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Catalytic Gasification of Large Particle Size Biomass with Loaded Aaems Under Oxygen-Steam Atmosphere

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SSRN 2023年

作者： Ren, Jiyun Yang, Kaixuan Li, Yuhang Bai, Yang Jiang, Jiahao Huang, Xiaole Deng, Lei Che, Defu State Key Laboratory of Multiphase Flow in Power Engineering School of Energy and Power Engineering Xi’an Jiaotong University Xi’an710049 China Shanghai Power Equipment Research Institute Co. Ltd. Shanghai200240 China Xi’an Thermal Power Research Institue Co. Ltd. Xi’an710032 China

To evaluate the effect of alkali and alkaline earth metals species (AAEMs) on the catalytic gasification of large particle size biomass, a vertical fixed-bed reactor is conducted for candlenut wood gasification under the oxygen-stream atmosphere. The gasification chars derived from gasification are characterized by SEM, X-ray CT, BET, and FTIR. Tar and syngas are analyzed via GC-MS and GC respectively. Advanced X-ray CT technology provides beneficial visualization to assist in the interpretation of the catalytic gasification of large particle size biomass loaded with AAEMs. The results indicate a progressive augmentation of AAEMs content along the radial direction and end surface for all loaded samples and gasification chars, which could also be visualized from the 3D reconstruction of X-ray CT. Many large pores (40-60 μm) aligned along the grain direction collapse after gasified and generate numerous micropores in gasification chars. 10-20 μm pores are more prominent in chars loaded with KCl and CaCl2. The char loaded with CaCl2 has more well-developed pores, a larger specific surface area, and -OH compounds, aldehydes, ketones and carboxylic acids. The addition of AAEMs facilitates the high generation of M1 compounds (contains 1 benzene ring) in the tar and suppresses the enhancement of other compounds, M4 compounds, and long-chain alkanes. H2 and CO concentrations augments and declines by loading AAEMs. The highest H2 concentration of 62.1% is detected by the addition of CaCl2. When loaded with KCl, the syngas calorific value reduces by 1.37%, while loaded with NaCl, CaCl2, and MgCl2 show an augmentation of 11.48%, 10.56%, and 2.55%, respectively. A decrement of CnHx concentration in syngas derived from samples loaded with KCl and MgCl2 and an increment one loaded with NaCl and CaCl2 are acquired. © 2023, The Authors. All rights reserved.

关键词： Oxygen

Effects of Combustor Wall Temperature on the Outer Recirculation Zone Combustion Modes Transition in Lean Premixed Dme/Air Swirl Flames

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SSRN 2024年

作者： Lin, Wenjun Zhang, Weijie An, Zhenhua Wang, Jinhua Huang, Zuohua Zhang, Huangwei State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xi’an710049 China Department of Mechanical Engineering National University of Singapore 9 Engineering Drive 1 Singapore117576 Singapore Department of Mechanical Engineering and Science Kyoto University Kyoto daigakuKatsura Nishikyo-ku Kyoto615-8540 Japan

In this study, the effects of wall thermal conditions on the ORZ combustion modes transition in the DME/air swirl flames are investigated using the Large Eddy Simulation (LES) and Flamelet Generated Manifold (FGM) method. The results show that the ORZ chemistry and temperature are highly sensitive to the wall thermal condition. Based on the correlation between the temperature and species observed in the time-averaged numerical results, the relation between the combustion mode and temperature in the ORZ is discovered. Through temporal analysis of species and heat release rate in the ORZ, the stable Mode II and Mode IV as well as the unstable Mode III are identified. The chemical reaction pathway analysis for typical probe in the ORZ reveals that different combustion modes undergo distinct (lowtemperature or high-temperature) chemical reaction pathways. Afterwards, the definition of combustion modes used in experiments is refined by utilizing the chemical reaction data from the simulations. And it is applied to identify the combustion mode across the entire computational domain. The results confirm the consistency between the combustion modes determined in experiments based on OH and CH2O and those determined in simulations using chemical reaction rates. Finally, this explains the mechanism of the flickering flame in Mode III is the competition between the low-temperature and high-temperature reaction in the ORZ. Whereas the unstable Mode III can be stabilized by changing the wall temperature to reach the Mode II or Mode IV. © 2024, The Authors. All rights reserved.

