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SSRN 2023年

作者： He, Qian Xu, Chaokai Tan, Shengdong Tang, Yaxin Xi, Shibo Yao, Bingqing Wade, Austin Zhao, Binbin Lu, Shangchen Tian, Mingjiao He, Chi Ma, Lu Fu, Xingjie Shi, Jiwei Lu, Jiong Howe, Alexander G.R. Dai, Sheng Luo, Guangfu Du, Yankun Department of Material Science and Engineering College of Design and Engineering National University of Singapore 9 Engineering Drive 1 EA #03-09 Singapore117575 Singapore Department of Materials Science and Engineering Guangdong Provincial Key Laboratory of Computational Science and Material Design Southern University of Science and Technology Guangdong Shenzhen518055 China 1 Pesek Road Jurong Island 627833 Singapore Thermo Fisher Scientific 5350 NW Dawson Creek Drive HillsboroOR United States State Key Laboratory of Multiphase Flow in Power Engineering School of Energy and Power Engineering Xi’an Jiaotong University Shaanxi Xi’an710049 China Brookhaven National Laboratory UptonNY11973 United States Department of Chemistry National University of Singapore 12 Science Drive 2 117549 Singapore Key Laboratory for Advanced Materials Joint International Research Laboratory of Precision Chemistry and Molecular Engineering School of Chemistry and Molecular Engineering East China University of Science & Technology Shanghai200237 China

We investigated the industrially important PtSn/Al2O3 catalysts prepared with uniform particle sizes (~ 1 nm) and varied compositions using molecular complexes of Pt(II) and Sn(II). Our best catalyst, with a Sn:Pt ratio of around 2, exhibited a high initial propylene productivity of about 1.1 mol C3H6 (g catalyst)-1 h-1. Elaborate electron microscopy studies revealed significant compositional variations in the catalyst, highlighting the practical challenges in achieving or confirming the theoretically predicted optimum Sn:Pt ratio. It is also found that the catalytic activities correlate well with the Pt dispersion, suggesting the structure-insensitive nature of the dehydrogenation reaction applies in these ultrasmall Pt-Sn nanoparticles. The presence of Pt-rich particles in the catalysts did not produce noticeable degradations in the reaction selectivity, indicating a wide composition range for Pt-Sn nanoparticles to be effective at the 1 nm size range. These findings emphasize the importance of detailed analysis of compositional distributions for understanding nanoalloys. © 2023, The Authors. All rights reserved.

关键词： Electron microscopy

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Comparison of Gelatinous and Calcined Magnesia Supported Ni or/And Co-Based Catalysts for Aqueous Bioglycerol Phase Reforming

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SSRN 2021年

作者： Liu, Dashuai Dou, Binlin Zhang, Hua Wu, Kai Zhao, Longfei Zeng, Pingchao Chen, Haisheng Xu, Yujie School of Energy and Power Engineering Shanghai Key Laboratory of Multiphase Flow and Heat Transfer in Power Engineering University of Shanghai for Science and Technology Shanghai200093 China Institute of Engineering Thermophysics Chinese Academy of Sciences Beijing100190 China

In this study, glycerol aqueous phase reforming was carried out in a batch reactor. The gases produced were H2, CO, CH4, and CO2 during the experiment. The catalysts used included Ni or/and Co catalysts supported by MgO. Meanwhile, two different MgO supporters were prepared by the sol-gel method and calcining method, and the active metal was added by an initial wet impregnation (IWI) method. The catalysts were characterized by BET, BJH, TEM, and XRD. In order to achieve the purpose of comparison, the activity of different types of catalysts was tested under similar conditions. It was found that the amount of hydrogen produced by the catalyst containing gelatinous MgO supporter is more than 1.5 times that of other catalysts, and the Ni-Co-MgO had the best catalytic effect among the same types of catalysts. The activity of the Ni-Co-MgO catalyst was tested under different temperatures, concentrations, and CaO conditions. We found that Ni-Co bimetallic catalyst supported on gelatinous MgO has the best highest gas production, while the catalyst containing calcined MgO support usually has a better hydrogen selectivity. Through the stability study of the Ni-Co-MgO catalyst, we found that the bimetallic catalyst supported by gelatinous MgO support has better catalytic stability. © 2021, The Authors. All rights reserved.

