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SSRN 2024年

作者： Hu, Laigang Wang, Weiwei Miao, Xiaozeng Hu, Min Luo, Dong Wu, Wenhao Lin, Daohui Yang, Kun Department of Environmental Science Zhejiang University Hangzhou310058 China ZJU-Hangzhou Global Scientific and Technological Innovation Center Zhejiang University Hangzhou311215 China Key Laboratory of Environmental Pollution and Ecological Health of Ministry of Education Hangzhou310058 China Zhejiang Provincial Key Laboratory of Organic Pollution Process and Control Hangzhou310058 China College of Chemistry and Materials Science Guangdong Provincial Key Laboratory of Functional Supramolecular Coordination Materials and Applications Jinan University Guangzhou510632 China

Benzene (Bz) vapor is harmful for human health, even at trace concentration. Besides, Bz and cyclohexane (Cy) separation is very difficult, due to their similar kinetic diameter and boiling points. Designing an adsorption-separation material, having stronger interactions with Bz than Cy, could be a potential strategy for trace Bz adsorption and Bz/Cy separation. Herein, a novel Al-based metal-organic framework ZJU-521(Al), consisted by tetrakis(4-carboxyphenyl)methane and helical chain [Al5(OH)7(—COO)8]∞ secondary building unit, with simplest net of linking one-way rods and tetrahedra, is synthesized. It is with uniform micropore size of 7.23 Å and specific surface area of 1248 m2 g–1, having excellent trace Bz adsorption (4.18 mmol g–1) at P/P0 = 0.01, due to its straight channel and orthogonal-array pocket pore structure. The values of ideal adsorbed solution theory selectivity and separation factor of ZJU-521(Al) for Bz/Cy are 22.50 and 6.20, respectively, indicating that it is a potential material for Bz/Cy separation. From multi-component simulation, Bz molecules can be preferentially adsorbed in the pocket, because of the stronger interactions including Al–π and π ... π interactions, while Cy molecules are rapid breakthrough the channels due to weaker C–H...π interactions, resulting to Bz/Cy separation. © 2024, The Authors. All rights reserved.

关键词： Benzene

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Characteristics and Source of Ambient Volatile organic Compounds (Vocs) at a Regional Background Site, Yrd Region, China: Significant Influence of Solvent Evaporation and Biogenic Emission During Hot Months

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SSRN 2022年

作者： Xu, Zhengning Zou, Qiaoli Jin, Lingling Shen, Jiasi Qu, Fangqi Zhang, Fei Xu, Jiawei Pei, Xiangyu Xie, Guangzhao Kuang, Binyu Huang, Xin Tian, Xudong Wang, Zhibin College of Environmental and Resource Sciences Zhejiang Provincial Key Laboratory of Organic Pollution Process and Control Zhejiang University Hangzhou310058 China ZJU-Hangzhou Global Scientific and Technological Innovation Center Hangzhou311200 China Zhejiang Ecological and Environmental Monitoring Center Hangzhou310012 China School of Atmospheric Sciences Nanjing University Nanjing210093 China Zhejiang Key Laboratory of Ecological and Environmental Monitoring Forewarning and Quality Control 310058 China

Continuous measurement of 98 volatile organic compounds (VOCs) was conducted during 2017-2019 at a regional background site (Shanxi) located at northeast of zhejiang Province, YRD region, China. The average concentration of total VOCs (TVOCs) was 25.4±18.4 ppbv, and an increasing trend (+12.2%) was observed. Alkanes were the most abundant VOC group among all seasons, accounting for 43.5% of TVOCs. Oxygenated VOCs (OVOCs), aromatics, halides and alkenes contributed 15.9%, 15.7%, 11.7% and 10.3% of TVOCs concentration, respectively. Biogenic VOCs (BVOCs) and OVOCs showed distinguished diurnal cycle from primary anthropogenic VOCs. Photochemical reactivity analysis based on ozone formation potential (OFP) and OH loss rate (L OH ) indicated that aromatics and alkenes were the most significant contributor, respectively. Toluene, xylene (m/p- and o-), ethene and propene were the largest contributor of annual OFP, with the mean OFP being 33.8±44.3 μg/m 3 , 31.9±32.1 μg/m 3 , 9.29±11.4 μg/m 3 , 22.1±21.3 μg/m 3 and 12.8±19.5μg/m 3 , respectively. Seven sources were identified with positive matrix factorization (PMF): petrochemical industry (13.8%), biogenic emission (1.0%), solvent usage-toluene (16.9%), vehicular exhaust (43.8%), Integrated circuits industry (3.8%), solvent usage-C8 aromatics (10.9%), and gasoline evaporation (9.8%). Vehicular exhaust was the most significant source (43.8%) during the whole measurement period. Solvent usage, petrochemical industry, and gasoline evaporation showed high temperature dependency. The integrated contribution of solvent usage and industrial processes were higher than vehicular exhaust during hot months. These sources also have higher chemical reactivities and can contribute more on O 3 formation. Our results are helpful on determining the control strategies aiming at alleviating O 3 pollution. © 2022, The Authors. All rights reserved.

