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Antioxidant system alterations and oxidative stress caused by polyfluoroalkyl substances (PFAS) in exposed biota: a review

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Science of the Total Environment 2025年 977卷 179395页

作者： Soares, Lorena Oliveira Souza de Araujo, Gabriel Farias Gomes, Thais Braga Júnior, Sidney Fernandes Sales Cuprys, Agnieszka Katarzyna Soares, Raquel Moraes Saggioro, Enrico Mendes Laboratory of Environmental Health Assessment and Promotion Oswaldo Cruz Institute Oswaldo Cruz Foundation Av. Brasil 4365 RJ Rio de Janeiro21045-900 Brazil Post-Graduate Program in Public Health and Environment Sergio Arouca National School of Public Health Oswaldo Cruz Foundation Av. Leopoldo Bulhões 1480 RJ Rio de Janeiro21041-210 Brazil Faculty of Science and Technology Norwegian University of Life Sciences P.O. Box 5003 Ås1432 Norway Post-Graduate Program in Environmental Technology and Water Resources Department of Civil and Environmental Engineering – FT University of Brasília Darcy Ribeiro Campus Via L3 Norte DF Brasília70910-900 Brazil

Contamination of aquatic and terrestrial organisms by Perfluoroalkyl substances (PFAS), emerging contaminants, is widespread, as these compounds are present in water, soil, air, and food, owing to their environmental persistence. PFAS exposure induces biochemical process alterations associated with the disruption of the antioxidant defense system in several species. This review aims to discuss how PFAS-induced antioxidant system alterations lead to changes in biochemical processes in different organisms exposed to these pollutants. This disruption, then leads to an imbalance in antioxidant defense systems, contributing to the formation of reactive oxidative species (ROS), which, in turn, can be exacerbate oxidative stress, induce cellular damage, enhance lipid peroxidation, destabilize lysosomal membranes, and cause genotoxic effects, ultimately compromising DNA integrity. In acute tests, PFAS have led to mortality, growth inhibition, diminished behavioral and locomotor abilities, and reproductive impairment. PFAS-induced effects differ with varying species or types of substances, and further bioaccumulation through food chains exacerbates environmental contamination, carrying considerable risks. These findings demonstrate the complex and enduring impact of PFAS on environmental health, emphasizing the importance of this review in corroborating studies on sub-lethal toxicity in exposed organisms and how these effects reflect on the environment. © 2025 Elsevier B.V.

关键词： Biotic

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Drought propagation in an Andean basin in South America: a spatio-temporal analysis approach with monitoring indices

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Arabian Journal of Geosciences 2025年第3期18卷 1-21页

作者： Ocampo-Marulanda, Camilo Mera-Franco, Julián David Lizcano, Víctor Augusto Carvajal-Escobar, Yesid Canchala, Teresita Zorrilla-Millan, Daniel Felipe Caicedo-Bravo, Eduardo Water Resources Engineering and Soil Research Group (IREHISA) School of Natural Resources and Environmental Engineering Universidad del Valle Cali Colombia Graduate Program in Biometrics and Applied Statistics Department of Statistics and Informatics Federal Rural University of Pernambuco Recife Brazil School of Exact Sciences and Engineering Universidad Sergio Arboleda Bogotá Colombia Programa de Ingeniería Ambiental Facultad de Ingeniería Universidad Mariana Pasto Colombia School of Electrical and Electronic Engineering Universidad del Valle Cali Colombia

Drought is a climatic phenomenon that has increased in severity over time. This study analyzed drought spread in the Alto Patía basin (13,047 km2) in South America, applying the Standardized Precipitation Index (SPI), Vegetation Health Index (VHI), and Streamflow Drought Index (SDI) to assess meteorological, agricultural, and hydrological drought, respectively. Synchronous and asynchronous correlations were estimated, and Wavelet analysis was conducted to verify relationships among drought types. Results show that the lag between drought types varies based on the intensity, temporal continuity, and spatial extent of meteorological drought. A lag of zero months (1–2 months) was observed between meteorological and hydrological drought when moderate (severe) meteorological drought partially (fully) covers the basin. Agricultural drought, however, does not always correspond to meteorological drought during isolated rainfall events. As the first study in Colombia to systematically connect these drought types, this research addresses a gap in understanding how drought impacts progress across systems in regions with complex rainfall patterns. These findings offer critical insights into the interdependencies among drought types, supporting enhanced drought monitoring and early warning systems in similar climatic regions. By identifying specific lags between meteorological and hydrological droughts, this study provides practical guidance for land management, water conservation, and crop planning, offering a foundation for future research on drought resilience strategies.

