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Regulating crystallization and retarding oxidation in Sn-Pb perovskite via 1D cation engineering for high performance all-perovskite tandem solar cells

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Journal of Energy Chemistry 2025年第1期100卷 646-652页

作者： Ranran Liu Xin Zheng Zaiwei Wang Miaomiao Zeng Chunxiang Lan Shaomin Yang Shangzhi Li Awen Wang Min Li Jing Guo Xuefei Weng Yaoguang Rong Xiong Li Michael Grätzel Center for Mesoscopic Solar Cells Wuhan National Laboratory for OptoelectronicsHuazhong University of Science and TechnologyWuhan 430074HubeiChina Institute of Technology for Carbon Neutrality Shenzhen Institute of Advanced TechnologyChinese Academy of SciencesShenzhen 518055GuangdongChina School of Chemistry Chemical Engineering and Life SciencesState Key Laboratory of Advanced Technology for Materials Synthesis and ProcessingWuhan University of Technology430070HubeiChina Suzhou Institute of Nano-Tech and Nano-Bionics(SINANO) Chinese Academy of SciencesSuzhou 215123JiangsuChina School of Physics and Optoelectronic Engineering Hainan UniversityHaikou 570228HainanChina

All-perovskite tandem solar cells have the potential to surpass the theoretical efficiency limit of single junction solar cells by reducing thermalization ***,the challenges encompass the oxidation of Sn^(2+)to Sn^(4+)and uncontrolled crystallization kinetics in Sn-Pb perovskites,leading to nonradiative recombination and compositional heterogeneity to decrease photovoltaic efficiency and operational ***,we introduced an ionic liquid additive,1-ethyl-3-methylimidazolium iodide (EMIMI) into Sn-Pb perovskite precursor to form low-dimensional Sn-rich/pure-Sn perovskites at grain boundaries,which mitigates oxidation of Sn^(2+)to Sn^(4+)and regulates the film-forming dynamics of Sn/Pb-based perovskite *** optimized single-junction Sn-Pb perovskite devices incorporating EMIMI achieved a high efficiency of 22.87%.Furthermore,combined with wide-bandgap perovskite sub-cells in tandem device,we demonstrate 2-terminal all-perovskite tandem solar cells with a power conversion efficiency of 28.34%,achieving improved operational stability.

关键词： All-perovskite tandem solar cells Sn-Pb perovskite 1D Regulated crystallization Antioxidation

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Ultra-low power MoS2 optoelectronic synapse with wavelength sensitivity for color target recognition

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Science China(Information Sciences) 2025年第4期68卷 187-196页

作者： Bo WEI Yabo CHEN Xiaotong HAN Yan KANG Bujia LIANG Cheng LI Xiaokuo YANG Liang FANG Yuanxi PENG Institute for Quantum Information & State Key Laboratory of High Performance Computing College of ComputerNational University of Defense Technology Fundamentals Department Air Force Engineering University College of Advanced Interdisciplinary Studies National University of Defense Technology Institute of Quantum Information Science and Technology College of ScienceNational University of Defense Technology College of Computer National University of Defense Technology

Optoelectronic synapses that integrate visual perception and pre-processing hold significant potential for neuromorphic vision systems（NVSs）. However, due to a lack of wavelength sensitivity, existing NVS mainly focuses on gray-scale image processing, making it challenging to recognize color images. Additionally, the high power consumption of optoelectronic synapses, compared to the 10 fJ energy consumption of biological synapses, limits their broader application. To address these challenges, an energy-efficient NVS capable of color target recognition in a noisy environment was developed,utilizing a MoS2optoelectronic synapse with wavelength sensitivity. Benefiting from the distinct photon capture capabilities of 450, 535, and 650 nm light, the optoelectronic synapse exhibits wavelength-dependent synaptic plasticity, including excitatory postsynaptic current（EPSC）, paired-pulse facilitation（PPF）, and long-term plasticity（LTP）. These properties can effectively mimic the visual memory and color discrimination functions of the human vision system. Results demonstrate that the NVS, based on MoS2optoelectronic synapses, can eliminate the color noise at the sensor level, increasing color image recognition accuracy from 50% to 90%. Importantly, the optoelectronic synapse operates at a low voltage spike of0.0005 V, consuming only 0.075 fJ per spike, surpassing the energy efficiency of both existing optoelectronic and biological synapses. This ultra-low power, color-sensitive device eliminates the need for color filters and offers great promise for future deployment in filter-free NVS.