关键词： Volatile organic compounds

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Engineered Bacillus subtilis alleviates intestinal oxidative injury through Nrf2-Keap1 pathway in enterotoxigenic Escherichia coli(ETEC) K88-infected piglet

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Journal of zhejiang University-Science B(Biomedicine & Biotechnology) 2023年第6期24卷 496-509页

作者： Chaoyue WEN Hong ZHANG Qiuping GUO Yehui DUAN Sisi CHEN Mengmeng HAN Fengna LI Mingliang JIN Yizhen WANG Institute of Feed Science Key Laboratory of Animal Feed and Nutrition of Zhejiang ProvinceKey Laboratory of Molecular Animal NutritionMinistry of EducationKey Laboratory of Animal Nutrition and Feed Science in Eastern ChinaMinistry of AgricultureCollege of Animal SciencesZhejiang UniversityHangzhou 310058China Hunan Provincial Key Laboratory of Animal Nutritional Physiology and Metabolic Process CAS Key Laboratory of Agro-Ecological Processes in Subtropical RegionNational Engineering Laboratory for Pollution Control and Waste Utilization in Livestock and Poultry ProductionInstitute of Subtropical AgricultureChinese Academy of SciencesChangsha 410125China College of Advanced Agricultural Science University of Chinese Academy of SciencesBejing 100039China

Engineered probiotics can serve as therapeutics based on their ability of produce recombinant immune-stimulating *** this study,we built the recombinant Bacillus subtilis WB800 expressing antimicrobial peptide KR32(WB800-KR32)using genetic engineering methods and investigated its protective effects of nuclear factor-E2-related factor 2(Nrf2)-Kelch-like ECH-associated protein 1(Keap1)pathway activation in intestinal oxidative disturbance induced by enterotoxigenic Escherichia coli(ETEC)K88 in weaned ***-eight weaned piglets were randomly distributed into four treatment groups with seven replicates fed with a basal *** feed of the control group(CON)was infused with normal sterilized saline;meanwhile,the ETEC,ETEC+WB800,and ETEC+WB800-KR32 groups were orally administered normal sterilized saline,5×10^(10)CFU(CFU:colony forming units)WB800,and 5×10^(10)CFU WB800-KR32,respectively,on Days 1-14 and all infused with ETEC K881×10^(10)CFU on Days *** results showed that pretreatment with WB800-KR32 attenuated ETEC-induced intestinal disturbance,improved the mucosal activity of antioxidant enzyme(catalase(CAT),superoxide dismutase(SOD),and glutathione peroxidase(GPx))and decreased the content of malondialdehyde(MDA).More importantly,WB800-KR32 downregulated genes involved in antioxidant defense(GPx and SOD1).Interestingly,WB800-KR32 upregulated the protein expression of Nrf2 and downregulated the protein expression of Keap1 in the ***800-KR32 markedly changed the richness estimators(Ace and Chao)of gut microbiota and increased the abundance of Eubacterium_rectale_ATCC_33656 in the *** results suggested that WB800-KR32 may alleviate ETEC-induced intestinal oxidative injury through the Nrf2-Keap1 pathway,providing a new perspective for WB800-KR32 as potential therapeutics to regulate intestinal oxidative disturbance in ETEC K88 infection.

