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What have we known so far for fluorescence staining and quantification of microplastics:A tutorial review

Frontiers of Environmental science & Engineering 2022年第1期16卷 37-50页

作者： Shengdong Liu Enxiang Shang Jingnan Liu Yining Wang Nanthi Bolan MBKirkham Yang Li Key Laboratory of Water and Sediment Sciences of Ministry of Education State Key Laboratory of Water Environment SimulationSchool of EnvironmentBeijing Normal UniversityBeijing 100875China College of Science and Technology Hebei Agricultural UniversityHuanghua 061100China School of Agriculture and Environment The University of Western AustraliaPerthWA 6001Australia The UWA Institute of Agriculture The University of Western AustraliaPerthWA 6001Australia Global Innovative Centre for Advanced Nanomaterials College of EngineeringScience and EnvironmentUniversity of NewcastleCallaghanNSW 2308Australia Department of Agronomy Throckmorton Plant Sciences CenterKansas State UniversityManhattanKS 66506USA

Understanding the fate and toxicity of microplastics(MPs,<5 mm plastic particles)is limited by quantification *** paper summarizes the methods in use and presents new ***,sampling and pretreatment processes ofMPs,including sample collection,digestion,density separation,and quality control are *** the promising and convenient staining procedures and quantification methods for MPs using fluorescence dyes are *** factors that influence the staining of MPs,including their physicochemical properties,are summarized to provide an optimal operation *** general,the digestion step is crucial to eliminate natural organic matter(NOM)to avoid interference in *** was reported to be the most appropriate solvent,and 10–20μg/mL are recommended as optimal dye *** addition,a heating and cooling procedure is recommended to maintain the fluorescence intensity of MPs for two *** staining,a fluorescence microscope is usually used to characterize the morphology,mass,or number of MPs,but compositional analysis cannot be determined with *** fluorescence staining methods have been implemented to study MP abundance,transport,and toxicity and have been combined with other chemical characterization techniques,such as Fourier transform infrared spectroscopy and Raman *** studies are needed to focus on the synthesis of novel dyes to avoid NOM’s *** need to be combined with other spectroscopic techniques to characterize plastic composition and to develop image-analysis *** stability of stained MPs needs to be improved.

关键词： Plastic particles Fluorescence dyes Identification Concentration quantification

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Layer Hall Detection of the Néel Vector in Centrosymmetric Magnetoelectric Antiferromagnets

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Physical Review Letters 2024年第9期133卷 096803页

作者： L. L. Tao Qin Zhang Huinan Li Hong Jian Zhao Xianjie Wang Bo Song Evgeny Y. Tsymbal Laurent Bellaiche School of Physics Key Laboratory of Material Simulation Methods and Software of Ministry of Education College of Physics International Center of Future Science National Key Laboratory of Science and Technology on Advanced Composites in Special Environments Department of Physics and Astronomy & Nebraska Center for Materials and Nanoscience Smart Ferroic Materials Center Physics Department and Institute for Nanoscience and Engineering Department of Materials Science and Engineering Tel Aviv University Ramat Aviv Tel Aviv 6997801 Israel

The efficient detection of the Néel vector in antiferromagnets is one of the prerequisites toward antiferromagnetic spintronic devices and remains a challenging problem. Here, we propose that the layer Hall effect can be used to efficiently detect the Néel vector in centrosymmetric magnetoelectric antiferromagnets. Thanks to the robust surface magnetization of magnetoelectric antiferromagnets, the combination of sizable exchange field and an applied electric field results in the layer-locked spin-polarized band edges. Moreover, the Berry curvature can be engineered efficiently by an electric field, which consequently gives rise to the layer-locked Berry curvature responsible for the layer Hall effect. Importantly, it is demonstrated that the layer Hall conductivity strongly depends on the Néel vector orientation and exhibits rich electromagnetic responses, which can be used to detect the Néel vector reversal. Based on density functional theory calculations, we exemplify those phenomena in the prototypical Cr2O3 compound. A complete list of the magnetic point groups sustaining the layer Hall effect is presented, aiding the search for realistic materials. Our work proposes a novel approach to detect the Néel vector and holds great promise for antiferromagnetic spintronic applications.

