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Recent advances in elaborate interface regulation of BiVO_(4)photoanode for photoelectrochemical water splitting

Materials Reports(Energy) 2023年第4期3卷 3-18页

作者： Liming Wang Yaping Zhang Weibing Li Lei Wang Key Laboratory of Eco-chemical Engineering International Science and Technology Cooperation Base of Eco-chemical Engineering and Green ManufacturingCollege of Environment and Safety EngineeringQingdao University of Science and TechnologyQingdao266042PR China

Bismuth vanadate(BiVO_(4))is an excellent photoanode material for photoelectrochemical(PEC)water splitting system,possessing high theoretical photoelectrocatalytic conversion ***,the actual PEC activity and stability of BiVO_(4)are faced with great challenges due to factors such as severe charge recombination and slow water oxidation kinetics at the ***,various interface regulation strategies have been adopted to optimize the BiVO_(4)*** review provides an in-depth analysis for the mechanism of interface regulation strategies from the perspective of factors affecting the PEC performance of BiVO_(4)*** interface regulation strategies improve the PEC performance of BiVO_(4)photoanode by promoting charge separation and transfer,accelerating interfacial reaction kinetics,and enhancing *** research on the interface regulation strategies of BiVO_(4)photoanode is of great significance for promoting the development of PEC water splitting *** the same time,it also has inspiration for providing new ideas and methods for designing and preparing efficient and stable catalytic materials.

关键词： Photoelectrochemical water splitting BiVO_(4)photoanode Charge recombination Water oxidation reaction kinetics Interface regulation strategy

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Chemically bonded multi-nanolayer inorganic aerogel with a record-low thermal conductivity in a vacuum

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National Science Review 2023年第10期10卷 96-105页

作者： Hongxuan Yu Menglin Li Yuanpeng Deng Shubin Fu Jingran Guo Han Zhao Jianing Zhang Shixuan Dang Pengyu Zhang Jian Zhou Dizhou Liu Duola Wang Chuanwei Zhang Menglong Hao Xiang Xu Key Lab of Smart Prevention and Mitigation of Civil Engineering Disasters of the Ministry of Industry and Information Technology and Key Lab of Structures Dynamic Behavior and Control of the Ministry of Education Harbin Institute of Technology Key Laboratory of Energy Thermal Conversion and Control of Ministry of Education School of Energy and EnvironmentSoutheast University Key Lab of Aerospace Bearing Technology and Equipment of the Ministry of Industry and Information Technology Harbin Institute of Technology

Inorganic aerogels have exhibited many superior characteristics with extensive applications,but are still plagued by a nearly century-old tradeoff between their mechanical and thermal *** reducing thermal conductivity by ultralow density,inorganic aerogels generally suffer from large fragility due to their brittle nature or weak joint crosslinking,while enhancing the mechanical robustness by material design and structural engineering,they easily sacrifice thermal insulation and ***,we report a chemically bonded multi-nanolayer design and synthesis of a graphene/amorphous boron nitride aerogel to address this typical tradeoff to further enhance mechanical and thermal *** to the chemically bonded interface and coupled toughening effect,our aerogels display a low density of 0.8 mg cm-3with ultrahigh flexibility（elastic compressive strain up to 99% and bending strain up to 90%）,and exceptional thermostability（strength degradation <3% after sharp thermal shocks）,as well as the lowest thermal conductivities in a vacuum(only 1.57 mW m-1K-1at room temperature and 10.39 mW m-1K-1at500℃) among solid materials to *** unique combination of mechanical and thermal properties offers an attractive material system for thermal superinsulation at extreme conditions.

