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Continuous wildfires threaten public and ecosystem health under climate change across continents

Frontiers of Environmental science & engineering 2024年第10期18卷 165-174页

作者： Guochao Chen Minghao Qiu Peng Wang Yuqiang Zhang Drew Shindell Hongliang Zhang Department of Environmental Science and Engineering Fudan UniversityShanghai 200438China Doerr School of Sustainability and Center for Innovation in Global Health Stanford UniversityStanfordCA 94305USA School of Marine and Atmospheric Science and Program in Public HealthStony Brook UniversityStony BrookNY 11794USA Department of Atmospheric and Marine Sciences Fudan UniversityShanghai 200438China IRDR ICoE on Risk Interconnectivity and Governance on Weather/Climate Extremes Impact and Public Health Fudan UniversityShanghai 200438China Environment Research Institute Shandong UniversityQingdao 266237China Nicholas School of the Environment Duke UniversityDurhamNC 27708USA Institute of Eco-Chongming Shanghai 200062China

Wildfires burn approximately 3%-4% of the global land area annually,resulting in massive emissions of greenhouse gases and air *** the past two decades,there has been a declining trend in both global burned area and wildfire *** trend is largely attributed to a decrease in wildfire activity in Africa,which accounts for a substantial portion of the total burned area and ***,the northern high-latitude regions of Asia and North America have witnessed substantial interannual variability in wildfire activity,with several severe events occurring in recent *** plays a pivotal role in influencing wildfire activity and has led to more wildfires in high-latitude *** wildfires pose significant threats to climate,ecosystems,and human *** recent changes in wildfire patterns and their impacts,it is critical to understand the contributors of wildfires,focus on deteriorating high-latitude areas,and address health risks in poorly managed areas tomitigate wildfire effects.

关键词： Wildfire activity Wildfire emissions Climate change Airquality

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Land Suitability Evaluation of New Settlement for Citizen Affected by the Construction of Cisokan Reservoir in West Bandung 4

Land Suitability Evaluation of New Settlement for Citizen Af...

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4th International Conference on sustainability science, CSS 2020

作者： Padhlulloh, Luthpi Parikesit Hadi, Firman Environment Science Program Postgraduate School Universitas Padjadjaran Indonesia Center for Environment and Sustainability Science Padjadjaran University Indonesia Lecture at Geodesy Engineering Department Faculty of Engineering Universitas Diponegoro Indonesia

The construction of the Cisokan Reservoir caused residents who previously lived and carried out activities around the land that would be inundated to have to move to another place. Based on the Land Acquisition and Relocation report, 10 locations were selected and already occupied by residents affected by the construction of the Cisokan Reservoir to be used as new residential land. An increase in the population of a space in a certain period of time is accompanied by an increase in the need for land, especially for housing needs. In an agrarian society, land is also needed for a production function. Land use for settlements must be regulated by taking into account ecological aspects so as not to cause problems and disasters in the future. With the Geographical Information System approach with the spatial scoring technique, the final results obtained at the research location were 3 land suitability classes, namely S1, S2, and S3 classes. The land suitability class N was not found in the study area. Meanwhile, for the resettlement locations of residents affected by the construction of the Cisokan reservoir from the 10 locations, all locations are in areas with land suitability class S2. © The Authors, published by EDP sciences, 2021.

关键词： Location

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Theoretical insights into metal-doped nanostructured hematite catalyst supported by graphene underlayer for photoelectrochemical water splitting applications

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Discover Catalysis 2025年第1期2卷 1-27页

作者： Bhattacharya, Labanya Caspary Toroker, Maytal Department of Materials Science and Engineering Technion-Israel Institute of Technology Haifa Israel The Nancy and Stephen Grand Technion Energy Program Technion-Israel Institute of Technology Haifa Israel Resnick Sustainability Center for Catalysis Technion-Israel Institute of Technology Haifa Israel

