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Regulating energy storage performances of 0.85NaNbO_(3)-0.15Bi(Zn_(2/3)Nb_(1/3))O_(3) ceramics using BaTiO_(3)

Journal of Materiomics 2022年第1期8卷 166-173页

作者： Dongyu Lai Zhonghua Yao Wei You Biao Gao Qinghu Guo Ping Lu Amjad Ullah Hua Hao Minghe Cao Hanxing Liu State Key Laboratory of Advanced Technology for Materials Synthesis and Processing School of Material Science and EngineeringWuhan University of TechnologyWuhan430070China International School of Material Science and Engineering Wuhan University of TechnologyWuhan430070China

Recently,NaNbO_(3)-based ceramics with excellent energy storage performances(ESPs)and fast chargedischarge characteristics have attracted great *** this case,BaTiO_(3) modified 0.85NaNbO_(3)-0.15Bi(Zn_(2/3)Nb_(1/3))O_(3)(0.85NN-0.15BZN-yBT)ceramics were designed and successfully fabricated using solid state *** discharge storage density of the ceramics increases from 1.22 J/cm^(3) at y=0-1.84 J/cm^(3) at y=8%,which is 1.5 times higher than pure 0.85NN-0.15BZN *** ceramic reveals excellent temperature stability up to 150℃,good discharge cycling after 10^(5) cycles and high discharge speed of 2.0μs,broadening the scope of NaNbO_(3)-based ceramics for energy storage applications.

关键词： Perovskites Ceramics Dielectric properties Energy storage Capacitors

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FeNi@CNS nanocomposite as an efficient electrochemical catalyst for N_(2)-to-NH_(3) conversion under ambient conditions

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Journal of materials Science & technology 2022年第8期103卷 59-66页

作者： Tayiba Ilyas Fazal Raziq Nasir Ilyas Liuxin Yang Sharafat Ali Amir Zada Syedul Hasnain Bakhtiar Yong Wang Huahai Shen Liang Qiao School of Physics University of Electronic Science and Technology of ChinaChengdu 610054China State Key Laboratory of New Ceramics and Fine Processing School of Materials Science and EngineeringTsinghua UniversityBeijing 10084China Department of Chemistry Abdul Wali Khan University of MardanMardanKPK 23200Pakistan Laboratory of Living Materials at the State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070China Institute of Nuclear Physics and Chemistry Chinese Academy of Engineering PhysicsMianyang 621900China

The electrocatalytic nitrogen reduction reaction(NRR)has emerged as a promising renewable energy source and a feasible strategy as an alternative to Haber-Bosch ammonia(NH_(3))***,finding an efficient and cost-effective robust catalyst to activate and cleave the extremely strong triple bond in nitrogen(N_(2))for electrocatalytic NRR is still a ***,a FeNi@CNS nanocomposite as an efficient catalyst for N_(2) fixation under ambient conditions is *** FeNi@CNS nanocomposite was prepared by a simple water bath process and *** FeNi@CNS is demonstrated to be a highly efficient NRR catalyst,which exhibits better NRR performance with exceptional Faradaic efficiency of 9.83%and an NH_(3) yield of 16.52μg h^(−1) cm^(−2) in 0.1 M Na_(2)SO_(4) aqueous ***,high stability and reproducibility with consecutive 6 cycles for two hours are also demonstrated throughout the NRR electrocatalytic process for 12 ***,the FeNi@CNS catalyst encourages N_(2) adsorption and activation as well as effectively suppressing competitive ***,this earth-abundant FeNi@CNS catalyst with a subtle balance of activity and stability has excellent potential in NRR industrial applications.