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How different spatial resolutions of digital models affects the geospatial distribution evaluation of the Index of Connectivity

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Journal of South American Earth Sciences 2025年 163卷

作者： Eberval Marchioro Geraldo André Rosseto Barreto Ialy Gomes Ferreira Adelsom Soares Filho Diogo Costa Buarque Department of Geography (DGEO) Graduate Program in Geography (PPGG) Federal University of Espírito Santo/Brazil (UFES) Coordinator of the Laboratory for Monitoring and Modeling Environmental Systems (Lamosa) Brazil Graduate Program in Management and Regulation of Water Resources (ProfÁgua/UFES) Brazil Graduate Program in Geography at UFES Brazil Graduate Program in Civil Engineering at UFV Brazil Department of Geography Graduate Program in Geography Federal University of Grande Dourados (UFGD) Brazil Department of Environmental Engineering Graduate Program in Environmental Engineering (PPGEA) Professional Master's in Water Resources Management and Regulation (ProfÁgua/UFES) Federal University of Espírito Santo/Brazil (UFES) Brazil

Digital Terrain Models (DTM) and Digital Elevation Models (DEM) are important for obtaining the Index of Connectivity, as they provide valuable information to assess the possibility of sediments reaching the riverbed in watershed basins. This is crucial for proactive management, as it allows the adoption of preventive and mitigating measures. Therefore, this study aims to analyze the effect of the spatial resolution of DEMs with resolutions of 5 m and 2 m, and between the DTM and DEM at 2 m, in determining the Index of Connectivity (IC). Additionally, it was investigated whether it is possible to use only one spatial resolution of digital models to assess the geospatial distribution of IC for all hydrogeomorphological landscapes of the Duas Bocas River watershed, located in the Metropolitan Region of Greater Vitória, in the state of Espírito Santo, Southeast Brazil. For this study, the Borselli Index of Connectivity model (et al., 2008) was used, originally developed for rural areas of Italy and widely applied in different regions worldwide. The data used, including Digital Elevation and Terrain Models and land use and cover information, were obtained from the Integrated Geospatial Base System of the State of Espírito Santo (Brazil), which is publicly *** results indicate that a better geospatial representation of IC occurs when changing the spatial resolution of DEMs from a 5 m pixel to a 2 m pixel and when using the 2 m DTM instead of the 2 m DEM. When analyzing the relationship between IC and the hydrogeomorphological landscapes in the basin, it was observed that, in the absence of models with an even finer pixel resolution, the 2 m DTM is the most suitable option, as it presented IC values consistent within and between landscapes in the Escalated Terraces of Southern Espírito Santo, Coastal Hills and Massifs, and Coastal Plateaus sectors. The exception was the fluvio-lagoon plain, which requires an even finer pixel resolution, necessitating further st

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Effectiveness of Predicting Event-Level Interception Losses Across Diverse Vegetated Sites Using Statistical Models

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Ecohydrology 2025年第3期18卷

作者： Abigail G. Sandquist Stephen P. Good Gabriel Barinas Scott T. Allen Graduate Program of Hydrologic Sciences University of Nevada Reno Reno Nevada USA Department of Natural Resources and Environmental Science University of Nevada Reno Reno Nevada USA Water Resources Graduate Program Oregon State University Corvallis Oregon USA Biological & Ecological Engineering Department Oregon State University Corvallis Oregon USA

