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Chinese Chemical Letters 2024年第8期35卷 25-35页

作者： Yatian Deng Dao Wang Jinglan Cheng Yunkun Zhao Zongbao Li Chunyan Zang Jian Li Lichao Jia School of Materials Science and Engineering State Key Lab of Material Processing and Die&Mould TechnologyHuazhong University of Science and TechnologyWuhan 430074China College of Science Qiongtai Normal UniversityHaikou 571127China Kunming Sino-Platinum Metals Catalyst Co. Ltd.Kunming 650106China State Key Laboratory of Advanced Electromagnetic Technology Huazhong University of Science and TechnologyWuhan 430074China

Catalyst with high performance has drawn increasing attention recently due to its significant advantages in chemical reactions such as speeding up the reaction,lowering the reaction temperature or pressure,and proceeding without itself being *** the superior catalytic performance of precious metal catalysts,transition metal oxides offer a promising route for substitution of precious metals in catalysis arising from their low cost,intrinsic activity and sufficient ***-type oxide SmMn_(2)O_(5) exhibits a unique crystal structure containing double crystalline fields,and nowadays is used widely as the catalyst in different chemical reactions,including the reactions of vehicle emissions reduction and oxygen evolution reaction,gas sensors,and metal-air batteries,promoting attention in catalytic perfor-mance *** our knowledge,there is no review article covering the comprehensive informa-tion of SmMn2 O 5 and its *** we review the recent progress in understanding of the crys-tal structure of SmMn_(2)O_(5) and its basic physical *** then summarize the catalytic sources of SmMn_(2)O_(5) and reaction mechanisms,while the strategies to improve catalytic performance of SmMn_(2)O_(5) are further ***,we provide a perspective on how to make further progress in catalytic applications.

关键词： Catalyst SmMn_(2)O_(5) Mullite-type oxide Catalytic oxidation Oxygen reduction reaction Oxygen evolution reaction Reaction mechanisms

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DDP-Fsim: Efficient and Scalable Fault Simulation for Deterministic Patterns with Two-Dimensional Parallelism 24

DDP-Fsim: Efficient and Scalable Fault Simulation for Determ...

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43rd International Conference on Computer-Aided Design, ICCAD 2024

作者： Gu, Feng Wang, Mingjun Mu, Jianan Liu, Zizhen Tang, Jiaping Wang, Hui Wang, Yonghao Ye, Jing Li, Huawei Li, Xiaowei State Key Lab of Processors Institute of Computing Technology CAS China University of Chinese Academy of Sciences China CASTEST Beijing China

ISBN: (纸本)9798400710773

Fault simulation is a fundamental component in the design for testability (DFT) processes, especially in automatic test pattern generation (ATPG). Various approaches have been proposed to enhance the efficiency of fault simulation on multi-core systems. However, these approaches have not taken full consideration of the intrinsic characteristics of deterministic patterns. Deterministic patterns are generated by ATPG and are predominantly employed in practical applications rather than random patterns. In this paper, we introduce DDP-Fsim, a fast and scalable fault simulator on multi-core systems. DDP-Fsim capitalizes on the distinctive nature of deterministic patterns, wherein a small subset of patterns can effectively detect the majority of faults. Initially, DDP-Fsim parallels in fault dimension by dynamically scheduling fanout-free regions (FFR) to handle easy-to-detect faults. Subsequently, it parallels in pattern dimension by dynamically scheduling patterns to address the remaining hard-to-detect faults. Experiments demonstrate that on a 24-core system, DDP-Fsim is 10× faster than the commercial tools for full-scan circuits and deterministic patterns. Additionally, DDP-Fsim with 24 cores achieves an average speed-up of 16× compared to its single-core execution, while the commercial tools with 24 cores achieves only 3×-6× speed-up than their single-core execution. This indicates the significantly superior scalability for DDP-Fsim. © 2024 Copyright is held by the owner/author(s).

