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DeCarbon 2024年第4期6卷 66-66页

作者： Youtao Yao Jiahui Lyu Xingchuan Li Cheng Chen Francis Verpoort John Wang Zhenghui Pan Zongkui Kou State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan430070PR China Sanya Science and Education Innovation Park of Wuhan University of Technology Sanya572000PR China Hubei Key Laboratory of Fuel Cell Wuhan University of TechnologyWuhan430070PR China Department of Materials Science and Engineering National University of Singapore117574SingaporeSingapore Institute of Materials Research and Engineering(IMRE) A*STAR(Agency for ScienceTechnology and Research)2 Fusionopolis WaySingapore138634Singapore National University of Singapore(Chongqing)Research Institute Chongqing401123PR China School of Materials Science and Engineering Tongji UniversityShanghai201804PR China

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Biomemory: Phototunable Biomemory Based on Light-Mediated Charge Trap (Adv. Sci. 9/2018)

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advanced Science 2018年第9期5卷 1870051-1870051页

作者： Ziyu Lv Yan Wang Zhonghui Chen Long Sun Junjie Wang Meng Chen Zhenting Xu Qiufan Liao Li Zhou Xiaoli Chen Jieni Li Kui Zhou Ye Zhou Yu-Jia Zeng Su-Ting Han Vellaisamy A. L. Roy College of Electronic Science and Technology Shenzhen University Shenzhen 518060 P. R. China Department of Materials Science and Engineering and State Key Laboratory of Millimeter Waves City University of Hong Kong Tat Chee Avenue Kowloon Hong Kong SAR 999077 China State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of Technology 122 Luoshi Road Wuhan 430070 P. R. China State Key Laboratory of Transducer Technology Shanghai Institute of Microsystem and Information Technology Chinese Academy of Sciences Shanghai 200050 China Institute for Advanced Study Shenzhen University Shenzhen 518060 P. R. China College of Optoelectronic Engineering Shenzhen University Shenzhen 518060 P. R. China

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Ultra-High Proportion of Grain Boundaries in Zinc Metal Anode Spontaneously Inhibiting Dendrites Growth

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Angewandte Chemie 2024年第32期136卷

作者： Sitian Lian Zhijun Cai Prof. Mengyu Yan Prof. Congli Sun Nianyao Chai Bomian Zhang Kesong Yu Ming Xu Dr. Jiexin Zhu Dr. Xuelei Pan Dr. Yuhang Dai Jiazhao Huang Bo Mai Ling Qin Wenchao Shi Qiqi Xin Xiangyu Chen Dr. Kai Fu Prof. Qinyou An Dr. Qiang Yu Prof. Liang Zhou Dr. Wen Luo Dr. Kangning Zhao Prof. Xuewen Wang Prof. Liqiang Mai State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of Technology Wuhan 430070 P. R. China Department of Physics The Chinese University of Hong Kong Shatin New Territories Hong Kong 999077 P. R. China Advanced Technology Institute University of Surrey Guildford Surrey GU2 7XH UK State Key Laboratory of Materials Processing and Die & Mould Technology School of Materials Science and Engineering Huazhong University of Science and Technology Wuhan Hubei 430074 P. R. China Minhang Hospital Shanghai Medical College of Fudan University Shanghai 201199 P. R. China Laoshan Laboratory Qingdao 266237 P. R. China School of Physical Sciences Great Bay University Dongguan 523808 P. R. China

Aqueous Zn-ion batteries are an attractive electrochemical energy storage solution for their budget and safe properties. However, dendrites and uncontrolled side reactions in anodes detract the cycle life and energy density of the batteries. Grain boundaries in metals are generally considered as the source of the above problems but we present a diverse result. This study introduces an ultra-high proportion of grain boundaries on zinc electrodes through femtosecond laser bombardment to enhance stability of zinc metal/electrolyte interface. The ultra-high proportion of grain boundaries promotes the homogenization of zinc growth potential, to achieve uniform nucleation and growth, thereby suppressing dendrite formation. Additionally, the abundant active sites mitigate the side reactions during the electrochemical process. Consequently, the 15 μm Fs−Zn||MnO 2 pouch cell achieves an energy density of 249.4 Wh kg −1 and operates for over 60 cycles at a depth-of-discharge of 23 %. The recognition of the favorable influence exerted by UP-GBs paves a new way for other metal batteries.

