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中华核医学与分子影像杂志 2025年第2期45卷 125-128页

作者：赵舒文张景展康晓静新疆医科大学研究生学院乌鲁木齐830001 新疆维吾尔自治区人民医院皮肤性病医学诊疗中心、新疆皮肤性病临床医学研究中心、新疆皮肤病研究重点实验室乌鲁木齐830001

皮肤恶性肿瘤多发生在光暴露部位。早期诊断并治疗可有效提高患者的生存率。组织病理学检查是临床诊断皮肤恶性肿瘤的"金标准",但该检查是一种侵入性操作,耗时较长且可能出现切口感染、瘢痕形成等风险。近年来,光谱学技术迅... 详细信息

皮肤恶性肿瘤多发生在光暴露部位。早期诊断并治疗可有效提高患者的生存率。组织病理学检查是临床诊断皮肤恶性肿瘤的"金标准",但该检查是一种侵入性操作,耗时较长且可能出现切口感染、瘢痕形成等风险。近年来,光谱学技术迅速发展,光谱学检测具有非侵入、操作简便、实时检测、高灵敏度等特点,已逐渐应用于皮肤恶性肿瘤的辅助诊断中。该文综述荧光光谱、拉曼光谱、红外光谱等光谱学技术在皮肤恶性肿瘤诊断中的最新研究进展。

关键词：皮肤肿瘤光谱法,荧光光谱分析,拉曼谱学,近红外线发展趋势

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A Hydrazine-Water Galvanic Cell-Inspired Self-Powered High-Rate Hydrogen Production via Overall Hydrazine Electrosplitting

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ADVANCED FUNCTIONAL MATERIALS 2025年第19期35卷

作者： Zhang, Linjie Li, Man Sun, Chen Wang, Hsiao-Tsu Xiao, Yi Ma, Ke Cai, Yimeng Lee, Cheng-You Shao, Yu-Cheng Wang, Chia-Hsin zhao, shuwen Ishii, Hirofumi Hiraoka, Nozomu Wang, Xiuyun Pao, Chih-Wen Han, Lili Chinese Acad Sci Fujian Inst Res Struct Matter State Key Lab Struct Chem Fuzhou 350002 Peoples R China Univ Chinese Acad Sci Sch Chem Sci Beijing 101408 Peoples R China Tamkang Univ Dept Phys New Taipei City 251301 Taiwan Natl Synchrotron Radiat Res Ctr Hsinchu 30076 Taiwan Fuzhou Univ Natl Engn Res Ctr Chem Fertilizer Catalyst Fuzhou 350002 Peoples R China

Exploring advanced electrolysis techniques for attaining scene-adaptive and on-site green H2 production is an imperative matter of utmost practical significance but grand challenge remains. Herein, drawn inspiration from a spontaneous hydrazine-H2O galvanic cell configured on a low-valence Ru single atoms-loaded Mo2C electrode (RuSA/v-Mo2C), an alternative H2 energy solution utilizing self-powered electrochemical hydrazine splitting (N2H4 -> 2H2 + N2) instead of the stereotyped electricity-consumed water splitting for green H2 production is proposed. This solution highlights a pH-decoupled hydrazine-H2O primary battery with notable open-circuit voltage of 1.37 V and energy density up to 358 Wh gN2H4-1, which powerfully propels an alkaline hydrazine splitting cell, leading to bilateral H2 harvest with a remarkable rate of 18 mol h-1 m-2, i.e., 403.2 L h-1 m-2, setting a new record for the self-sustaining electricity-powered H2 production systems. The success of RuSA/v-Mo2C for this solution is further decoded by tandem theoretical and in situ spectroscopic studies, cross-verifying a Ru-Mo dual-site synergy in streamlining the overall energy barriers, thereby enhancing the kinetics of electrode reactions. This pioneering work, showcasing electrochemical H2 production free from both external energy and feedstock inputs, opens up a new horizon on way of the ultimate H2 energy solution.

关键词： electrocatalysis energy conversion hydrogen evolution hydrazine oxidation self-powered

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A Multi-Regional Coordinated Peer-to-Peer Energy Trading Market Mechanism in Distribution Networks

A Multi-Regional Coordinated Peer-to-Peer Energy Trading Mar...