关键词： Engineered probiotics Intestine Oxidative injury Weaned piglets Nuclear factor-E2-related factor 2(Nrf2)-Kelch-like ECH-associated protein 1(Keap1)pathway

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Effect and Mechanism of Pyrophosphoric Acid Anodizing Technological Parameters on the Superhydrophilicity Coupled Corrosion Resistance of Aluminum Alloy Distillation Desalination Tubes

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SSRN 2023年

作者： Lv, Jiang Chen, Zhi-Li Tang, Jin Chen, Li Xie, Wen-Jing Sun, Meng-Xi Huang, Xiao-Jun Yang, Yue-Ping College of Environmental Science and Engineering Guilin University of Technology Guilin541000 China Guangdong Provincial Key Laboratory of Petrochemical Pollution Process and Control Key Laboratory of Petrochemical Pollution Control of Guangdong Higher Education Institutes School of Environmental Science and Engineering Guangdong University of Petrochemical Technology Maoming525000 China Department of Polymer Science and Engineering Zhejiang University Hangzhou310027 China

The distillation desalination tube prepared by using aluminum alloy instead of traditional copper/titanium alloy can not only significantly reduce the desalination device investment cost, but also considerably improve the energy utilization and water production efficiency of desalination by surface superhydrophilic modification. However, the restrict relationship between superhydrophilicity and corrosion resistance of this surface has become an important problem limiting the application of superhydrophilic modified aluminum alloy distillation desalination tubes. With a simple, economical, and practical anodizing technology of pyrophosphoric acid, this research performs superhydrophilic modification on 5052 aluminum alloy, and investigates the effect and mechanism of anodizing technological parameters (time, voltage and electrolyte temperature) on the superhydrophilicity coupled corrosion resistance of aluminum alloy surface. An equivalent circuit corresponding to the electrochemical impedance spectrum of the superhydrophilic anodic oxide film is proposed, and the corrosion resistance mechanism of the superhydrophilic anodic oxide film is revealed by fitting and analysis. Then, an effective method to enhance its corrosion resistance is proposed. The results show that the corrosion resistance of superhydrophilic anodic oxide film is independent of overall film thickness, but closely related to its internal barrier layer thickness. Moreover, increasing the constant voltage during anodizing can effectively increase its internal barrier layer thickness and thereby substantially improve the corrosion resistance of the superhydrophilic anodic oxide film. When anodizing the sample at the optimum 15 ℃ electrolyte temperature for 20 min and the applied constant voltage increasing from 30 V to 70 V, the corrosion potential of superhydrophilic anodic oxide film shifts to the positive direction by 0.18V, the corrosion current density reduces by 16.32 μA/cm2, and the film corrosi

关键词： Corrosion resistance

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Plant Response and Phosphorus Uptake is Better Predicted by Ion Exchange Desorption than Chemical Extraction for Soils Under Different Land Uses

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SSRN 2024年

作者： Zhang, Yaqi Chen, Dingjiang Zhu, Lizhong Zhou, Wenxiang Campbell, Shane Wang, Peng Menzies, Neal W. Dalal, Ram C. Zhejiang University College of Environmental & Resource Sciences Zhejiang Province Hangzhou310058 China ZJU-Hangzhou Global Scientific and Technological Innovation Center Zhejiang Province Hangzhou311200 China Zhejiang University Ministry of Education Key Laboratory of Environment Remediation and Ecological Health Zhejiang Province Hangzhou310058 China The University of Queensland School of Agriculture and Food Sustainability St LuciaQLD4072 Australia Zhejiang University Zhejiang Provincial Key Laboratory of Agricultural Resources and Environment Zhejiang Province Hangzhou310058 China Zhejiang Provincial Key Laboratory of Organic Pollution Process and Control Zhejiang Province Hangzhou310058 China College of Resources and Environmental Sciences Nanjing Agricultural University Nanjing210095 China

