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Revealing the unexpected promotion effect of EuO_x on Pt/CeO_2 catalysts for catalytic combustion of toluene

Chinese Journal of Catalysis 2019年第4期40卷 543-552,M0003页

作者： Baoming Zhao Yanfei Jian Zeyu Jiang Chi He Xi’an Modern Chemistry Research Institute Xi’an 710065ShaanxiChina State Key Laboratory of Multiphase Flow in Power Engineering School of Energy and Power EngineeringXi'an Jiaotong UniversityXi'an 710049ShaanxiChina Department of Chemistry College of ScienceImam Abdulrahman Bin Faisal UniversityP.O.Box 1982Dammam 31441Saudi Arabia National Engineering Laboratory for VOCs Pollution Control Material & Technology University of Chinese Academy of SciencesBeijing 101408China

Pt/Eu2O3-CeO2 materials with different Eu concentrations were prepared and applied to toluene destruction,and the remarkable promotion impact of EuOx on Pt/CeO2 can be *** characterization results reveal that the presence of EuOx significantly enhances the redox property,lattice O concentration,and Ce3+ ratio of the Pt/CeO2 material,which facilitates the dispersion and activity of Pt active sites and thus accelerates the decomposition process of *** all catalysts,a sample with an Eu content of 2.5 at.%(Pt/EC-2.5)possesses the best catalytic activity with 0.09 vol% of toluene completely destructed at 200 ℃ under a relatively high GHSV of 50000 h^-*** possible reaction pathway and mechanism of toluene combustion over Pt/Eu2O3-CeO2 samples are presented according to in-situ DRIFTS,which confirms that the toluene oxidation process obeys the Mars-van Krevelen mechanism with aldehydes and ketones as primary organic intermediates.

关键词： Pt/Eu2O3-CeO2 material Promotion effect Toluene Catalytic oxidation In-situ DRIFTS Reaction mechanism

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A study of a computational BVP for heat transfer and friction drag in magnetohydrodynamics viscous flow of a nanofluid subject to the curved surface

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Proceedings of the Institution of Mechanical Engineers, Part E: Journal of Process Mechanical engineering 2021年

作者： Khan, M Riaz Saleel, C Ahamed Saeed, Tareq Allehiany, F.M. El-Refaey, Adel M Jing, Dengwei Mahmoud, Emad E LSEC and ICMSEC Academy of Mathematics and Systems Science Chinese Academy of Sciences China School of Mathematical Science University of Chinese Academy of Sciences China Department of Mechanical Engineering College of Engineering King Khalid University Saudi Arabia -Research Group Department of Mathematics Faculty of Science King Abdulaziz University Saudi Arabia Department of Mathematical Sciences College of Applied Sciences Umm Al-Qura University Saudi Arabia Department of Basic and Applied Science College of Engineering and Technology Arab Academy for Science Technology Maritime Transport Smart Village Campus Egypt State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University China Department of Mathematics and Statistics College of Science Taif University Taif Saudi Arabia

The ongoing work investigates the features of Joule heating and convective condition over a magnetohydrodynamic stagnation point flow of (Formula presented.) nanofluid moving across a curved surface. Moreover, mass suction is supposed through the stretching/shrinking surface. The initially developed model of partial differential equations is transformed into the ordinary ones assisted by suitable similarity variables. Subsequently, the ultimate nonlinear model of ordinary differential equations is solved with the help of a built-in function bvp4c package in MATLAB. Several graphical results are plotted to see the influence of various dimensionless parameters over the velocity, temperature, heat transfer, and friction drag. We found that there exists an escalation in temperature with increasing values of curvature, Eckert number, Hartmann number, and Biot number;however, the velocity profile declines with large curvature, ratio parameter, and high concentration of nanoparticles. It is also important to note that the friction drag rises with the mass suction, and reduces with vast curvature, whereas the rate of heat transfer improves with suction and Biot number but lowers with Eckert number and Hartmann number. © IMechE 2021.