关键词： Temperature

Thermal-Hydraulic Characteristics of Helical Cruciform Single Rod Based on Cfd Investigation

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SSRN 2024年

作者： Chen, Yiwen Zhang, Dalin Jiang, Dianqiang Deng, Jian Zhang, Xisi Wang, Xinan Tian, Wenxi Qiu, Suizheng Su, Guanghui State Key Laboratory of Multiphase Flow in Power Engineering Shaanxi Key Laboratory of Advanced Nuclear Energy and Technology School of Nuclear Science and Technology Xi’an Jiaotong University Xi’an710049 China Nuclear Power Institute of China 328 Changshun Avenue Chengdu610213 China Science and Technology on Reactor System Design Technology Laboratory Nuclear Power Institute of China Chengdu610213 China China Institute of Atomic Energy Beijing611731 China

To increase power density in nuclear reactors, the helical cruciform fuel (HCF) is designed as a fundamental element. HCF takes advantages of strong mixing effects, self-supporting features, and strengthened heat transfer, potential to increase the fuel performance in nuclear reactors. In this paper, friction factor and heat transfer coefficient empirical correlations of HCF single rod cooled by water were proposed using a geometric dimensionless number based on numerical simulation. The velocity field, and temperature distribution were obtained to discuss influences of geometric sizes on the fuel performance. Finally, correlations with a geometric dimensionless number were validated with various cases, whose application conditions were also proposed and discussed. This paper provides a guide for study of heat transfer and fluid flow in helical structures, and a reference for establishment of reactor system model using helical cruciform fuels. © 2024, The Authors. All rights reserved.

关键词： Heat transfer coefficients

Numerical study on oxy-fuel co-combustion of semi-coke and coal in utility boiler: Insight into NOx emission and combustion efficiency 7

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Numerical study on oxy-fuel co-combustion of semi-coke and c...

7th International Conference on power engineering, ICOPE 2019

作者： Feng, Qinqin Wang, Chang'an Lv, Qiang Zhao, Lin Du, Yongbo Wang, Pengqian Zhang, Jingwen Che, Defu State Key Laboratory of Multiphase Flow in Power Engineering School of Energy and Power Engineering Xi'an Jiaotong University Xi'an710049 China

Oxy-fuel combustion is clean and efficient combustion technology, which not only benefits the large-scale capture of CO2 but also reduces NOx emission, and then promotes the efficient and clean utilization of carbon-based solid fuels. This study mainly aimed at the oxy-fuel co-combustion of semi-coke and coal in utility boiler with special insight into NOx emission and combustion efficiency. The simulation results showed that when the blending ratio of semi-coke was 45%, the NOx concentration at the furnace outlet under oxy-fuel condition was increased with the oxygen content. The flue gas circulation modes ("dry" versus "wet") had insignificant impact on the NOx emission when the initial oxygen concentration was set as 24% and 27%. When the blending ratio of semi-coke was 70%, the differences of NOx emission between "dry" and "wet" flue gas circulation modes were enlarged with rise in oxygen content under oxy-fuel condition. For oxy-fuel cases, despite of the growth of burnout ratio, the carbon content in fly ash first increased and then decreased with the rise of oxygen content. With the oxygen concentration increased to 30%, lower carbon content in fly ash and higher burnout ratio could be observed in comparison to the cases under air condition. © ICOPE 2019 - 7th International Conference on power engineering, Proceedings. All rights reserved.

关键词： Fly ash

Numerical Simulation for Non-Uniform Ptco Catalyst Degradation Under Constant Voltage Condition and its Impact on Pemfc Performance

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SSRN 2023年

作者： Yang, Yunjie Bai, Minli Zhou, Zhifu Wu, Wei-Tao Hu, Chengzhi Gao, Linsong Li, Yang Li, Yubai Song, Yongchen Key Laboratory of Ocean Energy Utilization and Energy Conservation of Ministry of Education Dalian University of Technology Dalian116023 China State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'An710049 China School of Mechanical Engineering Nanjing University of Science and Technology Nanjing210094 China

PtCo alloys are commonly utilized as catalysts in proton exchange membrane fuel cell (PEMFC) to reduce Pt loading and to achieve higher oxygen reduction reaction (ORR) activity. However, long-time operation can result in a reduction in electrochemical surface area (ECSA) in PEMFC. Meanwhile, the dissolved Co2+ may also contribute to additional local oxygen transport resistance. In this study, catalyst aging model and Co2+ transport and its effect on oxygen transport model have been integrated with the 3D single phase PEMFC performance model to develop a long-term performance model for investigating the impact of non-uniform catalyst degradation and Co2+ contamination on PEMFC performance during constant voltage operation. The results show that Co2+ contamination causes additional mass transfer losses and reduces the peak power of PEMFC. And it is found that the non-uniform degradation of catalyst and Co2+ contamination eventually affects the current density distribution in aged PEMFCs. In addition, the model is also applied to study a 50 cm2 PEMFC under long time constant voltage operation. The predicted ECSA loss is 73.1% and 62.0%, and output power reduction is 55.9% and 43.0% after 80,000 hours at a constant voltage of 0.75 V and 0.65 V, respectively. © 2023, The Authors. All rights reserved.