关键词： Anomalous Hall effect Magnetoelectric effect Transport phenomena Antiferromagnets Multiferroics First-principles calculations k dot p method

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Applications of MXenes in human-like sensors and actuators

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Nano Research 2023年第4期16卷 5767-5795页

作者： Jinbo Pang Songang Peng Chongyang Hou Xiao Wang Ting Wang Yu Cao Weijia Zhou Ding Sun Kai Wang Mark H.Rümmeli Gianaurelio Cuniberti Hong Liu Institute for Advanced Interdisciplinary Research(iAIR) Collaborative Innovation Center of Technology and Equipment for Biological Diagnosis and Therapy in Universities of ShandongUniversity of JinanJinan 250022China Institute for Materials Science and Max Bergmann Center of Biomaterials Technische Universität DresdenDresden 01069Germany Center for Advancing Electronics Dresden Technische Universität DresdenDresden 01069Germany Dresden Center for Computational Materials Science Technische Universität DresdenDresden 01062Germany Dresden Center for Intelligent Materials(GCL DCIM) Technische Universität DresdenDresden 01062Germany High-Frequency High-Voltage Device and Integrated Circuits R&D Center Institute of MicroelectronicsChinese Academy of SciencesBeijing 100029China Key Laboratory of Microelectronic Devices&Integrated Technology Institute of MicroelectronicsChinese Academy of SciencesBeijing 100029China Shenzhen Key Laboratory of Nanobiomechanics Shenzhen Institute of Advanced TechnologyChinese Academy of SciencesShenzhen 518055China State Key Laboratory of Biobased Material and Green Papermaking Qilu University of TechnologyShandong Academy of SciencesJinan 250353China School of Bioengineering Qilu University of TechnologyShandong Academy of ScienceJinan 250353China Key Laboratory of Modern Power System Simulation and Control&Renewable Energy Technology(Ministry of Education) Northeast Electric Power UniversityJilin 132012China School of Electrical Engineering Northeast Electric Power UniversityJilin 132012China School of Electrical Engineering Weihai Innovation Research InstituteQingdao UniversityQingdao 266000China School of Electrical and Computer Engineering Jilin Jianzhu UniversityChangchun 130118China Institute for Complex Materials Leibniz Institute for Solid State and Materials Research Dresden(IFW Dresden)20 Helmholtz StrasseDresden 01069Germany College of Energy Soochow Institute for Energy and Materials Innovations Soochow UniversitySuzhou 215006China Key L

Human beings perceive the world through the senses of sight,hearing,smell,taste,touch,space,and *** first five senses are prerequisites for people to *** sensing organs upload information to the nervous systems,including the brain,for interpreting the surrounding ***,the brain sends commands to muscles reflexively to react to stimuli,including light,gas,chemicals,sound,and ***,as an emerging two-dimensional material,has been intensively adopted in the applications of various sensors and *** this review,we update the sensors to mimic five primary senses and actuators for stimulating muscles,which employ MXene-based film,membrane,and composite with other functional ***,a brief introduction is delivered for the structure,properties,and synthesis methods of ***,we feed the readers the recent reports on the MXene-derived image sensors as artificial retinas,gas sensors,chemical biosensors,acoustic devices,and tactile sensors for electronic ***,the actuators of MXene-based composite are ***,future opportunities are given to MXene research based on the requirements of artificial intelligence and humanoid robot,which may induce prospects in accompanying healthcare and biomedical engineering applications.

关键词： MXenes sensors actuators gas sensors biosensors tactile sensors sound sensors artificial retina

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The impact of the atmospheric turbulence-development tendency on new particle formation: a common finding on three continents

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National science Review 2021年第3期8卷 140-150页