Understanding evaporation from wet canopies across ecosystems is challenged by its spatiotemporal variability and associated observational challenges. Precipitation and throughfall were measured at 22 sites of the National Ecological Observatory Network using consistent methodologies across diverse climates and ecosystems, providing a novel opportunity to examine the performance of statistical models in predicting interception loss from meteorological and canopy-structure data. We used those data to quantify event-level interception losses and found wide variation; median interception loss of small storms (< 10 mm) was 37.7% (39% inter-quartile range), and of large storms (> 50 mm) was 19.8% (20% interquartile range). We found storm gross-precipitation depth was the most important variable for predicting the amount of interception loss (predicting ~70% of the variation), followed by mean canopy height and air temperature. Storm gross-precipitation depth was also an important predictor of interception loss as a percent of storm depth, but much less variation was explained ( R 2 = 0.11, RMSE = 24%). Prediction of percent interception loss improved ( R 2 = 0.32 and RMSE = 19%) by including additional meteorological and vegetation structure characteristics in a random forest model. In addition to demonstrating the greater importance of storm traits over vegetation traits in predicting event interception losses, this analysis showed that relationships between storm traits and interception losses differed among sites; these inconsistent relationships across sites limited the ability for any statistical model to perform well in predicting event-level interception losses across sites, which may justify the use of alternative approaches (e.g. process-based models).

关键词： rainfall partitioning remote sensing throughfall vegetation structure

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Implications of technological improvement and circular agriculture on environmental sustainability of sugarcane production

Cleaner Environmental Systems

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Cleaner environmental Systems 2025年 18卷

作者： Aakriti Deuja Min Hein Khant Thapat Silalertruksa Shabbir H. Gheewala Trakarn Prapaspongsa Graduate Program in Environmental and Water Resources Engineering Department of Civil and Environmental Engineering Faculty of Engineering Mahidol University Nakhon Pathom Thailand Department of Environmental Engineering Faculty of Engineering King Mongkut's University of Technology Thonburi Bangkok Thailand The Joint Graduate School of Energy and Environment King Mongkut's University of Technology Thonburi Bangkok Thailand Centre of Excellence on Energy Technology and Environment Ministry of Higher Education Science Research and Innovation Bangkok Thailand

The spatially differentiated environmental impacts and associated costs of technological improvement and circular agricultural practices in sugarcane production were assessed. Analysis of the cause-effect relationship between the key processes and substances each helped develop alternative scenarios for impact reduction. PM 2.5 emissions contributed to 92 % of the total human health impacts from open burning of field residues. Freshwater ecotoxicity, mainly due to ametryn emissions from pesticide application, contributed to 47 % of the total damage to the ecosystem. The environmental costs were 116 % higher than the value of sugarcane production, signifying the critical importance of adopting alternative pathways that provide economic benefits from environmental cost reduction compared to the production value. Scenarios considering green cane harvesting and waste management approaches demonstrated high potential for total impact reduction of 99 % and 97 %, respectively, and economic gains of 202 and 225 billion THB, respectively (5.76 and 6.42 billion USD, respectively). The economic benefits of waste utilization were 137 % higher than the value of sugarcane production, demonstrating the potential benefits of product substitution to help mitigate impacts. The core findings highlight the significance of the PM 2.5 impact-related external costs and underscore the benefits of adopting green cane harvesting in conjunction with on-field waste utilization to mitigate the impact of open burning and produce value-added products. Technological improvement and circular agricultural practices coupled with valuation of spatially differentiated impacts can provide useful and more accurate information to policymakers, to prioritize the implementation of mitigation strategies for enhancing the environmental sustainability of sugarcane production.

关键词： Life cycle assessment On-site and supply chain emissions Human health Ecosystem environmental cost environmental sustainability

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A novel open-source framework for automatic flocculation kinetics and retention time modelling using image analysis and swarm intelligence

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Journal of water Process engineering 2025年 74卷

作者： Bankole, Abayomi O. Moruzzi, Rodrigo Negri, Rogério G. Campos, Luiza C. Department of Civil and Environmental Engineering São Paulo State University (UNESP) Bauru Campus São Paulo Brazil Institute of Science and Technology São Paulo State University (UNESP) São Paulo São José dos Campos Brazil Department of Water Resources Management and Agrometeorology COLERM Federal University of Agriculture Abeokuta Nigeria Graduate Program in Natural Disasters (UNESP/CEMADEN) São Paulo São José dos Campos Brazil Centre for Urban Sustainability and Resilience Department of Civil Environmental and Geomatic Engineering University College London Gower Street London WC1E 6BT United Kingdom