关键词： Numerical models

A Comprehensive Review on Multi-Dimensional Heat Conduction of Multi-Layer and Composite Structures:Analytical Solutions

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Journal of Thermal Science 2021年第6期30卷 1875-1907页

作者： AMIRI DELOUEI Amin EMAMIAN Amin SAJJADI Hasan ATASHAFROOZ Meysam LI Yueming WANG Lian-Ping JING Dengwei XIE Gongnan Department of Mechanical Engineering University of BojnordBojnordIran Mechanical Engineering Department Shahrood University of TechnologyShahroodIran Department of Mechanical Engineering Siijan University of TechnologySiijanIran School of Aerospace Engineering Xi’an Jiaotong UniversityXi’an 710049China Guangdong Provincial Key Laboratory of Turbulence Research and Applications Center for Complex Flows and Soft Matter Research and Department of Mechanics and Aerospace EngineeringSouthern University of Science and TechnologyShenzhen 518055China Department of Mechanical Engineering University of DelawareNewarkDelaware19711USA International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power EngineeringXi’an Jiaotong UniversityXi’an 710049China Department of Mechanical and Power Engineering Northwestern Polytechnical UniversityXi'an 710072China

Heat conduction in multi-layer and composite materials is one of the fundamental heat transfer problems in many industrial *** to different materials types,interface conditions,and various geometries of these laminates,the heat conduction mechanism is more complicated than that of one-layer isotropic *** solutions are the best ways to study and understand such problems in *** this study,different existing analytical solutions for heat conduction in multi-layer and composite materials are reviewed and classified in rectangular,cylindrical,spherical,and conical *** boundary conditions,internal heat source,and thermal contact resistance as the most critical parameters in the solution complexity investigated in the literature,are discussed and summarized in different *** types of multi-layer structures such as isotropic,anisotropic,orthotropic,and reinforced laminates are included in this *** is found that although more than half a century has passed since the beginning of the research on heat transfer in multi-layer composites,new researches that can help with a better understanding in this area are still being *** challenges and shortcomings in this area are also discussed to guide future researches.

关键词： multi-dimensional heat conduction composite laminates multi-layer structures analytical solutions interface contact resistance

Theoretical and experimental advances on heat transfer and flow characteristics of metal foams

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Science China(Technological Sciences) 2020年第5期63卷 705-718页

作者： WANG Hui GUO LieJin CHEN Kang School of Environmental Science and Engineering Donghua UniversityShanghai 201620China State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong UniversityXi’an 710049China Institute of Solar Engineering Technology Northwest Engineering Corporation LimitedPowerChinaXi’an 710065China

Open cell metal foam can be applied to greatly improve thermal performance of heat sink and heat exchanger,so that it has been widely used in the fields of thermal(or heat)control system of aerospace vehicle and energy utilization system and become a very important topic for research in the aerospace thermophysics field,and more and more attentions have been *** optimal design of metal foam heat transfer devices is based on the understanding the flow and heat transfer characteristics in metal *** article reviews some recent progresses of theoretical and experimental researches on heat transfer enhancement and flow characteristics of metal *** found that the pore cell simplification models of metal foams generally fall into four categories,among which the most commonly used cell model is Kelivin *** exploratory works performed by the current authors are also introduced,such as the effect of boundary conditions on the heat transfer enhancement;the theoretical modelling of interfacial convective heat transfer taking into account heat conduction between foam ligaments;and the flow characteristics under relatively high *** analytical results show that the flow characteristics of metal foam at relatively high speed are completely different from those at low speed,a further thorough study of the heat transfer and flow characteristics of metal foam is necessarily *** this paper,two types of partial filling techniques are *** heat transfer performance of partially filled tubes was evaluated by both the performance evaluation criteria and the performance evaluation plot of enhanced heat transfer techniques oriented for *** results show that the filling type of metal foam have a significant impact on its heat transfer enhancement ***,the filling method of metal foam should be further studied,in order to optimize the thermophysical properties of heat transfer devices.