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2021 IEEE Sustainable Power and Energy Conference, iSPEC 2021

作者： zhao, shuwen Wu, Zhi Wang, Jianhua Zheng, Shu zhao, Jingtao Wu, Yuanxi Southeast University School of Electrical Engineering Nanjing China Nari Technology Development Co. Ltd Nanjing China

ISBN: (纸本)9781665414395

Regional distribution network operation can be conducive for privacy protection, efficient calculation, grid modularity, and network scalability, which awfully tally with decentralized energy trade mechanism - peer-to-peer (P2P) market. This article proposes a multi-regional coordinated P2P energy trading market mechanism to achieve consensus by exchanging coupled information. At the regional grid level, lower level distribution systems operators (DSOs) coordinate the P2P market and ancillary service to attain market clear according to the coupled information shared by adjacent regions, such as the distribution locational marginal prices (DLMPs) and voltage of regional slack bus. In distribution grid levels, each region achieves consensus upon power flow by alternating direction method of multipliers (ADMM). The distribution grid model is established by Distflow-based linearized model and sensitivity factors to eliminate the higher nonlinearities in power flow. Finally, the case studies demonstrate the economic efficiency of the proposed multiregional market mechanism. © 2021 IEEE.

关键词： Electric load flow

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Interfacial electronic engineering of heterostructured Co2P-MoNiP/NF nano-sea-urchin catalysts for efficient and stable hydrogen evolution via water/seawater splitting

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CHEMICAL ENGINEERING JOURNAL 2023年 477卷

作者： zhao, Yifan Zhang, Hua Chen, Ji zhao, shuwen Xi, Min Yang, Lingfeng Long, Youyu Ni, Zitao Zhou, Yao Chen, Anran Yunnan Univ Sch Mat & Energy Kunming 650091 Peoples R China Yunnan Univ Electron Microscopy Ctr Kunming 650091 Yunnan Peoples R China Jiangnan Univ Sch Internet Things Engn Wuxi 214122 Peoples R China Univ Edinburgh Sch Engn South Bridge Edinburgh EH8 9YL Scotland

Using hydrogen as a fuel is an effective way to combat the energy crisis, at the same time, reduce greenhouse gas emissions. Designing high-performance and low-cost catalysts for the hydrogen evolution reaction (HER) is critical for commercial seawater electrolysis. Here, we designed a heterostructured Co2P-MoNiP/NF nano-sea-urchin catalyst that only showed an overpotential of 46 mV for 10 mA cm-2 to actuate HER in alkaline elec-trolytes along with superior stability. Theoretical calculations demonstrate that the constructed heterogeneous interfaces effectively promote the redistribution of the charge density and optimize the adsorbed hydrogen in-termediates, lowering the hydrogen adsorption free energy barrier and promoting H2 desorption, thus boosting the HER activity. Moreover, the assembled two-electrode electrolyzer only required ultra-low voltages of 1.51 and 1.66 V to deliver current densities of 10 and 100 mA cm-2, respectively. The solar-driven water electrolysis system achieves a high and stable solar-to-hydrogen (STH) conversion efficiency of 19.68 %.

关键词： Heterostructure Nano-sea-urchin Hydrogen evolution reaction Solar-to-hydrogen Seawater splitting

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Datasets for the CMIP6 Scenario Model Intercomparison Project (ScenarioMIP) Simulations with the Coupled Model CAS FGOALS-f3-L

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Advances in Atmospheric Sciences 2021年第2期38卷 329-339页

作者： shuwen zhao Yongqiang YU Pengfei LIN Hailong LIU Bian HE Qing BAO Yuyang GUO Lijuan HUA Kangjun CHEN Xiaowei WANG State Key Laboratory of Numerical Modeling for Atmospheric Sciences and Geophysical Fluid Dynamics(LASG) Institute of Atmospheric PhysicsChinese Academy of SciencesBeijing 100029China University of Chinese Academy of Sciences Beijing 100049China Center for ocean Mega-Science Chinese Academy of SciencesQingdao 266071China Chinese Academy of Meteorological Sciences Beijing 100081China Yunnan University Kunming 650091China

