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Experimental and kinetic study on laminar flame speeds of ammonia/syngas/air at a high temperature and elevated pressure

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Frontiers in Energy 2022年第2期16卷 263-276页

作者： Geyuan YIN Chaojun WANG Meng ZHOU Yajie ZHOU Erjiang HU Zuohua HUANG State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong UniversityXi’an 710049China Key Laboratory for Thermal Science and Power Engineering of the Ministry of Education Department of Thermal EngineeringTsinghua UniversityBeijing 100084China

The laminar flame speeds of ammonia mixed with syngas at a high pressure, temperature, and different syngas ratios were measured. The data obtained were fitted at different pressures, temperatures, syngas ratios, and equivalence ratios. Four kinetic models (the Glarborg model, Shrestha model, Mei model, and Han model) were compared and validated with experimental data. Pathway, sensitivity and radical pool analysis are conducted to find out the deep kinetic insight on ammonia oxidation and NO formation. The pathway analysis shows that H abstraction reactions and NHi combination reactions play important roles in ammonia oxidation. NO formation is closely related to H, OH, the O radical produced, and formation reactions. NO is mainly formed from reaction, HNO+ H= NO+ H2. Furthermore, both ammonia oxidation and NO formation are sensitive to small radical reactions and ammonia related reactions.

关键词： ammonia mixed with syngas laminar flame speed kinetic model sensitivity analysis pathway analysis

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Multi-objective optimization research of open and closed air brayton cycle

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International Journal of Advanced Nuclear Reactor Design and Technology 2024年第1期6卷 21-31页

作者： Song, Meihui Qian, Yiran Leng, Yuyang Liu, Tao Yu, Lianyun Chen, Weixiong State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Shaanxi Xi'an710049 China Reactor Engineering Technology Research Institute China Institute of Atomic Energy Beijing102413 China

Air Brayton cycle obtains the significant advantages of high efficiency, compact structure, easy medium requirement and so on, which is one of the most suitable choices for the mobile nuclear power conversion system. In this paper, system-component combined design method is used to establish the open and closed air Brayton cycle of diverse configurations. Based on performance and compactness targets, the multi-objective optimization is carried out to find the optimal design by nondominated sorting genetic algorithm II and entropy weight method. According to the analysis, the closed intercooling reheating recuperating cycle is the configuration with the best comprehensive performance, with cycle efficiency of 33.58 %, power density of 175.39 kW m−3 and power mass ratio of 68.60 kW t−1. The open simple recuperating cycle is the configuration with the smallest volume and mass, with cycle efficiency of 20.01 %, system volume of 6.56 m3 and system mass of 19.98 t. The closed intercooling recuperating cycle is the most balanced configuration, with cycle efficiency of 31.33 %, volume of 9.06 m3 and system mass of 24.97 t. Based on the optimal results, off-design performance analysis of different environmental conditions is also carried out for the configurations above. © 2024 Xi'an Jiaotong University

关键词： Brayton cycle

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Study on iterative algorithm of full plate cross-flow and counter-flow printed circuit heat exchanger for fluoride-salt-cooled high-temperature advanced reactor

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International Journal of Advanced Nuclear Reactor Design and Technology 2023年第2期5卷 86-96页

作者： Li, Xinze Zhang, Dalin Li, Xinyu Tian, Wenxi Qiu, Suizheng Su, G.H. State Key Laboratory of Multiphase Flow in Power Engineering Shaanxi Key Laboratory of Advanced Nuclear Energy and Technology School of Nuclear Science and Technology Xi'an Jiaotong University Xi'an710049 China

In the concept of Fluoride-Salt-cooled high-Temperature Advanced Reactor (FuSTAR), the Printed Circuit Heat Exchanger (PCHE) is mainly considered in its supercritical carbon dioxide (S–CO2) Brayton cycle secondary loop. The design of the PCHE is based on the property of working fluid provided by the Brayton cycle system design. Therefore, a fast and iterative PCHE design method is required. In this study, a mathematical model based on Picard's iterative method is proposed. The model can solve full plate temperature field with complex boundary conditions and initial values including cross-flow and counter-flow PCHE in parallel. Based on FuSTAR Brayton cycle design conditions, three sizes of cross-flow and counter-flow PCHEs are simulated respectively by the mathematical model. Compared with Computational Fluid Dynamics (CFD) models, a one and three-dimensional coupling model and a three-dimensional model, the mathematical model reduced the computing time from 1 to 10 h to 1–10 s, and the maximum temperature mean deviation is 18.6% for the smallest size case because of the edge effect and local disturbance, but 8.4% for other size. Taking secondary loop recuperator design as example, the computing speed and accuracy of the mathematical model can meet the design requirements of FuSTAR PCHE. © 2023 Xi'an Jiaotong University

关键词： Carbon dioxide

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EFFECT OF INNER FIN TUBE STRUCTURE ON COMPREHENSIVE PERFORMANCE OF SUPERCRITICAL CARBON DIOXIDE AND LEAD BISMUTH EUTECTIC HEAT EXCHANGER

EFFECT OF INNER FIN TUBE STRUCTURE ON COMPREHENSIVE PERFORMA...