Plant availability of soil phosphorus (P) is controlled by P concentration in the soil solution (intensity factor), quantity of plant available P (quantity factor), the rate of P desorbed from sorbents to replenish / maintain P in the soil solution as P is taken up by plant roots (rate factor), and the P buffer power to sustain the quantity of plant available P (buffer power) during plant growth. The relative importance of these P availability factors for growing plants in soils under different land uses is rarely evaluated. We quantified the relative significance of P availability factors to plant growth on three soils (0-10 cm), initially under native vegetation and converted to cropping, pasture, and plantation for up to 115 years, which provided eight soil / land-use combinations providing a wide range in soil P values. Soil P availability parameters were measured by the widely used sodium bicarbonate test (Olsen P, Colwell P), anion exchange membranes (AEM) and anion + cation exchange membranes (ACEM) either saturated by NaHCO3 or KCl solution. Plant P parameters measured were dry matter yield (DM), relative yield (RY), and P uptake by Rhodes grass (Chloris gayana). We found that the initial P concentration (intensity factor) measured either by bicarbonate-AEM or NaHCO3-ACEM accounted for > 92 % variability in DM yield and P uptake, respectively, whereas the rate of P desorption measured by NaHCO3-ACEM accounted for > 93 % variability in RY. Thus, either AEM or ACEM saturated with NaHCO3 provided superior performance in predicting the availability of soil P to plants compared to the routinely used soil test under different land uses. However, wider use of these ion exchange membranes must be studied in different environments and soils to validate these findings for increasing the phosphorus use efficiency in the face of decreasing P reserves. © 2024, The Authors. All rights reserved.

关键词： Chlorine compounds

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Enhanced Precipitation Responses Over the Tibetan Plateau Following Future Tambora-Size Volcanic Eruption

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SSRN 2024年

作者： Gan, Xin-Jun Yang, Lin-Shan Zuo, Meng Liu, Fei Gao, Chao-Chao College of Environmental and Resource Science Zhejiang University Hangzhou310058 China Zhejiang Provincial Key Laboratory of Organic Pollution Process and Control Hangzhou310058 China State Key Laboratory of Severe Weather Institute of Tibetan Plateau Meteorology Chinese Academy of Meteorological Sciences Beijing100081 China School of Atmospheric Sciences Sun Yat-Sen University Key Laboratory of Tropical Atmosphere-Ocean System Ministry of Education Southern Marine Science and Engineering Guangdong Laboratory Zhuhai519082 China

Summer precipitation over the Tibetan Plateau (TP) sustains the "Water tower of Asia" and has notable influences on the climate and subsequently eco-environment of the Northern Hemisphere. Due to its high elevation and complex topography, hydroclimate in TP is found to be highly sensitive to anthropogenic warming, and a recent study shows volcanism during the past millennium caused substantial rainfall reduction over southern TP. How would a future eruption affect TP precipitation under an anthropogenic warming climate, however, remains largely untackled. Here we show, based on the Community Earth System Model ensemble simulations under the preindustrial and RCP8.5 scenarios, that a Tambora-size volcanic perturbation leads to severe rainfall reduction over south TP in the following summer (June - August). Evaporation response contributes a minor and relatively constent share of precipitation reduction following the Clausius-Clapeyron scaling, whereas dynamic processes play the essential role by triggering an El Niño-like response in eastern equatorial Pacific, which suppresses Walker and Hadley circulation and contributes to the drying anomalies in south TP. Global Warming renders the hydroclimatic responses 30% more severe, due to the increased climatological moisture content and intensified El Niño response which enhancing hydroclimate sensitivity and attenuating the monsoon circulation. Our results demonstrate the high climate sensitivity of TP and the importance of climate internal modes and feedbacks in modulating the system responses to external forcing. © 2024, The Authors. All rights reserved.

关键词： Rain

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Corrigendum to "The significance of environmentally bioavailable antimicrobials in driving antimicrobial resistance in soils" [Environ. Int. 190 (2024) 108830]

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Environment international 2024年 191卷 108959页

作者： Han Yeong Kaw Jing Yu Xuejing Ma Qi Yang Lizhong Zhu Wei Wang Department of Environmental Science Zhejiang University Hangzhou Zhejiang Province 310058 China Zhejiang Provincial Key Laboratory of Organic Pollution Process and Control Hangzhou Zhejiang Province 310058 China. Zhejiang Provincial Key Laboratory of Organic Pollution Process and Control Hangzhou Zhejiang Province 310058 China. Electronic address: ww1@***.