作者： Hao Wu Zhanqing Li Hanqing Li Kun Luo Yuying Wang Peng Yan Fei Hu Fang Zhang Yele Sun Dongjie Shang Chunsheng Liang Dongmei Zhang Jing Wei Tong Wu Xiaoai Jin Xinxin Fan Maureen Cribb Marc L.Fischer Markku Kulmala Tuukka Pet?j? State Key Laboratory of Remote Sensing Science College of Global Change and Earth System ScienceBeijing Normal University ESSIC and Department of Atmospheric Science University of MarylandCollege Park State Key Laboratory of Clean Energy Utilization Zhejiang University School of Atmospheric Physics Nanjing University of Information Science and Technology Meteorological Observation Center China Meteorological Administration State Key Laboratory of Atmospheric Boundary Layer Physics and Atmospheric Chemistry Institute of Atmospheric Physics Chinese Academy of Sciences State Key Joint Laboratory of Environmental Simulation and Pollution Control College of Environmental Sciences and Engineering Peking University State Key Joint Laboratory of Environment Simulation and Pollution Control School of Environment Tsinghua University Lawrence Berkeley National Laboratory Institute for Atmospheric and Earth System Research/Physics Faculty of ScienceUniversity of Helsinki Aerosol and Haze Laboratory Beijing Advanced Innovation Center for Soft Matter Science and Engineering Beijing University of Chemical Technology Joint International Research Laboratory of Atmospheric and Earth System Sciences School of Atmospheric Sciences Nanjing University

A new mechanism of new particle formation(NPF) is investigated using comprehensive measurements of aerosol physicochemical quantities and meteorological variables made in three continents,including Beijing,China;the Southern Great Plains site in the USA;and SMEAR Ⅱ Station in Hyytiala,Finland.D espite the considerably different emissions of chemical species among the sites,a common relationship was found between the characteristics of NPF and the stability *** stability parameter(ζ=Z/L,where Z is the height above ground and L is the Monin-Obukhov length) is found to play an important role;it drops significantly before NPF as the atmosphere becomes more unstable,which may serve as an indicator of nucleation *** the atmosphere becomes unstable,the NPF duration is closely related to the tendency for turbulence development,which influences the evolution of the condensation ***,the unstable atmosphere may dilute pre-existing particles,effectively reducing the condensation sink,especially at coarse mode to foster *** new mechanism is confirmed by model simulations using a molecular dynamic model that mimics the impact of turbulence development on nucleation by inducing and intensifying homogeneous nucleation events.

关键词： new particle formation turbulence development molecular dynamic

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Generation of complete graph states in a spin-1/2 Heisenberg chain with a globally optimized magnetic field

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Physical Review A 2024年第4期109卷 042604-042604页

作者： X. X. Li D. X. Li X. Q. Shao Sino-European Institute of Aviation Engineering Civil Aviation University of China Tianjin 300300 China College of Physics Science and Technology Shenyang Normal University Shenyang 110034 China Center for Quantum Sciences and School of Physics Northeast Normal University Changchun 130024 China Center for Advanced Optoelectronic Functional Materials Research and Key Laboratory for UV Light-Emitting Materials and Technology of Ministry of Education Northeast Normal University Changchun 130024 China

Graph states possess significant practical value in measurement-based quantum computation, with complete graph states that exhibit exceptional performance in quantum metrology. In this work, we introduce a method for generating multiparticle complete graph states using a spin-1/2 Heisenberg XX chain subjected to a time-varying magnetic field, which applies to a wide range of systems. Our scheme relies exclusively on nearest-neighbor interactions between atoms, with real-time magnetic field formation facilitated by quantum optimal control theory. We focus specifically on neutral-atom systems, finding that multiparticle complete graph states with N=3–6 can be achieved in less than 0.25µs, using a hopping amplitude of J/(2π)=−2.443MHz. This assumes an initial state provided by an equal-weight superposition of all spin states that are encoded by the dipolar-interacting Rydberg states. Furthermore, we thoroughly address various experimental imperfections and showcase the robustness of our approach against atomic vibrations, fluctuations in pulse amplitude, and spontaneous emission of Rydberg states. Taking into account the common occurrence of disturbances in the experimental setups of neutral-atom systems, our one-step strategy to achieve such graph states emerges as a viable alternative to techniques based on controlled-Z gates.

