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Decentralized Federated Learning Algorithm Under Adversary Eavesdropping

IEEE/CAA Journal of Automatica Sinica 2025年第2期12卷 448-456页

作者： Lei Xu Danya Xu Xinlei Yi Chao Deng Tianyou Chai Tao Yang the State Key Laboratory of Synthetical Automation for Process Industries Northeastern University the Department of Mechanical Engineering University of Victoria Shanghai Institute of Intelligent Science and Technology Tongji University IEEE the Institute of Advanced Technology Nanjing University of Posts and Telecommunications

In this paper, we study the decentralized federated learning problem, which involves the collaborative training of a global model among multiple devices while ensuring data *** classical federated learning, the communication channel between the devices poses a potential risk of compromising private information. To reduce the risk of adversary eavesdropping in the communication channel, we propose TRADE(transmit difference weight) concept. This concept replaces the decentralized federated learning algorithm's transmitted weight parameters with differential weight parameters, enhancing the privacy data against eavesdropping. Subsequently, by integrating the TRADE concept with the primal-dual stochastic gradient descent(SGD)algorithm, we propose a decentralized TRADE primal-dual SGD algorithm. We demonstrate that our proposed algorithm's convergence properties are the same as those of the primal-dual SGD algorithm while providing enhanced privacy protection. We validate the algorithm's performance on fault diagnosis task using the Case Western Reserve University dataset, and image classification tasks using the CIFAR-10 and CIFAR-100 datasets,revealing model accuracy comparable to centralized federated learning. Additionally, the experiments confirm the algorithm's privacy protection capability.

关键词： Adversary eavesdropping decentralized federated learning privacy protection stochastic gradient descent

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The analysis and assessment of DC-Link voltage control loop dynamics on the transient synchronization stability of grid-following converters

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Electric Power Systems Research 2025年 247卷

作者： Xie, Chenyang Lin, Xinchun Sun, Huiqiang Wei, Juntian Zhang, Jiayan State Key Laboratory of Advanced Electromagnetic Engineering and Technology Huazhong University of Science and Technology Wuhan China

The transient synchronization stability of grid-following voltage source converters has been extensively investigated, but most of the previous literature has only studied the transient dynamics of the phase-locked loop (PLL) while ignoring the dynamics of the DC-link voltage control (DVC) loop. When the bandwidths of the PLL and DVC are relatively close to each other, erroneous conclusions will be derived if neglecting the transient influence of the DVC loop. This paper first takes into account the transient dynamics of the DVC loop while applying the improved equal-area criterion (EAC) analysis, which reveals how the DVC loop affects the transient synchronization stability. Then, a fourth-order model considering the DVC dynamics is obtained to quantitatively determine a reasonable range of bandwidth and damping ratio for the DVC loop. Moreover, the extent of the influence of DVC on transient synchronization stability with variation of grid strength is analyzed. © 2025

关键词： Transient analysis

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Niobium oxide/MXene heterostructure for simultaneous production of ammonia and energy via rechargeable Zn-N2 battery system

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Journal of Energy Chemistry 2025年第4期103卷 448-457页

作者： Xinyu Dai Wei Zhang Ying Sun Zhenyi Du Zhanliang Tao Jingang Wang Wenhui Fang Xuehan Xing Yang Chen Hui Li Hao Zheng Jieshan Qiu Tianyi Ma Institute of Clean Energy Chemistry Key Laboratory for Green Synthesis and Preparative Chemistry of Advanced Materials of Liaoning Province College of ChemistryLiaoning University State Key Laboratory of Clean and Efficient Coal Utilization Taiyuan University of Technology Key Laboratory of Advanced Energy Materials Chemistry (Ministry of Education) Renewable Energy Conversion and Storage Center College of Chemistry Nankai University College of Science Liaoning Petrochemical University College of Chemical Engineering State Key Laboratory of Chemical Resource Engineering Beijing University of Chemical Technology Centre for Atomaterials and Nanomanufacturing (CAN) School of Science RMIT University ARC Industrial Transformation Research Hub for Intelligent Energy Efficiency in Future Protected Cropping (E2Crop) College of Chemical State Key Laboratory of Chemical Resource Engineering Beijing University of Chemical Technology

