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An electron-transfer-tuning strategy at the graphene/metal interface for improving acidic water electrolysis in proton exchange membrane electrolyzers

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Journal of Energy Chemistry 2025年第4期103卷 344-352页

作者： Yue Xu Shuaidong Li Yingjian He Fumiya Shiokawa Samuel Jeong Aimi Asilah Haji Tajuddin Zeyu Xi Yoshikazu Ito Jingzi Zhang Zeyun Cai Xi Lin Kailong Hu School of Materials Science and Engineering and Institute of Materials Genome & Big Data Harbin Institute of Technology Institute of Applied Physics Graduate School of Pure and Applied Sciences University of Tsukuba Institute of Special Environments Physical Sciences Harbin Institute of Technology School of Computer Science and Technology Harbin Institute of Technology

Graphene encapsulation has been shown to be an effective technique for improving the corrosion resistance of non-noble metal catalysts for the acidic water *** key challenge lies in enhancing the electrocatalytic activity of graphene-encapsulated metals while maintaining their durability in acidic ***,an electron-transfer-tuning strategy is investigated at the graphene/NiMo interface,aiming to improve the hydrogen evolution reaction（HER） performance of graphene-encapsulated NiMo *** doping of Ti,a low electronegativity element,into NiMo substrate was confirmed to increase electron transfer from the metal core toward the *** electron-rich state on graphene facilitates the adsorption of positively charged protons on graphene,thereby enabling a Pt/C-comparable performance in 0.5 M H2SO4,with only a 3.8% degradation in performance over a 120-h continuous *** proton exchange membrane（PEM） water electrolyzer assembled by the N-doped grapheneencapsulated Ti-doped NiMo exhibits a smaller cell voltage to achieve a current density of 2.0 A cm-2,in comparison to the Pt/C based *** study proposes a novel electron-transfer-tuning strategy to improve the HER activity of graphene-encapsulated non-noble metal catalysts without sacrificing durability in acidic electrolytes.

关键词： Acidic media Graphene encapsulation Hydrogen evolution Interface Proton exchange membrane

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Soft-GNN:towards robust graph neural networks via self-adaptive data utilization

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Frontiers of Computer science 2025年第4期19卷 1-12页

作者： Yao WU Hong HUANG Yu SONG Hai JIN National Engineering Research Center for Big Data Technology and System Service Computing Technology and System LabCluster and Grid Computing LabSchool of Computer Science and TechnologyHuazhong University of Science and TechnologyWuhan 430074China College of Information and Communication National University of Defense TechnologyWuhan 430019China Department of Computer Science and Operations Research Universitéde MontréalMontreal H3C 3J7Canada

Graph neural networks(GNNs)have gained traction and have been applied to various graph-based data analysis tasks due to their high ***,a major concern is their robustness,particularly when faced with graph data that has been deliberately or accidentally polluted with *** presents a challenge in learning robust GNNs under noisy *** address this issue,we propose a novel framework called Soft-GNN,which mitigates the influence of label noise by adapting the data utilized in *** approach employs a dynamic data utilization strategy that estimates adaptive weights based on prediction deviation,local deviation,and global *** better utilizing significant training samples and reducing the impact of label noise through dynamic data selection,GNNs are trained to be more *** evaluate the performance,robustness,generality,and complexity of our model on five real-world datasets,and our experimental results demonstrate the superiority of our approach over existing methods.

关键词： graph neural networks node classification label noise robustness

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ELLIPTIC EQUATION WITH CRITICAL EXPONENT AND DIPOLE POTENTIAL: EXISTENCE AND DECAY ESTIMATES

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Acta Mathematica Scientia 2025年第2期45卷 636-658页

作者： Yu SU Zhisu LIU Senli LIU School of Mathematics and Big Data Anhui University of Science and TechnologyHuainan 232001China School of Mathematics and Physics China University of GeosciencesWuhan 430074China Institute for Advanced Marine Research China University of GeosciencesGuangzhou 511462China College of Mathematics and Computing Science Hunan University of Science and TechnologyXiangtan 411201China

The paper is concerned with a class of elliptic equation with critical exponent and Dipole *** precisely,we make use of the refined Sobolev inequality with Morrey norm to obtain the existence and decay properties of n... 详细信息

关键词： Dipole potential decay estimation Hardy Sobolev critical exponent Henon Sobolev critical exponent

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Area Coverage Reliability Evaluation for Collaborative Intelligence and Meta-Computing of Decentralized Industrial Internet of Things

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IEEE Internet of Things Journal 2025年第10期12卷 13734-13745页