Catalysis is pivotal in the production of green hydrogen through water splitting to meet the goal of carbon neutrality. Hematite (Fe2O3) is an excellent catalyst and benchmarked photoanode materials in photoelectrochemical water splitting. Among the metal dopants, aluminum (Al) substitution in hematite is found intrinsically. In this study, we investigate Al doped nanostructured hematite as a photoanode material and a catalyst in water oxidation mechanism using density functional theory+ U methodology. We have found that Al doping in hematite monolayer leads to unfavorable increase in theoretical overpotential value by 0.19 V. To improve the efficiency of oxygen evolution reaction, we consider heterostructuring of Al doped nanostructured hematite with pristine graphene and nitrogen (N) doped graphene as an underlayer material. Nitrogen doped graphene underlayer leads to the lowest overpotential value of 0.54 V compared to Al doped hematite catalyst (0.96 V) and graphene-Al doped hematite catalyst (0.63 V). The work function is notably reduced after nitrogen doping by 1.41 eV and 1.12 eV as compared to graphene-Al doped hematite and Al doped hematite, respectively. Charge density difference and Bader charge analysis confirm that nitrogen doped graphene underlayer induces delocalized charge density and lowers the activity of the surface states in the *O intermediate. Nitrogen doped graphene-Al doped hematite heterostructure has nearly zero band gap and has the highest cumulative probability of charge transport at photoanode’s surface. Our theoretical study provides mechanistic insights into improving the catalytic efficiency of Al doped nanostructured hematite by heterostructuring with pristine and N doped graphene.

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Advanced TiO2/Al2O3 Bilayer ALD Coatings for Improved Lithium-Rich Layered Oxide Electrodes

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ACS Applied Materials and Interfaces 2024年第10期16卷 13029-13040页

作者： Chen, Wei-Ming Hsieh, Hsin-Yu Wu, Dong-Ze Tang, Horng-Yi Chang-Liao, Kuei-Shu Chi, Po-Wei Wu, Phillip M. Wu, Maw-Kuen Institute of Physics Academia Sinica 128 Section 2 Academia Road Taipei11529 Taiwan Nano Science and Technology Program Taiwan International Graduate Program Academia Sinica and National Tsing Hua University 128 Section 2 Academia Road Taipei11529 Taiwan Department of Engineering and System Science National Tsing Hua University 101 Section 2 Kuang-Fu Road Hsinchu300044 Taiwan Graduate Institute of Energy and Sustainability Technology National Taiwan University of Science and Technology 43 Keelung Road Sec 4 Taipei10607 Taiwan Department of Applied Chemistry National Chi Nan University 1 University Road Puli Nantou545301 Taiwan College of Science National Chung Hsing University 145 Xingda Rd. South Dist. Taichung City402 Taiwan

Surface modification is a highly effective strategy for addressing issues in lithium-rich layered oxide (LLO) cathodes, including phase transformation, particle cracking, oxygen gas release, and transition-metal ion dissolution. Existing single-/double-layer coating strategies face drawbacks such as poor component contact and complexity. Herein, we present the results of a low-temperature atomic layer deposition (ALD) process for creating a TiO2/Al2O3 bilayer on composite cathodes made of AS200 (Li1.08Ni0.34Co0.08Mn0.5O2). Electrochemical analysis demonstrates that TiO2/Al2O3-coated LLO electrodes exhibit improved discharge capacities and enhanced capacity retention compared with uncoated samples. The TAA-5/AS200 bilayer-coated electrode, in particular, demonstrates exceptional capacity retention (∼90.4%) and a specific discharge capacity of 146 mAh g-1 after 100 cycles at 1C within the voltage range of 2.2 to 4.6 V. The coated electrodes also show reduced voltage decay, lower surface film resistance, and improved interfacial charge transfer resistances, contributing to enhanced stability. The ALD-deposited TiO2/Al2O3 bilayer coatings exhibit promising potential for advancing the electrochemical performance of lithium-rich layered oxide cathodes in lithium-ion batteries. © 2024 The Authors. Published by American Chemical Society.