Aqueous Zn-N2batteries with unique configuration are of potential for simultaneous N2electro reduction and electricity generation,in which the electrocatalysts are critical for improving the NH3yield and the energy ***,a heterostructure Nb2O5/Nb2CTXwith abundant exposed Nb active sites and tuned electron density has been synthesized by in situ formation and anchoring of Nb2O5nanoparticles on the surface of Nb2CTXMXene,which shows an enhanced N2adsorption/activation *** heterostructure Nb2O5/Nb2CTXwas used as the cathode of Zn-N2battery that can deliver a peak power density of 1.25 mW cm-2in 1.0 M KOH and can continuously produce NH3with a yield of3.62 μg *** NH3formed in the battery system can be easily collected as a net product without circulating the ***,the Nb2O5/Nb2CTXhas a long durability,evidenced by 70 h of operation at-0.4 V *** hydrogen electrode,which is the highest among the MXene-based electrocatalysts reported thus *** work may provide a new methodology based on Zn-N2battery for sustainable and large-scale NH3production with minimal energy consumption.

关键词： NH 3 production Zn-N 2 battery N 2 Electroreduction Nb 2 O 5 /Nb 2 CT X heterostructure

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Nonflammable electrolyte with weak-solvation structure for stable NCM811 cathode under high temperature

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Journal of Energy Chemistry 2025年第5期104卷 111-117页

作者： Dawei Xu Chao Yang Ailing Yang Xiaowei Liu Meilong Wang Jin Han Tiefeng Liu Ya You State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of Technology International School of Materials Science and Engineering School of Materials Science and Microelectronics Wuhan University of Technology College of Chemical and Biological Engineering Zhejiang University Quzhou Institute of Power Battery and Grid Energy Storage

High-nickel cathode LiNi0.8Co0.1Mn0.1O2（NCM811） could enable lithium-ion batteries （LIBs） with high energy ***,excessive decomposition of the electrolyte would happen in the high operating voltage *** addition,the utilization of flammable organic solvents would increase safety risks in the high temperature ***,an electrolyte consisting of flame-retardant solvents with lower highest occupied molecular orbital （HOMO） level and LiDFOB salt is proposed to address above two *** a result,a thin and robust cathode-electrolyte interface containing rich LiF and Li-B-O compounds is formed on the cathode to effectively suppress electrolyte decomposition in the high operating *** NCM811||Li cell paired with this designed electrolyte possesses a capacity retention of 72% after 300 cycles at 55℃.This work provides insights into developing electrolyte for stable high-nickel cathode operated in the high temperature.

关键词： Electrolyte engineering High temperature High-nickel cathode Safety Weak solvation

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Numerical Study of the Current Density on the Armature and Rail Interface with Dynamic Contact

Numerical Study of the Current Density on the Armature and R...

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International Conference of Electrical, Electronic and Networked Energy Systems, EENES 2024

作者： Xu, Jinghan Xia, Shengguo Chen, Lixue Ministry of Education Hubei Wuhan430074 China State Key Laboratory of Advanced Electromagnetic Engineering and Technology Hubei Wuhan430074 China School of Electrical and Electronic Engineering Huazhong University of Science and Technology Wuhan430074 China

ISBN: (纸本)9789819620791

The electrical contact between the armature and rail is acknowledged as imperfect electrical contact (ImPEC), exhibiting characteristics distinct from bulk behavior. It is important to understand the current distribution of the ImPEC for future design and optimization. This paper proposes ImPEC boundary conditions by combining the contact layer model (CLM) and the Cooper-Mikic-Yoranovich model (CMYM), and the current distribution is numerically studied. Variations in the contact pressure and current density with time are analyzed. The results show a rapid increase in the contact pressure and area during the current ramp-up stage, being constant in the flat stage, and a gradual decline in the current ramp-down stage. The current path changes with the contact area, and the current shifts from the trailing edge to the leading edge over time. Additionally, comparative calculations are performed to analyze current variations under dynamic contact. Results suggest that the current distribution is influenced by magnetic diffusion and forced shifts of current caused by dynamic contact. © Beijing Paike Culture Commu. Co., Ltd. 2025.