关键词： Automatic test pattern generation

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Revealing the interaction mechanism of pulsed laser processing with the application of acoustic emission

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Frontiers of Optoelectronics 2023年第2期16卷 91-101页

作者： Weinan Liu Youmin Rong Ranwu Yang Congyi Wu Guojun Zhang Yu Huang State Key Lab of Digital Manufacturing Equipment and Technology Huazhong University of Science and TechnologyWuhan 430074China School of Mechanical Science and Engineering Huazhong University of Science and TechnologyWuhan 430074China

The mechanisms of interaction between pulsed laser and materials are complex and indistinct,severely infuencing the stability and quality of laser *** paper proposes an intelligent method based on the acoustic emission(AE)technique to monitor laser processing and explore the interaction *** validation experiment is designed to perform nanosecond laser dotting on foat *** parameters are set diferently to generate various outcomes:ablated pits and irregular-shaped *** the signal processing stage,we divide the AE signals into two bands,main and tail bands,according to the laser processing duration,to study the laser ablation and crack behavior,*** parameters extracted by a method that combines framework and frame energy calculation of AE signals can efectively reveal the mechanisms of pulsed laser *** main band features evaluate the degree of laser ablation from the time and intensity scales,and the tail band characteristics demonstrate that the cracks occur after laser *** addition,from the analysis of the parameters of the tail band very large cracks can be efciently *** intelligent AE monitoring method was successfully applied in exploring the interaction mechanism of nanosecond laser dotting foat glass and can be used in other pulsed laser processing felds.

关键词： Laser dotting Acoustic emission Monitoring Laser ablation Cracks

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An effective'salt in dimethyl sulfoxide/water'electrolyte enables high-voltage supercapacitor operated at-50℃

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Journal of Energy Chemistry 2024年第6期93卷 361-367,I0009页

作者： Yingbin Liu Chang Yu Xuedan Song Siyi Hou Shuqin Lan Jinhe Yu Yuanyang Xie Jieshan Qiu State Key Lab of Fine Chemicals Frontier Science Center for Smart MaterialsSchool of Chemical EngineeringLiaoning Key Lab for Energy Materials and Chemical EngineeringDalian University of TechnologyDalian 116024LiaoningChina School of Chemistry Frontier Science Center for Smart MaterialsLiaoning Key Lab for Energy Materials and Chemical EngineeringDalian University of TechnologyDalian 116024LiaoningChina College of Chemical Engineering State Key Laboratory of Chemical Resource EngineeringBeijing University of Chemical TechnologyBeijing 100029China

Compared with organic electrolytes,aqueous electrolytes exhibit significantly higher ionic conductivity and possess inherent safety features,showcasing unique advantages in ***,challenges remain for low-salt aqueous electrolytes operating at high voltage and low ***,we report a low-salt(0.87 m,m means mol kg^(-1))'salt in dimethyl sulfoxide/water'hybrid electrolyte with non-flammability via hybridizing aqueous electrolyte with an organic co-solvent of dimethyl sulfoxide(hydrogen bond acceptor).As a result,the 0.87 m hybrid electrolyte exhibits enhanced electrochemical stability,a freezing temperature below-50℃,and an outstanding ionic conductivity of 0.52mS cm~(-1)at-50℃.Dimethyl sulfoxide can anchor water molecules through intermolecular hydrogen bond interaction,effectively reinforcing the stability of water in the hybrid ***,the interaction between dimethyl sulfoxide and water molecules diminishes the involvement of water in the generation of ordered ice crystals,finally facilitating the low-temperature performance of the hybrid *** paired with the 0.87 m'salt in dimethyl sulfoxide/water'hybrid electrolyte,the symmetric supercapacitor presents a 2.0 V high operating voltage at 25℃,and can operate stably at-50℃.Importantly,the suppressed electrochemical reaction of water at-50℃further leads to the symmetric supercapacitor operated at a higher voltage of 2.6 *** modification strategy opens an effective avenue to develop low-salt electrolytes for high-voltage and low-temperature aqueous supercapacitors.