关键词： Sol-gel process

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Physics-Based Probabilistic Assessment of Creep-Fatigue Failure for Pressurized Components by Extended Direct Steady Cycle Analysis-Driven Neural Network

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SSRN 2022年

作者： Wang, Xiaoxiao Ma, Zhiyuan Yang, Jie Chen, Haofeng Xuan, Fuzhen Department of Mechanical & Aerospace Engineering University of Strathclyde James Weir Building 75 Montrose Street GlasgowG1 1XJ United Kingdom Shanghai Key Laboratory of Multiphase Flow and Heat Transfer in Power Engineering School of Energy and Power Engineering University of Shanghai for Science and Technology Shanghai200093 China School of Mechanical and Power Engineering East China University of Science and Technology Shanghai200237 China

To achieve a high-reliability design with a feasible balance between accuracy and efficiency, the physics-based probabilistic assessment for creep-fatigue failure is proposed under the probabilistic Linear Matching Method (pLMM) framework. At the physical level, the structural failure mechanism is reflected in the prepared training database, which is generated by the direct method, extended Direct Steady Cycle Analysis (eDSCA) procedures. And to efficiently express the relationship between design parameters and structural responses implicitly, the extended DSCA-driven neural network (EDDNN) is built with the superior fitting quality of damage and lifetime. With the benchmarks of pressurized structures provided, the applicability of the proposed probabilistic analysis approach in solving practical problems is demonstrated, where the reliability-based evaluation diagram is established according to different requirements. Furthermore, a novel data classification scheme is proposed to deal with the randomness in creep damage-dominated probabilistic assessment. © 2022, The Authors. All rights reserved.

关键词： Failure (mechanical)

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RECENT ADVANCES OF SURFACE WETTABILITY EFFECT ON flow BOILING HEAT TRANSFER PERFORMANCE

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Frontiers in Heat and Mass Transfer 2021年 17卷

作者： Cao, Shuang Yang, Hui Zhao, Luxing Wang, Tao Xie, Jian School of Energy and Power Engineering Zhengzhou University of Light Industry Zhengzhou450002 China Beijing Key Laboratory of Multiphase Flow and Heat Transfer for Low Grade Energy Utilization North China Electric Power University Beijing102206 China

flow boiling heat transfer is an effective way to fulfill the energy transfer. The wettability of boiling surface influences the liquid spreading ability and the growth, departure, and release frequency of bubbles, which determines the heat transfer performance. According to the wettability and combination forms, boiling surface are classified into weak wetting surface, strong wetting surface, and heterogeneous wetting surface. Fabricating by physical, chemical method or coating the original surface with a layer of low surface energy, the weak wetting surface has more effective activation point and nucleation center density to improve heat transfer performance at low heat flux. The strong wetting surface always formed by physical or chemical treatment to enhance the rapid rewetting of the wall surface. It has a smaller bubble separation diameter, higher separation frequency and higher CHF. The heterogeneous wetting surface, having the synthetic effects of the strong and weak surface wettabilities, is a hot issue of recent study. But its composition and heat transfer enhancement mechanism are very complicated which need to study thoroughly. Furthermore, the intelligent wetting surface, having the dynamics wettability function, is also briefly analyzed in this paper. Despite the advances in this aspect, the boiling surfaces can be further optimized by fabricate effective wettability to achieve a strong stability, high heat transfer performance and realize the synergistic effect of flow pattern and heat transfer. © 2021, Global Digital Central. All rights reserved.

关键词： Wetting

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Experimental Investigation on Critical Heat Flux for Water flowing in a Vertical Uniformly Heated Rifled Tube under Near-critical Pressures

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Journal of Thermal Science 2018年第6期27卷 527-540页

作者： XIE Haiyan YANG Dong ZHAO Yunjie JIANG Huiqing QU Mofeng State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University

This study experimentally investigated the critical heat flux(CHF) of departure from nucleate boiling(DNB) of water flowing under near-critical pressures in a 2 m-long vertical upward rifled tube with the size of Φ35 × 5.67 mm. Operating conditions included pressures of 18–21 MPa, mass fluxes of 475–1000 kg·m^(-2)·s^(-1), inlet subcooling temperatures of 3–5°C, and wall heat fluxes of 40–960 kW·m^(-2). Tube wall temperature distribution and heat transfer performance in different test conditions were obtained. The effects of the operating parameters on CHF were analyzed. Four heat transfer coefficient correlations were evaluated against our experimental data for further investigation of the two-phase heat transfer characteristics. A heat transfer correlation based on Martinelli number utilized in two-phase region and two empirical correlations used to predict the CHF in rifled tube at near-critical pressures were proposed. Meanwhile, experimental CHF data in rifled tube were compared with six widely used correlations and a CHF look-up table. The CHF enhancement effect in rifled tube is obvious as compared with the CHF data in smooth tube. Results show that DNB occurs at low vapor quality and subcooled region in the rifled tube at near-critical pressures. The increase in pressure leads to the early occurrence of DNB and the decrease in CHF, whereas the increase in mass flux delays the occurrence of DNB and results in the increase in CHF. DNB presents a tendency to move toward the inlet of the rifled tube. At individual operating conditions, DNB and dryout coexist at different sections of the rifled tube.