关键词： Threshold current density

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Hierarchical hollow microspheres assembled from carbon nanosheets integrated with molybdenum carbide nanoparticles for boosting microwave absorption properties

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Nano Research 2025年第1期18卷 10-20页

作者： Zongsheng Chen Yahui Wang Yi Liu Zhigang Li Xiangyin Lv Liping Liu Yajing Chang Jiaming Shi Xiao Zhang State Key Laboratory of Pulsed Power Laser Technology School of Electronic EngineeringNational University of Defense TechnologyHefei 230037China Anhui Provincial Laboratory of Advanced Laser Technology School of Electronic EngineeringNational University of Defense TechnologyHefei 230037China Centre for Environmental and Energy Nanomaterials Anhui Key Laboratory of Nanomaterials and NanotechnologyCAS Centre for Excellence in NanoscienceInstitute of Solid State PhysicsHefei Institutes of Physical ScienceChinese Academy of SciencesHefei 230031China

Hierarchical hollow structure has demonstrated potential for enhancing electromagnetic(EM)attenuation and improving impedance matching,garnering significant attention for ***,we have successfully implemented compositional and structural engineering to fabricate hollow Mo2C/C microspheres with controllable composition by coupling interaction between dopamine hydrochloride and ammonium *** the synergistic effect of composition and hollow structure,the strongest reflection loss intensity and broadest effective absorption of the optimized sample reach-70.2 dB and 6.2 GHz,*** formation of hollow heterogeneous structures not only favors impedance matching feature,but also generates considerable contribution to EM attenuation ***,radar cross-section simulation data indicate that hollow Mo2C/C microspheres with compositional optimization and heterogeneous structures have broad prospects for practical applications.

关键词： electromagnetic absorption Mo2C/C microwave absorption hollow structure

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Microstructure and mechanical properties of nickel-based wrought superalloys under thermal-mechanical coupling: A review with Inconel 718,625 as main cases

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Progress in Natural Science:Materials International 2025年第1期35卷 65-82页

作者： Kai Cao Jiangkun Fan Xudong Liu Jianing Zhang Dian Jiao Yuelin Song Fulong Chen Jun Wang Bin Tang Hongchao Kou Jinshan Li State Key Laboratory of Solidification Processing Northwestern Polytechnical University National & Local Joint Engineering Research Center for Precision Thermoforming Technology of Advanced Metal Materials Chongqing Innovation Center Northwestern Polytechnical University AVIC Manufacturing Technology Institute

The typical processing and in-service behaviors of nickel-based wrought superalloys involve complex thermal-mechanical coupling effects, including elastic and plastic deformations, phase transformations, and other microstructural evolutions, directly impacting the mechanical properties. This review article provides an in-depth discussion on the microstructural evolution of these superalloys under thermal-mechanical coupling, focusing on two key aspects: the thermoplastic deformation behavior, and the phase transformation behavior in temperature/stress coupled field. The dynamic recrystallization(DRX) behavior during hot deformation and its improvement strategies are discussed in detail. The differences in phase precipitation behavior under conventional heat treatment and thermal-mechanical coupling conditions are compared. The mechanisms driving changes in precipitate characteristics are explored, enabling precise control of precipitates. This article further investigates the intricate relationship between the mechanical properties of nickel-based wrought superalloys and the characteristics of their precipitates, offering guidance for current and future optimizations. It also delves into the latest research advancements in precisely tailoring the precipitates through thermal-mechanical coupling methods to optimize these mechanical properties. Finally, it outlines several promising future research directions in this field.

关键词： Dynamic recrystallization

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Unveiling the confined dispersion mechanism of nanomaterials by stereocomplex cross-linked networks in polylactic acid

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Journal of Materials Science and technology 2025年 235卷 293-301页

作者： Su, Xiaolong Pan, Qingchun Zhai, Yaling Jia, Chao Wang, Jinqi Xu, Zhe Li, Jiaxin Zhao, Jian Xiang, Hengxue Wei, Xiaoding Zhu, Meifang State Key Laboratory of Advanced Fiber Materials College of Material Science and Engineering Donghua University Shanghai201620 China State Key Laboratory for Turbulence and Complex System Department of Mechanics and Engineering Science College of Engineering Beijing Innovation Center for Engineering Science and Advanced Technology Peking University Beijing100871 China College of Material Science and Engineering Xinjiang University Urumqi830046 China

Nanomaterials are extensively utilized in a multitude of sectors, but their propensity to aggregate can considerably diminish the efficacy of functional materials. A pivotal challenge in this domain is achieving a homogenous distribution of nanomaterials, which is essential for enhancing their performance while also reducing production costs. In this work, we achieve uniform and stable dispersion of various nanomaterials through the confinement effect generated by the stereocomplex cross-linked network formed by the combination of poly (L-lactic) acid and poly (D-lactic) acid. The unique confinement effect of polylactic acid (PLA) isomers is universal and significantly enhances the dispersion of nanomaterials in both PLA solutions and films. To demonstrate the efficacy of our approach, we disperse aggregation-induced emission (AIE) molecules within PLA, which leads to the production of PLA films exhibiting improved fluorescence property. This work provides an effective solution for the preparation of nanocomposite materials that are both high-performing and cost-efficient. © 2025

