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ASME 2023 Heat Transfer Summer Conference, HT 2023

作者： Shuhan, Liu Ji’an, Liu Qingjiang, Liu Xianliang, Lei State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an China

ISBN: (纸本)9780791887165

In the combined system of lead cooled fast reactor (LFR) and supercritical carbon dioxide (S-CO2) Brayton cycle, the intermediate heat exchanger plays a key role in the whole power system. However, the existing heat exchanger can not meet the trend of miniaturization of lead cooled fast reactor. Considering the thermo-physical properties and heat transfer behaviors in both S-CO2 and liquid lead bismuth eutectic (LBE) are significantly different, an asymmetric compact coupled heat exchanger learning from Honeycomb structure is proposed. Through numerical simulation, it is found that the thermal resistance mainly exists in the cold side. In order to enhance the heat transfer at the S-CO2 side, the fin tube is adopted at the cold side. The results show that the heat transfer performance and friction factor of the heat exchanger increase with the increase of fin height, width and number of fins due to the increase of heat transfer area. When the fin height is increased, PEC gradually increases at low inlet velocity, and then decreases at high inlet velocity;When the fin width is increased, PEC increases first and then decreases at low inlet velocity, and decreases gradually at high inlet velocity;With the increase of the number of fins, PEC showed an increasing trend at different inlet velocities. © 2023 by ASME.

关键词： Supercritical fluid extraction

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Progress and challenge of functional single-atom catalysts for the catalytic oxidation of volatile organic compounds

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Chinese Chemical Letters 2024年第9期35卷 83-91页

作者： Zeyu Jiang Yadi Wang Changwei Chen Chi He Department of Environmental Science and Engineering Xi’an Jiaotong UniversityXi’an 710049China State Key Laboratory of Multiphase Flow in Power Engineering School of Energy and Power EngineeringXi’an Jiaotong UniversityXi’an 710049China National Engineering Laboratory for VOCs Pollution Control Material&Technology University of Chinese Academy of SciencesBeijing 101408China

The catalytic oxidation of volatile organic compounds(VOCs)is of considerable significance for the sustainable development of the chemical industry;thus,considerable efforts have been devoted to the exploration of efficient catalysts for use in this *** this regard,the development and utilization of single-atom catalysts(SACs)in VOCs decomposition is a rapidly expanding research *** can be employed as potential catalysts for oxidizing VOC molecules due to their optimal utilization efficiency,unique atomic bonding structures,and unsaturated *** has been achieved,while the challenges surrounding precise regulation of the microstructures of SACs for improving their low-temperature efficiency,stability,and product selectivity under practical conditions are ***,elucidating structure-performance relationships and establishing intrinsic modulating mechanisms are urgently required for guiding researchers on how to synthesize effective and stable functional SACs ***,recent advances in the design and synthesis of functional SACs for application in the catalytic oxidation of VOCs are *** experimental and theoretical studies revealing higher efficiency,stability,and selectivity of as-prepared functional SACs are being ***,the future perspectives in terms of promising catalysts with multi-sized composite active sites and the illustration of intrinsic mechanism are *** rapid intelligent screening of applicable SACs and their industrial applications are also discussed.

关键词： Single-atom catalysts VOCs catalytic oxidation Hydrocarbon activation Oxygen species transformation Surface chemistry Intrinsic mechanism

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NUMERICAL SIMULATION OF FLUID-STRUCTURE COUPLING FOR THE MAIN PUMP OF LEAD COOLED FAST REACTOR 30

NUMERICAL SIMULATION OF FLUID-STRUCTURE COUPLING FOR THE MAI...

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30th International Conference on Nuclear engineering, ICONE 2023

作者： Xiang, Zutao Li, Liangxing Zhao, Jiayuan Xu, Xiangyang State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Xi'an China

ISBN: (纸本)9784888982566

The main pump blades of lead cooled fast reactor have complex mechanical characteristics, and there are complex fluid-structure coupling problems in the structural analysis of the impeller. In this paper, CFX software is mainly used for numerical simulation to carry out one-way fluid-structure coupling research on the moving blade of the main pump. Generally, three kinds of materials as Ti3SiC2, T91 steel and 304 stainless steel are considered for the moving blade of main pump and the deformation distribution and equivalent stress distribution of the three models under the three moving blade materials are analyzed respectively. Finally, the modal analysis of the moving blade of the main pump is carried out. The results show that the resistance to deformation of moving blade made in Ti3SiC2 is better than those of T91 steel and 304 stainless steel;The equivalent stress on the pressure surface of Ti3SiC2 is slightly higher than those of T91 steel and 304 stainless steel, and the maximum equivalent stress on the pressure surface of moving blade occurs on the inner edge of the blade. This research can provide reference for the design of moving blades, and help to improve the service life of the main pump. © 2023 by JSME.