关键词： Cathodes

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Preparation of LFP-based cathode materials for lithium-ion battery applications

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Materials Today: Proceedings 2022年 65卷 2347-2350页

作者： Suttison, Suchanat Pengpat, Kamonpan Intatha, Uraiwan Fan, Jinchen Zhang, Wei Eitssayeam, Sukum Master's Degree Program in Materials Science Faculty of Science Chiang Mai University Chiang Mai 50200 Thailand Graduate School Chiang Mai University Chiang Mai Thailand Department of Physics and Materials Science Faculty of Science Chiang Mai University Thailand Center of Innovative Materials for Sustainability School of Science Mae Fah Luang University Chiang Rai 57100 Thailand School of Materials and Chemistry University of Shanghai for Science and Technology Shanghai 200093 China Department of Engineering Mechanics Dalian University of Technology Dalian 116024 China

Lithium-ion batteries (LIB) have developed into the mainstream power source of energy storage devices due to their advantages: high power density, high power, long service life, and less pollution. This materials development for LFP batteries was considered successful in synthesizing powder. Here we show that three synthesis conditions were performed. LFP doped NiO, NMC, and (NH4)2HPO4 were synthesized by the nitrogen gas flow method. LFP-doped NiO was burned at 600 °C and 700 °C for five h. NMC doped with LFP burned at 550 °C for five h, and NMC-doped LFP and (NH4)2HPO4 were burned at 550 °C and 600 °C for five h. The structure and morphology of the material were examined by X-ray diffraction (XRD) and scanning electron microscopy (SEM). © 2022

关键词： Lithium-ion batteries

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Comprehensive assessment of water and sediment quality to support sustainable management practices and mitigate potential risks of trace metal pollution in the Johor River Basin, South Peninsular Malaysia

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Ecohydrology and Hydrobiology 2025年第2期25卷 315-329页

作者： Mazilamani, Lelavathy S. Annammala, Kogila V. Martin, Patrick Qi, Liang Y. Sugumaran, Dhinesh Ling, Yong E. Reynard, P.S. Nurhidayat, Agus Syawal, Muhamad S. Sutapa, Ignasius D.A. Department of Water & Environmental Engineering Faculty of Civil Engineering Universiti Teknologi Malaysia Johor Bahru Malaysia Disaster Preparedness and Prevention Centre Universiti Teknologi Malaysia Kuala Lumpur Malaysia Asian School of the Environment Nanyang Technological University Singapore Centre of Environmental Sustainability & Water Security (IPASA) Research Institute for Sustainable Environment (RISE) Universiti Teknologi Malaysia Johor Bahru Malaysia Faculty of Engineering – Industrial Engineering International Study Program University of Indonesia Indonesia Asia Pacific Centre for Ecohydrology (APCE) – UNESCO C2C Indonesia Research Centre for Limnology and Water Resources – NRIA Indonesia Faculty of Environmental Science and Technology – Soegijapranata Catholic University (SCU) Semarang Indonesia

Human activities have caused concerns over the contamination of trace elements in aquatic systems due to their toxicity, long-lasting nature, and ability to accumulate in living organisms. This study evaluated the spatial pattern, environmental hazard, and potential health hazard of 13 trace metals in water and sediment samples collected from the Johor River basin using multivariate statistical techniques in order to identify the impact of both natural and human-related factors on the presence of trace metals in the area. The increased levels of metals in Station S1 indicated a significant impact from municipal, domestic, and industrial waste. The Geo-accumulation Index (I_geo) values for pollution and ecological indices in the sediment of the Johor River Basin ranged from -9.44 to 6.27. The Pollution Load Index (PLI) values ranged from 0.05 to 0.18, and the Potential Ecological Risk Assessment (RI) values ranged from 2.15 to 11.18. These results indicate that the sediments in the Johor River Basin have a low risk of contamination from trace metals. The water's hazard quotient (HQ) had an average value of 0.0001, while the hazard index (HI) had an average value of 0.0003. It is important to increase stakeholders' understanding and concerns regarding the potential long-term human health and ecological implications associated with trace metals in Johor River water. The results of this study offer essential initial information for government entities to implement sustainable management strategies, reducing the likelihood of future trace metal contamination issues in the Johor River basin and similar regions. © 2024 European Regional Centre for Ecohydrology of the Polish Academy of sciences

