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Au@SiO_2 core/shell nanoparticle-decorated TiO_2 nanorod arrays for enhanced photoelectrochemical water splitting

Chinese Science Bulletin 2014年第18期59卷 2191-2198页

作者： Jianan Chen Miao Yu Yuhao Wang Shaohua Shen Meng Wang Liejin Guo International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power EngineeringXi’an Jiaotong University School of Chemical Engineering and Technology Harbin Institute of Technology

To improve the separation efficiency of photoinduced charge carries,Au@SiO2nanoparticles(NPs)with core–shell structure were loaded onto the surface of TiO2nanorods grown on fluorine-doped tin oxide substrate by a facile two-step *** resulted Au@SiO2/TiO2photoanodes were characterized by X-ray diffraction,scanning electron microscopy,transmission electron microscopy,as well as photoelectrochemical *** with pristine TiO2nanorod film,the Au@SiO2/TiO2films showed remarkable enhancement in photoelectrochemical water splitting,with incident photonto-current conversion efficiency increasing from 31%to37%at 380 nm at 0.7 V versus saturated calomel *** could be interpreted by the effect of metallic surface plasmon resonance of Au@SiO2NPs,which would generate an intense electromagnetic field with spatially nonhomogenous distributed *** a result,the charge carriers generated in the near-surface region of TiO2nanorods could be easily *** modification method based on the effect of metallic surface plasmon resonance for promoted charge carrier separation provides a promising way to develop semiconductor photoelectrodes with high solar water-splitting performance.

关键词：二氧化硅纳米粒子二氧化钛纳米棒电解水表面等离子体共振效应纳米颗粒金属 TiO2薄膜

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Experimental and modeling study on auto-ignition of DME/ n -butane blends under engine relevant pressure

Experimental and modeling study on auto-ignition of DME/ n -...

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SAE 2014 World Congress and Exhibition

作者： Jiang, Xue Zhang, Yingjia Pan, Lun Man, Xingjia Huang, Zuohua State Key Laboratory of Multiphase Flow in Power Engineering Xi'An Jiaotong University Xi'an 710049 China

In this study, the ignition delay times of DME/n-C4H 10 fuel blends (neat DME, 50/50 and neat n-C4H 10) diluted with argon were measured behind reflected shock waves. The experiments were performed in the temperature range of 1250 - 1600 K, at pressure of 2.0 MPa and equivalence ratios from 0.5 to 2.0. A latest kinetic mechanism NUIG Aramco Mech 1.3 was validated against the present ignition data and used to conducted chemical kinetic analysis. Different equivalence-ratio- dependent was exhibited at different temperature regimes for DME, n-C 4H10, and their blend. Fuel flux analysis, sensitive analysis and mole fraction analysis were carried out for understanding the interaction between the ignition chemistries of DME and n-C4H 10. Copyright © 2014 SAE International.

关键词： Shock waves

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Experimental and modeling study on ignition delay times of dimethyl ether/ n -butane blends at a pressure of 2.0 MPa

Experimental and modeling study on ignition delay times of d...

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作者： Jiang, Xue Zhang, Yingjia Man, Xingjia Pan, Lun Huang, Zuohua State Key Laboratory of Multiphase Flow in Power Engineering Xi'An Jiaotong University Xi'an 710049 China

In this study, the ignition delay times of dimethyl ether (DME)/n-C 4H10 fuel blends, neat DME, and neat n-C4H 10 diluted with argon were measured behind reflected shock waves. The experiments were performed in the temperature range of 1100-1600 K, at a pressure of 2.0 MPa, and equivalence ratios from 0.5 to 2.0. A latest kinetic mechanism NUIG Aramco Mech 1.3 was validated against the measured ignition data and used to conduct the chemical kinetic analysis. Results showed that different equivalence ratio-dependent behaviors were exhibited at different temperature regimes for DME, n-C4H10, and their blend. The ignition delay time of neat n-C4H10 was increased with an increase in the equivalence ratio. A strong inhibiting trend was exhibited at high temperatures. For the neat DME, however, an opposite influencing tendency from the equivalence ratio was presented in comparison to that on n-C 4H10. Ignition promotion becomes significant at relatively low temperatures. A 50% DME/50% n-C4H10 blend show a combined behavior of both n-butane and DME. Fuel reaction flux analysis, sensitive analysis, and mole fraction analysis were conducted for the understanding of the interaction between the ignition chemistries of DME and n-C4H10 at a pressure of 2.0 MPa. © 2014 American Chemical Society.

关键词： Ethers

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Convective heat transfer characteristics of supercritical hydrocarbon fuel in small non-circular cross-section Channels 11

Convective heat transfer characteristics of supercritical hy...