关键词： zinc anode grain boundary femtosecond laser aqueous battery nucleation mode

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Bifunctional Electrocatalysts: Cobalt−Iron Oxide Nanosheets for High‐Efficiency Solar‐Driven CO2−H2O Coupling Electrocatalytic Reactions (Adv. Funct. Mater. 31/2020)

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advanced Functional materials 2020年第31期30卷

作者： Yuying Mi Yuan Qiu Yifan Liu Xianyin Peng Min Hu Shunzheng Zhao Huanqi Cao Longchao Zhuo Hongyi Li Junqiang Ren Xijun Liu Jun Luo Center for Electron Microscopy Tianjin Key Lab of Advanced Functional Porous Materials Institute for New Energy Materials and Low‐Carbon Technologies School of Materials Science and Engineering Tianjin University of Technology Tianjin 300384 China Key Laboratory of Optoelectronic Devices and Systems of Ministry of Education and Guangdong Province Shenzhen University Shenzhen 518060 China Department of Environmental Engineering University of Science and Technology Beijing Beijing 100083 China Key Laboratory of Display Materials and Photoelectric Devices (Ministry of Education) School of Materials Science and Engineering Tianjin University of Technology Tianjin 300384 China School of Materials Science and Engineering Xi'an University of Technology Xi'an 710048 China Qualification of Products Supervision & Inspection Institute of Technology Xinjiang Uygurs Autonomous Region Urumqi 830011 China State Key Laboratory of Advanced Processing and Recycling of Nonferrous Metals Lanzhou University of Technology Lanzhou 730050 China

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Applications of hierarchically structured porous materials from energy storage and conversion, catalysis, photocatalysis, adsorption, separation, and sensing to biomedicine

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Chemical Society reviews 2016年第12期45卷 3479-563页

作者： Ming-Hui Sun Shao-Zhuan Huang Li-Hua Chen Yu Li Xiao-Yu Yang Zhong-Yong Yuan Bao-Lian Su State Key Laboratory of Advanced Technology for Material Synthesis and Processing Wuhan University of Technology Luoshi Road 122 Wuhan 430070 China. chenlihua@*** baoliansu@***. Collaborat Innovat. Ctr. Chem. Sci. & Engn. Tianjin Key Lab. Adv. Energy Mat. Chem. Minist. Educ. Coll. Chem. Nankai Univ. Tianjin 300071 China. State Key Laboratory of Advanced Technology for Material Synthesis and Processing Wuhan University of Technology Luoshi Road 122 Wuhan 430070 China. chenlihua@*** baoliansu@*** and Laboratory of Inorganic Materials Chemistry (CMI) University of Namur 61 rue de Bruxelles B-5000 Namur Belgium. bao-lian.su@unamur.be and Clare Hall University of Cambridge Cambridge CB2 1EW UK. bls26@cam.ac.uk.

Over the last decade, significant effort has been devoted to the applications of hierarchically structured porous materials owing to their outstanding properties such as high surface area, excellent accessibility to active sites, and enhanced mass transport and diffusion. The hierarchy of porosity, structural, morphological and component levels in these materials is key for their high performance in all kinds of applications. The introduction of hierarchical porosity into materials has led to a significant improvement in the performance of materials. Herein, recent progress in the applications of hierarchically structured porous materials from energy conversion and storage, catalysis, photocatalysis, adsorption, separation, and sensing to biomedicine is reviewed. Their potential future applications are also highlighted. We particularly dwell on the relationship between hierarchically porous structures and properties, with examples of each type of hierarchically structured porous material according to its chemical composition and physical characteristics. The present review aims to open up a new avenue to guide the readers to quickly obtain in-depth knowledge of applications of hierarchically porous materials and to have a good idea about selecting and designing suitable hierarchically porous materials for a specific application. In addition to focusing on the applications of hierarchically porous materials, this comprehensive review could stimulate researchers to synthesize new advanced hierarchically porous solids.