关键词： Dimethyl sulfoxide Co-solvent High voltage Low temperature Supercapacitors

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Intrinsic pentagon defect engineering in multiple spatial-scale carbon frameworks for efficient triiodide reduction

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Journal of Energy Chemistry 2024年第8期95卷 20-28,I0002页

作者： Siyi Hou Xuedan Song Chang Yu Jiangwei Chang Yiwang Ding Yingbin Liu Xiubo Zhang Weizhe Liu Jieshan Qiu State Key Lab of Fine Chemicals Liaoning Key Lab for Energy Materials and Chemical EngineeringFrontier Science Center for Smart MaterialsSchool of Chemical EngineeringDalian University of TechnologyDalian 116024LiaoningChina Liaoning Key Lab for Energy Materials and Chemical Engineering Frontier Science Center for Smart MaterialsSchool of ChemistryDalian University of TechnologyDalian 116024LiaoningChina State Key Laboratory of Chemical Resource Engineering College of Chemical EngineeringBeijing University of Chemical TechnologyBeijing 100029China

Intrinsic topological defect engineering has been proven as a promising strategy to elevate the electrocatalytic activity of carbon ***,the controllable construction of high-density and specific topological defects in carbon frameworks to reveal the relationship between reactivity and defect structure remains a challenging ***,the intrinsic pentagon carbon sites that can favor electron overflow and enhance their binding affinity towards the intermediates of catalytic reaction are firstly presented by the work function and the p-band center *** experimentally verify this,the cage-opening reaction of fullerene is proposed and utilized for synthesizing carbon quantum dots with specific pentagon configuration(CQDs-P),subsequently utilizing CQDs-P to modulate the micro-scale defect density of three-dimensional reduced graphene oxide(rGO)viaπ-π*** multiple spatial-scale rGO-conjugated CQDs-P structure simultaneously possesses abundant pentagon and edge defects as catalytic active sites and long-range-orderedπelectron delocalization system as conductive *** defects-rich CQDs-P/rGO-4 all-carbon-based catalyst exhibits superb catalytic activity for triiodide reduction reaction with a high photoelectric conversion efficiency of 8.40%,superior to the Pt reference(7.97%).Theoretical calculations suggest that pentagon defects in the carbon frameworks can promote charge transfer and modulate the adsorption/dissociation behavior of the reaction intermediates,thus enhancing the electrocatalytic activity of the *** work confirms the role of intrinsic pentagon defects in catalytic reactions and provides a new insight into the synthesis of defects-rich carbon catalysts.

关键词： Defect engineering Pentagon carbon Carbon quantum dots Electrocatalytic activity Triiodide reduction

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Formation and evolution of supercritical geofluid

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science china Earth sciences 2025年第1期68卷 39-51页

作者： Huaiwei NI Yilin XIAO Xiaolin XIONG Xiandong LIU Chunxiao GAO Yi-Xiang CHEN Yunguo LI Wan-Cai LI Xuan GUO Yang-Yang WANG Dong-Bo TAN Li ZHANG State Key Laboratory of Lithospheric and Environmental Coevolution University of Science and Technology of ChinaHefei230026China Deep Space Exploration Laboratory/School of Earth and Space Sciences University of Science and Technology of ChinaHefei230026China Guangzhou Institute of Geochemistry Chinese Academy of SciencesGuangzhou510640China School of Earth Sciences and Engineering Nanjing UniversityNanjing210023China State Key Lab of Superhard Materials Jilin UniversityChangchun130012China

In this work,we provide a comprehensive review on the formation,evolution,properties,and effects of supercritical *** Earth's interior,enhanced miscibility between H_(2)O and silicate by the addition of special components or by the increase of pressure and temperature gives rise to supercritical geofluid with a significant amount of both H_(2)O and silicate *** formation of supercritical geofluid in magmatic-hydrothermal systems,typified by pegmatite system,is governed by meltfluid critical *** formation of supercritical geofluid in metamorphic systems,typified by subducted slab,is governed by the second critical end *** results suggest that the presence of boron and fluorine in pegmatite system makes it possible to form supercritical geofluid at crustal depths,but the release of supercritical geofluid from subducted slab is withheld until almost 100 km depth.A major presence of both H_(2)O and depolymerized structural units(monomers,dimers,etc.)endows supercritical geofluid with unique physical properties including low density,low elastic moduli,low viscosity,high diffusivity,and high electrical *** geofluid can effectively mobilize a variety of elements even including high field strength elements and heavy rare earth *** chemical signatures of supercritical geofluid can be inherited by metasomatized mantle and mantle-derived melts,and this could give an explanation of the oxidation of arc *** separation of supercritical geofluid through the mechanism of spinodal decomposition leads to formation of a melt *** fluid inclusions recovered from subduction zone rocks and pegmatites are possible relics of supercritical *** geofluid can cause electrical anomaly and low seismic velocity near the top of subducted slab,and can be linked with intermediate-focus *** geofluid may have played a crucial role in the formation of pegmatites and associ