关键词： Magnetohydrodynamics

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Experimental Study on Deliquification with Atomizing Nozzle in Gas Well

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IOP Conference Series: Earth and Environmental Science 2020年第1期555卷

作者： Yutang Gao Xiaobai Li Peng Chang Lei Liu State Key Laboratory of Multiphase Flow in Power Engineering Xi'an 710049 Shaanxi P.R. China

Gas is a clean energy resource in comparison with oil and coal. Liquid-loading problem is frequently encountered in the process of gas production. It would directly cause the production of gas wells decreasing, even off production. A number of deliquification techniques have been suggested for solving this kind of problem, but the available techniques are not yet widely applicable. Based on the analysis, the method of deliquification with atomizing nozzle in gas wells was put forward. The test bench was designed for studying the atomization of nozzles and the liquid entrainment of gas flow. The size distribution of atomized droplets was measured by Malvern laser grain size analyzer. The Sauter mean diameters of atomized droplets were analysed under different two-phase flow conditions. The results indicate that the designed nozzles have good atomization performances and show potential application for reducing liquid loading in gas wells.

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Vapor condensation with low air mass fraction inside water seal branch tube under free convection

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Nuclear engineering and Design 2021年 379卷

作者： Bing Tan Xi Wang Y.W. Wu W.X. Tian S.Z. Qiu G.H. Su School of Nuclear Science and Technology State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University 28 Xianning West Road Xi an 710049 China School of Electric Power South China University of Technology Guangzhou 510640 China

The pressure vessel has used a newly designed water seal structure, and the sealed water is from condensation at low hydrogen concentration. To get the condensation capacity of the water seal branch tube under the pressure vessel normal operation, the experimental loop named WASETEL was constructed, which is aimed at studying the heat transfer during the process of air-steam mixture condensation inside the inclined branch tube at the condition of low air mass fraction. The inner tube is diameter 0.134 m with length 0.68 m which is connected with diameter 1.4 m, high 2.5 m pressure vessel. A canon camera was set to record the images and videos of the condensate height through glass tube in communicating vessel liquidometer. The experiment was conducted under the pressure ranged from 0.2 to 0.6 MPa, air mass concentration ranged from 0.49 to 6.42% and wall subcooling ranged from 11 to 40 K. The test showed HTC (heat transfer coefficient) would sharply deteriorate with the small air fraction, compared with pure steam condensation, about 0.49% mass fraction of the air will reduce heat transfer coefficient by 70–80%. When air concentration is relatively small, those widely used relations can not predict the condensation well, therefore, a new heat transfer empirical correlation with air mass fraction, pressure and subcooling is proposed, covered all the experimental data within the error band ±13%.

关键词： Natural condensation New empirical correlation Water seal

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Photocatalytic water oxidation over BiVO_4 with interface energetics engineered by Co and Ni-metallated dicyanamides

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Chinese Journal of Catalysis 2018年第3期39卷 502-509页

作者： Yi Shang Fujun Niu Shaohua Shen International Research Centre for Renewable Energy State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong UniversityXi’an 710049 Shaanxi China

Photocatalytic water oxidation based on semiconductors usually suffers from poor charge transfer from the bulk to the interface,which is necessary for oxygen ***,we construct a hybrid artificial photosynthesis system for photocatalytic water *** system consists of BiVO4as the light harvester,a transitional metal complex(M(dca)2,M=Co,Ni,dca:dicyanamide)as the water oxidation catalyst,and S2O82?as a sacrificial electron *** system exhibits enhanced oxygen evolution activity when M(dca)2is *** BiVO4/Co(dca)2and Bi‐VO4/Ni(dca)2systems exhibit excellent oxygen evolution rates of508.1and297.7μmol/(h·g)compared to the pure BiVO4which shows a photocatalytic oxygen evolution rate of252.2μmol/(h·g)during6h of photocatalytic ***(dca)2is found to be more effective than Ni(dca)2as a water oxidation *** enhanced photocatalytic performance is ascribed to the M(dca)2‐engineered BiVO4/electrolyte interface energetics,and to the M(dca)2‐catalyzed surface water *** two factors lead to a decrease in the energy barrier for hole transfer from the bulk to the surface of BiVO4,which promotes the water oxidation kinetics.

关键词： Metal complex BiVO4 Water oxidation Photocatalysis Interfacial kinetics

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Construction of Pd-M （M = Ni, Ag, Cu） alloy surfaces for catalytic applications

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Nano Research 2018年第2期11卷 780-790页

作者： Xiang Li Xixi Wang Maochang Liu Hongyang Liu Qiang Chen Yadong Yin Mingshang Jin Frontier Institute of Science and Technology (FIST) School of Chemical Engineering and Technology and State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xi’an China Shenyang National Laboratory for Materials Science Institute of Metal Research Chinese Academy of Sciences Shenyang China State Key Laboratory of Chemical Resource Engineering Beijing University of Chemical Technology Beijing China Department of Chemistry University of California Riverside USA

