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2022 IET International Conference on engineering Technologies and Applications, IET-ICETA 2022

作者： Yang, Tsung-Ying Kuo, Mei-Yan Chang, Edward-Yi National Yang Ming Chiao Tung University International College of Semiconductor Technology Hsinchu Taiwan National Yang Ming Chiao Tung University Graduate Program for Nanotechnology Department of Materials Science and Engineering Hsinchu Taiwan

ISBN: (数字)9781665491389

ISBN: (纸本)9781665491389

In this work, cyclic atomic layer etching (ALE) was used to etch silicon nitride (SiN) to find its working conditions. To understand the mechanism behind it, we tested the ALE adsorption effect and the removal effect of the ALE working window. Also, we made a comparison with the etching RMS of normal etching ICP and showed that ALE has better etch flatness. This demonstrates that ALE has a potential ability to become a reliable and stable etching technology in the future. © 2022 IEEE.

关键词： Silicon nitride

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Quaternary ammonium-functionalized polysilsesquioxanes for antifogging coating

RSC Applied Polymers

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RSC Applied Polymers 2024年第1期3卷 92-96页

作者： Hamada, Takashi Sugimoto, Tetsuya Tanaka, Arata Maeda, Tetsuya Katsura, Daiji Koga, Hiroyuki Ohshita, Joji Collaborative Research Laboratory Graduate School of Advanced Science and Engineering Hiroshima University 1-4-1 Kagamiyama Higashi-Hiroshima Hiroshima 739-8527 Japan Quantum Materials and Applications Research Center Takasaki Institute for Advanced Quantum Science National Institutes for Quantum Science and Technology (QST) 1233 Watanuki-machi Takasaki Gunma 370-1292 Japan Technical Research Center Mazda Motor Corporation Aki-gun Hiroshima 730-8670 Japan Smart Innovation Program Graduate School of Advanced Science and Engineering Hiroshima University 1-4-1 Kagamiyama Higashi-Hiroshima Hiroshima 739-8527 Japan Division of Materials Model-Based Research Digital Monozukuri (Manufacturing) Education and Research Center Hiroshima University 3-10-32 Kagamiyama Higashi-Hiroshima Hiroshima 739-0046 Japan

Aiming to develop antifogging materials with enhanced antifogging properties and scratch resistance, polysilsesquioxane films containing quaternary ammonium groups were prepared via a sol-gel reaction and quaternization. Owing to their high water uptake, scratch hardness, and transparency, the prepared quaternary ammonium-functionalized polysilsesquioxane films are promising for application in antifogging coatings. © 2025 RSC.

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Resolving Contradictory Estimates of Band Gaps of Bulk PdSe2: A Wannier-Localized Optimally-Tuned Screened Range-Separated Hybrid Density Functional Theory Study

arXiv

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arXiv 2025年

作者： Florio, Fred Camarasa-Gómez, María Ohad, Guy Naveh, Doron Kronik, Leeor Ramasubramaniam, Ashwin Department of Mechanical and Industrial Engineering University of Massachusetts Amherst AmherstMA01003 United States Department of Molecular Chemistry and Materials Science Weizmann Institute of Science Rehovoth7610001 Israel Institute for Nanotechnology and Advanced Materials Bar-Ilan University Ramat Gan52900 Israel Materials Science and Engineering Graduate Program University of Massachusetts Amherst AmherstMA01003 United States

Palladium diselenide (PdSe2)—a layered van der Waals material—is attracting significant attention for optoelectronics due to the wide tunability of its band gap from the infrared through the visible range as a function of the number of layers. However, there continues to be disagreement over the precise nature and value of the optical band gap of bulk PdSe2, owing to the rather small value of this gap that complicates experimental measurements and their interpretation. Here, we design and employ a Wannier-localized optimally-tuned screened range-separated hybrid (WOT-SRSH) functional to investigate the electronic bandstructures and optical absorption spectra of bulk and monolayer PdSe2. In particular, we account carefully for the finite exciton center-of-mass momentum within a time-dependent WOT-SRSH framework to calculate the indirect optical gap and absorption onset accurately. Our results agree well with the best available photoconductivity measurements, as well as with state-of-the-art many-body perturbation theory calculations, confirming that bulk PdSe2 has an optical gap in the mid-infrared (upper-bound of 0.44 eV). More generally, this work further bolsters the utility of the WOT-SRSH approach for predictive modeling of layered semiconductors. Copyright © 2025, The Authors. All rights reserved.