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ASME 2023 Heat Transfer Summer Conference, HT 2023

作者： Shuhan, Liu Ji’an, Liu Qingjiang, Liu Xianliang, Lei State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an China

ISBN: (纸本)9780791887165

In the combined system of lead cooled fast reactor (LFR) and supercritical carbon dioxide (S-CO2) Brayton cycle, the intermediate heat exchanger plays a key role in the whole power system. However, the existing heat exchanger can not meet the trend of miniaturization of lead cooled fast reactor. Considering the thermo-physical properties and heat transfer behaviors in both S-CO2 and liquid lead bismuth eutectic (LBE) are significantly different, an asymmetric compact coupled heat exchanger learning from Honeycomb structure is proposed. Through numerical simulation, it is found that the thermal resistance mainly exists in the cold side. In order to enhance the heat transfer at the S-CO2 side, the fin tube is adopted at the cold side. The results show that the heat transfer performance and friction factor of the heat exchanger increase with the increase of fin height, width and number of fins due to the increase of heat transfer area. When the fin height is increased, PEC gradually increases at low inlet velocity, and then decreases at high inlet velocity;When the fin width is increased, PEC increases first and then decreases at low inlet velocity, and decreases gradually at high inlet velocity;With the increase of the number of fins, PEC showed an increasing trend at different inlet velocities. © 2023 by ASME.

关键词： Supercritical fluid extraction

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Progress and challenge of functional single-atom catalysts for the catalytic oxidation of volatile organic compounds

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Chinese Chemical Letters 2024年第9期35卷 83-91页

作者： Zeyu Jiang Yadi Wang Changwei Chen Chi He Department of Environmental Science and Engineering Xi’an Jiaotong UniversityXi’an 710049China State Key Laboratory of Multiphase Flow in Power Engineering School of Energy and Power EngineeringXi’an Jiaotong UniversityXi’an 710049China National Engineering Laboratory for VOCs Pollution Control Material&Technology University of Chinese Academy of SciencesBeijing 101408China

The catalytic oxidation of volatile organic compounds(VOCs)is of considerable significance for the sustainable development of the chemical industry;thus,considerable efforts have been devoted to the exploration of efficient catalysts for use in this *** this regard,the development and utilization of single-atom catalysts(SACs)in VOCs decomposition is a rapidly expanding research *** can be employed as potential catalysts for oxidizing VOC molecules due to their optimal utilization efficiency,unique atomic bonding structures,and unsaturated *** has been achieved,while the challenges surrounding precise regulation of the microstructures of SACs for improving their low-temperature efficiency,stability,and product selectivity under practical conditions are ***,elucidating structure-performance relationships and establishing intrinsic modulating mechanisms are urgently required for guiding researchers on how to synthesize effective and stable functional SACs ***,recent advances in the design and synthesis of functional SACs for application in the catalytic oxidation of VOCs are *** experimental and theoretical studies revealing higher efficiency,stability,and selectivity of as-prepared functional SACs are being ***,the future perspectives in terms of promising catalysts with multi-sized composite active sites and the illustration of intrinsic mechanism are *** rapid intelligent screening of applicable SACs and their industrial applications are also discussed.

关键词： Single-atom catalysts VOCs catalytic oxidation Hydrocarbon activation Oxygen species transformation Surface chemistry Intrinsic mechanism

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NUMERICAL SIMULATION OF FLUID-STRUCTURE COUPLING FOR THE MAIN PUMP OF LEAD COOLED FAST REACTOR 30

NUMERICAL SIMULATION OF FLUID-STRUCTURE COUPLING FOR THE MAI...