关键词： Electric dipole-dipole interactions Quantum control Quantum information theory Zeeman effect Rydberg atoms & molecules Two-level models

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First-principles study of the Pr-doped bilayer nickelate La3Ni2O7

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Physical Review B 2025年第19期111卷 195118-195118页

作者： Zihao Huo Peng Zhang Haoliang Shi Xiaochun Yan Defang Duan Tian Cui Key Laboratory of Material Simulation Methods and Software of Ministry of Education State Key Laboratory of Superhard Materials College of Physics Jilin University Changchun 130012 China MOE Key Laboratory for Non-equilibrium Synthesis and Modulation of Condensed Matter Shaanxi Province Key Laboratory of Advanced Functional Materials and Mesoscopic Physics School of Physics Xi'an Jiaotong University Xi'an 710049 China Institute of High Pressure Physics School of Physical Science and Technology Ningbo University Ningbo 315211 China

Recently, the Pr-doped Ruddlesden-Popper (RP) phase of bilayer nickelate La3Ni2O7 has been reported to exhibit a superconducting transition temperature (Tc) of 82.5 K and a superconducting volume fraction of about 57% at high pressure. However, the effect of Pr doping on La3Ni2O7 remains unclear. Here, we studied the crystal structures and electronic properties of Pr-doped La3Ni2O7 at 0 and 15 GPa based on the first-principles calculations to explore the doping effect of Pr. Our findings indicate that the praseodymium atoms prefer to occupy the outer La-O layers site. We then investigated the evolution of crystal structures in both the ambient pressure phase and the high-pressure phase of La3Ni2O7 as a function of doping concentration, revealing inconsistent trends in their evolution with increasing doping levels. Finally, by fitting the bilayer two-orbital model, we propose that doping Pr may reduce the required pressure for the superconductivity of La3Ni2O7. These results not only can help the further experimental search of RP phase nickelate at lower pressure, but also provide a helpful guide for understanding the effect of chemical pressure in an isovalent-doped RP phase nickelate superconductor.

关键词： Crystal atomic structure

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key Techniques on Unified Identity Authentication in OpenMBEE Integration 4

Key Techniques on Unified Identity Authentication in OpenMBE...

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4th IEEE International Conference on Electronics and Communication Engineering, ICECE 2021

作者： Xue, Junjie Zhou, Junhua Shi, Guoqiang Feng, Chaoqun Liu, Penghua Quan, Hongyan Beijing Complex Product Advanced Manufacturing Engineering Research Center Beijing Simulation Center Beijing China State Key Laboratory of Intelligent Manufacturing System Technology Beijing China Institute of Electronic System Engineering Beijing China Beijing Complex Product Advanced Manufacturing Engineering Research Center Beijing Simulation Center Beijing China Science and Technology on Space System Simulation Laboratory Beijing Simulation Center Beijing China School of Computer Science and Technology East China Normal University Shanghai China

ISBN: (纸本)9781728194226

In order to make full use of the concept of model-based systems engineering (MBSE) and the collaborative design capability of the open model-based engineering environment (OpenMBEE) in establishing complex product development platform, we propose an effective method to solve the problem of unified identity authentication in OpenMBEE integration. The proposed method is based on the Model View Controller(MVC) architecture in OpenMBEE, which has the characteristics strong plasticity and can be benefit for expanding the function in the controller layer. In our research, we make full use of the Software Development Kit (SDK) of OpenMBEE to expand the existing functions in the controller layer, and increase the function of communicating with the application development platform, then realize the function of sharing user authentication information between the development platform and OpenMBEE. After expansion, the system includes three modules, including the Front-end Service Module(FSM), MQ based Information Receiving Service Module(IFRSM), and the OpenMBEE Back-end Server Module(BSM). The effectiveness of the proposed strategies is verified by some practical instances, which verifies that our study can provide an effective design idea for the identity authentication in OpenMBEE integration. ©2021 IEEE

关键词： Integration

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Radar signal recognition based on deep residual network with attention mechanism 4

Radar signal recognition based on deep residual network with...