关键词： Electrocatalytic nitrogen reduction Transition-metal alloy FeNi@CNS catalyst N_(2)fixation to NH_(3)

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Cu-N-C support confinement stabilizes active Co sites in oxygen reduction reaction

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Nano Research 2025年第5期18卷 134-144页

作者： Longyang Zhang Wei Sang Tingting Wang Xiaoyu Wei Zihan Li Cheng Chen Zongkui Kou Shichun Mu State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070China Sanya Science and Education Innovation Park of Wuhan University of Technology Sanya 572000China School of Mathematical and Physical Sciences Wuhan Textile UniversityWuhan 430200China

Strengthening the operational durability of oxygen reduction reaction(ORR)catalysts is essential for advancing both fuel cells and metal-air ***,developing highly active and durable catalysts remains a significant *** this study,a catalyst(Co/Cu-N-C)featuring uniformly distributed Co nanoparticles(NPs)and Co/Cu sites has been synthesized via a facile complex-assisted pyrolysis *** observed that Cu-N-C support effectively confines the growth and leaching of Co NPs during both synthesis and ORR catalysis,thereby boosting the stability of the ***,the presence of Co NPs and Cu sites slightly contributes to the ORR activity by optimizing the ^(*)OH *** assembled zinc-air battery(ZAB)demonstrates a superhigh power density of 256.1 mW·cm^(−2)and a long-term operational stability exceeding 500 *** work not only underscores the potential of bimetallic systems and NPs in enhancing catalyst stability but also provides valuable insights for the synthesis of high-performance ORR electrocatalysts.

关键词： metal nitrogen-doped carbon materials(M-N-C) stability oxygen reduction reaction(ORR) zinc-air batteries(ZABs) fuel cells

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Design and Dynamic Experiment of Al-Cu Graded materials Impactor with Strain Rate of 10^(4)–10^(5)/s

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稀有金属材料与工程 2025年第3期54卷 581-586页

作者： Hu Jianian Zhou Zizheng Li Yidi Chen Xiang Yang Gang Liu Jintao Zhang Jian State Key Laboratory of Precision Blasting Jianghan UniversityWuhan 430056China Hubei Key Laboratory of Blasting Engineering Jianghan UniversityWuhan 430056China Luoyang Ship Material Research Institute Luoyang 471023China State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070China

Based on simplified calculations of one-dimensional wave systems,loading pressure platform curves of Al-Cu gradient materials(GMs)impactor were *** Al-Cu GMs were prepared using tape-pressing sintering,and their acoustic properties were characterized to match the design *** parallelism of the Al-Cu GM was confirmed using a three-dimensional surface profilometry machine.A one-stage light-gas gun was used to launch the Al-Cu GM,impacting an Al-LiF target at a velocity of 400 m/*** results of the experimental strain rate demonstrate that the Al-Cu GMs can realize the precise control of the strain rate within the range of 10^(4)‒10^(5)/s in the high-speed impact experiments.

关键词： high strain rate Al-Cu graded materials impactor acoustic impedance gas gun experiment

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Iron anode-based aqueous electrochemical energy storage devices: Recent advances and future perspectives

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Interdisciplinary materials 2022年第1期1卷 116-139页

作者： Jian Jiang Jinping Liu Chongqing Key Lab for Advanced Materials and Clean Energies of Technologies School of Materials and EnergySouthwest UniversityChongqingChina State Key Laboratory of Advanced Technology for Materials Synthesis and Processing School of ChemistryChemical Engineering and Life ScienceWuhan University of TechnologyWuhanChina Key Laboratory for Photonic and Electronic Bandgap Materials Ministry of EducationSchool of Physics and Electronic EngineeringHarbin Normal UniversityHarbinChina