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30th International Conference on Nuclear engineering, ICONE 2023

作者： Xiang, Zutao Li, Liangxing Zhao, Jiayuan Xu, Xiangyang State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an China

ISBN: (纸本)9784888982566

The main pump blades of lead cooled fast reactor have complex mechanical characteristics, and there are complex fluid-structure coupling problems in the structural analysis of the impeller. In this paper, CFX software is mainly used for numerical simulation to carry out one-way fluid-structure coupling research on the moving blade of the main pump. Generally, three kinds of materials as Ti3SiC2, T91 steel and 304 stainless steel are considered for the moving blade of main pump and the deformation distribution and equivalent stress distribution of the three models under the three moving blade materials are analyzed respectively. Finally, the modal analysis of the moving blade of the main pump is carried out. The results show that the resistance to deformation of moving blade made in Ti3SiC2 is better than those of T91 steel and 304 stainless steel;The equivalent stress on the pressure surface of Ti3SiC2 is slightly higher than those of T91 steel and 304 stainless steel, and the maximum equivalent stress on the pressure surface of moving blade occurs on the inner edge of the blade. This research can provide reference for the design of moving blades, and help to improve the service life of the main pump. © 2023 by JSME.

关键词： Numerical models

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Performance comparison investigation on different pulse tube position heat pumps with power recovery displacer

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International Journal of Refrigeration 2025年 176卷 1-16页

作者： Zhu, Shenglin Chen, Xi Zhu, Yifan Qi, Yingxia School of Energy and Power Engineering University of Shanghai for Science and Technology 516 Jungong Road Shanghai200093 China Shanghai Key Laboratory of Multiphase Flow and Heat Transfer in Power Engineering University of Shanghai for Science and Technology 516 Jungong Road Shanghai200093 China

Spacecraft waste heat is dissipated into space primarily by radiation. To improve the heat dissipation efficiency of spacecraft radiators in high-temperature environments and reduce heat wastage in spaceflight thermal control systems, thermoacoustic heat pumps (TAHP) are considered a viable method for increasing radiator cooling temperatures and recovering waste heat. In this study, one-dimensional simulations are used to optimize the geometrical parameters of the 100-watt work recovery thermoacoustic heat pump (WRTAHP) for various pulse tube positions. The performances of the two systems are compared at a cold-end temperature of 293 K and a hot-end temperature of 353 K. The results reveal that a heating capacity of 256 W with a relative Carnot efficiency of 35.01 % is achieved for the pulse tube front-type thermoacoustic heat pump (FTTAHP), whereas the pulse tube back-type thermoacoustic heat pump (BTTAHP) obtains a heating capacity of 225 W with a relative Carnot efficiency of 30.59 %. As the cold-end temperature decreases, the coefficient of performance is reduced for FTTAHP, while the performance of BTTAHP shows a substantial improvement. At a cold end temperature of 233 K and a hot-cold end temperature difference of 60 K, a heating capacity of 268 W with a relative Carnot efficiency of 50.57 % is achieved for BTTAHP. Furthermore, the heating capacity of the BTTAHP is not significantly increased by adopting the active phase adjustment structure. In summary, the FTTAHP is suitable for spacecraft radiator applications and avoids high temperatures affecting compressor operation, whereas the BTTAHP is better suited for low-temperature heating. © 2025 Elsevier Ltd and IIR

关键词： Waste heat utilization

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Base-or acid-assisted polystyrene plastic degradation in supercritical CO_(2)

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Waste Disposal and Sustainable Energy 2023年第2期5卷 165-175页

作者： Yanbing Liu Jinwen Shi Liuhao Mao Bingru Lu Xing Kang Hui Jin International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power EngineeringXi’an Jiaotong University28 West Xianning RoadXi’an710049ShaanxiChina

Plastic has caused serious"white pollution"to the environment,and the highly inert characteristics of plastic bring a major challenge for *** fluids have unique physical properties and have been widely used in various *** this work,supercritical CO_(2)(Sc-CO_(2))with mild conditions was selected and assisted by NaOH/HCl solution to degrade polystyrene(PS)plastic,and the reaction model was designed using response surface methodology(RSM).It was found that,regardless of the types of assistance solutions,the factors affecting PS degradation efficiencies were reaction temperature,reaction time,and NaOH/HCl *** the temperature of 400℃,time of 120 min,and base/acid concentration of 5%(in weight),0.15 g PS produced 126.88/116.99±5 mL of gases with 74.18/62.78±5 mL of H2,and consumed 81.2/71.5±5 mL of CO_(2).Sc-CO_(2)created a homogeneous environment,which made PS highly dispersed and uniformly heated,thus promoting the degradation of ***,Sc-CO_(2)also reacted with the degradation products to produce new CO and more CH_(4)and C_(2)H_(x)(x=4,6).Adding NaOH/HCl solution not only improved the solubility of PS in Sc-CO_(2),but also provided a base/acid environment that reduced the activation energy of the reaction,and effectively improved the degradation efficiencies of *** short,degrading PS in Sc-CO_(2)is feasible,and better results are obtained with the assistance of base/acid solution,which can provide a reference for the disposal of waste plastics in the future.