关键词： Layered semiconductors

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Surface Characterization of Sodium Cholate Treated CVD Graphene

Surface Characterization of Sodium Cholate Treated CVD Graph...

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IEEE Conference on Nanotechnology

作者： Evans Addo-Mensah Janet Obaemo Katie Welch Yang Tian Shiva Dolatabadi Hugh Churchill Uchechukwu Wejinya Materials Science and Engineering Graduate Program University of Arkansas Microelectronics and Photonics Program University of Arkansas Department of Physics University of Arkansas Fayetteville Arkansas Department of Mechanical Engineering University of Arkansas Fayetteville Arkansas

The advancement of graphene has created a need in exploring its properties for different applications. One way to explore its properties is by reducing its hydrophobicity. To overcome hydrophobicity of graphene, surfactants have been used in functionalization, hence improving the surface properties of the graphene monolayer. Therefore, investigating surfactant treatment for CVD graphene becomes useful in understanding the surface property effects on graphene. This study utilizes CVD graphene on silicon substrates. Its treatment was done with varying concentrations of Sodium Cholate (SC) for different treatment times. These samples were then characterized using Atomic Force Microscopy (AFM) to investigate the surface properties of the samples before and after treatment. To be optimized, the graphene must remain attached to the silicon substrate. The result shows that the integrity of the graphene, which is basically the Sp2 structure, is preserved as there was no delamination from the substrate even after treatment for as long as 2 hours in 1% weight/volume concentration of the SC solution.

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Thermodynamic and Environmental Assessment of Low-GWP Alternative Refrigerants for Domestic Cooling

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Journal of The Institution of Engineers (India): Series C 2023年第2期104卷 377-383页

作者： Islam, Md. Amirul Rupam, Tahmid Hasan Hosan, Shahadat Saha, Bidyut Baran Institute for Materials Chemistry and Engineering Kyushu University Kasuga-Koen 6-1 Kasuga-Shi Fukuoka816-8580 Japan Department of Electrical and Electronics Engineering Bangabandhu Sheikh Mujibur Rahman Science and Technology University Gopalganj8100 Bangladesh Kyushu University 744 Motooka Nishi-Ku Fukuoka819-0395 Japan Kyushu University Program for Leading Graduate School Green Asia Education Center Kyushu University Fukuoka Japan Department of Mechanical Engineering Kyushu University 744 Motooka Nishi-Ku Fukuoka819-0395 Japan

Nearly two billion air-conditioning (AC) units are currently being used for space cooling worldwide. The majority of these ACs use R134a as the working fluid, a greenhouse gas (GHG) with a global warming potential (GWP) of 1300 kg-CO2-eq. According to the rules set by the world environment safety organizations, the GWP of domestic air-conditioning systems must not exceed 750 kg-CO2-eq. Hence, the R134a must be phased out by 2025, and an alternative refrigerant with similar thermodynamic properties yet low GWP is required. Therefore, the authors have investigated several potential binary/ternary refrigerant blends in this study. Among the studied refrigerants, R445A, R30A, and NPB2 (newly proposed blend: 8% R152a + 92% R1234yf) can reduce 90–99% global warming impact (more than 200 million tonnes of CO2 emission equivalent) caused by the domestic air-conditioning systems every year. © 2023, The Institution of Engineers (India).

