the mechanism of the cavity buffeting noise is studied based on a simple cavity model firstly,and then the effects of the incoming boundary layer thicknesses and the incoming boundary layer shapes on the cavity buffeting noise are *** results show that:theΩmethod clearly captures the processes of the vortex generation,development,collision and fragmentation,verifying that the generation of the cavity buffeting noise is related to the free shear layer oscillation and the periodic vortex shedding;as the thickness of the incoming boundary layer increases,the free shear layer becomes more stable and the Helmholtz resonance is avoided effectively,thereby the cavity buffeting noise is reduced effectively,adding a convexity upstream of the cavity opening to interfere the shape of the incoming boundary layer to reduce the acoustic feedback effect can reduce the cavity buffeting noise effectively.

关键词： Vortex identification Omega(Ω) buffeting noise boundary layer

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simulation Research on Dynamic Characteristics of Hydraulic Mount

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Chinese Journal of Mechanical Engineering 2021年第3期34卷 336-344页

作者： Yanhua Liu Xin Guan Pingping Lu Rui Guo State Key Laboratory of Automobile Simulation and Control Jilin UniversityChangchun 130022China

At present,research on hydraulic mounts has mainly focused on the prediction of the dynamic stiffness and loss *** to the traditional finite element analysis method,the programming method can be used to analyze hydraulic mounts for a rapid and accurate understanding of the influence of the different mounting parameters on the dynamic stiffness and loss *** aims of this study were to investigate the nonlinear dynamic characteristics of a hydraulic mount,and to identify the parameters that affect the dynamic stiffness and loss angle using MATLAB software programs to obtain the influence curves of the parameters,so as to use suitable parameters as the basis for vibration analysis.A nonlinear mechanical model of a hydraulic mount was established according to the basic principles of fluid *** dynamic stiffness and loss angle of the dimensionless expression were proposed.A numerical calculation method for the dynamic performance evaluation index of the hydraulic mount was derived.A one-to-one correspondence was established between the structural parameters and peak frequency of the evaluation *** accuracy and applicability of the mechanical model were verified by the test *** results demonstrated the accuracy of the nonlinear mechanical model of the hydraulic mount,and the vehicle driving comfort was greatly improved by the optimization of the structural parameters.

关键词： Hydraulic mount Vibration analysis Dynamic characteristics Calculation method

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Research on key Issues of Consistency Analysis of Vehicle Steering Characteristics

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Chinese Journal of Mechanical Engineering 2021年第2期34卷 123-134页

作者： Yanhua Liu Xin Guan Pingping Lu Rui Guo State Key laboratory of Automobile Simulation and Control Jilin UniversityChangchun 200240China

Given the global lack of effective analysis methods for the impact of design parameter tolerance on performance deviation in the vehicle proof-of-concept stage,it is difficult to decompose performance tolerance to design parameter *** study proposes a set of consistency analysis methods for vehicle steering *** process of consistency analysis and control of automotive performance in the conceptual design phase is proposed for the first time.A vehicle dynamics model is constructed,and the multi-objective optimization software Isight is used to optimize the steering performance of the *** analysis is used to optimize the design performance *** tolerance interval of the performance is obtained by comparing the original car performance value with the optimized *** the help of layer-by-layer decomposition theory and interval mathematics,automotive performance tolerance has been decomposed into design parameter *** simulation and real vehicle experiments,the validity of the consistency analysis and control method presented in this paper are *** decomposition from parameter tolerance to performance tolerance can be achieved at the conceptual design stage.

关键词： Interval mathematical theory Layer by layer decomposition theory Consistency of performance Multi-objective optimization

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Sludge-based biochar adsorbent:pore tuning mechanisms,challenges,and role in carbon sequestration

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Biochar 2023年第1期5卷 1419-1441页

作者： Md Manik Mian Wenya Ao Shubo Deng State Key Joint Laboratory of Environment Simulation and Pollution Control(SKLESPC) Beijing Key Laboratory for Emerging Organic Contaminants ControlSchool of EnvironmentTsinghua UniversityBeijing 100084China