Automatic detection of flocculation kinetic mechanisms and total hydraulic retention time (THRT) in multi-chamber systems in series is essential for seamless water treatment modelling. This study presents the first open-source tool for modelling flocculation kinetics and THRT in multi-chambers systems, with their sensitivity to image analysis. This study introduces three key novelties: (1) a non-derivative Secant method for simulating THRT, (2) use of Particle Swarm Optimization (PSO) algorithm to facilitate curve fitting technique for modelling flocculation kinetic coefficients, and (3) automatic retention time modelling directly from floc images, including sensitivity to threshold-based image segmentation. The proposed Secant method demonstrated greater robustness compared to the existing Newton-Raphson method (N-R), as it avoided convergence in cases where the N-R produced negative retention times. The PSO algorithm produced results comparable to the Bayesian approach, with aggregation coefficients of 2.773 × 10⁻⁴ and 1.905 × 10⁻⁴, and breakage coefficients of 1.186 × 10⁻⁶ and 2.656 × 10⁻⁶, at low and high velocity gradients (G), respectively. Flocculation kinetics at low G has steady aggregation followed by a dynamic equilibrium, while high G exhibited rapid formation of fragile flocs, followed by dominant breakage mechanism, and a later lower equilibrium. Scaled G for multi-chamber systems showed that reactor configurations with an immediate low G in the second chamber resulted in an average 50 % decrease in THRT. Finally, aggregation and breakage coefficients were sensitive to image segmentation thresholds, but THRT sensitivity is limited. The deployed model is accessible to improve flocculation modelling for multi-chambers in series (https://***). © 2025 Elsevier Ltd

关键词： Aggregation and breakage coefficients Completely stirred tank reactor Flocculation kinetics Intelligent water treatment monitoring System automation

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Characterization and Modification of a Clay Mineral Used in Adsorption Tests

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Journal of Minerals and Materials Characterization and engineering 2015年第4期3卷 277-288页

作者： Natália Costa Dias Patrícia Arns Steiner Maria Cristina Borba Braga Water Resources and Environmental Engineering Post-Graduate Program Department of Hydraulics and Sani-tation Parana Federal University Curitiba Brazil

Clay minerals are widespread in natural systems and have been widely used for the removal of pollutants. In this study, natural expanded vermiculite was used in adsorption tests to remove ammonium nitrogen from landfill leachate. The modification of vermiculite was carried out using NaOH and HCl, and for both modifications the best concentration was 0.1 mol/L. The results produced by XRD (X-ray diffraction) showed that Al replaced K after modification of the vermiculite using HCl and that Mg and Na replaced K after modification using NaOH. It was observed that the adsorption capacity increased as the percentage in mass of K diminished. The Langmuir is the isotherm that presents the best fit of the data, and the values of RL (the Langmuir coefficient) suggest that the adsorption is linear. The thermodynamic parameters indicate that the process is spontaneous and endothermic, that there is a high affinity between the adsorbate and the adsorbent, and that physical adsorption is prevalent.

关键词： Adsorption Isotherms Adsorption Thermodynamics Clay Minerals Expanded Vermiculite Landfill Leachate Vermiculite

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Seasonal Inflow Forecasts Based on Non-Homogeneous Hidden Markov Models: The Case of Orós Reservoir, Northeastern Brazil 18

Seasonal Inflow Forecasts Based on Non-Homogeneous Hidden Ma...

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18th World environmental and water resources Congress 2018: watershed Management, Irrigation and Drainage, and water resources Planning and Management

作者： Hernández, Luis Carlos Hernández Reis, Dirceu Silveira Environmental Technology and Water Resources Graduate Program Dept. of Civil and Environmental Engineering Univ. of Brasilia Brasília Brazil Dept. of Civil and Environmental Engineering Univ. of Brasilia Brasília Brazil