关键词： Refrigerants

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Rational effect of CuSe2phase with octadecyl amine modified reduced graphene composite for dual-mode sensing of environmental hazardous anthelminthic drug in aquatic and biological samples

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Journal of Environmental Chemical engineering 2023年第1期11卷

作者： Hwa, Kuo-Yuan Ganguly, Anindita Santhan, Aravindan Department of Molecular Science and Engineering National Taipei University of Technology Taipei Taiwan International Graduate Program in Energy and Optoelectronic Materials National Taipei University of Technology Taipei Taiwan

The increasing usage of antihelminthic drug mebendazole (MEB) in humans and livestock poses serious threat and is considered a significant environmental pollutant. Hence, monitoring the MEB residues in environmental samples, and human fluids is essential to decrease the ecological risk and improve the health of humans. In this work, copper selenide (CuSe2) nano/microspheres were hydrothermally synthesized and ultrasonically treated with rGO surface modified with ODA alkyl amine (rGO-ODA). The optical, structural, morphological, and functional analysis were performed which revealed the CuSe2 in marcasite phase, orthorhombic pattern with Pnnm space group, and substantial composite formation. The morphological studies revealed sphere structure of the CuSe2 and wrinkled sheets of rGO-ODA. A sensor that detects MEB using the cyclic voltammetry (CV), differential pulse voltammetry (DPV) and UV-Vis absorbance techniques was developed. For DPV analysis, the sensor exhibited a very low value for limit of detection 13.55 nM and a sensitivity of 9.4871 μA M-1cm-2. For UV-Vis, the sensor demonstrated a very low limit of detection 22.3 nM. The use of this sensor was validated in real-time analysis with aquatic and biological real samples. The results suggested > 90% of analyte recovery and enhanced efficiency for MEB detection with a potential for commercialization in future. © 2022 Elsevier Ltd.

关键词： Copper compounds

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Perspective on the perovskite quantum dots for flexible photovoltaics

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Journal of Energy Chemistry 2021年第11期30卷 505-507,I0011页

作者： Jiabei Yuan Nopporn Rujisamphan Wanli Ma Jianyu Yuan Youyong Li Shuit-Tong Lee Institute of Functional Nano&Soft Materials(FUNSOM) Jiangsu Key Laboratory of Carbon-Based Functional Materials and DevicesSoochow UniversitySuzhou 215123JiangsuChina Macao Institute of Materials Science and Engineering Macao University of Science and TechnologyTaipa 999078MacaoChina Nanoscience and Nanotechnology Graduate Program Faculty of ScienceKing Mongkut’s University of Technology ThonburiBangkok 10140Thailand

Owing to the ever-increasing charging demand for portable electronics,display devices and wearable electronic textiles,flexible and lightweight solar cells are highly urgent to be ***-generation solution-processable photovoltaic(PV)devices attracted great attentions due to their unique properties of low-cost,lightweight,and large-area printing compatibility with flexible substrates[1].

关键词： printing perovskite compatibility

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Layer-by-Layer Assembly of Chitosan and Quince Seed Gum Polyelectrolytes as a Ph-Responsive, On-Off Switchable Multilayer Film for Controlled Release of Ibuprofen

SSRN

引用

SSRN 2024年

作者： Kaviani, Alireza Pircheraghi, Gholamreza Bagheri, Reza Azizi Saadatlou, Ghazaleh Demirel, A. Levent Department of Materials Science and Engineering Sharif University of Technology P.O. Box: 11365‐9466 Tehran Iran Materials Science & Engineering Graduate Program Koç University Sarıyer Istanbul34450 Turkey Chemistry Department Koç University Sarıyer Istanbul34450 Turkey