关键词： optoelectronic synapse neuromorphic vision system color recognition 2D materials image pre-processing

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Machine learning assisted screening of binary alloys for metal-based anode materials

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Journal of Energy Chemistry 2025年第5期104卷 62-68页

作者： Xingyue Shi Linming Zhou Yuhui Huang Chaohui Wu Yongjun Wu Juan Li Zijian Hong State Key Laboratory of Silicon and Advanced Semiconductor Materials School of Materials Science and EngineeringZhejiang UniversityHangzhou 310058ZhejiangChina Nanhu Brain-Computer Interface Institute Hangzhou 311100ZhejiangChina Zhejiang Key Laboratory of Advanced Solid State Energy Storage Technology and Applications Research Institute of Zhejiang University-TaizhouTaizhou 318000ZhejiangChina Inner Mongolia Electric Power Economic and Technological Research Institute Hohhot 010010Inner MongoliaChina College of Materials Science and Engineering Zhejiang University of TechnologyHangzhou 310014ZhejiangChina School of Engineering Hangzhou City UniversityHangzhou 310015ZhejiangChina Institute of Fundamental and Transdisciplinary Research Zhejiang UniversityHangzhou 311121China

Metal alloy anode materials with high specific capacity and low voltage have recently gained significant attention due to their excellent electrochemical performance and the ability to suppress dendrite ***,experimental investigations of metal alloys can be time-consuming and expensive,often requiring extensive experimental design and *** this study,we developed a machine learning model based on the Crystal Graph Convolutional Neural Network(CGCNN)to screen alloy anode materials for seven battery systems,including lithium(Li),sodium(Na),potassium(K),zinc(Zn),magnesium(Mg),calcium(Ca),and aluminum(Al).We utilized data with tens of thousands of alloy materials from the Materials Project(MP)and Automatic FLOW for Materials Discovery(AFLOW)*** any experimental voltage input,we identified over 30 alloy systems that have been experimentally validated with good ***,we predicted over 100 alloy anodes with low potential and high specific *** hope this work to spur further interest in employing advanced machine learning models for the design of battery materials.

关键词： CGCNN Alloy anodes Machine learning Metal-based batteries

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Special issue on progress of real-time confocal microscopy study on steelmaking and phase transformation in metallic materials

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Journal of Iron and Steel Research International 2025年第2期32卷 313-314页

作者： Wangzhong Mu Ying Ren Tong-sheng Zhang Deepoo Kumar Susanne Michelic Bryan Webler Key Laboratory of Electromagnetic Processing of Materials(Ministry of Education) Northeastern UniversityShenyang 110819LiaoningChina Department of Materials Science and Engineering KTH Royal Institute of TechnologyStockholm 10044Sweden School of Metallurgical and Ecological Engineering University of Science and Technology Beijing(USTB)Beijing 100083China School of Materials Science and Engineering Shanghai UniversityShanghai 200444China Department of Metallurgical Engineering and Materials Science IIT BombayPowaiMumbaiIndia Christian Doppler Laboratory for Inclusion Metallurgy in Advanced Steelmaking Montanuniversitaet LeobenLeoben 8700Austria Department of Materials Science and Engineering Carnegie Mellon UniversityPittsburgh 15213PAUSA

High-temperature confocal laser scanning microscopy(HT-CLSM)is a robust characterization tool which can provide in situ real-time studies of materials *** facility has been applied in investigating interfacial phenomena in ironmaking and steelmaking as well as phase transformations during heat treatment of metallic *** pioneering work on the application of HTCLSM dates back to twenty-five years ago,to directly observe the crystallization of undercooled steel melt.

关键词： transformation materials steel

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Nonflammable electrolyte with weak-solvation structure for stable NCM811 cathode under high temperature

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Journal of Energy Chemistry 2025年第5期104卷 111-117页

作者： Dawei Xu Chao Yang Ailing Yang Xiaowei Liu Meilong Wang Jin Han Tiefeng Liu Ya You State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070HubeiChina International School of Materials Science and Engineering School of Materials Science and MicroelectronicsWuhan University of TechnologyWuhan 430070HubeiChina College of Chemical and Biological Engineering Zhejiang UniversityHangzhou 310058ZhejiangChina Quzhou Institute of Power Battery and Grid Energy Storage Quzhou 324000ZhejiangChina