作者： Zhu, Chenlu Fan, Xiaoxuan Deng, Xianjun Liu, Shenghao Yin, Duan Gao, Hanjun Yang, Laurence T. Huazhong University of Science and Technology Hubei Key Laboratory of Distributed System Security Hubei Engineering Research Center on Big Data Security School of Cyber Science and Engineering Wuhan China China Mobile Communications Group Terminal Co Beijing China CNNC Wuhan Nuclear Power Operation Technology Co Wuhan China

Industrial Internet of Things (IIoT) is evolving towards decentralization and autonomous operation. Nodes in decentralized IIoT collaboratively sense data and communicate to participate in meta-computing and provide diverse intelligent services. Area coverage reliability evaluates the information collaborative intelligence sensing and communication capabilities of nodes in decentralized IIoT for a target area. It serves as a crucial performance evaluation metric for the meta-computing and intelligent services of decentralized IIoT. Existing area coverage reliability evaluation algorithms do not consider the dynamic node states in decentralized IIoT, and overlook the capability of nodes to collaborate in meta-computing. To address these issues, this paper proposes a novel Confident Information Coverage (CIC)-based area coverage reliability metric (CACREL), which comprehensively considers node multistate, node collaboration, network coverage rate, and network connectivity. To effectively evaluate CACREL, a CIC-based coverage reliability evaluation algorithm (CACR) is proposed. Specifically, CACR transforms complex networks into grid networks and utilizes a Coverage Table (CT) to describe different coverage states of each grid, which reduces the complexity of the area coverage reliability evaluation. Additionally, CACR employs a reliable path algorithm to converge the CT of each grid to the sink node based on grid connectivity. Simulation results demonstrate that the proposed CACR can accurately evaluate the area coverage reliability of decentralized IIoT and enhance its service performance. © 2014 IEEE.

关键词： Decentralized finance

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FlexIM: Efficient and Verifiable Index Management in Blockchain

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IEEE Transactions on Knowledge and data engineering 2025年第6期37卷 3399-3412页

作者： Li, Binhong Lin, Licheng Zhang, Shijie Xu, Jianliang Xiao, Jiang Li, Bo Jin, Hai Huazhong University of Science and Technology National Engineering Research Center for Big Data Technology and System Services Computing Technology and System Laboratory The Cluster and Grid Computing Laboratory School of Computer Science and Technology Wuhan430074 China Hong Kong Baptist University School of Computer Science Hong Kong Hong Kong University of Science and Technology Department of Computer Science and Engineering Hong Kong999077 Hong Kong

Blockchain-based query with its traceability and data provenance has become increasingly popular and widely adopted in numerous applications. Yet existing index-based query approaches are only efficient under static blockchain query workloads where the query attribute or type must be fixed. It turns out to be particularly challenging to construct an efficient index for dynamic workloads due to prohibitively long construction time and excessive storage consumption. In this paper, we present FlexIM, the first efficient and verifiable index management system for blockchain dynamic queries. The key innovation in FlexIM is to uncover the inherent characteristics of blockchain, i.e., data distribution and block access frequency, and then to optimally choose the index by utilizing reinforcement learning technique under varying workloads. In addition, we enhance and facilitate verifiability with low storage overhead by leveraging Root Merkle Tree (RMT) and Bloom Filter Merkle Tree (BMT). Our comprehensive evaluations demonstrate that FlexIM outperforms the state-of-the-art blockchain query mechanism, vChain+, by achieving a 26.5% speedup while consuming 94.2% less storage, on average, over real-world Bitcoin datasets. © 1989-2012 IEEE.

关键词： Structured Query Language

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An overview on IRS-enabled sensing and communications for 6G: architectures, fundamental limits, and joint beamforming designs

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science China(Information sciences) 2025年第5期68卷 170-193页

作者： Xianxin SONG Yuan FANG Feng WANG Zixiang REN Xianghao YU Ye ZHANG Fan LIU Jie XU Derrick Wing Kwan NG Rui ZHANG Shuguang CUI School of Science and Engineering (SSE) Shenzhen Future Network of Intelligence Institute (FNii-Shenzhen)and Guangdong Provincial Key Laboratory of Future Networks of Intelligence The Chinese University of Hong Kong Department of Electrical Engineering City University of Hong Kong School of Information Engineering Guangdong University of Technology Key Laboratory of Wireless-Optical Communications Chinese Academy of Sciences School of Information Science and Technology University of Science and Technology of China Computer School Beijing Information Science and Technology University National Mobile Communications Research Laboratory School of Information Science and Engineering Southeast University School of Electrical Engineering and Telecommunications University of New South Wales School of Science and Engineering Shenzhen Research Institute of Big Data The Chinese University of Hong Kong Department of Electrical and Computer Engineering National University of Singapore