关键词： critical heat flux near-critical pressure rifled tube DNB heat transfer

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Study of thermophysical properties of binary mixtures of N-phenyl ethanolammonium based protic ionic liquids with water and ethanol solvents

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Journal of Ionic Liquids 2022年第1期2卷

作者： Chennuri, Bharath Kumar Losetty, Venkatramana Sreenivasulu, K. Gardas, Ramesh L. Sivakumar, K. A.P. Tirupati517502 India Department of Chemistry VelTech Rangarajan Dr. Sagunthala R&D Institute of Science and Technology Avadi Chennai600062 India Department of Chemistry State Key Laboratory of Multiphase Flow in Power Engineering Xian Jiaotong University Xian710049 China Department of Chemistry Indian Institute of Technology Madras Chennai600036 India

This work reveals that the physicochemical properties such as density, ρ and speed of sound, u for the binary mixtures of N-phenylethanolammonium formate ([NPEA][For]) and N-phenylethanolammonium acetate ([NPEA][Ace] with water and ethanol solvents were experimentally measured for the temperature ranges from 293.15 K to 318.15 K at atmosphere pressure. The apparent molar volume, VΦ and apparent molar isentropic compressibility, κs,Φ were estimated from the experimental data. Redlich-Mayer type empirical equation was applied to calculate the limiting apparent molar properties at infinite dilution (Vω∞ and k∞) and corresponding empirical parameters (Sv, Bv, Sk and Bk). The type of interaction either IL-solvent or IL-IL or solvent-solvent occurring in solution were determined from the data of empirical parameters. Furthermore, the temperature dependent apparent molar volume at infinite dilution, V∞ was used to calculate the apparent molar expansibility at infinite dilution, E∞. Moreover, these E∞ values of the studied binary solutions were found to be positive. The making and breaking structure ability of both PILs were analyzed at all experimental conditions. © 2021 The Authors

关键词： Dilution

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Numerical Study of Percolation and Seepage Behaviors in Ion-Adsorption-Type Rare Earth Ore Leaching Process

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Mathematical Problems in engineering 2023年第1期2023卷

作者： Dianyu, E. Su, Zhongfang Zeng, Jia Yang, Liuyimei Li, Jing Xu, Qiang Wang, Lin Cui, Jiaxin Jiangxi Provincial Key Laboratory for Simulation and Modelling of Particulate Systems Jiangxi University of Science and Technology Nanchang330013 China International Institute for Innovation Jiangxi University of Science and Technology Nanchang330013 China Ganjiang Innovation Academy Chinese Academy of Sciences Ganzhou341000 China ARC Research Hub for Computational Particle Technology Department of Chemical and Biological Engineering Monash University ClaytonVIC3800 Australia State Key Laboratory of Multiphase Flow in Power Engineering Xi'An Jiaotong University Xi'an710049 China Delft University of Technology Delft Netherlands

Ionic rare earth ore is a type of featured rare earth ore in China. Its mining process suffers from a long leaching cycle and considerable consumption of leaching agents. Improving mining efficiency requires a sound physical understanding of the leaching process. In this study, the CFD-based numerical model is used to analyze the physical process of leaching through porous media formed by particles. The simulation results indicate that a lower packing porosity and smaller particles packed granular porous medium result in much larger energy dissipation during seepage, and the energy dissipation increases with seepage velocity. It is found that when the seepage velocity increases to a certain high value, the energy dissipation exceeds the value predicted by Darcy's law, which is mainly caused by liquid turbulence. Additionally, the effect of particle shape is examined. The results show that the granular medium composed of prolate particles causes larger energy dissipation than oblate particles, and spherical particles play the least role. This phenomenon may result from the particle shape affecting the area of the frontal contact surface between particles and liquid. The results provide new insights into the fundamental understanding of percolation and seepage behaviors in the ion-adsorption-type rare earth ore leaching process. © 2023 E. Dianyu et al.

关键词： Energy dissipation

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Effects of Flue Gas Recirculation on Combustion and Heat Flux Distribution in 660 Mw Double-Reheat Tower-Type Boiler

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SSRN 2022年

作者： Deng, Lei Dong, Lingxiao Bai, Yang Wu, Yuhao Liu, Hu Belošević, Srdjan Tomanović, Ivan Che, Defu State Key Laboratory of Multiphase Flow in Power Engineering School of Energy and Power Engineering Xi’an Jiaotong University Xi’an710049 China Guoshen Institute of Technology CHN ENERGY Xi'An710065 China Department of Thermal Engineering and Energy "VINČA" Institute of Nuclear Sciences National Institute of thе Republic of Serbia University of Belgrade Mike Petrovića Alasa 12-14 11351 Vinča PO Box 522 Belgrade11001 Serbia