The fabrication of ultrathin alloy shells as heterogeneous catalysts to increase the utilization efficiency and enhance the catalytic activity of metal atoms has been recognized as an effective method for the construction of efficient metal nanocatalysts, particularly noble-metal nanocatalysts. In this study, we demonstrate the successful formation of Pd-M （M = Ni, Ag, Cu） alloy shells with a tunable thickness on preformed nanoscale Pd seeds. The success of this synthesis mainly relies on the combination of the slow reduction of ＂M＂ ions and the subsequent diffusion of M ad-atoms into the surface lattice of Pd seeds. The composition of the Pd-M alloy shell is easily tuned by changing the type and amount of the added precursor, and the shell thickness is manipulated according to the reaction time. More significantl the surface structure of these alloy shells is maintained after the reaction, implying that any desired surface structure of Pd-M alloy shells can be prepared by using the appropriate starting materials. Further catalytic evaluation of the hydrogenation of chloronitrobenzenes shows that these alloy surfaces exhibit significantly improved selectivity compared to the Pd seeds. The Pd-Ni alloy surfaces exhibit much better catalytic selectivity （as high as 〉 99%） than Pd catalysts.

关键词： Pd allo3 catalyst shape control hydrogenation

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Cavitation characteristics of rotary vane pump in aeroengine lubricating oil system and their effects on pump performance

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Hangkong Dongli Xuebao/Journal of Aerospace power 2025年第7期40卷

作者： Wang, Ge Wang, Yijin He, Denghui Yang, Lina Cao, Ming Bai, Bofeng State Key Laboratory of Eco-hydraulic in Northwest Arid Region of China Xi’an University of Technology Xi’an710048 China Department of Power Engineering Institute of Water Resources and Hydro-electric Engineering Xi’an University of Technology Xi’an710048 China State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xi’an710049 China Commercial Aircraft Engine Company Limited Aero Engine Corporation of China Shanghai200241 China Shanghai Center of Research for Commercial Aircraft Engine Engineering Techniques Shanghai200241 China

To meet the demand for high-performance oil pumps in the lubricating oil system of high thrust and high-speed aeroengines, numerical simulation was conducted on a new high-speed rotary vane oil pump. The Mixture multiphase flow model, Singhal full cavitation model, and renormalization group（RNG） k-Ε turbulence model were employed for numerical calculation, and the reliability of the numerical simulation method was verified through experiments. Then, cavitation characteristics of the rotary vane pump and its impact on pump performance under different inlet pressure and oil temperature conditions were analyzed. The results showed that the cavitation gas was mainly distributed in the volume chamber on the oil suction side, as well as on the suction surface of the rotary vane and near the inner wall of the rotor. With the decrease of inlet pressure and the increase of oil temperature, the cavitation phenomenon inside the rotary vane pump intensified, and the cavitation gas increased, which in turn led to a decrease in the average oil discharge flow rate at the pump outlet and a decrease in volumetric efficiency. When the inlet pressure dropped to 40 kPa and the temperature rose to 373.15 K, the average oil discharge flow rate and volumetric efficiency at the pump outlet both significantly decreased. The pressure pulsation at the monitoring point exhibited low-frequency and high-amplitude pulsation characteristics. The cavitation of the rotary vane pump affected not only its oil discharge and volumetric efficiency, but also the stable and reliable operation of the pump. © 2025 Beijing University of Aeronautics and Astronautics (BUAA). All rights reserved.

关键词： Vane pumps

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Synthesis of AgI/Bi2MoO6 nano-heterostructure with enhanced visible-light photocatalytic property

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Progress in Natural Science:Materials International 2018年第2期28卷 235-241页

作者： Li Zhang Hongcheng Teng Jiancheng Zhou Yueming Sun Naixu Li Maochang Liu Dengwei Jing School of Chemistry and Chemical Engineering Southeast University Department of Chemical and Pharmaceutical Engineering Southeast University Chengxian College Jiangsu Province Hi-Tech Key Laboratory for Bio-medical Research Southeast University International Research Center for Renewable Energy & State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Suzhou Academy of Xi'an Jiaotong University

A novel nano-heterostructure of Ag I/Bi2MoO6photocatalyst was successfully synthesized via a facile depositionprecipitation method. The samples were systematically characterized by X-ray diffraction, scanning and transmission electron microscopy, X-ray photoemission spectroscopy, UV–Vis absorption spectroscopy, and photoluminescence spectra. While sole Bi2MoO6or Ag I showed poor activity toward photocatalytic rhodamine B degradation, the nano-heterostructure was found with superior performance. The AgI/Bi2MoO6composite with an optimal content of 20 wt% Ag I exhibited the highest photocatalytic degradation rate. Rhodamine B was totally degraded within 75 min visible-light irradiation. Moreover, the hybrid photocatalyst also showed a fairly good stability for several-cycle reuse. This study indicates that the AgI/Bi2MoO6nano-heterostructure can be used as an effective candidate for photocatalytic degradation of organic pollutants.