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AIAA AVIATION 2014 -11th AIAA/ASME Joint Thermophysics and Heat Transfer Conference 2014

作者： Guo, Yong Yang, Zhuqiang Jiang, Lei Liu, Zhaohui Bi, Qincheng State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an 710049 China

ISBN: (数字)9781624102813

ISBN: (纸本)9781624102813

Convective heat transfer characteristics of supercritical pressure hydrocarbon fuel were experimentally investigated in electrically heated small non-circular channels with hydraulic diameter ranging from 2.00 to 3.00 mm. In this research, the system pressure and fuel mass velocity were maintained at supercritical (3.0 MPa) and 840.0 kg/(m2·s), while fuel inlet temperature varied from 200.0 ~ 450.0 °C. Heat transfer characteristics of various cross-section channels were obtained in view of the temperature profiles on the channel outside surface. Experimental results were compared among different non-circular channels. The effects of inlet fuel temperature, heat flux, aspect ratio or length to diameter ratio on the convective heat transfer characteristics were discussed. Due to the varieties of length to diameter ratio, the unique heat transfer characteristics of non-circular cross-section channels seemed to make them suitable for the application of hypersonic vehicle. However, this study did not consider the pyrolytic reaction in the high temperature range. The coking characteristics of small non-circular channels under high temperature may trade off the benefits acquired in the heat transfer characteristics.

关键词： Aspect ratio

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Heat transfer characteristics of hydrocarbon fuel in a horizontal small tube under different pressures 11

Heat transfer characteristics of hydrocarbon fuel in a horiz...

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AIAA AVIATION 2014 -11th AIAA/ASME Joint Thermophysics and Heat Transfer Conference 2014

作者： Yang, Zhuqiang Bi, Qincheng Guo, Yong Liu, Zhaohui Jiang, Lei State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi' an 710049 China

ISBN: (数字)9781624102813

ISBN: (纸本)9781624102813

Experiments for heat transfer of a kerosene hydrocarbon fuel in a small horizontal tube have been conducted at subcritical and supercritical pressures. Parameters included the pressure of 2.0-5.0 MPa, mass flux of 822-2466 kg/ (m2·s) and heat flux up to 1500 kW/m2. The wall temperature and heat transfer performance at various operating conditions were captured in the experiments. Based on the results, the normal, improved and deteriorated heat transfer characteristics of the fuel were analyzed in detail. The effects of heat flux, pressure and mass flux on the heat transfer were discussed respectively. The heat transfer performed better when working pressure approached critical pressure. The deterioration in the large change of thermophysical properties region didn't occur at supercritical pressures. In the test, the increase of mass flux could enhance the heat transfer. But the effect of the enhancement decreased with mass flux increase. As to the pressure drop characteristics, low pressure and high mass flux both contributed to the increase of flow resistance.

关键词： Heat flux

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Visualization investigation of secondary flow on heat transfer deterioration in horizontal heat tube 22

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2014 22nd International Conference on Nuclear engineering, ICONE 2014

作者： Wu, Chao Li, Hui-Xiong Qian, Zhang State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an Shaanxi China

ISBN: (纸本)9780791845905

Mixed convection heat transfer in heated tubes has been studied extensively in the past decades, which is widely used in various industrial fields such as cooling of a nuclear reactor core. The secondary flow, which is induced by buoyancy force, has been found in previous research to have profound influence on the heat transfer difference on circumferential position and occurrence of heat transfer deterioration in horizontal heated channel. Therefore, understanding the secondary flow velocity field has important implications to prevent heat transfer deterioration and ensure the safe operation of nuclear power plants. Numerical methods have been adopted in literature to analyze the complex interaction between secondary flow and heat transfer deterioration. However, to the knowledge of the author, experimental measurement of secondary flow in the radial cross-section of a horizontal tube does not exist.. Copyright © 2014 by ASME.

关键词： Numerical methods

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Flame-front instabilities of outwardly expanding isooctane/ n -butanol blend-air flames at elevated pressures

Flame-front instabilities of outwardly expanding isooctane/ ...

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作者： Zhang, Xinyi Tang, Chenglong Yu, Huibin Huang, Zuohua State Key Laboratory of Multiphase Flow in Power Engineering Xi'An Jiaotong University Xi'an 710049 China

Experiments were conducted in a constant volume bomb filled with isooctane/n-butanol blend-air mixtures over a wide range of n-butanol blending ratios, equivalence ratios, and initial pressures. High-speed schlieren photography was used to measure the critical radius for the onset of flame-front instability. Results show that, for a given n-butanol blending ratio, cellular instabilities appear earlier and the critical Peclet number, which represents the onset of instability, is decreased with the increase of the initial pressure and equivalence ratio. Under fuel-rich conditions, the critical Peclet number increases with the increase of the n-butanol blending ratio. Theoretical calculation of the critical Peclet number was also conducted to interpret the effects of n-butanol on the flame-front instabilities of the blends. Results show that, for rich mixture conditions, with the increase of the n-butanol blending ratio, the overall activation energy of the mixtures is decreased and, thus, the thermal-diffusional instabilities are suppressed. While under fuel-lean conditions, the thermal-diffusional instabilities are favored. As a consequence, with an increasing n-butanol blending ratio, the critical Peclet number is expected to be decreased under fuel-lean conditions and increased under fuel-rich conditions. © 2014 American Chemical Society.