关键词： Health assessment Johor river basin Multivariate analysis Sediment quality Trace metals Water quality

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MOF-Derived Bimetal-Embedded Carbon with Etched Morphologies as an Efficient Activator of Peroxymonosulfate for Eliminate Emerging Contaminants

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Korean Journal of Chemical engineering 2024年第6期41卷 1815-1831页

作者： Chen, Yi-Chun Jiang, Xin-Yu Lin, Jia-Yin Thanh, Bui Xuan Wang, Haitao Huang, Chao-Wei Ghotekar, Suresh Huang, Chih-Feng Lin, Kun-Yi Andrew Department of Biotechnology National Formosa University Yunlin63208 Taiwan Department of Environmental Engineering & amp Innovation and Development Center of Sustainable Agriculture National Chung Hsing University Taichung Taiwan Semiconductor and Green Technology Program National Chung Hsing University 250 Kuo-Kuang Road Taichung Taiwan Ho Chi Minh City Viet Nam Ho Chi Minh City700000 Viet Nam Key Laboratory of Pollution Processes and Environmental Criteria College of Environmental Science and Engineering Nankai University Tianjin300071 China Department of Engineering Science National Cheng Kung University Tainan70101 Taiwan Centre for Herbal Pharmacology and Environmental Sustainability Chettinad Hospital and Research Institute Chettinad Academy of Research and Education Kelambakkam Tamil Nadu Chennai603103 India Department of Chemical Engineering National Chung Hsing University Taichung Taiwan Institute of Analytical and Environmental Sciences National Tsing Hua University Hsinchu Taiwan Department of Civil Engineering National Taipei University of Technology Taipei City Taiwan

As bis(4-hydroxyphenyl)methanone (BHP) is one of the most common UV light stabilizers (UVLS), but exhibits endocrine disrupting toxicity, this study aims to develop useful sulfate radical-based techniques to eliminate BHP from water by activating peroxymonosulfate (PMS). Hence, while cobalt (Co) exhibits efficacy as a transition metal for the activation of PMS, the utilization of manganese/cobalt (Mn/Co) bimetallic oxides presents an even more encouraging prospect as heterogeneous catalysts for PMS activation. In this study, we have successfully produced N-doped carbon-supported Mn/Co nanoparticles (NCMC) with a distinctive hollow-engineered nanostructure. The synthesis involved the utilization of Co-MOF as a precursor, followed by easy etching and Mn doping to achieve the desired composition of Mn/Co bimetallic oxide nanoparticles. The inclusion of Mn dopant facilitates the integration of Mn/Co nanoparticles into the hollow-structured N-doped carbon matrix. NCMC demonstrates much higher activity compared to NCC and the benchmark catalyst, Co3O4 NP, in terms of PMS activation for the degradation of BHP. The findings of the eco-toxicity study indicate that the degradation of BHP by NCMC + PMS does not yield hazardous or extremely toxic byproducts, so establishing NCMC as a potentially effective heterogeneous catalyst for activating PMS in the degradation of BHP. © The Author(s), under exclusive licence to Korean Institute of Chemical Engineers, Seoul, Korea 2024.