The ultra-supercritical double-reheat boiler has attracted more attention because of high parameters, low pollution and large capacity. However, there are some difficulties in the development of this technology, such as adjusting the reheat steam temperature. In this study, computational fluid dynamics simulation is used to analyze a 660 MW double-reheat tower-type pulverized coal-fired boiler. The influence of flue gas recirculation (FGR) on heat transfer characteristics and combustion process in the furnace (including heating surfaces in the upper parts of the furnace) are evaluated. The user-defined function approach predicates CO reduction effect on NO x . The results show that the flow at the horizontal section through the centerline of recirculating flus gas nozzles is rotating. The velocity distribution changes into an elliptical rotating flow when FGR ratio is 20%. At higher FGR ratios, the high-temperature area (1565-1700 K) shrinks and both the NO x concentration at the low-temperature superheater outlet and oxygen concentration in the furnace descend. Oxygen concentration at low-temperature superheater outlet first increases and then decreases. In the main combustion zone, the heat flux peak of water-cooled wall is about 330 kW m -2 . As FGR ratio increases from 0% to 20%, the rate of water-cooled wall heat absorption to total boiler decreases by 3.50%. This rate for reheater and superheater increases by 2.53% and 2.13%, respectively. © 2022, The Authors. All rights reserved.

关键词： Temperature

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Numerical Simulation of Acoustic Propagation in Gas Ultrasonic flowmeter

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SSRN 2022年

作者： Xiao, Yongqing Zhang, Meng Li, Dong Yang, Yueming Ma, Bingkun Qi, Jianhui School of Energy and Power Engineering Shandong University Jinan250061 China Beijing Key Laboratory of Multiphase Flow and Heat Transfer for Low Grade Energy Utilization North China Electric Power University Beijing102206 China Suzhou Research Institute Shandong University Suzhou215123 China Shandon Academy of Sciences China

Ultrasonic flowmeter has been widely used in chemical smelting, industrial production and other fields. Through the COMSOL Multiphysics software, the non-linear trajectory of the rays in the non-invasive and intrusive UFW is first simulated by the ray tracing method. Then, the transient ultrasonic propagation process is simulated to analyze the reasons for the error of ultrasonic propagation. Finally, the cause of the error of the transducer is analyzed by the sound pressure signal at the receiving end. It was found that it is precisely because of the high-speed flow that the ultrasonic propagation is distorted, which is manifested as the non-linear trajectory and downstream drift of the sound beam. The signal at the receiving end also fails to hit the correct position due to beam drift, resulting in sound pressure falling below the detected value. © 2022, The Authors. All rights reserved.

关键词： flow measurement

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Activated Overall Water Splitting Over a Ni-Fe Layered Double Hydroxide Electrocatalyst by V Doping and Sulfuration

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SSRN 2023年

作者： Wu, Wentong Peng, Lei Min, Boya Huang, Jie Liu, Saiya Lu, Kejian Lu, Shijian Jing, Dengwei Zheng, Mingsheng Liu, Maochang International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Shaanxi Xi’an710049 China No. 8 Oil Production Plant of PetroChina Changqing Oilfield Company Shaanxi Xi’an710016 China Carbon Neutrality Institute Jiangsu Key Laboratory of Coal-based Greenhouse Gas Control and Utilization China University of Mining and Technology Jiangsu Xuzhou221008 China Gree Altairnano New Energy Inc Zhuhai519040 China School of Chemistry and Biological Engineering University of Science and Technology Beijing Beijing100083 China

Ni-Fe layered double hydroxide (NiFe-LDH) is regarded as one of the promising non-noble electrocatalyst. However, the limited number of active sites and poor electrical conductivity impede its further development. Herein, we report the synthesis of a Ni foam supported NiFe-LDH electrocatalyst modified by V doping and vulcanization (NiFeV-S/NF). This modification endows the catalyst excellent property toward hydrogen evolution reaction (HER), oxygen evolution reaction (OER), and overall water splitting. Only 211 mV and 127 mV of the overpotentials are required to achieve the current density of 10 mA cm-2 for OER and HER in 1 M KOH electrolyte, respectively. Particularly, the prepared NiFeV-S/NF could serve as a bifunctional electrocatalyst for overall water splitting, with a cell voltage of 1.573 V to reach a current density of 10 mA cm-2. In principle, the success relies on the intrinsically improved conductivity, increased specific surface area and the number of active sites, as well as the heterojunction structure of the catalyst. Therefore, this work provides a new idea for the design and preparation of more efficient noble-metal-free bifunctional electrocatalysts. © 2023, The Authors. All rights reserved.

关键词： Electrocatalysts

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