关键词： Numerical models

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Base-or acid-assisted polystyrene plastic degradation in supercritical CO_(2)

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Waste Disposal and Sustainable Energy 2023年第2期5卷 165-175页

作者： Yanbing Liu Jinwen Shi Liuhao Mao Bingru Lu Xing Kang Hui Jin International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power EngineeringXi’an Jiaotong University28 West Xianning RoadXi’an710049ShaanxiChina

Plastic has caused serious"white pollution"to the environment,and the highly inert characteristics of plastic bring a major challenge for *** fluids have unique physical properties and have been widely used in various *** this work,supercritical CO_(2)(Sc-CO_(2))with mild conditions was selected and assisted by NaOH/HCl solution to degrade polystyrene(PS)plastic,and the reaction model was designed using response surface methodology(RSM).It was found that,regardless of the types of assistance solutions,the factors affecting PS degradation efficiencies were reaction temperature,reaction time,and NaOH/HCl *** the temperature of 400℃,time of 120 min,and base/acid concentration of 5%(in weight),0.15 g PS produced 126.88/116.99±5 mL of gases with 74.18/62.78±5 mL of H2,and consumed 81.2/71.5±5 mL of CO_(2).Sc-CO_(2)created a homogeneous environment,which made PS highly dispersed and uniformly heated,thus promoting the degradation of ***,Sc-CO_(2)also reacted with the degradation products to produce new CO and more CH_(4)and C_(2)H_(x)(x=4,6).Adding NaOH/HCl solution not only improved the solubility of PS in Sc-CO_(2),but also provided a base/acid environment that reduced the activation energy of the reaction,and effectively improved the degradation efficiencies of *** short,degrading PS in Sc-CO_(2)is feasible,and better results are obtained with the assistance of base/acid solution,which can provide a reference for the disposal of waste plastics in the future.

关键词： Plastic degradation Polystyrene Supercritical CO_(2) NaOH HCl

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Experimental investigation on the gravity driven discharge of cohesive particles from a silo with two outlets

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Particuology 2024年第6期89卷 11-21页

作者： Li Dai Zhulin Yuan Fengxian Fan Conghui Gu School of Energy and Power Engineering University of Shanghai for Science and TechnologyShanghai 200093China Key Laboratory of Energy Thermal Conversion and Control of Ministry of Education School of Energy and EnvironmentSoutheast UniversityNanjing 210096China Shanghai Key Laboratory of Multiphase Flow and Heat Transfer in Power Engineering University of Shanghai for Science and TechnologyShanghai 200093China School of Energy and Power Jiangsu University of Science and TechnologyZhenjiang 212100China

An experimental study on the gravity driven discharge of cohesive particles from a silo with two outlets was *** discharge behaviors under the conditions that a single outlet was open and two outlets were open were investigated by varying the moisture content of the particles and the filling height of the particles in the *** results show that the discharge rate of the cohesive particles increases gradually at the beginning,then almost keeps constant,and finally drops *** discharge rate in case of two openings is around 1.1–1.6 times that in case of a single *** filling height leads to lower discharge rate in case of a single opening but results in higher discharge rate in case of two ***,the avalanche dynamics in case of a single opening was examined,and the mixing behavior of the cohesive particles was *** is observed that the discharge flow is promoted by the avalanche phenomenon in the silo,generating a general trend that the normalized mass of discharge increases with the filling height at higher moisture *** case of a single opening,the transition from mass flow to funnel flow favors the particle mixing,resulting in an increasing mixing index as the moisture content *** general,a better performance of mixing can be achieved in case of a single opening compared with in case of two *** study provides vital information for fundamental understanding of the gravity driven discharge of cohesive particles from the silo with multiple outlets.