关键词： Mixtures

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Preliminary safety analysis of the PWR with accident-tolerant fuels during severe accident conditions

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Annals of Nuclear Energy 2015年 80卷 1-13页

作者： Xiaoli Wu Wei Li Yang Wang Yapei Zhang Wenxi Tian Guanghui Su Suizheng Qiu Tong Liu Yongjun Deng Heng Huang State Key Laboratory of Multiphase Flow in Power Engineering School of Nuclear Science and Technology Xi’an Jiaotong University No. 28 Xianning West Road Xi’an Shanxi 710049 China China Nuclear Power Technology Research Institute A-1101 Fengde Plaza No. 6 Hangkong Road Chengdu Sichuan 610000 China

Experience gained in decades of nuclear safety research and previous nuclear accidents direct to the investigation of passive safety system design and accident-tolerant fuel (ATF) system which is now becoming a hot research point in the nuclear energy field. The ATF system is aimed at upgrading safety characteristics of the nuclear fuel and cladding in a reactor core where active cooling has been lost, and is preferable or comparable to the current UO 2 –Zr system when the reactor is in normal operation. By virtue of advanced materials with improved properties, the ATF system will obviously slow down the progression of accidents, allowing wider margin of time for the mitigation measures to work. Specifically, the simulation and analysis of a large break loss of coolant accident (LBLOCA) without ECCS and extended station blackout (SBO) severe accident are performed for a pressurized water reactor (PWR) loaded with ATF candidates, to reflect the accident-tolerance of ATF.

关键词： Safety analysis Accident-tolerant Severe accident

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Pool boiling heat transfer enhancement by γ-Al2O3 /FC-72 nanofluids on a smooth surface 15

Pool boiling heat transfer enhancement by γ-Al2O3 /FC-72 na...

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15th International Heat Transfer Conference, IHTC 2014

作者： Kong, Xin Wei, Jinjia Ding, Jie Zhang, Yonghai State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong Uniersity Xi'an Shaanxi710049 China

The influence of γ-Al2O3/FC-72 nanofluids on pooling boiling heat transfer with a smooth surface was experimentally investigated. The fluorocarbon surfactant FSO-100 was also used in the experiment. In order to distinguish the effects of surfactant, four groups of contrast tests were designed as follows: base fluids (FC-72), base fluids with nanoparticles (γ-Al2O3+FC-72), base fluids with surfactant (FC-72+FSO-100) and nanofluids with surfactant (γ-Al2O3/FC-72+FSO-100). The results of nanofluids with surfactant showed that the heat transfer performance is enhanced compared with base fluid, but will weaken with the increase of particle concentration. In general, nanofluids can enhance the boiling heat transfer to some extent, and the enhancement is affected by the adjunction of surfactant and the sedimentation of nano-particules. Nanofluids prepared with only nanoparticles were not stable due to nonuniform distribution of the particles. The adjunction of surfactant (without nanoparticules) will lead to a significant deterioration in both heat transfer coefficient and CHF (Critical Heat Flux), but it can keep nanofluids stable and homogeneous to some degree for heat transfer enhancement.

关键词： Nanoparticles

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Effect of anolyte pH and cathode Pt loading on electricity and hydrogen co-production performance of the bio-electrochemical system

Effect of anolyte pH and cathode Pt loading on electricity a...

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作者： Liu, Ya-Peng Wang, Yun-Hai Wang, Bai-Shi Chen, Qing-Yun Department of Environmental Engineering State Key Laboratory of Multiphase Flow in Power Engineering Xi'An Jiaotong University Xi'an 710049 China

In a novel bio-electrochemical system (BES) for hydrogen and electricity co-production with acetate substrate, the anolyte pH and cathode Pt loading effects are investigated to improve the cell performance for hydrogen and electricity co-production and reduce the cost. The optimized anolyte pH is 9. The maximum hydrogen production rate of 0.55 m3 m-3 d -1 and COD removal of 76% are obtained under optimal anolyte pH in the present BES. Over high or over low anolyte pH decreases the hydrogen production rate and COD removal. In addition, the experiments show that there is no considerable difference for the power density output and steady state current when the Pt catalyst loading is above 0.1 mg cm-2. But when the Pt catalyst loading is lower than 0.1 mg cm-2, the power density output and current decreases significantly. About 1.7 W m-3 power density output can be obtained by using 0.1 mg cm-2 Pt catalyst in the present research. © 2014, Hydrogen Energy Publications, LLC. Published by Elsevier Ltd. All rights reserved.

关键词： Hydrogen production

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