关键词： Transition metals

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Spatially differentiated life cycle assessment of Thailand's transport: The implications from country-specific factors and alternative technologies

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Sustainable Production and Consumption 2025年 57卷 319-340页

作者： Vitoon Chotanapund Shabbir H. Gheewala Vladimir Strezov Nazmul Huda Jitti Mungkalasiri Trakarn Prapaspongsa Graduate Program in Environmental and Water Resources Engineering Department of Civil and Environmental Engineering Faculty of Engineering Mahidol University Nakhon Pathom Thailand School of Natural Sciences Faculty of Science and Engineering Macquarie University NSW 2109 Australia The Joint Graduate School of Energy and Environment (JGSEE) King Mongkut's University of Technology Thonburi Bangkok Thailand Center of Excellence on Energy Technology and Environment Ministry of Higher Education Science Research and Innovation Ministry of Education Bangkok Thailand School of Engineering Faculty of Science and Engineering Macquarie University NSW 2109 Australia Technology and Informatics Institute for Sustainability (TIIS) National Metal and Materials Technology Center (MTEC) National Science and Technology Development Agency (NSTDA) Pathum Thani Thailand

This study proposed country-specific characterisation factors (CFs) for Thailand by modifying the Thai Spatially Differentiated Life Cycle Impact Assessment (ThaiSD) method and introducing monetary conversion factors to express environmental impacts in Thai Baht. Five impact categories were fully parameterised, including fine particulate matter formation (PMF), human toxicity (both cancer and non-cancer) (HT c and HT nc ), freshwater ecotoxicity (FET), and water scarcity (WS). Other spatialised CFs were selected from regionalisation models in ReCiPe2016 and IMPACT World+. When comparing the use of country-specific CFs with global average, the impact scores for PMF, HT c , HT nc , FET, photochemical ozone formation and terrestrial acidification demonstrated notably different levels, ranging from ±25 to ±50 %. The developed method was then applied to assess environmental impacts and costs of Thailand's transport sector, encompassing freight and passenger transport across roadway, railway, waterway, and aviation. Climate change (CC) was significantly attributed to human health and ecosystem quality impacts, while the major contributor to resource scarcity impact was fossil resource scarcity (FS). In some scenarios, non-exhaust emissions, particularly from freight trucks, accounted for 40–60 % of the total PMF impacts. Environmental costs of freight and passenger transport in Thailand were 0.08–3.64 Thai Baht per tonne-kilometre and 0.01–0.81 Thai Baht per passenger-kilometre, respectively. Among transport modes, trains were found to be the most environmentally favourable option for both passenger and freight transport, while aviation had the highest environmental impact for freight transport. In contrast, passenger aviation had a comparable environmental burden to passenger cars due to optimised occupancy rates. Despite the efficiency of modern internal combustion engine vehicles (ICEVs), particularly Euro 5 and 6, employing blended biodiesel was less effective in comp

关键词： Life cycle assessment Thai Spatially Differentiated Life Cycle Impact Assessment Freight transport Passenger transport Transport technologies

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Electrospun Aligned PCL/Gelatin Scaffolds Mimicking the Skin ECM for Effective Antimicrobial Wound Dressings

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Advanced Fiber Materials 2023年第1期5卷 235-251页

作者： Erfan Rezvani Ghomi Rajamani Lakshminarayanan Vijila Chellappan Navin Kumar Verma Amutha Chinnappan Rasoul Esmaeely Neisiany Kottaiswamy Amuthavalli Zhi Sheng Poh Brandon Han Siang Wong Nileshkumar Dubey Roger Narayan Seeram Ramakrishna Department of Mechanical Engineering Center for Nanotechnology and SustainabilityNational University of SingaporeSingapore 117581Singapore Ocular Infections and Antimicrobials Research Group Singapore Eye Research InstituteThe Academia20 College RoadDiscovery TowerSingapore 169856Singapore Institute of Materials Research and Engineering(IMRE) Agency for Science Technology and Research(A*STAR)#08‑032 Fusionopolis WayInnovisSingapore 138634Singapore Lee Kong Chian School of Medicine Nanyang Technological University SingaporeClinical Sciences Building11 Mandalay RoadSingapore 308232Singapore Department of Pharmacy National University of Singapore18 Science Drive 4Singapore 117543Singapore Academic Clinical Program in Ophthalmology and Visual Sciences Academic Clinical Program Duke-NUS Medical SchoolSingapore 169857Singapore National Skin Centre 1 Mandalay RoadSingapore 308205Singapore Department of Materials and Polymer Engineering Faculty of EngineeringHakim Sabzevari UniversitySabzevar ***Iran Faculty of Dentistry National University of SingaporeSingapore 119085Singapore ORCHIDS:Oral Care Health Innovations and Designs Singapore National University of SingaporeSingaporeSingapore 119085Singapore Department of Biomedical Engineering University of North Carolina at Chapel HillChapel HillNC 27514USA

