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Electrospinning engineering of gas electrodes for high-performance lithium-gas batteries

Carbon Energy 2024年第10期6卷 353-398页

作者： Jingzhao Wang Xin Chen Jianan Wang Xiangming Cui Ze Wang Guangpeng Zhang Wei Lyu Maxim Shkunov S.Ravi P.Silva Yaozu Liao Kai Yang Wei Yan State Key Laboratory of Multiphase Flow in Power Engineering Department of Environmental Science and EngineeringSchool of Energy and Power EngineeringXi'an Jiaotong UniversityXi'anChina Advanced Technology Institute University of SurreyGuildfordSurreyUK State Key Laboratory for Modification of Chemical Fibers and Polymer Materials College of Materials Science and EngineeringDonghua UniversityShanghaiChina

Lithium-gas batteries(LGBs)have garnered significant attention due to their impressive high-energy densities and unique gas conversion ***,the practical application of LGBs faces substantial challenges,including sluggish gas conversion kinetics inducing in low-rate performance and high overpotential,along with limited electrochemical reversibility leading to poor cycle *** imperative task is to develop gas electrodes with remarkable catalytic activity,abundant active sites,and exceptional electrochemical ***,a versatile and well-established technique for fabricating fibrous nanomaterials,has been extensively explored in LGB *** this work,we emphasize the critical structure-property for ideal gas electrodes and summarize the advancement of employing electrospun nanofibers(NFs)for performance enhancement in *** elucidating the fundamental principles of LGBs and the electrospinning technique,we focus on the systematic design of electrospun NF-based gas electrodes regarding optimal structural fabrication,catalyst handling and activation,and catalytic site optimization,as well as considerations for large-scale *** demonstrated principles and regulations for electrode design are expected to inspire broad applications in catalyst-based energy applications.

关键词： carbon nanofibers electrocatalyst electrospinning gas electrodes metal-gas batteries

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Numerical simukation of nitrogen condensation flow in acryogeni nozzle 24

Numerical simukation of nitrogen condensation flow in acryog...

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24th IIR International Congress of Refrigeration, ICR 2015

作者： Wan, Sun Guoqing, Liu Lu, Niu Shuangtao, Chen Yu, Hou State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University 710049 China

ISBN: (纸本)9782362150128

2-D numerical simulations on the nitrogen expansion flow with spontaneous condensation in a nozzle were conducted based on the equilibrium model and the non-equilibrium model respectively. In the equilibrium model, the mass transfer between the liquid and vapor is determined by the saturation enthalpies of the liquid and vapor phases. The pressure distribution of the nozzle could be influenced slightly by the condensation process. In the non-equilibrium model, the classical nucleation model is used for the droplets formation. The flow is heated by the latent heat and consequently the decrease of pressure and the increase of Mach number are delayed. Meanwhile, due to the requirement of a certain supercooling level, the condensation onset point is pushed away from the nozzle inlet, and the nozzle outlet wetness fraction becomes smaller. Then, the influence of the nozzle inlet temperature and inlet pressure on gas supercooling, nucleation rate and wetness are analyzed.

关键词： Nucleation

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Design and simulation of a novel geothermalsolar combined chimney power plant

Design and simulation of a novel geothermalsolar combined ch...

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26th International Conference on Efficiency, Cost, Optimization, Simulation and Environmental Impact of Energy Systems, ECOS 2013

作者： Cao, Fei Ma, Qiuming Zhao, Liang Guo, Liejin State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an China

The solar chimney power plant (SCPP) is dominated by the solar radiation, and therefore its discontinuous operation is an unavoidable problem. In this paper, low temperature geothermal energy is introduced into the SCPP for overcoming this problem. Based on a developed mathematical model, theoretical analyses are carried out to investigate the performance of the geothermal-solar chimney power plant (GSCPP) with main dimensions the same as the Manzanares prototype in Spain. It is found that the GSCPP can attractively run in the full geothermal mode to deliver power continuously, which could solve the problem of the SCPP's running without sunlight in a long time, including at night. In addition, the introducing of geothermal energy into the SCPP can highly improve its power capacity.