关键词： Supercritical geofluid Miscibility Subduction zone Pegmatite

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Dual-photoconductivity in monolayer PtSe_(2) ribbons

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Nano Research 2024年第11期17卷 10189-10195页

作者： Zechen Li Honglin Wang Huaipeng Wang Jing Li Fangzhu Qing Xuesong Li Dan Xie Hongwei Zhu State Key Lab of New Ceramics and Fine Processing School of Materials Science and Engineering Tsinghua University Beijing 100084 China School of Integrated Circuits Beijing National Research Center for Information Science and Technology Tsinghua University Beijing 100084 China State Key Lab of Solid Waste Reuse for Building Materials Beijing Building Materials Academy of Science Research Beijing 100041 China Shenzhen Institute for Advanced Study University of Electronic Science and Technology of China Shenzhen 518110 China

Two-dimensional platinum diselenide (PtSe_(2)) has been explored for applications in visible and infrared photodetectors, owing to its tunable electrical and optoelectronic properties governed by layer-dependent bandgaps. Studies have explored both positive photoconductivity (PPC) and negative photoconductivity (NPC) behaviors in few-layer PtSe_(2) thin films, proposing mechanisms related to gas molecule adsorption. However, these proposed mechanisms, typically based on models with ideal limit structures, often lacked consistency with the structure and scale of polycrystalline thin films employed in actual experiments. Here, photodetectors utilizing monolayer PtSe_(2) ribbons were designed, demonstrating a significant NPC effect upon exposure to visible light in atmospheric conditions, with device resistance increasing to over threefold the initial state. Under vacuum conditions, the device demonstrated PPC characteristics. Density functional theory calculations indicated that oxygen molecules physically adsorbed at the edges of PtSe_(2) ribbons were integral. Laser irradiation prompted the detachment of oxygen molecules from the ribbon’s edges, leading to a decreased carrier concentration in channel conductivity. The abundant edge sites of the ribbons endowed the photodetectors with a pronounced NPC response. This study diverted from traditional multilayer PtSe_(2) films to explore monolayer PtSe_(2) ribbons. These ribbons, as limit structures, offered a more fundamental insight into the intrinsic photoconductivity properties of PtSe_(2). Photodetectors employing PtSe_(2) ribbons presented novel application prospects in low-power photodetection, gas detection, and additional fields.

关键词： platinum diselenide photodetector negative photoconductivity positive photoconductivity photoinduced desorption

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IVE: Accelerating Enumeration-Based Subgraph Matching via Exploring Isolated Vertices 40

IVE: Accelerating Enumeration-Based Subgraph Matching via Ex...

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40th IEEE International Conference on Data Engineering, ICDE 2024

作者： Jiang, Zite Zhang, Shuai Hou, Xingzhong Yuan, Mengting You, Haihang Institute of Computing Technology CAS State Key Lab of Processors Beijing China School of Computer Science and Technology University of Chinese Academy of Sciences Beijinz China Zhongguancun Laboratory Beijing China School of Computer Science Wuhan University Wuhan China

ISBN: (纸本)9798350317152

The performance of the enumeration-based sub-graph matching, which searches all isomorphic subgraphs in the data graph, is crucial to various applications. The upper bound of the complexity for the enumeration-based method is exponential to the number of query graph vertices, denoted as n. We propose a novel subgraph matching algorithm called the Isolated Vertices Exploration (IVE). The IVE leverages isolated vertices during the reordering and enumeration phases, thereby significantly accelerating the subgraph matching process. During the enumeration, the isolated vertices can be matched by using a quick bipartite graph matching algorithm. Consequently, the complexity of matching the remaining non-isolated vertices is exponential to the number of non-isolated vertices, denoted as n'. For the reordering, we designed the Maximum Deleted Edges (MDE) to minimize n'. MDE iteratively selects the query vertex with the maximum edges. According to the experimental results, n' is less than 0.8n for 99.8% of arbitrary graphs. Moreover, IVE outperforms the state-of-the-art algorithms in various scenarios with different sizes, sparsities and fields, achieving a performance speedup of up to 80.3x. © 2024 IEEE.