ISBN: (数字)9780784481400

ISBN: (纸本)9780784481400

This study explores the use of non-homogeneous hidden Markov models (NHMMs) to forecast streamflows into the Orós Reservoir, located in the State of Ceará, Northeastern Brazil. These models employ hydro-climatic information from a given year to predict the next year inflow. The Orós Reservoir is a key infrastructure in the water resources system of the state, where most rivers present very high temporal variability, which is a challenge for water managers. Streamflow forecast systems at the climate scale (months ahead) can be very useful for the challenging process of water allocation in the region. This paper explores the use of NHMMs to provide a probabilistic one-year ahead forecast of the mean annual flow for the Orós Reservoir. Results based on a forecast verification study based on 60 years of independent data show that NHMMs with two or three hidden states, employing the NINO3 climate index as exogenous variable, provides forecasts with an average value of the continuous ranked probability skill score of about 0.2-0.25, meaning that they are better than climatology. It is also evident that those models performed much better during dry years than during wet years, which may be related to lack of other climate indices. © 2018 American Society of Civil Engineers.

关键词： Hidden Markov models

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Prospecting toxicity of the avobenzone sunscreen in plants

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environmental Science and Pollution Research 2024年第31期31卷 44308-44317页

作者： Beijora, Sara Splendor Vaz, Thalia Aparecida Correia Santo, Diego Espirito de Almeida, Edson Araújo Junior, Osvaldo Valarini Parolin, Mauro da Silva Gonzalez, Regiane de Souza, Débora Cristina Peron, Ana Paula Chemical Engineering Course Federal Technological University of Paraná Campo Mourão Paraná Brazil Graduate Program in Environmental Engineering Federal Technological University of Paraná Paraná Francisco Beltrão Brazil Graduate Program in Chemistry State University of Maringá Paraná Maringá Brazil Academic Department of Food and Chemical Engineering Federal Technological University of Paraná Paraná Campo Mourão Brazil Graduate Program in Geography State University of Maringá Paraná Maringá Brazil Graduate Program in Food Technology Federal Technological University of Paraná Paraná Campo Mourão Brazil Graduate Program in Water Resources and Environmental Engineering Federal University of Paraná Paraná Brazil Graduate Program in Technological Innovations Federal Technological University of Paraná Via Rosalina Maria Dos Santos 1233 Paraná Campo Mourão87.301-899 Brazil

Avobenzone (AVO) is a sunscreen with high global production and is constantly released into the environment. Incorporating sewage biosolids for fertilization purposes, the leaching from cultivated soils, and the use of wastewater for irrigation explain its presence in the soil. There is a lack of information about the impact of this sunscreen on plants. In the present study, the ecotoxicity of AVO was tested at concentrations 1, 10, 100, and 1,000 ng/L. All concentrations caused a reduction in root growth of Allium cepa, Cucumis sativus, and Lycopersicum esculentum seeds, as well as a mitodepressive effect, changes in the mitotic spindle and a reduction in root growth of A. cepa bulbs. The cell cycle was disturbed because AVO disarmed the enzymatic defense system of root meristems, leading to an accumulation of hydroxyl radicals and superoxides, besides lipid peroxidation in cells. Therefore, AVO shows a high potential to cause damage to plants and can negatively affect agricultural production and the growth of non-cultivated plants. © The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2024.

关键词： Cell proliferation

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Assessing snow extent variations of Illimani mountain with Landsat NDSI 37

Assessing snow extent variations of Illimani mountain with L...

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37th Annual IEEE International Geoscience and Remote Sensing Symposium, IGARSS 2017

作者： Centeno, Jorge Antonio Silva Mitishita, Edson Aparecido Kishi, Regina Tiemy Federal University of Paraná Graduate Course in Geodetic Sciences Brazil Federal University of Paraná Graduate Program in Water Resources and Environmental Engineering Caixa Postal 19001 Curitiba Parana81.531-990 Brazil

ISBN: (纸本)9781509049516

Snow in the mountains is important because it keeps freshwater resources and supplies water for agriculture and human consumption. One of the most well-known mountains in Bolivia is the Illimani. In this paper the results of a multitemporal analysis of the snow cover at the Illimani are shown. Therefore, Landsat imagery of two years, 2010, and 1016 is presented. Snow cover is estimated from Landsat imagery using image processing and a snow-index. The temporal variation along a year is also compared to historical records. The results showed the seasonal variation of the snow cover area and that the glacier area is reducing. © 2017 IEEE.

关键词： Three-dimensional displays High definition video

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