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Corrigendum to “Silica coating with well-defined micro-nano hierarchy for universal and stable surface superhydrophobicity” [Chem. Phys. Lett. 730 (2019) 594–599]

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Chemical Physics Letters 2019年 735卷

作者： Huan Liu Wei Geng Cheng-Jing Jin Si-Ming Wu Yi Lu Jie Hu Hao-Zheng Yu Gang-Gang Chang Tian Zhao Ying Wan Zhi-Qiang Luo Ge Tian Xiao-Yu Yang State Key Laboratory Advanced Technology for Materials Synthesis and Processing & School of Materials Science and Engineering Wuhan University of Technology 122 Luoshi Road Wuhan 430070 China Chemical Engineering and Life Science School of Chemistry Wuhan University of Technology 122 Luoshi Road Wuhan 430070 China College of Life Science and Technology Huazhong University of Science and Technology 1037 Luoyu Road Wuhan 430074 China School of Engineering and Applied Sciences Harvard University Cambridge MA 02138 USA Southern Marine Science and Engineer Guangdong Laboratory (Zhuhai) Zhuhai 51900 China

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Enhanced Carrier Diffusion Enables Efficient Back-Contact Perovskite Photovoltaics

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Angewandte Chemie 2023年第27期135卷

作者： Boya Zhao Dr. Lara V. Gillan Dr. Andrew D. Scully Dr. Anthony S. R. Chesman Dr. Boer Tan Dr. Xiongfeng Lin Dr. Jingying Liu Dr. Kevin J. Rietwyk Siqi Deng Dr. Christopher Bailey Prof. Yi-Bing Cheng Prof. Dane R. McCamey Prof. Udo Bach Department of Chemical and Biological Engineering Monash University Victoria 3800 Australia ARC Centre of Excellence in Exciton Science Australia School of Physics University of New South Wales New South Wales 2052 Australia CSIRO Manufacturing Victoria 3168 Australia Department of Materials Science and Engineering Monash University Victoria 3800 Australia State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of Technology Wuhan 430070 China Foshan Xianhu Laboratory Foshan 528216 China

Back-contact architectures offer a promising route to improve the record efficiencies of perovskite solar cells (PSCs) by eliminating parasitic light absorption. However, the performance of back-contact PSCs is limited by inadequate carrier diffusion in perovskite. Here, we report that perovskite films with a preferred out-of-plane orientation show improved carrier dynamic properties. With the addition of guanidine thiocyanate, the films exhibit carrier lifetimes and mobilities increased by 3–5 times, leading to diffusion lengths exceeding 7 μm. The enhanced carrier diffusion results from substantial suppression of nonradiative recombination and improves charge collection. Devices using such films achieve reproducible efficiencies reaching 11.2 %, among the best performances for back-contact PSCs. Our findings demonstrate the impact of carrier dynamics on back-contact PSCs and provide the basis for a new route to high-performance back-contact perovskite optoelectronic devices at low cost.