High-nickel cathode LiNi_(0.8)Co_(0.1)Mn_(0.1)O_(2)(NCM811)could enable lithium-ion batteries(LIBs)with high energy ***,excessive decomposition of the electrolyte would happen in the high operating voltage *** addition,the utilization of flammable organic solvents would increase safety risks in the high temperature ***,an electrolyte consisting of flame-retardant solvents with lower highest occupied molecular orbital(HOMO)level and LiDFOB salt is proposed to address above two *** a result,a thin and robust cathode-electrolyte interface containing rich LiF and Li-B-O compounds is formed on the cathode to effectively suppress electrolyte decomposition in the high operating *** NCM811||Li cell paired with this designed electrolyte possesses a capacity retention of 72%after 300 cycles at 55℃.This work provides insights into developing electrolyte for stable high-nickel cathode operated in the high temperature.

关键词： Electrolyte engineering Weak solvation High temperature Safety High-nickel cathode

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Massive GaN micro-LED array based underwater wireless optical communication

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Optics Express 2025年第9期33卷 19527-19534页

作者： Lv, Zhijian Liu, Xinyi Wu, Shuang Zhang, Wenwei Yue, C. Patrick Liu, Zhaojun Sino-German College of Intelligent Manufacturing Shenzhen Technology University Shenzhen China Department of Electrical and Electronic Engineering Southern University of Science and Technology Shenzhen China State Key Laboratory of Advanced Displays and Optoelectronics Technologies The Integrated Circuit Design Center Department of Electronic and Computer Engineering The Hong Kong University of Science and Technology Hong Kong

High-speed underwater wireless optical communication technology is a much-needed communication technology in current underwater applications, and micro-LED is a promising light source option. Considering the limitation of transmission distance due to the low optical power of a single micro-LED pixel, an underwater wireless optical communication system based on a novel massive GaN micro-LED array includes more than 5000 pixels fabricated via flip-chip technology is proposed, which can achieve 165-Mbps and 90-Mbps at 37.7 m and 73.5 m, respectively. Therefore, the feasibility of realizing a high data rate and long transmission distance in an underwater wireless optical communication system based on a novel massive micro-LED array is confirmed. © 2025 Optica Publishing Group under the terms of the Optica Open Access Publishing Agreement.

关键词： Fiber to the x

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Mid-infrared period doubled solitons in a few-mode fluoride fiber oscillator

Mid-infrared period doubled solitons in a few-mode fluoride ...

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2024 advanced Fiber Laser Conference, AFL 2024

作者： Yang, Ying Ma, Shuanglong Chen, Zifeng Luo, Xing Guo, Chunyu Ruan, Shuangchen Shenzhen Key Laboratory of Laser Engineering Guangdong Provincial Key Laboratory of Micro/Nano Optomechatronics Engineering Key Laboratory of Optoelectronic Devices and Systems of Ministry of Education and Guangdong Province State Key Laboratory of Radio Frequency Heterogeneous Integration College of Physics and Optoelectronic Engineering Shenzhen University Shenzhen518060 China Key Laboratory of Advanced Optical Precision Manufacturing Technology of Guangdong Higher Education Institutes Shenzhen Technology University Shenzhen518118 China

ISBN: (数字)9781510688889

ISBN: (纸本)9781510688872

Period doubling bifurcation (PDB) phenomenon, which is prevalent in nonlinear systems, has attracted considerable attention because of its potential application value. As an ideal platform for studying the pulse dynamics of nonlinear systems, the mode-locked fiber laser has been intensively investigated in the near-infrared (NIR) spectral region. However, there is a paucity of relevant reports of pulse dynamics in the mid-infrared (MIR) spectral region. Especially for the MIR large-mode-area (LMA) fluoride fiber oscillator, the existence of multiple transverse modes and a new spatial degree of freedom makes the pulse dynamics phenomenon is more complex, which needs to be further explored. In this paper, a soliton regime with a pulse duration of 404.5 fs, repetition frequency of 45.02 MHz, and average output power of 105.3 mW is obtained in a few-mode fluoride fiber oscillator mode-locked by the nonlinear polarization rotation (NPR) technique. By merely increasing the power of the pump, a period doubled soliton with the pulse intensity varying between two different values can be obtained. This work facilitates a more profound comprehension of the nonlinear dynamics in the mid-infrared multimode fluoride fiber laser, and opens up new opportunities for the chaos, optical frequency combs and all-optical modulation. © 2025 SPIE.