The ever-growing demands for green and sustainable power sources for ap-plications in grid-scale energy storage and portable/wearable devices have enabled the continual development of advanced aqueous electrochemical energy storage(EES)*** batteries and supercapacitors made of iron-based anodes are one of the most promising options due to the remark-able electrochemical features and natural abundance,pretty low cost and good environmental friendliness of ferruginous *** impressive ad-vances in developing the state-of-the-art ferruginous anodes and designing various full-cell aqueous devices have been made,there still remain key issues and challenges on the way to practical applications,which urgently need discussing to put forwards possible *** this review,rather than focusing on the detailed methods to optimize the iron anode,electrolyte,and device performance,we first give a comprehensive review on the charge storage mechanisms for ferruginous anodes in different electrolyte systems,as well as the newly developed iron-based aqueous EES *** deep in-sights,involving the inherent failure mechanisms and corresponding modification/optimization strategies toward iron anodes for the development of high-performance aqueous EES devices,will then be *** advances in applying iron-based aqueous EES devices for emerging fields such as flexible/wearable electronics and functionalized building materials will be further ***,future research trends and perspectives for maximizing the potential of current iron anodes and devices as well as exploiting brand-new iron-based aqueous EES systems are put forward.

关键词： aqueous batteries battolyser charge storage mechanism hybrid supercapacitors iron anode

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Single-atom metal-nitrogen-carbon catalysts energize single molecule detection for biosensing

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InfoMat 2023年第6期5卷 44-65页

作者： Xianyang Zhang Pengfei Chen Siwuxie He Bowen Jiang Yong Wang Yonghua Cheng Jian Peng Francis Verpoort John Wang Zongkui Kou State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhanthe People's Republic of China “ZhuCai”Center of Innovation and Entrepreneurship Wuhan University of TechnologyWuhanthe People's Republic of China West China School of Pharmacy Sichuan UniversityChengduthe People's Republic of China Department of Materials Science and Engineering Faculty of EngineeringNational University of SingaporeSingapore Institute of Materials Research and Engineering A*StarSingapore

Biosensors featuring single molecule detection present huge opportunities as well as challenges in food safety inspection,disease diagnosis,and environmental ***-molecule detection is largely lacking of high enough activity,precision molecule selectivity,and understanding in the exact operating ***-atom catalysts(SACs),especially those metals-nitrogen-carbon that mimic the natural metalloenzyme structure,and with well-defined metal atom bond configurations,high level of molecular selectivity,and easy fabrication,endow single molecule detections with practical-use *** recent advances in single-atom catalysts also present new pathways in the key mechanism *** this short review,we will first visit the brief history and advantages of SACs that have been explored only recently for molecule-scale biosensors,where they are analogous and also differentiated from those nanozymes and natural *** applications in electrochemical,photochemical,and photoelectrochemical sensors are then discussed comprehensively by focusing on the different molecule-scale sensing modes in achieving local coordination-modulated signal ***,we identify new opportunities and challenges faced by these SACs-based single molecule detections in the further development of biosensors.

关键词： biosensors metal-nitrogen-carbon nanozyme single molecule detection single-atom catalysts

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Green synthesis of luminescent La-MOF nanoparticle from waste poly(ethylene terephthalate) for high-performance in Fe(Ⅲ) detection

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Rare Metals 2024年第8期43卷 3833-3843页

作者： Zhi Gong Zhi-Kui Dai Zhi-Yue Dong Qiu-Xuan Liu Valentin A.Milichko Hua-Jian Liu Jie Liu Ran Niu Jiang Gong Key Laboratory of Material Chemistry for Energy Conversion and Storage Hubei Key Laboratory of Material Chemistry and Service FailureHubei Engineering Research Center for Biomaterials and Medical Protective MaterialsSemiconductor Chemistry CenterSchool of Chemistry and Chemical EngineeringMinistry of EducationHuazhong University of Science and TechnologyWuhan 430074China School of Chemical Engineering and Pharmacy Wuhan Institute of TechnologyWuhan 430073China Collaborative Innovation Center for Advanced Organic Chemical Materials Co-constructed by the Province and Ministry Ministry of Education Key Laboratory for the Synthesis and Application of Organic Functional Molecules and College of Chemistry and Chemical EngineeringHubei UniversityWuhan 430062China School of Physics and Engineering ITMO UniversitySt.Petersburg197101Russia School of Materials Science and Engineering Hubei UniversityWuhan430062China Guangdong Provincial Key Laboratory of Technique and Equipment for Macromolecular Advanced Manufacturing School of Mechanical and Automotive EngineeringKey Laboratory of Polymer Processing EngineeringMinistry of EducationSouth China University of TechnologyGuangzhou 510641China