This study presents an overview on intelligent reflecting surface(IRS)-enabled sensing and communication for the forthcoming sixth-generation(6G) wireless networks, in which IRSs are strategically deployed to proactively reconfigure wireless environments to improve both sensing and communication(S&C) performance. First, we exploit a single IRS to enable wireless sensing in the base station's(BS's) non-line-of-sight(NLoS) area. In particular, we present three IRS-enabled NLoS target sensing architectures with fully-passive, semi-passive, and active IRSs, respectively. We compare their pros and cons by analyzing the fundamental sensing performance limits for target detection and parameter estimation. Next, we consider a single IRS to facilitate integrated sensing and communication(ISAC), in which the transmit signals at the BS are used for achieving both S&C functionalities, aided by the IRS through reflective beamforming. We present joint transmit signal and receiver processing designs for realizing efficient ISAC, and jointly optimize the transmit beamforming at the BS and reflective beamforming at the IRS to balance the fundamental performance tradeoff between S&C. Furthermore, we discuss multi-IRS networked ISAC, by particularly focusing on multi-IRS-enabled multi-link ISAC, multi-region ISAC, and ISAC signal routing, respectively. Finally, we highlight various promising research topics in this area to motivate future work.

关键词： integrated sensing and communication (ISAC) intelligent reflecting surface (IRS) non-line-of-sight (NLoS) sensing sensing and communication tradeoff

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A sharding blockchain-based UAV system for search and rescue missions

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Frontiers of Computer science 2025年第3期19卷 103-118页

作者： Xihan ZHANG Jiashuo ZHANG Jianbo GAO Libin XIA Zhi GUAN Hao HU Zhong CHEN School of Computer Science Peking UniversityBeijing 100871China Peking University Chongqing Research Institute of Big Data Chongqing 401329China National Engineering Research Center for Software Engineering Peking UniversityBeijing 100871China State Key Lab for Novel Software Technology Nanjing UniversityNanjing 210023China

Sharding is a promising technique to tackle the critical weakness of scalability in blockchain-based unmanned aerial vehicle(UAV)search and rescue(SAR)*** breaking up the blockchain network into smaller partitions called shards that run independently and in parallel,shardingbased UAV systems can support a large number of search and rescue UAVs with improved scalability,thereby enhancing the rescue ***,the lack of adaptability and interoperability still hinder the application of sharded blockchain in UAV SAR *** refers to making adjustments to the blockchain towards real-time surrounding situations,while interoperability refers to making cross-shard interactions at the mission *** address the above challenges,we propose a blockchain UAV system for SAR missions based on dynamic sharding *** from the benefits in scalability brought by sharding,our system improves adaptability by dynamically creating configurable and mission-exclusive shards,and improves interoperability by supporting calls between smart contracts that are deployed on different *** implement a prototype of our system based on Quorum,give an analysis of the improved adaptability and interoperability,and conduct experiments to evaluate the *** results show our system can achieve the above goals and overcome the weakness of blockchain-based UAV systems in SAR scenarios.

关键词： blockchain sharding unmanned aerial vehicle search and rescue blockchain interoperability

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Successive Interference Cancellation-Enabled Timely Status Update in Linear Multi-hop Wireless Networks

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IEEE Transactions on Mobile Computing 2025年第6期24卷 5298-5311页

作者： Han, Xinhui Pan, Haoyuan Wang, Zhaorui Li, Jianqiang Shenzhen University College of Computer Science and Software Engineering Shenzhen China Future Network of Intelligence Institute The School of Science and Engineering Shenzhen China Shenzhen University National Engineering Laboratory for Big Data System Computing Technology The College of Computer Science and Software Engineering Shenzhen China

We investigate the timely status update in linear multi-hop wireless networks, where a source tries to deliver status update packets to a destination through a sequence of half-duplex relays. Timeliness is measured by the age of information (AoI) metric. Maintaining a low AoI at the destination typically necessitates frequent transmission of update packets from the source. However, high packet transmission frequency in multi-hop scenarios can result in mutual wireless interference at intermediate relays. Specifically, when an intermediate relay receives wireless signals of a new packet from its previous node, simultaneous transmission of an old packet by its subsequent node to the next hop may cause wireless signals to interfere at the intermediate relay, conventionally leading to packet collision. A key motivation to solve this issue is that the intermediate relay has previously received the old packet (which can thus be forwarded to the subsequent node for further relaying). Hence, successive interference cancellation (SIC) can be employed to mitigate interference of the old packet and recover the new packet. This paper designs an SIC-enabled packet relaying scheme tailored to low AoI. Initially focusing on a three-hop network, we subsequently extend our approach to general multi-hop networks. We model the multi-hop relaying scheme using a Markov chain to derive the theoretical average AoI. Theoretical and simulation results indicate that the SIC-enabled packet relaying scheme significantly reduces the average AoI compared to the non-SIC approaches, owing to an increased packet transmission frequency at the source and the effectiveness of SIC techniques at the relays. © 2002-2012 IEEE.