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Carbon Reduction Performance of Inter-Regional Uhvdc Renewable Power Transmission Projects in China from 2016 to 2021

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SSRN 2023年

作者： Gao, Chaochao Zhang, Yijia Liu, Ti Yao, Lin Lu, Yinying College of Environmental and Resource Science Zhejiang University Hangzhou China Zhejiang Provincial Key Laboratory of Organic Pollution Process and Control Hangzhou310058 China State Grid Zhejiang Electric Power Co. Ltd. Construction Company Hangzhou310016 China China Energy Engineering Group Zhejiang Electric Power Design Institute Co. Ltd. Hangzhou310014 China Environmental Science Research & Design Institute of Zhejiang Province Zhejiang Hangzhou310007 China

Renewable energy is the cornerstone to the decarbonization of the power system, whereas inter-regional power transmission accelerates renewable energy integration. Build on a previous assessment of material and thus emissions cost of the UHVDC renewable transmission infrastructure in China, here we evaluate the actual emission gains of the 17 UHVDC projects during 13th Five Year Plan. Results showed that, the renewable power transmitted through the UHVDC projects contributed a net reduction of 654.9 Mt CO2, but with a declining annual share. Six non-hydro power transmission projects actually induced additional emission costs, counterbalancing 8.23% of the total emission gains, due to the low renewable penetration rates and relatively high thermal power carbon intensity in the exporting regions. These projects need to either reduce thermal power emission factor by 4.3% to 36.9%, or to increase renewable energy above 37.1% to achieve net-zero emissions, and some optimization strategies are provided. © 2023, The Authors. All rights reserved.

关键词： Power transmission

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Bioresponses of Earthworm-Microbiota Symbionts to Polychlorinated Biphenyls in the Presence of Nano Zero Valent Iron in Soil

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SSRN 2022年

作者： Zhang, Jianying Zhang, Lei He, Mengyang Wang, Yifan Zhang, Chunlong Lin, Daohui College of Environmental and Resource Sciences Zhejiang University 866 Yuhangtang Road Hangzhou310058 China National Demonstration Center for Experimental Environment and Resources Education Zhejiang University Hangzhou310058 China Department of Environmental Sciences University of Houston-Clear Lake HoustonTX77058 United States Institute of Environmental Health Zhejiang University 866 Yuhangtang Road Hangzhou310058 China Zhejiang Provincial Key Laboratory of Organic Pollution Process and Control Hangzhou310058 China

Both earthworms and nano zero-valent iron (nZVI) have been recently regarded as important approaches for in-situ remediation of polychlorinated biphenyls (PCBs) in soil. However, the combined action of earthworms and nZVI toward PCBs, and the biological responses of earthworm-microbiota symbionts to nZVI-PCBs co-exposure in soil remediation systems remain unclear. In this study, an orthogonally designed 28-d exposure with different levels of polychlorinated biphenyls (PCBs) and nZVI was applied to earthworm Eisenia fetida in an agricultural soil. Both physiological responses of earthworms and their surrounding microbiota in gut and soil were examined. Kinetic modelling parameters showed a doubled PCB accumulation in earthworms with the presence of nZVI. Meanwhile, nZVI-PCBs coexposure synergistically stimulated the activities of superoxide dismutase (SOD) and catalase (CAT), along with the elevated levels of reactive oxygen species (ROS), malondialdehyde (MDA) and glutathione (GSH) in earthworms. Based on integrated metabolomic and 16S rRNA analysis, it was found that earthworms provided certain metabolites, e.g., S-(2-hydroxyethyl)glutathione, 16-hydroxypalmitic acid, and formamide, beneficial to PCB-degrading microbiota (Novosphingobium and Achromobacter) in the intestine. Our findings show the active role of earthworm-microbiota symbionts in the defense of PCB-nZVI exposure, and the promise of combining earthworms with nZVI for the remediation of PCBs-contaminated soil. © 2022, The Authors. All rights reserved.