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4th IEEE International Conference on Electronic Information and Communication technology, ICEICT 2021

作者： Jin, Xiaolin Ma, Jing Ye, Fang College of Infomation and Communication Engineering Harbin Engineering University Harbin150001 China Key Laboratory of Advanced Marine Communication and Information Technology Ministry of Industry and Information Technology Beijing100854 China Science and Technology on Special System Simulation Laboratory Beijing100854 China

ISBN: (纸本)9781665432030

To address the problem of poor recognition success rate (RSR) of low probability of intercept (LPI) radar signals such as polyphase codes at low signal-to-noise ratio (SNR), In this paper, we propose a method of deep neural network with attention mechanism for modulation recognition of radar signals. The method first transforms the received radar signal into a two-dimensional time-frequency image(TFI), and then we obtain a binary time-frequency image by threshold segmentation，and resize TFIs through bicubic interpolation. While a deep residual network with Convolutional Block Attention Module (CBAM) is designed to recognize the radar signals. We take advantage of the attention mechanism to find the effective feature information in the noise and increase the effective information weight to further improve the recognition success rate of radar signals under low SNR. Finally, the average RSR of the method is nearly 96% for 7 signals at -6dB. © 2021 IEEE

关键词： Deep neural networks

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CMAS + sea salt corrosion to thermal barrier coatings

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Corrosion science 2023年第1期218卷

作者： Guo, Lei Zhang, Xinmu Liu, Mingguang Yang, Shuo Dai, JianWei School of Materials Science and Engineering Tianjin University Tianjin300072 China Tianjin Key Laboratory of Advanced Joining Technology Key Lab of Advanced Ceramics and Machining Technology of Ministry of Education Tianjin300072 China Naval Logistics Academy Tianjin300450 China Center for analysis and Test Tianjin University 300072 China Key laboratory for advanced corrosion and protection of aviation materials AECC Beijing Institute of Aeronautical Materials Beijing100095 China

In marine environment, sea salt and calcium-magnesium-alumina-silicate (CMAS) coexist largely endangering thermal barrier coatings (TBCs) service safety. In this study, the corrosion behavior of synthetic sea salt and CMAS to TBCs was investigated. Sea salt changed the CMAS structure, thereby decreasing its melting temperature and high-temperature viscosity. At 1200 ℃, CMAS + sea salt completely melted but CMAS did not;at 1250 ℃, both melted while CMAS + sea salt had stronger penetration ability in TBCs than CMAS. Thus, TBCs which have not been or are less affected by CMAS may be damaged due to CMAS + sea salt attack. © 2023 Elsevier Ltd

关键词： Alumina

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Enhancing particle heat resistance of the silicon-oxygen network skeleton in silica aerogel via Y/Yb dual-doping for thermal insulation

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Ceramics International 2025年

作者： Wu, Sijia Yu, Yuxi Luo, Zhong Huang, Liuying Fu, Zhongyi Zhao, Shuyuan College of Materials Xiamen University Xiamen361005 China China Aviation Power Machinery Research Institute Zhuzhou412002 China College of Naval Architecture & Ocean Engineering Naval University of Engineering Wuhan430033 China National Key Laboratory of Science and Technology on Advanced Composites in Special Environments Harbin Institute of Technology Harbin150080 China

SiO2 aerogels are nanoporous thermal insulation materials composed of a network of interconnected nanoparticles, but they are easy to crack and collapse above 800 °C which resulting in failure of thermal insulation. To improve the temperature resistance of nanoparticles, rare earth elements yttrium (Y) and ytterbium (Yb) were introduced as an enhancement system by sol-gel method to change the chemical interaction on the chemical structure and molecular bonding, together with improving the thermal stability. TEOS as the silicon source, yttrium nitrate and ytterbium nitrate as the rare earth sources, aerogel material with a density of 0.0904 g/cm3 was prepared by adjusting the finally chosen molar ratio of Si:Y:Yb = 1:0.05:0.05. By investigating the influence of RE on the microstructure, Y and Yb were found to be involved in the molecular bonding forming Si-O-Y and Si-O-Yb and changing the surface of primary particles. The thermal stability showed that the phase transition process after 573 °C was greatly inhibited by the introduction of single or dual RE. By analyzing the high temperature microstructural evolution, the shrinkage was decreased 25 % when at 1200 °C. The Cristobalite phase above 1200 °C was inhibited due to the Y/Yb dual-doping system. Furthermore, the decomposition stability was enhanced and the crack formation was significantly reduced at 1000 °C with thermal conductivity reducing from 0.2111W/(m·K) to 0.1187 W/(m·K) after heat treatment at 1000 °C. © 2025 Elsevier Ltd and Techna Group S.r.l.

关键词： Sol-gel process

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