Developing luminescent metal-organic frameworks(MOFs) capable of high-efficiency Fe^(3+)sensing has aroused great attraction in the fields of biology,chemistry,***,previous solvothermal methods are limited by organic solvent usage,time consuming,high pressure,and high-energy ***,we propose the waste-toMOF strategy towards the scale-up production of La-MOF nanoparticles through the ball milling of recycled poly(-ethylene terephthalate)(PET) bottles and La(NO_(3))_(3)·_(6)H_(2)*** goes on alkaline hydrolysis to form 1,4-benzenedicarboxylic acid sodium salt(Na_(2)BDC) and ethylene glycol by ball ***,BDC reacts with La^(3+)to form *** as-prepared La-MOF crystal nanoparticles possess a rod-like morphology with the size of few hundred ***,La-MOF nanoparticles display high selectivity and sensitivity for Fe^(3+)*** quenching constant and limit of detection are 5.29×10^(3)(mol·L^(-1))^(-1) and 0.147 μmol·L^(-1),respectively,thus surpassing many advanced Fe^(3+) *** to the result of density functional theory,the high Fe^(3+) detection performance of La-MOF is related to the complexing of Fe^(3+)with La-MOF,which leads to the gradual dissociation of the coordination bond between terephthalic acid and La^(3+).It is anticipated that the mechanochemistry milling-based wasteto-MOF strategy provides a new platform for the massive production of functional MOFs in a green manner.

关键词： Metal-organic framework Waste polyester Mechanochemistry milling Fluorescence sensor

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Advances in ultra-high temperature ceramics,composites,and coatings

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Journal of advanced Ceramics 2022年第1期11卷 1-56页

作者： Dewei NI Yuan CHENG Jiaping ZHANG Ji-Xuan LIU Ji ZOU Bowen CHEN Haoyang WU Hejun LI Shaoming DONG Jiecai HAN Xinghong ZHANG Qiangang FU Guo-Jun ZHANG State Key Laboratory of High Performance Ceramics&Superfine Microstructure Structural Ceramics and Composites Engineering Research CenterShanghai Institute of CeramicsChinese Academy of SciencesShanghai 200050China National Key Laboratory of Science and Technology on Advanced Composites in Special Environments Center for Composite Materials and StructuresHarbin Institute of TechnologyHarbin 150001China Shaanxi Key Laboratory of Fiber Reinforced Light Composite Materials Northwestern Polytechnical UniversityXi’an 710072China State Key Laboratory for Modification of Chemical Fibers and Polymer Materials Institute of Functional MaterialsDonghua UniversityShanghai 201620China State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070China University of Chinese Academy of Sciences Beijing 100049China

Ultra-high temperature ceramics(UHTCs)are generally referred to the carbides,nitrides,and borides of the transition metals,with the Group IVB compounds(Zr&Hf)and TaC as the main *** UHTCs are endowed with ultra-high melting points,excellent mechanical properties,and ablation resistance at elevated *** unique combinations of properties make them promising materials for extremely environmental structural applications in rocket and hypersonic vehicles,particularly nozzles,leading edges,and engine components,*** addition to bulk UHTCs,UHTC coatings and fiber reinforced UHTC composites are extensively developed and applied to avoid the intrinsic brittleness and poor thermal shock resistance of bulk ***,high-entropy UHTCs are developed rapidly and attract a lot of attention as an emerging direction for ultra-high temperature *** review presents the state of the art of processing approaches,microstructure design and properties of UHTCs from bulk materials to composites and coatings,as well as the future directions.