关键词： organic pollutants

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Emerging contaminants:A One Health perspective

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The Innovation 2024年第4期5卷 140-170,139页

作者： Fang Wang Leilei Xiang Kelvin Sze-Yin Leung Martin Elsner Ying Zhang Yuming Guo Bo Pan Hongwen Sun Taicheng An Guangguo Ying Bryan WBrooks Deyi Hou Damian EHelbling Jianqiang Sun Hao Qiu Timothy MVogel Wei Zhang Yanzheng Gao Myrna JSimpson Yi Luo Scott XChang Guanyong Su Bryan MWong Tzung-May Fu Dong Zhu Karl JJobst Chengjun Ge Frederic Coulon Jean Damascene Harindintwali Xiankui Zeng Haijun Wang Yuhao Fu Zhong Wei Rainer Lohmann Changer Chen Yang Song Concepcion Sanchez-Cid Yu Wang Ali El-Naggar Yiming Yao Yanran Huang Japhet Cheuk-Fung Law Chenggang Gu Huizhong Shen Yanpeng Gao Chao Qin Hao Li Tong Zhang Natàlia Corcoll Min Liu Daniel SAlessi Hui Li Kristian KBrandt Yolanda Pico Cheng Gu Jianhua Guo Jianqiang Su Philippe Corvini Mao Ye Teresa Rocha-Santos Huan He Yi Yang Meiping Tong Weina Zhang Fidèle Suanon Ferdi Brahushi Zhenyu Wang Syed AHashsham Marko Virta Qingbin Yuan Gaofei Jiang Louis A.Tremblay Qingwei Bu Jichun Wu Willie Peijnenburg Edward Topp Xinde Cao Xin Jiang Minghui Zheng Taolin Zhang Yongming Luo Lizhong Zhu Xiangdong Li DamiàBarceló Jianmin Chen Baoshan Xing Wulf Amelung Zongwei Cai Ravi Naidu Qirong Shen Janusz Pawliszyn Yong-guan Zhu Andreas Schaeffer Matthias C.Rillig Fengchang Wu Gang Yu James M.Tiedje State Key Laboratory of Soil and Sustainable Agriculture Institute of Soil ScienceChinese Academy of SciencesNanjing 210008China University of Chinese Academy of Sciences Beijing 100049China Department of Chemistry Hong Kong Baptist UniversityHong KongChina HKBU Institute of Research and Continuing Education Shenzhen Virtual University ParkShenzhenChina Technical University of Munich TUM School of Natural SciencesInstitute of Hydrochemistry85748 GarchingGermany School of Resources&Environment Northeast Agricultural UniversityHarbin 150030China Climate Air Quality Research UnitSchool of Public Health and Preventive MedicineMonash UniversityMelbourneVICAustralia Faculty of Environmental Science&Engineering Kunming University of Science&TechnologyKunming 650500China Ministry of Education Key Laboratory of Pollution Processes and Environmental Criteria College of Environmental Science and EngineeringNankai UniversityTianjin 300350China Guangdong Key Laboratory of Environmental Catalysis and Health Risk Control School of Environmental Science and EngineeringInstitute of Environmental Health and Pollution ControlGuangdong University of TechnologyGuangzhou 510006China Ministry of Education Key Laboratory of Environmental Theoretical Chemistry South China Normal UniversityGuangzhouGuangdong 510006China Department of Environmental Science Baylor UniversityWacoTXUSA Center for Reservoir and Aquatic Systems Research(CRASR) Baylor UniversityWacoTXUSA School of Environment Tsinghua UniversityBeijing 100084China School of Civil and Environmental Engineering Cornell UniversityIthacaNY 14853USA Key Laboratory of Microbial Technology for Industrial Pollution Control of Zhejiang Province Zhejiang University of TechnologyHangzhou 310014China School of Environmental Science and Engineering Shanghai Jiao Tong UniversityShanghai 200240China Laboratoire d’Ecologie Microbienne Universite Claude Bernard Lyon 1UMR CNRS 5557UMR INRAE 1418VetAgro Sup69622 VilleurbanneFrance Department of Pla

Environmental pollution is escalating due to rapid global development that often prioritizes human needs over planetary *** global efforts to mitigate legacy pollutants,the continuous introduction of new substances remains a major threat to both people and the *** response,global initiatives are focusing on risk assessment and regulation of emerging contaminants,as demonstrated by the ongoing efforts to establish the UN’s Intergovernmental Science-Policy Panel on Chemicals,Waste,and pollution *** review identifies the sources and impacts of emerging contaminants on planetary health,emphasizing the importance of adopting a One Health *** for monitoring and addressing these pollutants are discussed,underscoring the need for robust and socially equitable environmental policies at both regional and international *** actions are needed to transition toward sustainable pollution management practices to safeguard our planet for future generations.

关键词： pollution planet contaminants

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