关键词： metal foam effective thermal conductivity interfacial convective heat transfer coefficient heat transfer enhancement thermal radiation

Laser-Synthesized Ligand-Free Cu Nanocatalysts in Electrochemical CO2 Reduction to Methane

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arXiv

arXiv 2025年

作者： Ye, Taiping Lactionov, Artyom Sozaev, Islam Popov, Anton Klimentov, Sergei Kabashin, Andrei V. Liu, Ya International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Shaanxi 710049 China National Research Nuclear University MEPhI Moscow115409 Russia CNRS LP3 Aix-Marseille Université Marseille13288 France

Electrochemical CO2 reduction (eCO2R) represents a pivotal strategy for mitigating global carbon emissions while simultaneously converting renewable energy into storable chemical fuels. Copper-based catalysts have been extensively explored in this field due to their unique capability to catalyze multi-carbon products. However, the intrinsic complexity of eCO2R pathways on Cu surfaces often leads to mixed product distributions, posing a significant challenge for achieving high selectivity toward a single desired hydrocarbon. Herein, we report a breakthrough in methane selectivity using laser-synthesized, ligand-free Cu nanomaterials. Unlike conventional Cu catalysts that produce diverse products, these ligand-free nanoparticles exhibit unprecedented selectivity for methane (CH4) with a Faradaic efficiency (FE) exceeding 70% at superior overpotentials. The absence of surface ligands, a direct consequence of the ultrafast laser ablation synthesis, ensures abundant exposed active sites with tailored electronic and geometric configurations. We attribute the exceptional methane selectivity to the synergistic effects of active sites-rich surfaces and optimized *CO intermediate binding energetics, which favor the protonation pathway toward CH4 rather than C–C coupling. This work not only resolves the longstanding selectivity dilemma in Cu-catalyzed eCO2R but also establishes laser-synthesized ligand-free nanomaterials as a versatile platform for designing high-performance electrocatalysts. Copyright © 2025, The Authors. All rights reserved.

关键词： Nanoparticles

Study on the Flame Structure and flow Field of Hydrogen-Enriched Combustion in Array Micro-Tube

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SSRN 2024年

作者： Tian, Liang Feng, Wenbin Han, Xiao Liu, Yuzhi Liu, Hongfang Cai, Xiao School of Energy and Environmental Engineering Hebei University of Technology Tianjin300401 China National Key Laboratory of Science and Technology on Aero-Engine Aero thermodynamics Research Institute of Aero-Engine Collaborative Innovation Center for Advanced Aero-Engine Beihang University Beijing100191 China State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi’an710049 China

Addressing climate change and reducing greenhouse gas emissions are critical priorities. Utilizing hydrogen-rich methane or pure hydrogen as fuels within gas turbines, facilitated by array micro-tube premixed combustion technology, is anticipated to markedly accelerate the decarbonization process of the energy sector. In this study, the flame structure of the array micro-tube premixed burner under various fuel compositions was examined using OH-Planar Laser-Induced Fluorescence (OH-PLIF) and Particle Image Velocimetry (PIV) measurement techniques. The effects of the equivalence ratio (φ) and the hydrogen power ratio (HPR) on the characteristics of the flame front, including its curvature, density, volume, and the associated flow field properties, were discussed. As φ and HPR increase, the wrinkled structure of the flame front is significantly enhanced, with a more pronounced effect on smaller scales. This enhancement leads to the separation of the unburned pockets from the main flame. Concurrently, both the flame length and flame area decrease with the augmentation of φ and HPR, indicating a more concentrated combustion process and increased combustion intensity under hydrogen-enriched and pure hydrogen conditions. The study also observed a slight increase in both the negative and positive curvatures of the flame front, with a more notable increase in negative curvature. The increased negative curvature results in an elevated degree of wrinkling and a higher value of Σ (flame surface density), reaching a maximum of 0.876 mm-1 under the conditions where φ is 0.8 and (mean progress variable) is 0.5, resulting in the smallest observed flame volume of 100.6 mm3. Upon coupling the flame with the flow field, it was discovered that the exit flow field of the array micro-tube exhibits symmetry and a characteristic conical flame shape. The burning velocity of the side flame brushes increases, and the velocity peak shifts upstream. The above findings confirms that the additio

关键词： flow fields