关键词： inorganic aerogels multi-nanolayer mechanical-thermal tradeoff flexibility thermal superinsulation

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2D phosphides heterostructures on titanium microfiltration membrane for enhanced ampere-level current density overall seawater splitting

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Nano Research 2025年第1期18卷 249-259页

作者： Wenjing Dai Xin Wang Yulong Ma Sisi He Ming Chen Zhaohui Yin Shuheng Tian Maolin Wang Shixiang Yu Hang Zhang Yuanzhe Wang Hong Wang Jianxin Li Faming Gao Bowen Cheng Yun Wang Zhen Yin Ding Ma Tianjin Key Laboratory of Brine Chemical Engineering and Resource Eco-utilization College of Chemical Engineering and Materials ScienceTianjin University of Science and TechnologyTianjin 300457China State Key Laboratory of Biobased Fiber Manufacturing Technology Tianjin University of Science and TechnologyTianjin 300457China Haian Institute of High-Tech Research Nanjing UniversityHaian 226600China Beijing National Laboratory for Molecular Sciences College of Chemistry and Molecular EngineeringPeking UniversityBeijing 100871China State Key Laboratory of Separation Membranes and Membrane Processes Separation Membrane Science and Technology International Joint Research CentreTiangong UniversityTianjin 300387China Centre for Catalysis and Clean Energy School of Environment and ScienceGold Coast CampusGriffith UniversitySouthportQueensland 4222Australia

The advancement of direct seawater electrolysis is a significant step towards sustainable hydrogen production,addressing the critical need for renewable energy sources and efficient resource ***,direct seawater electrolysis has to face several challenges posed by the corrosiveness of highly concentrated chloride and the competitive chlorine evolution reaction(ClER).To overcome these issues,we designed a novel NiP_(2)@CoP electrocatalyst on a porous titanium microfiltration(Ti MF)*** obtained bifunctional NiP_(2)@CoP catalyst outperforms the Pt/C and IrO_(2),as evidenced by its low overpotentials of 192 and 425 mV at a current density of 500 mA·cm^(-2) for hydrogen evolution reaction(HER)and oxygen evolution reaction(OER)in alkaline seawater(1 M KOH+0.5 M NaCl),***,only 231 and 569 mV overpotentials are required at the current density of 1500 mA·cm^(-2) towards HER and OER in alkaline seawater,*** importantly,no ClER was observed,demonstrating its excellent selectivity to *** selection of porous Ti MF membrane as an electrode substrate further enhances the performance by providing a robust structure that promotes the fast generation and release of gas *** promising outcomes obtained with NiP_(2)@CoP catalysts on Ti MF support,therefore,pave the way for the commercial viability of direct seawater electrolysis technologies at industrial-level current densities.

关键词： direct seawater electrolysis porous titanium microfiltration membrane phosphides heterostructures NiP_(2)@CoP electrocatalyst excellent selectivity to oxygen evolution reaction(OER)

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Developing modified k–εturbulence models for neutral atmospheric boundary layer flow simulation using OpenFOAM

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Building Simulation 2024年第12期17卷 2281-2295页

作者： Yuanbo Wang Jiqin Li Wei Liu Jiankai Dong Jing Liu School of Architecture Harbin Institute of TechnologyKey Laboratory of Cold Region Urban and Rural Human Settlement Environment Science and TechnologyMinistry of Industry and Information TechnologyHarbin 150090China Tianjin Key Laboratory of Indoor Air Environmental Quality Control School of Environmental Science and EngineeringTianjin University92 Weijin RoadTianjin 300072China Division of Sustainable Buildings Department of Civil and Architectural EngineeringKTH Royal Institute of TechnologyBrinellvägen 2310044 StockholmSweden