关键词： Plastic degradation Polystyrene Supercritical CO_(2) NaOH HCl

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Experimental investigation on the gravity driven discharge of cohesive particles from a silo with two outlets

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Particuology 2024年第6期89卷 11-21页

作者： Li Dai Zhulin Yuan Fengxian Fan Conghui Gu School of Energy and Power Engineering University of Shanghai for Science and TechnologyShanghai 200093China Key Laboratory of Energy Thermal Conversion and Control of Ministry of Education School of Energy and EnvironmentSoutheast UniversityNanjing 210096China Shanghai Key Laboratory of Multiphase Flow and Heat Transfer in Power Engineering University of Shanghai for Science and TechnologyShanghai 200093China School of Energy and Power Jiangsu University of Science and TechnologyZhenjiang 212100China

An experimental study on the gravity driven discharge of cohesive particles from a silo with two outlets was *** discharge behaviors under the conditions that a single outlet was open and two outlets were open were investigated by varying the moisture content of the particles and the filling height of the particles in the *** results show that the discharge rate of the cohesive particles increases gradually at the beginning,then almost keeps constant,and finally drops *** discharge rate in case of two openings is around 1.1–1.6 times that in case of a single *** filling height leads to lower discharge rate in case of a single opening but results in higher discharge rate in case of two ***,the avalanche dynamics in case of a single opening was examined,and the mixing behavior of the cohesive particles was *** is observed that the discharge flow is promoted by the avalanche phenomenon in the silo,generating a general trend that the normalized mass of discharge increases with the filling height at higher moisture *** case of a single opening,the transition from mass flow to funnel flow favors the particle mixing,resulting in an increasing mixing index as the moisture content *** general,a better performance of mixing can be achieved in case of a single opening compared with in case of two *** study provides vital information for fundamental understanding of the gravity driven discharge of cohesive particles from the silo with multiple outlets.

关键词： Cohesive particles Moisture content Discharge rate Avalanche Mixing

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Fabricating PdCe/OMS-2 catalysts with boosted low-temperature activity for toluene deep degradation

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Journal of Rare Earths 2023年第6期41卷 839-849,I0002页

作者： Lin Yue Zhihua Xu Minghua Hu Mingjiao Tian Mudi Ma Bijie Huang Chi He State Key Laboratory of Multiphase Flow in Power Engineering School of Energy and Power EngineeringXi'an Jiaotong UniversityXi'an 710049China State Key Laboratory of Precision Blasting and Hubei Key Laboratory of Industrial Fume and Dust Pollution Control Jianghan UniversityWuhan 430056China National Engineering Laboratory for VOCs Pollution Control Material&Technology University of Chinese Academy of SciencesBeijing 101408China

Porous cryptomelane-type octahedral molecular sieve(OMS-2)with mixed Mn valence and abundant lattice oxygen species has attracted much attention in volatile organic compounds(VOC)catalytic ***,complete conversion of arene over OMS-2 catalysts at relatively low temperature is still a challenge due to its limited crystal structure and inferior ***,a series of PdCe/OMS-2 catalysts with different Pd/Ce molar ratios was fabricated by a facile impregnation method and the physicochemical properties of which were extensively characterized by X-ray diffraction(XRD),scanning electron microscopy(SEM),high-resolution transmission electron microscopy(HR-TEM),B runauer-Emmett-Teller(BET)method,X-ray fluorescence(XRF),X-ray photoelectron spectroscopy(XPS),temperature programmed reduction of H2(H2-TPR),Raman,In situ diffused reflectance infrared Fourier transform spectra(DRIFTS),and density functional theory(DFT)*** show that the total conversion of toluene can be achieved at 207℃ over PdCe2 with apparent activation energy as low as 62.6 kJ/*** strong synergistic effect between Pd and Ce remarkably boosts the catalytic activity of OMS-2,attributed to the abundant Mn^(3+)-O bands and active surface oxygen *** results reveal that oxygen vacancy can be formed over PdCe2 much easily than that of Pd/OMS-2 and Ce/OMS-2 with the oxygen vacancy formation energy of2.42,2.83 and 2.68 eV,*** increasing the Pd content cannot promote the catalytic activity although PdO is a critical active center in toluene *** vacancy attributed to the integrative effect of Pd,Ce and Mn species plays a promine nt role over prepared catalysts in toluene activation *** findings reported in this work showed new insights into the designing of highly efficient OMS-2catalysts for VOC deep oxidation by tuning oxygen vacancy concentration.

关键词： PdCe/OMS-2 Toluene Catalytic oxidation Oxygen vacancy Rare earths

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