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Experimental Study on Supported MnO2-Based Catalysts for No Oxidation

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SSRN 2022年

作者： Wang, Denghui Li, Hui Wu, Feng Hui, Shien State Key Laboratory of Multiphase Flow in Power Engineering School of Energy and Power Engineering Xi’an Jiaotong University No. 28 Xianning West Rd. Xi’an710049 China

The selective catalytic oxidation (SCO) of NO in the flue gas to easily soluble NO2 has received extensive attention. In this paper, a single-phase supported MnO2/Al2O3 catalyst and Ce-doped MnCe/Al catalyst system were used for the NO-SCO experiment with MnO2 as the main active component. Combined with XRD, BET, XPS, SEM, O2-TPD, and H2-TPR characterization methods, the physicochemical state of the catalyst surface was analyzed. Furthermore, the effect of loading and Ce doping on active oxygen species and the important factors related to catalyst activity was revealed. The MnO2 catalyst obtained the best activity at 300 °C, corresponding to a NO conversion rate of 79.4%. After MnO2 was loaded on the γ-Al2O3, the activity of the Mn/Al catalysts was not as good as that of the MnO2 catalyst, and the temperature window of Mn/Al shifted to the high-temperature region with the increase of the loading ratio. The relative content of adsorbed oxygen Oα of Mn/Al catalysts was lower than that of MnO2, resulting in poor activity. Ce-doped Mn0.23Ce0.023/Al catalysts exhibited good low-temperature activity. The introduction of the Ce element enhanced the dispersion of Mn species on the catalyst surface, the relative content of surface adsorbed oxygen Oα increased, and the low-temperature activity and mobility of surface oxygen species were enhanced. The Mn0.23Ce0.023/Al catalyst was endowed with both a high specific surface area and good pore structure, as well as a large oxygen storage capacity and excellent surface oxygen species. © 2022, The Authors. All rights reserved.

关键词： Manganese oxide

Thermodynamics analyses on a novel CHP system integrated with multi-grade thermal energy storage

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Journal of Energy Storage 2025年 106卷

作者： Liu, Rongtang Zhang, Kezhen Qin, Yuanzhi Wan, Kaidi Xu, Can Liu, Ming Ningbo Institute of Technology Beihang University Ningbo315800 China Xi'an Thermal Power Research Institute Co. Ltd. Xi'an710054 China State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an710049 China Dongfang Boiler Co. Ltd. of Dongfang Electric Group Chengdu611731 China

The high penetration level of intermittent renewable power necessitates the crucial requirement for combined heat and power systems to possess both high efficiency and flexibility. However, the heat-controlled operation modes of traditional combined heat and power systems impose limitations on their efficiency and flexibility. Therefore, it is of great significance to develop a heat-power decoupling technology that exhibits exceptional efficiency and flexibility. A novel combined heat and power system integrated with multi-grade thermal energy storage is proposed in this study. Thermodynamic analysis models of all operational conditions are developed, and the comprehensive characteristics of efficiency and operational flexibility for the proposed system are assessed by taking a 330 MW system as an example. Results show that the proposed system can decrease/increase 16.05 MW/30.96 MW power loads comparing with the reference system during the charging/discharging periods under the design condition. Energy efficiency of the proposed system can reach 49.40 %, which is improved by 1.66 percentage points. Exergy analysis reveals the exergy destruction order for the proposed system, and shows that the combustion and heat transfer in the boiler are the major process of exergy dissipation. Moreover, operation strategies of the proposed system during charging-discharging cycle are explored and formulated under off-design condition, suggesting that thermodynamic performances of the novel system under various conditions even extreme conditions exhibits exceptional properties. The maximum heat load of the proposed system can be improved by 46.78 % comparing with the reference system, and the maximum improvement of power load capacity during charging-discharging cycle is 14.58 percentage points. This study provides a promising approach for multi-grade thermal energy storage to improve the comprehensive characteristics of combined heat and power systems. © 2024

关键词： Charge storage

Effect of Fuel System on the Heat Releasing Method and flow-Path Design of Rocket-Based Combined Cycle Engine

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Effect of Fuel System on the Heat Releasing Method and Flow-...

International Conference on Mechanical and Aerospace engineering (ICMAE)

作者： Xiao Liu Yinhu Wang Yiyan Yang Lei Shi Dekun Yan State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xi’an China Beijing Institute of Long March Vehicle Beijing China Science and Technology on Combustion Internal Flow and Thermal-structure Laboratory Northwestern Polytechnical University Xi’an China

Multi-components rocket-based combined cycle (RBCC) engine is widely applied in most two-stage-to-orbit program due to stable operation performance under variable flight conditions. Present researches numerically compared RBCC’s performance under ramjet mode and scramjet mode, respectively, by using two fuel system, hydrogen and kerosene together with a $\mathrm{k}-\omega$ SST turbulence model. Researches showed that the combustor area ratio should be increased to keep stable pressure difference balance between inflow and flame because of higher caloric value using hydrogen. Distributed heat addition method is benifit for overall performance improvement when using hydrogen. Different from using kerosene, head should be delayedly added in combustor downtream under scramjet mode. Moreover, the advanced heat addition amount should be decreased under ramjet mode to ensure effective isolator operation.