Sludge biochar,a carbonized product of raw sludge,contains porous architectures that can act as epicenters for adsorbing external molecules through physical or chemical *** biochar also immobilizes innate micropollutants,which is advantageous over conventional sludge disposal *** date,numerous strategies have been discovered to improve sludge biochar morphology,but the influential factors,pore tuning mechanisms,and process feasibility remain *** knowledge gap limits our ability to design a robust sludge-based ***,we present state-of-the-art sludge biochar synthesis methods with insight into structural and chemical transformation *** and novel concepts for improving sludge biochar porous architecture are *** the first time,sludge biochar properties,adsorption performances,and techno-economic perspectives were compared with commercial activated carbon(AC)to reveal the precise challenges in sludge biochar *** importantly,sludge biochar role in carbon sequestration is detailed to demonstrate the environmental significance of this ***,the review concludes with an overview of prospects and an outlook for developing sludge biochar-based research.

关键词： Sludge-based adsorbent Micropores Feasible methods Challenges Carbon sequestration

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Real-world identification of high-emitting vehicles based on near-road sensor measurement

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Frontiers of Environmental Science & Engineering 2025年第5期19卷 81-96页

作者： Bo Li Dongbin Wang Qiang Zhang Leqi Shi Mingliang Fu Hang Yin Jingkun Jiang State Key Joint Laboratory of Environment Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing 100084China Vehicle Emission Control Center Chinese Research Academy of Environmental SciencesBeijing 100012China

A small fraction of high-emitting vehicles make disproportionally large contributions to total fleet *** identifying high emitters under real driving conditions is *** this study,two portable sensor platforms for high-emitter identification were used for online roadside measurements of vehicle-emitted NO,particle number(PN),and CO_(2) concentrations in Tangshan and Chengdu,*** measured mean concentrations of vehicle-emitted NO,PN,and CO_(2) in Tangshan and Chengdu were 27.7-32.9 ppb,5.4×10^(3)-8.2×10^(3)#/cm^(3),and 7.3-8.2 ppm,*** on more than one month of second-by-second measured pollutant concentrations and passed vehicle information,a scheme was developed to identify high *** the 217000 and 43000 vehicles that passed the roadside sensor platforms at Tangshan and Chengdu,approximately 60%and 73%of vehicle exhaust plumes were successfully detected using the sensor *** NO and PN emission factors(EFs)tended to have log-normal distributions with the median values of 14.3 g/kg-fuel and 1.3×10^(15)#/kg-fuel,*** general,the percentages of high-emitters identified at the Tangshan and Chengdu sites were 8.7% and 12.2% of the total identified vehicles,*** these high-emitters,122 vehicles were randomly inspected on-site with the assistance of traffic officers,and the rate of correct identification was approximately 95%,which demonstrates that our methodology performs well in identifying real-world ***,its low cost,good mobility,strong adaptability,and high correct identification rate make this roadside sensor platform a promising approach for real-world high-emitter identification.

关键词： Real world High-emitter identification Roadside sensor measurement Nitrogen oxide Particle number

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Experimental Study on Impingement Processes of Fuel Sprays on Biomimetic Structured Surfaces

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Journal of Bionic Engineering 2024年第1期21卷 362-373页

作者： Yanling Chen Liang Guo Wanchen Sun Yuying Yan Rong Xuan Junfeng Zhang State Key Laboratory of Automotive Simulation and Control Jilin UniversityChangchun 130025China Faculty of Engineering University of NottinghamNottingham NG72RDUK

To improve the controllability of the wall-wetting process after the fuel spray-wall impingement in internal combustion engines,the methods of laser etching,chemical etching and surface free energy modification are used to prepare biomimetic structured surfaces with different *** impingement processes of diesel and n-butanol sprays on the walls under different conditions are experimentally *** the surface oleophilicity increases,the spreading radius of wall-impinging sprays *** about 5 s after the fuel injections,the fuel spray droplets hit the walls for the first time,and the secondary breakup and rebound *** mixture concentrations of different fuels hitting the various walls reach the peak *** a higher surface temperature,the peak value of the mixture concentration is mainly related to the heat flux to the fuel droplets in different boiling regimes from the metal *** concentration of the air–fuel mixture in the near wall region increases with increasing surface oleophilicity,increasing wall temperature and decreasing ambient *** with diesel,n-butanol presents a higher air–fuel mixture concentration in the near wall region.

关键词： Spray-wall impingement Morphological development Air-fuel mixture concentration Surface wettability Wall temperature:Ambient pressure

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