关键词： Infrared devices

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Crevice corrosion of reinforcing steel in carbonated simulated concrete pore solutions contaminated by chloride

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Journal of Iron and Steel Research International 2025年第1期32卷 293-311页

作者： Peng-peng Wu Yuan-pei Gong Shao-hua Zhang Yue-zhong Zhang Bao-sheng Liu Guang-ling Song College of Materials Science and Engineering Taiyuan University of Science and TechnologyTaiyuan030024ShanxiChina College of Chemical Engineering and Technology Taiyuan University of Science and TechnologyTaiyuan030024ShanxiChina Department of Ocean Science and Engineering Southern University of Science and TechnologyShenzhen518055GuangdongChina School of Mechanical and Mining Engineering Centre for Advanced Materials Processing and Manufacturing(AMPAM)The University of QueenslandSt LuciaQLD4072Australia State Key Laboratory of Physical Chemistry of Solid Surfaces Xiamen UniversityXiamen361005FujianChina

The crevice corrosion of the reinforcing steel in the carbonated simulated concrete pore solutions(SCPSs)containing 0.04 mol/L chloride was *** comparison,the steel without crevice covered on its surface was also *** showed that the crevice corrosion in the uncarbonated SCPS was not triggered and the steel remained passivity by suppressing the anodic dissolution in the crevice *** SCPS was carbonated to have pH values of 10.5 and 11.5,the crevice corrosion was easier to be activated than the widely reported pitting corrosion owing to the rapid oxygen depletion within the crevice,but the crevice corrosion damage might be alleviated to a certain extent due to the relative compact surface film formed inside the *** further carbonation led to the activation dissolution of both the crevice interior and exterior,causing the more serious corrosion *** process of the crevice corrosion was systematically analyzed by combining the electrochemical measurement results and Evens polarization diagram.

关键词： Crevice corrosion Reinforcing steel Carbonation Electrochemical test Rust Evens polarization diagram

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Suppression of microcracks in femtosecond laser grooving of aluminum using a flame environment

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Optics Letters 2025年第9期50卷 2836-2839页

作者： Guo, Sijia Jiang, Yuanfei Han, Jianhui Chen, Anmin Jin, Mingxing Institute of Atomic and Molecular Physics Jilin University Changchun130012 China Jilin Provincial Key Laboratory of Applied Atomic and Molecular Spectroscopy Jilin University Changchun130012 China State Key Laboratory of Advanced Space Propulsion Department of Aerospace Science and Technology Space Engineering University Beijing101416 China

Femtosecond laser machining of aluminum often suffers from microcrack formation and edge irregularities, affecting processing quality. This study explores the impact of a flame environment on groove characteristics. Results show that in ambient air, high-energy laser pulses induce microcracks, especially at high scanning speeds, while the flame environment suppresses microcracks and improves edge uniformity. The flame preheats the material, reduces thermal shock, and enhances material removal, leading to deeper and more consistent grooves. These findings provide insights for optimizing laser processing parameters to improve machining stability and surface quality. © 2025 Optica Publishing Group. All rights, including for text and data mining (TDM), Artificial Intelligence (AI) training, and similar technologies, are reserved.

关键词： Laser materials processing

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Preface to Special Issue on Optoelectronic Neuromorphic Devices

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Journal of Semiconductors 2025年第2期46卷 2-4页

作者： Zhenyi Ni Zhongqiang Wang Jia Huang Xiaodong Pi State key Laboratory of Silicon and Advanced Semiconductor Materials&School of Materials Science and Engineering Zhejiang UniversityHangzhou 310027China Shangyu Institute of Semiconductor Materials Shaoxing 312300China Key Laboratory of UV-Emitting Materials and Technology of Ministry of Education Northeast Normal UniversityChangchun 130024China School of Materials Science and Engineering&National Key Laboratory of Autonomous Intelligent Unmanned Systems Tongji UniversityShanghai 201804China Institute of Advanced Semiconductors&Zhejiang Provincial Key Laboratory of Power Semiconductor Materials and Devices ZJ-UHangzhou Global Scientific and Technological Innovation CenterZhejiang UniversityHangzhou 311200China

The rapid advancement of artificial intelligence(AI),recognized with Nobel Prizes in both Physics and Chemistry in 2024,has been revolutionizing countless aspects of modern life,driving innovations across diverse fields and reshaping how people interact with *** its great advances,the computing of AI systems is now approaching the limit of traditional computing based on the von Neumann architecture,which is characterized by separated memory and process units-a challenge known as the"von Neumann bottleneck".

关键词： approaching separated Neumann

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