Accurate turbulence modeling is essential for simulation studies of urban *** this study,the comprehensive atmospheric boundary layer(ABL)model involving a variable model coefficient and an additional turbulent dissipation source term was implemented using the open-source software *** with consistent inlet wind profiles and rough wall functions of different turbulence variables based on the aerodynamic roughness,the model maintained the horizontal homogeneity ***,a hybrid approach was introduced to consider buildings immersed in ABL flows,enabling automatic transformation of the turbulence model between the region around the buildings and the free flow region away from any ***,the effects of applying different model forms to the airflow field around buildings were evaluated in detail through three-dimensional building cases representing six urban prototypes based on three wind tunnel *** findings indicated that all modified k–εmodels perform well in reproducing the flow data of the CEDVAL and Architectural Institute of Japan(AIJ)experiments consisting of a single building,an array of buildings,and an isolated high-rise ***,the modified k–εmodel with an additional correction term performed poorly in the database of Niigata Institute of technology and the case of complex terrain and urban building configurations,because the correction term inhibited the generation of turbulent kinetic *** addition,from the comparison between the experimental data of all cases,the model with the original formulation of the coefficient performed the best in terms of prediction *** root mean square errors of the normalized velocity were 0.1250,0.0879,0.1145,0.1350,and 0.1492 in different cases,which proved the reliability of this turbulence model.

关键词： urban airflow computational fluid dynamics(CFD) atmospheric boundary layer OpenFOAM turbulence model

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The degradation of perovskite precursor

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Journal of Semiconductors 2023年第10期44卷 3-6页

作者： Mengjia Li Lixiu Zhang Cong Chen Jiangzhao Chen Liming Ding State Key Laboratory of Reliability and Intelligence of Electrical Equipment School of Materials Science and EngineeringHebei University of TechnologyTianjin 300401China Key Laboratory of Optoelectronic Technology&Systems(MoE) College of Optoelectronic EngineeringChongqing UniversityChongqing 400044China Center for Excellence in Nanoscience(CAS) Key Laboratory of Nanosystem and Hierarchical Fabrication(CAS)National Center for Nanoscience and TechnologyBeijing 100190China Macao Institute of Materials Science and Engineering(MIMSE) Macao University of Science and TechnologyMacao 999078China

Perovskite solar cells(PSCs)are taking a leading position in thin-film optoelectronic devices due to their excellent optical,physical and electrical properties[1-4].Nevertheless,the stability issue of metal halide perovskite precursor solution severely retards the future industrialization of PSCs[5-7].In stoichiometry,slight solution composition change will induce severe degradation of device performance.

关键词： perovskite halide film

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Mantle flow underneath the South China Sea revealed by seismic anisotropy

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National Science Review 2023年第10期10卷 54-61页

作者： Fansheng Kong Rui Gao Stephen S.Gao Kelly H.Liu Weiwei Ding Xiongwei Niu Aiguo Ruan Pingchuan Tan Jianke Fan Shaoping Lu Zhengyi Tong Liqun Cheng Wenfei Gong Yanghui Zhao Jiabiao Li Key Laboratory of Submarine Geosciences Second Institute of OceanographyMinistry of Natural Resources Southern Marine Science and Engineering Guangdong Laboratory Geology and Geophysics Program Department of Geosciences and Geological and Petroleum Engineering Missouri University of Science and Technology School of Earth Sciences and Engineering Sun Yat-sen University Key Laboratory of Marine Geology and Environment Institute of Oceanology Chinese Academy of Sciences

It has long been established that plastic flow in the asthenosphere interacts constantly with the overlying lithosphere and plays a pivotal role in controlling the occurrence of geohazards such as earthquakes and volcanic ***,accurately characterizing the direction and lateral extents of the mantle flow field is notoriously difficult,especially in oceanic areas where deployment of ocean bottom seismometers(OBSs) is expensive and thus *** this study,by applying shear wave splitting analyses to a dataset recorded by an OBS array that we deployed between mid-2019 and mid-2020 in the South China Sea(SCS),we show that the dominant mantle flow field has a NNW-SSE orientation,which can be attributed to mantle flow extruded from the Tibetan Plateau by the ongoing Indian-Eurasian *** addition,the results suggest that E-W oriented flow fields observed in South China and the Indochina Peninsula do not extend to the central SCS.