关键词： Heterostructure Photocatalyst RhB-degradation

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Radiation Effects of 500 MeV Kr+ ions on NiO/β-Ga2O3 heterojunction diodes

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IEEE Transactions on Nuclear Science 2025年

作者： Zhao, Penghui Chen, Hao Zhou, Leidang Ma, Teng Chen, Liang Yang, Tao Lei, Zhifeng Lu, Xing Zhou, Genshu Guo, Hui Ouyang, Xiaoping School of Materials Science and Engineering Xi’an Jiaotong University Xi’an710049 China Xi’an Jiaotong University School of Microelectronics Xi’an710049 China State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xi’an710049 China Xi’an Engineering Research Center of Advanced3D Vision Shaanxi Xi’an710000 China China Electronic Product Reliability and Environmental Testing Research Institute Science and Technology on Reliability Physics and Application of Electronic Component Laboratory Guangzhou510610 China Northwest Institute of Nuclear Technology Radiation Detection Research Center Xi’an710024 China Xi’an Jiaotong University School of Instrument Science and Technology Xi’an710049 China Sun Yat-sen University State Key Laboratory of Optoelectronic Materials and Technologies School of Electronics and Information Technology Guangzhou510275 China Xidian University School of Microelectronics Shaanxi Xi’an710016 China

This study investigates the in-situ radiation effects on NiO/β-Ga2O3 heterojunction diodes (HJDs) under 500 MeV Kr+ ions irradiation, with a fluence of 1×108 cm-2 at -200 V. The statistical results show that both the forward conductive and reverse blocking characteristics of the HJDs were degraded after the irradiation of Kr+ ions. Associated with the analysis of current-voltage characteristics and the SRIM simulation results, the performance degradations were attributed to the vacancies induced by Kr+ ions radiation in the β-Ga2O3 material. On the one hand, the Kr+ radiation-induced vacancies reduced the net carrier concentration of the β-Ga2O3 and increased the generation-recombination current, leading to increased specific on-resistance and ideality factor of the irradiated HJDs. On the other hand, an oxygen di-vacancies-related trap, set at 1.07±0.01 eV below the conduction band, was involved after Kr+ ions radiation, which enhanced the Poole-Frenkel emission process, dominating the higher leakage current of the irradiated HJDs beyond -300 V. These results provide valuable insights into the radiation damage and performance degradation mechanisms in β-Ga2O3-based devices for space applications. © 1963-2012 IEEE.

关键词： Radiation damage

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An efficient cellular flow model for cohesive particle flocculation in turbulence

arXiv

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arXiv 2020年

作者： Zhao, K. Vowinckel, Bernhard Hsu, T.-J. Köllner, T. Bai, B. Meiburg, E. Department of Mechanical Engineering UC Santa Barbara CA93106 United States State Key Laboratory of Multiphase Flow in Power Engineering Xi’an Jiaotong University Xi’an710049 China Leichtweiß-Institut für Wasserbau Technische Universität Braunschweig Braunschweig38106 Germany Center for Applied Coastal Research Department of Civil & Environmental Engineering University of Delaware NewarkDE19716 United States

We propose a one-way coupled model that tracks individual primary particles in a conceptually simple cellular flow setup to predict flocculation in turbulence. This computationally efficient model accounts for Stokes drag, lubrication, cohesive and direct contact forces on the primary spherical particles, and allows for a systematic simulation campaign that yields the transient mean floc size as a function of the governing dimensionless parameters. The simulations reproduce the growth of the cohesive flocs with time, and the emergence of a log-normal equilibrium distribution governed by the balance of aggregation and breakage. Flocculation proceeds most rapidly when the Stokes number of the primary particles is O(1). Results from this simple computational model are consistent with experimental observations, thus allowing us to propose a new analytical flocculation model that yields improved agreement with experimental data, especially during the transient stages. Copyright © 2020, The Authors. All rights reserved.

关键词： Turbulence

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