关键词： Cohesive particles Moisture content Discharge rate Avalanche Mixing

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BiOCl Atomic Layers with Electrons Enriched Active Sites Exposed for Efficient Photocatalytic CO_(2)Overall Splitting

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Nano-Micro Letters 2025年第9期17卷 400-415页

作者： Ting Peng Yiqing Wang Chung‑Li Dong Ta Thi Thuy Nga Binglan Wu Yiduo Wang Qingqing Guan Wenjie Zhang Shaohua Shen International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power EngineeringXi’an Jiaotong UniversityXi’an 710049People’s Republic of China Department of Physics Tamkang UniversityNew Taipei City 25137TaiwanPeople’s Republic of China

Given the limited exposure of active sites and the retarded separation of photogenerated charge carriers in those developed photocata-lysts,photocatalyticCO_(2)splitting into value-added chemicals has suffered from the poor activity and remained in great challenge for real ***,hydrothermally synthesized BiOCl with layered structure(BOC-NSs)was exfoliated into thickness reduced nanosheets(BOCNSs-w)and even atomic layers(BOCNSs-i)via ultrasonication in water and isopro-panol,*** comparison with the pristine BOCNSs,the exfoli-ated BiOCl,especially BOCNSs-i with atomically layered structure,exhibits much improved photocatalytic activity forCO_(2)overall splitting to produce CO andO_(2) at a stoichiometric ratio of 2:1,with CO evolution rate reaching 134.8µmolg^(-1)h^(-1) under simulated solar light(1.7 suns).By surpassing the photocatalytic performances of the state-of-the-artBi_(l)O_(m)X_(n)(X:Cl,Br,I)based photocatalysts,the CO evolution rate is further increased by 99 times,reaching 13.3 mmolg^(-1)h^(-1) under concentrated solar irradiation(34 suns).This excellent photocatalytic performance achieved over BOCNSs-i should be benefited from the shortened transfer distance and the increased built-in electric field intensity,which acceler-ates the migration of photogenerated charge carriers to ***,with oxygen vacancies(VO)introduced into the atomic layers,BOCNSs-i is exposed with the electrons enriched Bi active sites that could transfer electrons to activateCO_(2)molecules for highly efficient and selective CO production,by lowering the energy barrier of rate-determining step(RDS),*OH+*CO_(2)-→HCO_(3)-.It is also realized that theH_(2)O vapor supplied during photocatalytic reaction would exchange oxygen atoms withCO_(2),which could alter the reaction path-ways and further reduce the energy barrier of RDS,contributing to the dramatically improved photocatalytic performance forCO_(2)overall splitting to CO andO_(2).

关键词： Photocatalysis CO_(2)overall splitting BiOCl atomic layers Charge separation

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Fabricating PdCe/OMS-2 catalysts with boosted low-temperature activity for toluene deep degradation

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Journal of Rare Earths 2023年第6期41卷 839-849,I0002页

作者： Lin Yue Zhihua Xu Minghua Hu Mingjiao Tian Mudi Ma Bijie Huang Chi He State Key Laboratory of Multiphase Flow in Power Engineering School of Energy and Power EngineeringXi'an Jiaotong UniversityXi'an 710049China State Key Laboratory of Precision Blasting and Hubei Key Laboratory of Industrial Fume and Dust Pollution Control Jianghan UniversityWuhan 430056China National Engineering Laboratory for VOCs Pollution Control Material&Technology University of Chinese Academy of SciencesBeijing 101408China

Porous cryptomelane-type octahedral molecular sieve(OMS-2)with mixed Mn valence and abundant lattice oxygen species has attracted much attention in volatile organic compounds(VOC)catalytic ***,complete conversion of arene over OMS-2 catalysts at relatively low temperature is still a challenge due to its limited crystal structure and inferior ***,a series of PdCe/OMS-2 catalysts with different Pd/Ce molar ratios was fabricated by a facile impregnation method and the physicochemical properties of which were extensively characterized by X-ray diffraction(XRD),scanning electron microscopy(SEM),high-resolution transmission electron microscopy(HR-TEM),B runauer-Emmett-Teller(BET)method,X-ray fluorescence(XRF),X-ray photoelectron spectroscopy(XPS),temperature programmed reduction of H2(H2-TPR),Raman,In situ diffused reflectance infrared Fourier transform spectra(DRIFTS),and density functional theory(DFT)*** show that the total conversion of toluene can be achieved at 207℃ over PdCe2 with apparent activation energy as low as 62.6 kJ/*** strong synergistic effect between Pd and Ce remarkably boosts the catalytic activity of OMS-2,attributed to the abundant Mn^(3+)-O bands and active surface oxygen *** results reveal that oxygen vacancy can be formed over PdCe2 much easily than that of Pd/OMS-2 and Ce/OMS-2 with the oxygen vacancy formation energy of2.42,2.83 and 2.68 eV,*** increasing the Pd content cannot promote the catalytic activity although PdO is a critical active center in toluene *** vacancy attributed to the integrative effect of Pd,Ce and Mn species plays a promine nt role over prepared catalysts in toluene activation *** findings reported in this work showed new insights into the designing of highly efficient OMS-2catalysts for VOC deep oxidation by tuning oxygen vacancy concentration.