The datasets for the tier-1 Scenario Model Intercomparison Project(ScenarioMIP)experiments from the Chinese Academy of Sciences(CAS)Flexible Global Ocean-Atmosphere-Land System model,finite-volume version 3(CAS FGOALS-f3-L)are described in this *** is one of the core MIP experiments in phase 6 of the Coupled Model Intercomparison Project(CMIP6).Considering future CO2,CH4,N2O and other gases’concentrations,as well as land use,the design of ScenarioMIP involves eight pathways,including two tiers(tier-1 and tier-2)of ***-1 includes four combined Shared Socioeconomic Pathways(SSPs)with radiative forcing,i.e.,SSP1-2.6,SSP2-4.5,SSP3-7.0 and SSP5-8.5,in which the globally averaged radiative forcing at the top of the atmosphere around the year 2100 is approximately 2.6,4.5,7.0 and 8.5 W m−2,*** study provides an introduction to the ScenarioMIP datasets of this model,such as their storage location,sizes,variables,*** analysis indicates that surface air temperatures will increase by about 1.89℃,3.07℃,4.06℃ and 5.17℃ by around 2100 under these four scenarios,***,some other key climate variables,such as sea-ice extension,precipitation,heat content,and sea level rise,also show significant long-term trends associated with the radiative forcing *** datasets will help us understand how the climate will change under different anthropogenic and radiative forcings.

关键词： CMIP6 ScenarioMIP FGOALS-f3-L coupled model data description

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数字经济时代黑龙江省区域经济与物流业时空耦合演变研究

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物流技术 2023年第5期42卷 54-58页

作者：王莎赵淑雯齐齐哈尔大学经济与管理学院黑龙江齐齐哈尔161006

利用地理联系率、地理集中度、地理耦合度,选取黑龙江省2011-2019年的数据,从时间、空间两个角度分析在数字经济蓬勃发展的背景下,区域经济与物流产业之间的关联性和耦合关系。结果表明,二者在空间上具有中上水平的耦合关联特征,耦合关... 详细信息

利用地理联系率、地理集中度、地理耦合度,选取黑龙江省2011-2019年的数据,从时间、空间两个角度分析在数字经济蓬勃发展的背景下,区域经济与物流产业之间的关联性和耦合关系。结果表明,二者在空间上具有中上水平的耦合关联特征,耦合关联程度整体在波动中呈现上升的趋势,二者在地区上的差异性、不均衡性相似。在此基础上,提出黑龙江省应优化区域空间发展格局,推进数字经济下物流服务供应链创新,深化物流与区域经济的耦合协调高质量发展,使区域经济整体提质增效。

关键词：数字经济区域经济物流业时空演变高质量发展黑龙江

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Mo-doped NiCoP nanowire array grown in situ on Ni foam as a high-performance bifunctional electrocatalyst for overall water splitting

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JOURNAL OF ALLOYS AND COMPOUNDS 2022年 918卷

作者： zhao, Yifan Chen, Ji zhao, shuwen Zhou, Weijie Dai, Ruijie zhao, Xuan Chen, Zhengang Sun, Tao Zhang, Hua Chen, Anran Yunnan Univ Sch Mat & Energy Kunming 650091 Peoples R China

The development and application of durable and efficient non-precious metal-based electrocatalysts are particularly crucial for hydrogen production using overall water-splitting technology. Herein, a simple method was employed to synthesize Mo-doped NiCoP nanowires on a metallic 3D Ni foam (Mo-NiCoP/NF) for hydrogen evolution reaction (HER) and oxygen evolution reaction (OER). This long-term stable MoNiCoP/NF catalyst demonstrated comparatively low overpotentials and excellent dual-functional catalytic performances. The overpotentials for the HER and OER were 64 and 262 mV, respectively, to actuate a current density of 10 mA cm-2 in an alkaline environment (1 M KOH). Meanwhile, when this electrocatalyst was utilized for overall water splitting, a cell voltage of 1.56 V could supply a current density of 10 mA cm-2 for at least 50 h with a negligible performance drop. This work provides an advanced approach to developing non-noble metal phosphide nanostructures as monolithic dual-functional electrocatalysts for overall alkaline water splitting. (c) 2022 Elsevier B.V. All rights reserved.

关键词： Mo-NiCoP Electrocatalyst Hydrogen evolution Oxygen evolution Overall water splitting

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Polyvinyl Chloride Microplastics Disseminate Antibiotic Resistance Genes in Chinese Soil: A Metagenomic Analysis

SSRN

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SSRN 2024年

作者： zhao, shuwen Zhang, Qianru Huang, Qilan Zhang, Chuchen Li, Hongna Siddique, Kadambot H.M. State Key Laboratory of Efficient Utilization of Arid and Semi-arid Arable Land in Northern China Institute of Agricultural Resources and Regional Planning Chinese Academy of Agricultural Sciences Beijing100081 China Institute of Environment and Sustainable Development in Agriculture Chinese Academy of Agricultural Sciences Beijing100081 China The UWA Institute of Agriculture The University of Western Australia PerthWA6001 Australia