关键词： Nanoclay

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Nonlinear optical response of BiVO4 and its application for ultrafast pulsed fiber lasers

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Optics Express 2025年第3期33卷 6559-6566页

作者： Du, Ruonan Shi, Aokun Lian, Yudong Fang, Huajing Qi, Yaoyao Bai, Zhenxu Wang, Yulei Huang, Feng Ding, Jie Lu, Zhiwei Center for Advanced Laser Technology Hebei University of Technology Tianjin300401 China Hebei Key Laboratory of Advanced Laser Technology and Equipment Tianjin300401 China State Key Laboratory for Mechanical Behavior of Materials Xi’an Jiaotong University Xi’an710049 China College of Mechanical Engineering and Automation Fuzhou University Fuzhou350108 China

Herein, we present aN Er-doped all-fiber laser with BiVO4 as the saturable absorber (SA). To illustrate the nonlinear optical response, a two-dimensional model of monoclinic and its electronic structure was calculated. The nonlinear absorption properties were evaluated utilizing the Z-scan technique, and a saturable absorber was fabricated for integration into a fiber laser, resulting in a stable Q-switched output. At a maximum pump power of 600 mW, the fiber laser achieved an average output power of 25.23 mW and a pulse energy of 330.76 nJ. This research confirms that BiVO4 material exhibits outstanding nonlinear optical characteristics, thereby broadening its scope of application in the realm of ultrafast pulsed fiber lasers. © 2025 Optica Publishing Group under the terms of the Optica Open Access Publishing Agreement.

关键词： Optical depth

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Fe doping 1T phase MoS_(2)with enhanced zinc-ion storage ability and durability for high-performance aqueous zinc-ion batteries

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Rare Metals 2025年第1期44卷 253-263页

作者： Jing-Yi Liu Rong-Jie Zhe Zhan-Hong Peng Yi-Hui Song Lin-Xuan Yang Chen Qing Jun-Ling Guo Jin-Ping Liu Yunnan Key Laboratory of Opto-Electronic Information Technology College of Physics and Electronic Information TechnologyYunnan Normal UniversityKunming650000China Country State Center for International Cooperation on Designer Low-Carbon and Environmental Materials School of Materials Science and EngineeringZhengzhou UniversityZhengzhou450001China School of Chemistry Chemical Engineering and Life ScienceState Key Laboratory of Advanced Technology for Materials Synthesis and ProcessingWuhan University of TechnologyWuhan430070China

As a promising cathode material for aqueous zinc-ion batteries,1T-MoS_(2)has been extensively investigated because of its facile two-dimensional ion-diffusion channels and high electrical ***,the limited number of available Zn storage sites,i.e.,limited capacity,hinders its application because the inserted Zn^(2+),which form strong electrostatic interactions with 1T-MoS_(2),preventing subsequent Zn^(2+)***,the approach of enlarging the interlayer distance to reduce electrostatic interactions has been commonly used to enhance the capacity and reduce Zn^(2+)migration ***,an enlarged interlayer spacing can weaken the van der Waals force between 1T-MoS_(2)monolayers,easily disrupting the structural ***,to address this issue,an effective strategy based on Fe doping is proposed for 1T-MoS_(2)(Fe-1T-MoS_(2)).The theoretical calculations reveal that Fe doping can simultaneously moderate the rate of decrease in the adsorption energy after gradually increasing the number of stored atoms,and enhance the electron delocalization on metal-O ***,the experiment results show that Fe doping can simultaneously activate more Zn storage sites,thus enhancing the capacity,and stabilize the structural stability for improved cycling ***,Fe-1T-MoS_(2)exhibits a larger capacity(189 mAh·g^(-1)at 0.1 A·g^(-1))and superior cycling stability(78%capacity retention after 400 cycles at 2 A·g^(-1))than pure 1T-MoS_(2).This work may open up a new avenue for constructing high-performance MoS_(2)-based cathodes.

关键词： Aqueous zinc-ion battery 1T-MoS_(2) Fe doping More Zn storage sites Enhanced structural stability

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