关键词： mantle flow South China Sea Tibetan Plateau seismic anisotropy shear wave splitting

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Sequence structure controllable polymerization-induced self-assembly

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Science China Chemistry 2024年第1期67卷 390-397页

作者： Zi-Xuan Chang Ren-Man Zhu Chun-Yan Hong Wen-Jian Zhang Department of Polymer Science and Engineering University of Science and Technology of ChinaHefei 230026China Institute of Physical Science and Information Technology Anhui UniversityHefei 230601China Key Laboratory of Environment-Friendly Polymeric Materials of Anhui Province Anhui UniversityHefei 230601China

Polymerization-induced self-assembly(PISA)combines synthesis and self-assembly of artificial polymers in one-pot,which brings us one step closer to emulating ***,the reported PISA formulations primarily focus on developing nano-objects with new chemical compositions and rarely on structural regulation of polymers with specific ***,sequence structure controllable polymerization-induced self-assembly(SCPISA)is reported by using 7-(2-methacryloyloxyethoxy)-4-methylcoumarin(CMA)as a *** the copolymerization of 2-hydroxyethyl methacrylate(HEMA)and CMA,controlled incorporation of CMA units into the polymer chains can be realized by programmable light/heat ***-based P(HEMA-co-CMA)copolymers with the same composition but different sequence structures generate a range of ***,the morphologies of the resultant nano-objects can also be controlled by regulating the feed molar ratio of CMA and HEMA,which is similar to the conventional PISA,but the synthesis procedure is obviously simplified in *** versatility of the methodology is further demonstrated by the fabrication of different functional nano-objects with sequence structure-dependent morphologies in SCPISA systems with different functional monomers.

关键词： polymerization-induced self-assembly sequence-controlled polymers PET-RAFT polymerization

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A mechanically durable,excellent recyclable 3D hierarchical Ni_(3)S_(2)@Ni foam photothermal membrane

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Green Energy & environment 2022年第3期7卷 492-499页

作者： Zhongping Yao Kailun Yu Mengyao Pan Hongbo Xu Tianqi Zhao Zhaohua Jiang School of Chemistry and Chemical Engineering State Key Laboratory of Urban Water Resource and EnvironmentHarbin Institute of TechnologyHarbin150001China

Solar-driven water evaporation is considered to be a viable and very efficient technology for fresh water ***,the photothermal membrane has a low absorptivity,low photothermal conversion and poor recyclability,which are difficult to meet the demands of self-floating solar driven evaporators in practical ***,a hierarchical nanostructure Ni_(3)S_(2) has been prepared by in-situ growing method on Ni foam(NF),which shows excellent absorptivity,outstanding recyclable and high mechanically durable *** photothermal membrane was composed of hierarchical nanostructure Ni_(3)S_(2)@NF,which exhibited excellent solar absorption(93.13%) in the wavelength range of 250–2500 nm and sustained anti-corrosion capacity for one *** addition,the hierarchical nanostructure Ni_(3)S_(2)@NF has good hydrophilicity and strong binding force,indicating this photothermal membrane exhibits good stability and outstanding photothermal conversion *** evaporation system based on 3D Ni_(3)S_(2)@NF membrane exhibited excellent water evaporation ability,the highest water evaporation rate(1.53 kg m^(-2)h^(-1)) and the photothermal conversion efficiency(84.7%) under 1 sun *** the desalination experiment,the water evaporation rate and photothermal conversion efficiency almost keep constant over 5 cycles tests and do not decrease compared with the experiment in pure *** result demonstrated that the Ni_(3)S_(2)@NF membrane has shown good corrosion resistance and outstanding *** to the simple preparation method,low cost,outstanding recyclability and high mechanical durability in the sea water,this Ni_(3)S_(2)@NF membrane have great potential for long-term solar distillation applications.