关键词： Markov chains

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An Entorhinal-Hippocampal Loop Model Based on Non-negative Sparse Coding

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Journal of The Institution of Engineers (India): Series B 2025年第1期106卷 113-127页

作者： Zhao, Kaixin Ren, Menghui College of Computer Science and Technology Henan Institute of Technology Xinxiang453003 China School of Electrical and Information Engineering Zhengzhou University Zhengzhou450001 China Manufacturing IoT Big Data Engineering Technology Research Center of Henan Province Xinxiang453003 China

In our study, we investigate how the brain maps environmental spaces into understandable maps through hippocampal place cells and entorhinal cortex grid cells. We uncover that the hippocampus and entorhinal cortex are not just directly connected but also engage in a sophisticated feedback loop crucial for spatial encoding during navigation. We developed an innovative network model based on this feedback mechanism, linking entorhinal inputs to hippocampal spatial encoding cells through a non-negative sparse coding, using grid cells and weak spatial cells as inputs. Our findings demonstrate that the model learns and adjusts the characteristics of spatial encoding cells, successfully learning the specific spatial selectivities of place cells even with inputs from cells carrying weaker spatial information. This highlights the critical role of feedback encoding in refining spatial representations, an indispensable component of the brain’s navigation system. Moreover, experiments comparing our model with others validate our model’s exceptional ability in generating precise spatial encodings, underscoring its superiority. This research not only deepens our understanding of the brain’s navigational mechanisms but also offers a robust computational framework for future neuroscience studies, emphasizing the intricate interplay between feedback loops and spatial encoding in the brain’s navigation system. © The Institution of Engineers (India) 2024.

关键词： Brain

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Gupacker: Generalized Unpacking Framework for Android Malware

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IEEE Transactions on Information Forensics and Security 2025年 20卷 4338-4352页

作者： Zheng, Tao Hou, Qiyu Chen, Xingshu Ren, Hao Li, Meng Li, Hongwei Shen, Changxiang Sichuan University School of Cyber Science and Engineering Chengdu610065 China Sichuan University School of Cyber Science and Engineering Cyber Science Research Institute Key Laboratory of Data Protection and Intelligent Management Ministry of Education Chengdu610065 China Hefei University of Technology Key Laboratory of Knowledge Engineering with Big Data Ministry of Education Intelligent Interconnected Systems Laboratory of Anhui Province School of Computer Science and Information Engineering Hefei230002 China University of Padua Department of Mathematics HIT Center Padua35131 Italy University of Electronic Science and Technology of China School of Computer Science and Engineering Chengdu611731 China Sichuan University Cyber Science Research Institute Key Laboratory of Data Protection and Intelligent Management Ministry of Education Chengdu610065 China

Android malware authors often use packers to evade analysis. Although many unpacking tools have been proposed, they face two significant challenges: 1) They are easily impeded by anti-analysis techniques employed by packers, preventing efficient collection of hidden Dex data. 2) They are typically designed to unpack a specific packer and cannot handle malware packed with mixed packers. Consequently, many packed malware samples evade detection. To bridge this gap, we propose Gupacker , a novel generalized unpacking framework. Gupacker offers a generic solution for first-generation holistic packer by customizing the Android system source code. It identifies the type of packer and selects an appropriate unpacking function, constructs a deeper active call chain to achieve generic unpacking of second-generation function extraction packers, and uses JNI function and instruction monitoring to handle third-generation virtual obfuscation packer. On this basis, we counteract a diverse array of anti-analysis techniques. We conduct extensive experiments on 5K packed Android malware samples, comparing Gupacker with 2 commercial and 4 state-of-the-art academic unpacking tools. The results demonstrate that Gupacker significantly improves the efficiency of Android malware unpacking with acceptable system overhead. We analyze real packed applications based on Gupacker and found several are second-packed by attackers, including WPS for Android, with tens of millions of users. We receive and responsibly report 13 0day vulnerabilities and also assist in the remediation of all vulnerabilities. © 2005-2012 IEEE.

关键词： Android malware

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