The widespread prevalence of microplastics (MPs) in the environment poses concerns as they are vectors of antibiotic resistance genes (ARGs). The relationships between antibiotic resistomes and MPs remain unexplored in soil which was considered as the reservoirs of MPs and ARGs. This study investigated the effects of polyvinyl chloride (PVC) MPs on soil bacterial communities and ARG abundance which soil samples sourced from 20 provinces across China. We found that PVC significantly influences soil bacterial community structure and ARG abundance. Structural equation modeling revealed that PVC alters soil characteristics, ultimately affecting soil bacterial communities, including ARG-containing bacterial hosts, and the relative abundance of ARGs. This study enhances our understanding of how MPs influence the proliferation and hosts of ARGs within diverse soil environments, offering crucial insights for future strategies in plastic management and disposal. © 2024, The Authors. All rights reserved.

关键词： Polyvinyl chlorides

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Crystalline and amorphous phases: NiFeCo tri-metal phosphide as an efficient electrocatalyst to accelerate oxygen evolution reaction kinetics

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ELECTROCHIMICA ACTA 2022年 426卷

作者： zhao, shuwen zhao, Yifan Chen, Ji Dai, Ruijie Zhou, Weijie Yang, Jinpeng zhao, Xuan Chen, Zhengang Zhou, Yao Zhang, Hua Chen, Anran Yunnan Univ Sch Mat & Energy Kunming 650091 Peoples R China Univ Edinburgh Sch Engn Edinburgh EH8 9YL Scotland

To solve the problem of low hydrogen production efficiency from water electrolysis, increasing research is focusing on improving the efficiency of the complex oxygen evolution reaction (OER) that occurs at the anode. The preparation of high-efficiency OER electrocatalysts is key to improving the OER efficiency and the only way forward. In this work, a NiFeCo ternary OER high-efficiency electrocatalyst, NiFeCoP@CAP/NF, comprising coexisting crystalline and amorphous phases (CAP), was prepared on nickel foam (NF) by a simple one-step hydrothermal reaction and high-temperature gas-phase phosphating. The as-synthesized catalyst exhibits an ultralow overpotential of 202 mV (10 mA cm-2) in 1 M KOH solution with a Tafel slope (eta 10 = 202 mV) of 28.9 mV dec- 1. Further, it is understood that owing to the combination of the crystalline and amorphous phases, the catalyst can rapidly transform the amorphous phase into the true active (NiOOH) phase of the OER process while retaining the fast charge transport properties of the crystalline phase, as observed by in situ Raman analysis.

关键词： Oxygen evolution reaction Crystalline and amorphous phases NiFeCoP@CAP NF In situ Raman

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深水FPSO应急集合站结构抗爆炸设计分析

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工程机械 2025年第4期56卷 131-137,I0006,I0007页

作者：李娜赵淑文任晓芳中国海洋石油国际有限公司北京市100010 海洋石油工程股份有限公司

为了确保作业人员在火灾、爆炸事故时的避难、逃生安全,深水浮式生产储油卸油装置(FPSO)在船尾布置应急集合站。应用DNV PHAST软件分析了火炬燃烧热辐射,火炬塔和应急集合站的布置满足热辐射强度的衡准要求。基于FLUENT软件和DNV PHAST... 详细信息

为了确保作业人员在火灾、爆炸事故时的避难、逃生安全,深水浮式生产储油卸油装置(FPSO)在船尾布置应急集合站。应用DNV PHAST软件分析了火炬燃烧热辐射,火炬塔和应急集合站的布置满足热辐射强度的衡准要求。基于FLUENT软件和DNV PHAST软件,建立了上部模块油气处理系统泄漏天然气爆燃事故后果预测与分析模型,对油气爆燃进行模拟和风险定量分析。为确定应急集合站处的油气燃爆控制方案,开展了敏感性分析,研究在工艺处理上部模块后方加装防爆墙对FPSO船尾设施抗爆炸设计的影响。基于石油公司企业标准的要求,确定了应急集合站处结构设计爆炸压强,对应急集合站结构进行了抗爆炸工况线性和非线性分析,计算了结构强度和塑性应变,分析结果满足BV、DNV船级社规范和企业标准要求。

关键词：浮式生产储油卸油装置应急集合站抗爆炸线性分析非线性分析塑性应变

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