关键词： ultra-high temperature ceramics(UHTCs) coatings composites high-entropy ultra-high temperature ceramics

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Na_(3)Zr_(2)Si_(2)PO_(12) solid-state electrolyte with glass-like morphology for enhanced dendrite suppression

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Rare Metals 2022年第12期41卷 4086-4093页

作者： Hang Su Shi-Wei Zhang Yi-Meng Liu Chao Yang Li-Xiao Zhang Sen Xin Ya You State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070China CAS Key Laboratory of Molecular Nanostructure and Nanotechnology CAS Research/Education Center for Excellence in Molecular SciencesInstitute of ChemistryChinese Academy of Sciences(CAS)Beijing 100190China University of Chinese Academy of Sciences International School of Materials Science and Engineering Wuhan University of TechnologyWuhan 430070China

Rechargeable batteries based on solid-state electrolytes are of great interest and importance for the next-generation energy storage due to their high energy output and improved *** building the solid-state batteries,Na_(3)Zr_(2)Si_(2)PO_(12)(NZSP)represents a promising candidate as it features high chemical stability against air exposure and a high Na^(+)*** pellets were usually calcined at a high temperature,and the high volatility of Na and P elements easily led to the formation of impurity *** this work,the effects of calcination temperature and stoichiometry on the phase purity and ionic conductivity of the NZSP electrolyte were *** an elevated sintering temperature,the NZSP electrolyte showed a high ionic conductivity owing to decreased porosity,and the highest ionic conductivity at 30℃was observed to be 2.75×10^(-5)S·cm^(-1)with an activation energy of 0.41 *** the stoichiometry,the introduction of 5 mol%excessive P results in formation of more Na_(3)PO_(4) and glass-like phase at the grain boundary,which caused the blurred grain boundary and reduced grain barrier,and effectively suppressed Na dendrite growth,then accounted for improved cycling performance of a Na‖Na symmetric *** work provided insights on reasonable design and preparation of NZSP electrolyte towards practical realization of solid-state Na-metal batteries.

关键词： Na_(3)Zr_(2)Si_(2)PO_(12)(NZSP) Natrium superionic conductor(NASICON)solid-state electrolytes Grain boundary Ionic conductivity Glass-like morphology

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Thermoelectric Properties of an Individual Suspended Single-Crystalline Sb_(2)Se_(3)Nanowire

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Journal of Thermal Science 2022年第4期31卷 1106-1114页

作者： DU Yanzheng SHI Shaoyi MIAO Tingting MA Weigang MAI Liqiang ZHANG Xing Key Laboratory for Thermal Science and Power Engineering of Ministry of Education Department of Engineering Mechanics Tsinghua UniversityBeijing 100084China Beijing Key Laboratory of Process Fluid Filtration and Separation College of Mechanical and Transportation EngineeringChina University of PetroleumBeijing 102249China State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan430070China

Nanowires exhibit excellent thermoelectric performance,due to the stronger quantum confinement and phonon scattering effect compared to bulk ***,it is a challenge to accurately evaluate the thermoelectric performance of *** this paper,the thermoelectric properties of an individual suspended Sb_(2)Se_(3) nanowire have been characterized by comprehensive T-type method,including thermal conductivity,electrical conductivity,Seebeck coefficient and figure of *** thermal conductivity increases from 0.57 W/(m·K)to 3.69 W/(m·K)with temperature increasing from 80 K to 320 *** lattice vibration dominates the heat conduction process,and due to its flawless crystal structure,the thermal conductivity is not lower than the reported values of bulk Sb_(2)Se_(3).The electrical conductivity increases from 7.83 S/m to 688 S/m in the temperature range of 50 K–320 K,which is a great improvement compared with the corresponding bulk *** 294 K,the Seebeck coefficient of the Sb_(2)Se_(3) nanowire is–1120μV/K and the corresponding figure of merit is 0.064.

关键词： Sb_(2)Se_(3)nanowire thermoelectric properties thermal conductivity Seebeck coefficient electrical conductivity

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