关键词： corrosion durability illumination

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Wetting front migration model of ion-adsorption rare earth during the multi-hole unsaturated liquid injection

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Journal of Rock Mechanics and Geotechnical engineering 2024年第2期16卷 483-496页

作者： Yu Wang Xiaojun Wang Yuchen Qiu Hao Wang Gang Li Kaijian Hu Wen Zhong Zhongqun Guo Bing Li Chunlei Zhang Guangxiang Ye Jiangxi Key Laboratory of Mining Engineering Jiangxi University of Science and TechnologyGanzhou341000China School of Resources and Environment Engineering Jiangxi University of Science and TechnologyGanzhou341000China School of Civil Engineering and Surveying&Mapping Engineering Jiangxi University of Science and TechnologyGanzhou341000China Ganzhou Nonferrous Metallurgy Research Institute Ganzhou341000China

In the process of ion-adsorption rare earth ore leaching,the migration characteristics of the wetting front in multi-hole injection holes and the influence of wetting front intersection effect on the migration distance of wetting fronts are still ***,wetting front migration distance and leaching time are usually required to optimize the leaching *** this study,wetting front migration tests of ionadsorption rare earth ores during the multi-hole fluid injection(the spacing between injection holes was 10 cm,12 cm and 14 cm)and single-hole fluid injection were completed under the constant water head *** the pre-intersection stage,the wetting front migration laws of ion-adsorption rare earth ores during the multi-hole fluid injection and single-hole fluid injection were *** the postintersection stage,the intersection accelerated the wetting front *** using the Darcy’s law,the intersection effect of wetting fronts during the multi-hole liquid injection was transformed into the water head height directly above the ***,based on the Green-Ampt model,a wetting front migration model of ion-adsorption rare earth ores during the multi-hole unsaturated liquid injection was *** analysis results showed that the proposed model can accurately simulate the infiltration process under experimental *** research results enrich the infiltration law and theory of ion-adsorption rare earth ores during the multi-hole liquid injection,and this study provides a scientific basis for optimizing the liquid injection well pattern parameters of ion-adsorption rare earth in situ leaching in the future.

关键词： Ion-adsorption rare earth ore Multi-hole unsaturated liquid injection In situ leaching Intersection effect Calculation model

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A review on Bi_(2)WO_(6)-based photocatalysts synthesis, modification, and applications in environmental remediation, life medical, and clean energy

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Frontiers of environmental Science & engineering 2024年第7期18卷 87-108页

作者： Wei Mao Xuewu Shen Lixun Zhang Yang Liu Zehao Liu Yuntao Guan Guangdong Provincial Engineering Technology Research Center for Urban Water Cycle and Water Environment Safety Tsinghua Shenzhen International Graduate SchoolTsinghua UniversityShenzhen 518055China State Environmental Protection Key Laboratory of Microorganism Application and Risk Control School of EnvironmentTsinghua UniversityBeijing 100084China

Photocatalysis has emerged a promising strategy to remedy the current energy and environmental crisis due to its ability to directiy convert clean solar energy into chemical *** tungstate(Bi_(2)WO_(6))has been shown to be an excellent visible light response,a well-defined perovskite crystal structure,and an abundance of oxygen atoms(providing efficient channels for photogenerated carrier transfer)due to their suitable band gap,effective electron migration and separation,making them ideal *** has been extensively applied as photocatalyst in aspects including pollutant removal,carbon dioxide reduction,solar hydrogen production,ammonia synthesis by nitrogen photocatalytic reduction,and cancer *** this review,the fabrication and application of Bi_(2)WO_(6) in photocatalysis were comprehensively *** photocatalytic properties of BizwO-based materials were significantly enhanced by carbon modification,the construction of heterojunctions,and the atom doping to improve the photogenerated carrier migration rate,the number of surface active sites,and the photoexcitation ability of the *** addition,the potential development directions and the existing challenges to improve the photocatalytic performance of Bi_(2)WO_(6)-based materials were discussed.

关键词： Bismuth tungstate Synthesis and modification Photocatalytic application environmental remediation Clean energy Medical science

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