关键词： PdCe/OMS-2 Toluene Catalytic oxidation Oxygen vacancy Rare earths

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Boosting photocatalytic hydrogen production via interfacial engineering over a Z-scheme core/shell heterojunction

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Nano Research 2023年第1期16卷 352-359页

作者： Bing Luo Jinghua Li Wei Wang Chaoqian Ai Haihan Zhang Yuxin Zhao Dengwei Jing School of Chemical Engineering and Technology Xi'an Jiaotong UniversityXi'an 710049China International Research Center for Renewable Energy&State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong UniversityXi’an 710049China

Designing high efficacy photocatalysts is a promising way to improve solar fuel production *** this work,we prepared a core/shell composite of loose ZnCr layered double hydroxide nanosheets modified CdS nanorods for efficient visible light driven photocatalytic hydrogen *** highest hydrogen production rate achieved 425.8μmol·h^(−1) without adding any noble metal cocatalyst under the visible light stimulus,which is 22.4 times that of 1 wt.%Pt-modified *** corresponding apparent quantum yield is 13.9%at 420 *** is revealed that the synergistic actions of the interfacial redox shuttle of Cr^(3+)/Cr^(δ+)and the interfacial electric field enable the efficient separation of photoinduced charge carriers between two components via a Z-scheme energy band ***,with the hydrogen evolution contribution of Zn^(2+),a remarkable improvement in photocatalytic performance was achieved in contrast to bare *** work provides an effective methodology to construct highly efficient and economically viable photocatalysts for solar H_(2)production and mechanistic study.

关键词： photocatalysis heterojunction interfacial engineering noble metal free hydrogen production

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Experimental study on prediction model of wet gas pressure drop across single-orifice plate in horizontal pipes in the low gas phase Froude number region

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Chinese Journal of Chemical engineering 2022年第6期35卷 63-72页

作者： Youfang Ma Youfu Ma Junfu Lyu Weiye Liu Shanghai Key Laboratory of Multiphase Flow and Heat Transfer in Power Engineering School of Energy and Power EngineeringUniversity of Shanghai for Science and TechnologyShanghai 200093China Key Laboratory for Thermal Science and Power Engineering of Ministry of Education Department of Energy and Power EngineeringTsinghua UniversityBeijing 100084China

The pressure drop prediction of wet gas across single-orifice plate in horizontal pipes had been solved satisfactorily under an annular-mist flow in the upstream of orifice ***,this pressure drop prediction is still not clearly determined when the upstream is in an intermittent flow or stratified flow,which is corresponding to a region of low FrG(gas phase Froude number)in the flow pattern map of wet *** this study,the wet gas pressure drop across a single-orifice plate was experimentally investigated in the low FrG *** the experiment,the flow pattern transition in the downstream of single-orifice plates,as well as the effects of FrG and FrL(liquid phase Froude number)on UG(gas phase multiplier),were determined and compared when the upstream is in the flow pattern transition and the stratified flow region,*** performances were examined on the available pressure drop *** was found that no model could be capable of jointly predicting the wet gas pressure drop in the low FrG region with an acceptable *** a new method of correlating FrG and FrL simultaneously,new correlations were proposed for the low FrG *** which the modified Chisholm model shows the best prediction accuracies,with the prediction deviations of UG being within 7%and 3%when the upstream is in flow pattern transition and stratified flow region,respectively.

关键词： Gas-liquid flow Two-phase flow Wet gas Orifice plate Pressure drop Model

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Research and development of helium-xenon Brayton cycle technology:A review

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National Science Open 2024年第6期3卷 188-218页

作者： Weixiong Chen Meihui Song Yiran Qian Hongxing Yu Junjie Yan State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong UniversityXi’an 710049China Key Laboratory of Nuclear Reactor System Design Technology Nuclear Power Institute of ChinaChengdu 610200China

Helium-xenon Brayton cycle systems have significant potential as the energy conversion system for small-scale reactors in remote land,deep-sea,and space applications due to a range of advantages,including high cycle efficiency,compact system structures,and chemical *** objective of this review is to provide a comprehensive understanding of the helium-xenon Brayton cycle system based on the projects and ***,the basic information and development history are introduced,and a series of typical designs are ***,the system configurations,cycle parameter analysis and optimization are ***,the key components are classified,such as turbine,compressor,and heat ***,the dynamic processes and control strategies are introduced in different ***,the deficiency and prospect of current research are *** review covers the representative helium-xenon Brayton cycle systems,which could provide a reference for promoting the development of energy conversion systems.

关键词： helium-xenon Brayton cycle cycle analysis heat exchanger dynamic research

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