Bacterial infections and multidrug-resistant bacteria are major health burdens in wound *** antimicrobial agents,e.g.,ε-polylysine(ε-PL),provide a broad spectrum of antibacterial properties and support dermal cell ***,ε-PL was incorporated into polycaprolactone(PCL)/gelatin electrospun scaffolds collected at varying rotation ***,the samples were crosslinked using dopamine hydrochloride to provide highly proliferative dressings with broad antimicrobial *** morphological study showed that the electrospun wound dressings were smooth,continuous,and bead-free,with a mean diameter ranging from 267±7 to 331±8 nm for all random and aligned *** fiber alignment of the electrospun PCL/gelatin scaffolds improved their tensile strength and ***,nanofiber mats are highly hydro-philic,which is crucial for an efficient wound *** samples also demonstrated high antimicrobial properties against common wound bacterial strains,including methicillin-resistant Staphylococcus aureus(MRSA),Staphylococcus aureus(SA),Escherichia coli(EC),Acinetobacter baumannii(AB),and Pseudomonas aeruginosa(PA).Mammalian cell prolifera-tion and morphology assays involving primary human dermal fibroblasts(hDFs)and immortalized keratinocytes(HaCaT)showed excellent biocompatibility of the electrospun mats and remarkably aligned ***,aligned mats showed more cell migration than randomly oriented mats,which is desirable for more efficient wound ***,it can be concluded that aligned PCL/gelatin mats containingε-PL are promising for potential use in wound dressings.

关键词： Electrospinning Wound healing Fiber alignment Biomaterials Nanofiber dressing Bacterial infections

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Perception of Disasters and Land Reclamation in an Informal Settlement on Reclaimed Land:Case of the BASECO Compound,Manila,the Philippines

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International Journal of Disaster Risk science 2020年第5期11卷 640-654页

作者： Ven Paolo Bruno Valenzuela Miguel Esteban Onuki Motoharu Graduate Program in Sustainability Science-Global Leadership Initiative The University of TokyoKashiwaChiba 277-8563Japan Department of Civil and Environmental Engineering Waseda UniversityTokyo 169-8555Japan

Southeast Asia's coastal urban areas continue to grow,with land reclamation fast becoming an important option for megacities to address issues of economic growth and increasing population *** are divided over the advantages and disadvantages of land reclamation,though this process continues unabated,exposing settlements to coastal *** Bataan Shipping and engineering Company(BASECO)compound is an informal settlement on reclaimed land in Manila,the *** informal coastal settlements view disaster risk and their more pressing socioeconomic needs is crucial to understanding the potentials and repercussions of land *** a topographic survey,a questionnaire survey,and the protective action decision model,this study explored the perception of disasters and land reclamation of informal settlers who are living on reclaimed *** study found that people are aware of disaster risks,but are more concerned with everyday *** are divided on the issue of further land *** on the original non-reclaimed land view it as a coastal defense,while those on reclaimed land fear potential *** this,all locations in the community are concerned with the loss of jobs,economic opportunities,and eviction,rather than potential disasters.

关键词： Coastal hazards Flooding Informal settlements Land reclamation Philippines Risk perception Urbanization

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