关键词： Iterative methods

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Automatic Target Description File Generation

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Journal of Computer science & technology 2023年第6期38卷 1339-1355页

作者：耿洪娜吕方钟茗崔慧敏薛景玲冯晓兵 State Key Laboratory of Processors Institute of Computing TechnologyChinese Academy of SciencesBeijing 100190China University of Chinese Academy of Sciences Beijing 100049China School of Computer Science and Engineering University of New South WalesSydneyNSW 2052Australia

Agile hardware design is gaining increasing momentum and bringing new chips in larger quantities to the market ***,it also takes new challenges for compiler developers to retarget existing compilers to these new chips in shorter time than ever ***,retargeting a compiler backend,e.g.,an LLVM backend to a new target,requires compiler developers to write manually a set of target description files(totalling 10300+lines of code(LOC)for RISC-V in LLVM),which is error-prone and *** this paper,we introduce a new approach,Au-tomatic Target Description File Generation(ATG),which accelerates the generation of a compiler backend for a new tar-get by generating its target description files *** a new target,ATG proceeds in two ***,ATG synthesizes a small list of target-specific properties and a list of code-layout templates from the target description files of a set of existing targets with similar instruction set architectures(ISAs).Second,ATG requests compiler developers to fill in the information for each instruction in the new target in tabular form according to the list of target-specific properties syn-thesized and then generates its target description files automatically according to the list of code-layout templates *** first stage can often be reused by different new targets sharing similar *** evaluate ATG using nine RISC-V instruction sets drawn from a total of 1029 instructions in LLVM *** enables compiler developers to gen-erate compiler backends for these ISAs that emit the same assembly code as the existing compiler backends for RISC-V but with significantly less development effort(by specifying each instruction in terms of up to 61 target-specific properties only).

关键词： retargetability compiler target description target backend automatic generator

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A Hybrid Level Set Optimization Design Method of Functionally Graded Cellular Structures Considering Connectivity

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Computers, Materials & Continua 2024年第4期79卷 1-18页

作者： Yan Dong Kang Zhao Liang Gao Hao Li The State Key Lab of Digital Manufacturing Equipment and Technology Huazhong University of Science and TechnologyWuhan430074China Institute of Systems Engineering China Academy of Engineering PhysicsMianyang621900China

With the continuous advancement in topology optimization and additive manufacturing(AM)technology,the capability to fabricate functionally graded materials and intricate cellular structures with spatially varying microstructures has grown ***,a critical challenge is encountered in the design of these structures–the absence of robust interface connections between adjacent microstructures,potentially resulting in diminished efficiency or macroscopic failure.A Hybrid Level Set Method(HLSM)is proposed,specifically designed to enhance connectivity among non-uniform microstructures,contributing to the design of functionally graded cellular *** HLSM introduces a pioneering algorithm for effectively blending heterogeneous microstructure ***,an interpolation algorithm is presented to construct transition microstructures seamlessly connected on both ***,the algorithm enables the morphing of non-uniform unit cells to seamlessly adapt to interconnected adjacent *** method,seamlessly integrated into a multi-scale topology optimization framework using the level set method,exhibits its efficacy through numerical examples,showcasing its prowess in optimizing 2D and 3D functionally graded materials(FGM)and multi-scale topology *** essence,the pressing issue of interface connections in complex structure design is not only addressed but also a robust methodology is introduced,substantiated by numerical evidence,advancing optimization capabilities in the realm of functionally graded materials and cellular structures.

关键词： Hybrid level set method functionally graded cellular structure connectivity interpolated transition optimization design

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