关键词： Geothermal energy

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Manipulating metal-oxygen local atomic structures in singlejunctional p-Si/WO_(3) photocathodes for efficient solar hydrogen generation

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Nano Research 2021年第7期14卷 2285-2293页

作者： Wu Zhou Chung-Li Dong Yiqing Wang Yu-Cheng Huang Lingyun He Han-Wei Chang Shaohua Shen International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power EngineeringXi’an Jiaotong UniversityShaanxi 710049China Department of Physics Tamkang UniversityTamsui 25137TaiwanChina

Self-passivation in aqueous solution and sluggish surface reaction kinetics significantly limit the photoelectrochemical(PEC)performances of silicon-based ***,a WO_(3) thin layer is deposited on the p-Si substrate by pulsed laser deposition(PLD),acting as a photocathode for PEC hydrogen *** to bare p-Si,the single-junctional p-Si/WO_(3) photoelectrodes exhibit excellent and stable PEC performances with significantly increased cathodic photocurrent density and exceptional anodic shift in onset potential for water *** is revealed that the WO_(3) layer could reduce the charge transfer resistance across the electrode/electrolyte interface by eliminating the effect of Fermi level pinning on the surface of *** importantly,by varying the oxygen pressures during PLD,the collaborative modulation of W–O bond covalency and WO6 octahedral structure symmetry contributes to the promoted charge carrier transport and ***,a large band bending at the p-Si/WO_(3) junction,induced by the optimized O vacancy contents in WO_(3),could provide a photovoltage as high as~500 mV to efficiently drive charge transfer to overcome the water reduction ***,by manipulating W–O local atomic structures in the deposited WO_(3) layer,a great improvement in PEC performance could be achieved over the singlejunctional p-Si/WO_(3) photocathodes for solar hydrogen generation.

关键词： silicon local atomic structure water splitting photocathodes hydrogen generation

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A calculation method for evaluating thermal loss of solar cavity receiver

A calculation method for evaluating thermal loss of solar ca...

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2009 Asia-Pacific power and Energy engineering Conference, APPEEC 2009

作者： Jiabin, Fang Jinjia, Wei Xunwei, Dong Yueshe, Wang State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an China

ISBN: (纸本)9781424424870

One of the most important components of solar thermal power system is the solar central receiver, which performance is in direct relation to the efficiency of the whole power generation system. The calculation of internal surface heat flux and thermal efficiency of receiver therefore plays a very important role in receiver design. A calculation method of heat loass of a cavity receiver is put forward in this paper. The first step of this method is to use the Monte Carlo method to simulate the track of solar beam and compute surface heat flux inside the receiver. The second step is to employ the correlations of flow boiling heat transfer to figure out the convective heat transfer coefficient inside the tubes and then the wall temperature of the boiling tubes laid inside the receiver. The last step is to simulate the air flow field inside the receiver to calculate convective thermal loss of the receiver. As every step can not be independently done, all steps are coupled and an iterative scheme is needed. Internal surface heat flux and thermal efficiency of the receiver can be finally gained with this method, and the result can provide theoretical guide for receiver design. © 2009 IEEE.

关键词： Monte Carlo methods

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Experimental and modeling study of low temperature ignition characteristics of methylcyclohexane/ethanol binary fuel 12

Experimental and modeling study of low temperature ignition ...

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12th Asia-Pacific Conference on Combustion, ASPACC 2019

作者： Liu, Yang Tang, Chenglong Huang, Zuohua State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an China

The purpose of this work is to investigate the effect of ethanol blending into methylcyclohexane during the ignition at low temperatures. The ignition delay times of the binary fuels with ethanol blending ratio varied from 0% to 100% at = 1.0, Pc = 20 bar, Tc = 680 - 890 K were measured with the rapid compression machine, and the mechanism of Bissoonauth et al. (Proc Combust Inst 2018) well predicts the experimental results. Based on the high quality of the model, the effects of ethanol blending on the pressure and heat release are studied. Both of the maximum pressure and the heat release during the ignition decrease with the ethanol blending ratio increases. The interaction of MCH and ethanol happens in the competition of active radicals like OH, and MCH dominates the ignition process as it occupies about two thirds of the OH to form the fuel radical. © Asia-Pacific Conference on Combustion, ASPACC *** right reserved.

关键词： Ethanol

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A Novel One-step Hydrothermal Method for the Preparation of Cd1-xZnxS/Titanate Nanotubes Composites for Photocatalytic Hydrogen Production 18

A Novel One-step Hydrothermal Method for the Preparation of ...

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18th World Hydrogen Energy Conference, WHEC 2010

作者： Chen, Yubin Guo, Liejin State Key Laboratory of Multiphase Flow in Power Engineering School of Energy and Power Engineering Xi'an Jiaotong University China

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Base-or acid-assisted polystyrene plastic degradation in supercritical CO_(2)

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Waste Disposal and Sustainable Energy 2023年第2期5卷 165-175页

作者： Yanbing Liu Jinwen Shi Liuhao Mao Bingru Lu Xing Kang Hui Jin International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power EngineeringXi’an Jiaotong University28 West Xianning RoadXi’an710049ShaanxiChina