关键词： Back-Contact Architecture Carrier Dynamics Crystallographic Orientation Guanidine Thiocyanate Perovskite Solar Cells

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Inside Cover: Biofuel cells Based on the Immobilization of Photosynthetically Active Bioentities (ChemCatChem 3/2011)

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ChemCatChem 2011年第3期3卷 422-422页

作者： Dr. Christophe F. Meunier Dr. Xiao-Yu Yang Dr. Joanna C. Rooke Prof. Bao-Lian Su Laboratory of Inorganic Materials Chemistry (CMI) The University of Namur (FUNDP) 61 rue de Bruxelles B-5000 Namur (Belgium) Fax: (+32) 81-72-54-14 F.N.R.S. “ Chargé de Recherches ” Position Fonds National de la Recherche Scientifique 5 rue d'Egmont B-1050 Bruxelles (Belgium) State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of Technology 122 Luoshi Road Wuhan 430070 (China)

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Lösliche und röhrenförmige höhere Fullerene zur Verkapselung von Metallen†

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Angewandte Chemie 2012年第12期124卷

作者： Xing Lu Takeshi Akasaka Shigeru Nagase Life Science Center for Tsukuba Advanced Research Alliance University of Tsukuba Tennodai 1‐1‐1 Tsukuba Ibaraki 305‐8577 (Japan) State Key Lab of Materials Processing and Die & Mould Technology College of Materials Science and Engineering Huazhong University of Science and Technology (HUST) Wuhan 430074 (China) Department of Theoretical and Computational Molecular Science Institute for Molecular Science Okazaki Aichi 444‐8585 (Japan)

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A Facile Route for the synthesis of New 1D manganese(II) Coordination Polymer As Precursors for the Preparation of Nanostructures of Mn3O4: Crystallography, Hirshfeld Surface Analysis and Molecular Docking Studies

SSRN

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SSRN 2022年

作者： Gurbanov, Atash V. Pourshirband, Nafiseh Sharafi-Badr, Paria Rostamnia, Sadegh Hayati, Payam Souri, Bagher Eshghi, Fazlolah Kaminsky, Werner Mahmoudi, Ghodrat Verpoort, Francis Centro de Química Estrutural Institute of Molecular Sciences Instituto Superior Técnico Universidade de Lisboa Av. Rovisco Pais Lisboa1049-001 Portugal Department of Chemistry Baku State University Z. Khalilov Str. 23 BakuAZ 1148 Azerbaijan Department of Chemistry Shahreza Branch Islamic Azad University P.O. Box 311-86145 Shahreza Isfahan Iran Department of Pharmacognosy and Pharmaceutical Biotechnology School of Pharmacy Iran University of Medical Sciences Tehran Iran PO Box 16846-13114 Tehran Iran Department of Chemistry Faculty of Sciences University of Sistan and Baluchestan Zahedan Iran Department of Chemistry College of Sciences Shiraz University Shiraz Iran X-ray Crystallography Laboratory University of Washington United States Department of Chemistry Faculty of Science University of Maragheh P.O. Box 55136-83111 Maragheh Iran State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of Technology Wuhan430070 China

The novel metal-organic coordination polymers (MOCP) with the general chemical formula [Mn2L(SCN)2(OH)2]***3OH [L=1,5-bis(pyridine-4-ylmethylene) carbonohydrazide] {1} were synthesized by using two techniques, solvothermal and sonochemical ultrasonic-assisted. The effects of sonication power, reaction time, concentration of reactants, and temperature were examined on their impact on influencing the size and morphology of the *** findings have discovered that all parameters have an inverse impact on the size and morphology of 1. However, this study determined that temperature and sonication power do not control the crystals' size and morphology. SEM further analyzed the prepared microcrystals of MOCPs to examine the surface morphology and XRD, elemental evaluation composition, and FT-IR spectroscopy to clarify the functional groups of the prepared Mn-MOCPs. In the following, the calcination of 1 in the air atmosphere resulted in the production of Mn3O4 nanoparticles at 650 °C. The geometric and electronic structure of the MOCPs is evaluated in the density functional theory (DFT) framework. Molecular docking methodologies show that the best cavity of the human androgen receptor has −116.3 kJ mol−1 interaction energy involving bonding and non-bonding. © 2022, The Authors. All rights reserved.

关键词： Density functional theory

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