Polysaccharide-based multilayer films have shown substantial potential for drug delivery application. Herein, polyelectrolyte multilayers using Chitosan (CS) and Quince seed gum (QSG) are constructed and the effects of assembly pH, salt concentration, and post-assembly pH are systematically investigated. It was evident that both mass per unit area (10000 ng/cm2) and the wet thickness (107.8 nm) after the deposition of 5 bilayers were accurately estimated by viscoelastic model due to the highly swollen state of films. Atomic Force Microscopy (AFM) could feasibly demonstrate the development of globular structures during the layer-by-layer assembly. Ellipsometry analysis showed that the variation assembly pH resulted in conformational changes from extended to coiled. Consequently, different optical thicknesses as well as transitions from exponential to linear growth were observed. Moreover, extrinsic charge compensation was responsible for coiling or extensive counterion screening of polyelectrolyte chains depending on the NaCl concentration. CS/QSG films displayed pH-stimulus on–off switching behavior in pH 2 and 7.4 for 3 cycles. The constructed film could absorb 1200 ng/cm2 within 60 min at pH 7.4. The in vitro release kinetic from IBF-loaded samples showed pH dependency. The CS/QSG multilayer film can be considered as a smart and tunable pH stimuli system for drug loading/release applications. © 2024, The Authors. All rights reserved.

关键词： Chitosan

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SR-CLD: spatially-resolved chord length distributions for statistical description, visualization, and alignment of non-uniform microstructures

arXiv

引用

arXiv 2024年

作者： Whitman, Sheila E. Latypov, Marat I. Graduate Interdisciplinary Program in Applied Mathematics University of Arizona TucsonAZ85721 United States Department of Materials Science and Engineering University of Arizona TucsonAZ85721 United States

This study introduces the calculation of spatially-resolved chord length distribution (SR-CLD) as an efficient approach for quantifying and visualizing non-uniform microstructures in heterogeneous materials. SR-CLD enables detailed analysis of spatial variation of microstructure constituent sizes in different directions that can be overlooked with traditional descriptions. We present the calculation of SR-CLD using efficient scan-line algorithm that counts pixels in constituents along pixel rows or columns of microstructure images for detailed, high-resolution SR-CLD maps. We demonstrate the application of SR-CLD in two case studies: one on synthetic polycrystalline microstructures with known and intentionally created uniform and gradient spatial distributions of grain size;and one on experimental images of two-phase microstructures of additively manufactured Ti alloys with significant spatially non-uniform distributions of laths of one of the phases. Additionally, we present how SR-CLDs can enable automated, computationally efficient, and robust alignment of large sets of images for merging into accurate composite images of large microstructure areas. © 2024, CC BY.

关键词： Titanium alloys

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Terahertz Time-Domain Imaging for Radiotherapy Treatment Monitoring in Pancreatic Ductal Adenocarcinoma

Terahertz Time-Domain Imaging for Radiotherapy Treatment Mon...

引用

CLEO: Applications and Technology in CLEO 2024, CLEO: A and T 2024 - Part of Conference on Lasers and Electro-Optics

作者： Chakraborty, Debamitra Mills, Bradley N. Cheng, Jing Komissarov, Ivan Gerber, Scott Sobolewski, Roman Materials Science Graduate Program University of Rochester RochesterNY14627 United States Laboratory for Laser Energetics University of Rochester RochesterNY14623-1299 United States Department of Surgery University of Rochester Medical Center RochesterNY14642 United States Department of Electrical and Computer Engineering University of Rochester RochesterNY14627-0231 United States

ISBN: (纸本)9781957171395

Terahertz time-domain imaging was performed of stereotactic body radiotherapy-treated murine pancreatic ductal adenocarcinoma (PDAC) with a high spatial resolution. To generate 2D maps of the tissue samples, the refractive index and absorption coefficient were used as imaging markers extracted with the maximum a-posteriori probability (MAP) estimation algorithm. The results were then compared with the terahertz maps of untreated murine PDAC tissue samples and demonstrated that terahertz imaging can probe physical changes with high sensitivity in the tissue post treatment. © Optica Publishing Group 2024, © 2024 The Author(s)

关键词： Tissue

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