Plastic has caused serious"white pollution"to the environment,and the highly inert characteristics of plastic bring a major challenge for *** fluids have unique physical properties and have been widely used in various *** this work,supercritical CO_(2)(Sc-CO_(2))with mild conditions was selected and assisted by NaOH/HCl solution to degrade polystyrene(PS)plastic,and the reaction model was designed using response surface methodology(RSM).It was found that,regardless of the types of assistance solutions,the factors affecting PS degradation efficiencies were reaction temperature,reaction time,and NaOH/HCl *** the temperature of 400℃,time of 120 min,and base/acid concentration of 5%(in weight),0.15 g PS produced 126.88/116.99±5 mL of gases with 74.18/62.78±5 mL of H2,and consumed 81.2/71.5±5 mL of CO_(2).Sc-CO_(2)created a homogeneous environment,which made PS highly dispersed and uniformly heated,thus promoting the degradation of ***,Sc-CO_(2)also reacted with the degradation products to produce new CO and more CH_(4)and C_(2)H_(x)(x=4,6).Adding NaOH/HCl solution not only improved the solubility of PS in Sc-CO_(2),but also provided a base/acid environment that reduced the activation energy of the reaction,and effectively improved the degradation efficiencies of *** short,degrading PS in Sc-CO_(2)is feasible,and better results are obtained with the assistance of base/acid solution,which can provide a reference for the disposal of waste plastics in the future.

关键词： Plastic degradation Polystyrene Supercritical CO_(2) NaOH HCl

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Fabricating PdCe/OMS-2 catalysts with boosted low-temperature activity for toluene deep degradation

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Journal of Rare Earths 2023年第6期41卷 839-849,I0002页

作者： Lin Yue Zhihua Xu Minghua Hu Mingjiao Tian Mudi Ma Bijie Huang Chi He State Key Laboratory of Multiphase Flow in Power Engineering School of Energy and Power EngineeringXi'an Jiaotong UniversityXi'an 710049China State Key Laboratory of Precision Blasting and Hubei Key Laboratory of Industrial Fume and Dust Pollution Control Jianghan UniversityWuhan 430056China National Engineering Laboratory for VOCs Pollution Control Material&Technology University of Chinese Academy of SciencesBeijing 101408China

Porous cryptomelane-type octahedral molecular sieve(OMS-2)with mixed Mn valence and abundant lattice oxygen species has attracted much attention in volatile organic compounds(VOC)catalytic ***,complete conversion of arene over OMS-2 catalysts at relatively low temperature is still a challenge due to its limited crystal structure and inferior ***,a series of PdCe/OMS-2 catalysts with different Pd/Ce molar ratios was fabricated by a facile impregnation method and the physicochemical properties of which were extensively characterized by X-ray diffraction(XRD),scanning electron microscopy(SEM),high-resolution transmission electron microscopy(HR-TEM),B runauer-Emmett-Teller(BET)method,X-ray fluorescence(XRF),X-ray photoelectron spectroscopy(XPS),temperature programmed reduction of H2(H2-TPR),Raman,In situ diffused reflectance infrared Fourier transform spectra(DRIFTS),and density functional theory(DFT)*** show that the total conversion of toluene can be achieved at 207℃ over PdCe2 with apparent activation energy as low as 62.6 kJ/*** strong synergistic effect between Pd and Ce remarkably boosts the catalytic activity of OMS-2,attributed to the abundant Mn^(3+)-O bands and active surface oxygen *** results reveal that oxygen vacancy can be formed over PdCe2 much easily than that of Pd/OMS-2 and Ce/OMS-2 with the oxygen vacancy formation energy of2.42,2.83 and 2.68 eV,*** increasing the Pd content cannot promote the catalytic activity although PdO is a critical active center in toluene *** vacancy attributed to the integrative effect of Pd,Ce and Mn species plays a promine nt role over prepared catalysts in toluene activation *** findings reported in this work showed new insights into the designing of highly efficient OMS-2catalysts for VOC deep oxidation by tuning oxygen vacancy concentration.

关键词： PdCe/OMS-2 Toluene Catalytic oxidation Oxygen vacancy Rare earths

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Experimental study on a linear concentrating solar photovoltaic/thermal system

Experimental study on a linear concentrating solar photovolt...

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26th International Conference on Efficiency, Cost, Optimization, Simulation and Environmental Impact of Energy Systems, ECOS 2013

作者： Ma, Qiuming Cao, Fei Zhao, Liang State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an China

A set of solar photovoltaic and thermal combined (PV/T) system is installed and tested in the present study. The PV/T system is designed and constructed by integrating coiled-channel flat-plate collectors with polycrystalline silicon PV modules. The linear Fresnel lens acts as the concentrator. Three systems, i.e. the non-cooling PV system, the non-concentrating PV/T system and the concentrating PV/T system, are tested and analyzed. Experimental results show that a high thermal and electrical combined efficiency, over 65%, is achieved by the PV/T system. Water in the flat plate can significantly decrease the PV module temperature and improve the electricity-conversion efficiency. Comparing with the non-concentrating PV/T system, the concentrating PV/T system can increase the total utilization of solar energy.

关键词： Solar energy

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