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Prediction of Pressure Drop in Heavy Oil-Water Ring Two-Phase flow Based on Modified Two-Fluid Model

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SSRN 2024年

作者： Fu, Jiqiang Du, Mingjun Jing, Jiaqiang Sun, Jie Liu, Huichao Chen, Yongjiu State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xi’an710049 China China Petroleum Engineering & Construction Corp North Company Heibei Renqiu062552 China School of Oil & Natural Gas Engineering Southwest Petroleum University Sichuan Chengdu610500 China

Accurate prediction of pressure drop of the heavy oil-water ring flow in pipeline is of great significance for establishing an optimal drag reduction model and ensuring safe production. The effects of different factors on the flow pattern and pressure drop of heavy oil-water annular two-phase flow were systematically analyzed, and a standard two-fluid pressure drop prediction model for annular flow was established. By modifying the shear stress equation of oil-water interface and introducing the wave-flow theory to modify the shear stress equation of water wall, a pressure drop prediction model for the generalized concentric water ring was obtained to calculate the periodic fluctuations of oil phase. Furthermore, by introducing the comprehensive Reynolds number expression of eccentric water ring, the pressure drop prediction model for the generalized eccentric water ring was obtained to calculate the periodic fluctuations of oil phase. The results show that the pressure drop prediction accuracy of the concentric water ring for ultra-heavy oil is improved by 80 % by using the modified pressure drop prediction model. The comprehensive Reynolds number expression of eccentric water ring can effectively reflect the influence of eccentric effect on shear stress of water wall and the calculation error is less than 20 % by predicting the pressure drop of the generalized eccentric water ring with different density differences. © 2024, The Authors. All rights reserved.

关键词： Two phase flow

Multi-Objective Optimization and Configurations Comparison of Closed-Air Brayton Cycle

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SSRN 2023年

作者： Qian, Yiran Gu, Zhenzhen Song, Meihui Yang, Yi Zhao, Quanbin Chen, Weixiong Yan, Junjie State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xi’an710049 China China Institute of Atomic Energy P.O. Box 275-32 Beijing102413 China

Microreactor power system has characteristics of efficient, compact and high environmental adaptability. In this study, closed-air Brayton cycle (CABC) is proposed as the microreactor thermoelectric conversion system, and thermodynamic model of CABC with different configurations are established. The cycle parameters and component’s structure are designed using system-component combined design method. To obtained the optimal system design scheme, the Genetic Algorithm (GA) and the Non-dominated Sorting Genetic Algorithm II (NSGA-II) are separately applied for single-objective optimization and multi-objective optimization. According to multi-objective optimization results, the IRRC has the highest cycle efficiency of 35.4% and the ratio of power to mass of 59.1 kW·t-1 , respectively, and the RRC has the highest power density of 179.6 kW·m-3 . Similar performance with IRRC and simpler structure make the RRC the optimal configuration of CABC. Compared with single-objective optimization, the design results of multi-objective optimization are more balanced in terms of three performance indicators, meaning that the optimized design scheme has a better comprehensive performance. © 2023, The Authors. All rights reserved.

关键词： Multiobjective optimization

Transient Cooling Performance of R134a Flash-Evaporation Spray Enhanced by Cold Air Jet: A Novel Heat Transfer Enhancement Method in Laser Dermatology

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SSRN 2022年

作者： Li, Bufa Wang, Junfeng Tian, Jiameng Chen, Bin Xu, Haojie School of Energy and Power Engineering Jiangsu University Zhenjiang212013 China State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Shaanxi Xi’an710049 China

Nevus of Ota is a dermal hyperplastic pigmented disease with a morbidity rate of 0.1%–0.6% in the Asian population. Laser surgery with the assistance of cryogen spray cooling (CSC) is a potential clinical treatment for nevus of Ota. However, for Asians with high melanin content, it is necessary to enhance cooling capability without the increment of refrigerant amount. In this study, a R134a flash-evaporation cryogen spray cooling coupled with cold air jet (CSC-CAJ) was developed to improve the cooling capacity. Epoxy resin was employed as a skin phantom to investigate the heat transfer characteristics of CSC-CAJ with different air jet parameters. Air jet parameters of CSC-CAJ are recommended to be T a = -7 °C, V a = 3 m 3 /h Z a = 10 mm and Φ a = 30°. Compared to CSC, CSC-CAJ could reduce the minimum surface temperature from -39 °C to -42.1 °C, and the average value of convection heat transfer coefficient ( h ) of CSC-CAJ could increase from 8 W/(m 2 ·k) to 12.9 W/(m 2 ·k) or 61.3% for the recommended parameters. The liquid film residence time ( τ ) decreases from 301 ms to 234 ms or 23.3%. In addition, based on the visualization observation and surface heat transfer measurement, the frost formation phenomenon on the surface and the heat transfer enhancement mechanisms are well understood. Four modes, including Leidonfrost mode, no runoff mode, runoff mode and evaporation mode, are proposed to describe the four stages of CSC-CAJ. A non-dimensional correlation of normalized Nusselt number ( Nu *) and time ( t *) is summarized. The primary heat transfer enhancement mechanism of CSC-CAJ is found to be the increase in cryogen evaporation rate and the ratio of heat removal from the phantom surface to phase change latent heat. © 2022, The Authors. All rights reserved.

关键词： Evaporation

Dynamic simulation of coal-fired power plant integrated with trough solar collector operating in parallel with high pressure heaters

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Dynamic simulation of coal-fired power plant integrated with...

2019 Canadian Society for Civil engineering Annual Conference, CSCE 2019

作者： Yan, Hui Li, Xin Liu, Ming Chong, Daotong Yan, Junjie State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an China

ISBN: (纸本)9780791883747

Solar-aided coal-fired power plant (SACFPP) is a costeffective approach to overcome solar energy intermittency. SACFPPs frequently operate in dynamic processes due to power load and solar energy fluctuations. This study investigated the dynamic characteristics of SACFPPs;such characteristics are important for flexibility evaluation and control system design. The SACFPP used in this study was based on a 660 MW coalfired power plant, and a trough collector system (TCS) operates in parallel with high pressure (HP) heaters. After model development and validation, the dynamic performance of the SACFPP was analyzed under four load ratios of power plant, with disturbances of two parameters: direct normal irradiance (DNI) and mass flowrate ratio to TCS. The performance was also compared with three parallel TCS connection modes. Results showed that the magnitude and response time for power variation under DNI disturbance increased with load ratio. With 500 W/m2 DNI step increments, power increased by approximately 18.4, 21.2, 24.7, and 29.8 MW in 2200, 2330, 2550 and 2620 s at 70%, 80%, 90%, and 100% load ratios, respectively, when all the HP heaters were replaced. The serial number and the number of HP heaters replaced also increased the power variation and response time. Under mass flowrate ratio to TCS increase disturbance, the power rapidly changed to its maximum and then slowly decreased, but the variation value depended on the load ratio. Copyright © 2020 ASME.

关键词： Coal fired power plant

Characteristics of Bubble Dynamic Behavior on the Surface of Photoelectrode Under the Influence of a Vertical Magnetic Field

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SSRN 2023年

作者： Feng, Yuyang Wang, Yechun Zhang, Bo Cao, Zhenshan Liu, Miaomiao Zhen, Canghao Guo, Liejin State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xi’an710049 China Xinjin Weihua Institute of Clean Energy Research Nanhai District Guangdong Province Foshan City China

The magnetohydrodynamic (MHD) flow around the bubble induced by the Lorentz force owing to the applied magnetic field significantly affects the behavioral characteristics of the bubble on the electrode surface. However, the mechanism of the impact of a magnetic field perpendicular to the electrode on the dynamic behavior of bubbles remains unclear. In this study, the evolution law of a single oxygen bubble on the surface of a TiO2 photoelectrode under the influence of a vertical magnetic field with different magnetic induction intensities was investigated. The vertical magnetic field effectively promoted the rapid detachment of bubbles from the electrode surface, and greatly improved the gas evolution efficiency. The mass transfer was dominated by single-phase free convection during bubble evolution. Under the influence of the vertical magnetic field, the mass transfer coefficient near the electrode was enhanced, and the adverse effects of bubbles on mass transfer were counteracted when they entered the reaction-controlled growth phase. The further multiphysics simulation found that the MHD convection decreased the local supersaturation of reaction product oxygen molecules near the electrode, thereby reducing concentration overpotential and increasing the reaction rate. This study provides an experimental and theoretical basis for promoting the bubble detachment and the reaction rate on the gas evolving electrode surface during photoelectrochemical water splitting. © 2023, The Authors. All rights reserved.

关键词： Efficiency

Experimental Study on the flow Characteristics of a Plate with a Mechanically Choked Orifice

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Fluid Dynamics & Materials Processing 2021年第1期17卷 97-107页

作者： Ming Liu Xingkai Zhang Dong Wang State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong UniversityXi’an710049China Petroleum Engineering Technology Research Institute of Shengli Oilfield Company SINOPECDongying257000China Shandong Key Laboratory of Heavy Oil Production Technology Shengli Oilfield CompanySINOPECDongying257000China Petroleum Engineering College Yangtze UniversityWuhan430100China

The mechanically choked orifice plate (MCOP) is a new type of device for flow control by which choking conditionsfor incompressible fluids can be obtained with relatively small pressure losses. Given the lack of relevant results anddata in the literature, in the present study, we concentrate on the experimental determination of the flow coefficientfor the annular orifice, the pressure distribution in the MCOP, and the characteristics of the choked flow itself. Asconfirmed by the experimental results, the Reynolds number, the orifice plate thickness, the plug taper, and theeccentricity have an obvious influence on the aforementioned flow coefficient. The pressure drop in the MCOPis mainly generated near the orifice plate, and the pressure upstream of the orifice plate is slightly reduced in theflow direction, while the pressure downstream of the orifice plate displays a recovery trend. The choked flow rateof the MCOP can be adjusted by replacing the spring with a maximum flow control deviation of 4.91%.

关键词： Mechanical choked orifice plate flow control flow coefficient flow characteristics