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Superconductivity in Cubic La_(3)Al with Interstitial Anionic Electrons

Chinese Physics Letters 2025年第2期42卷 88-97页

作者： Zhijun Tu Peihan Sun Donghan Jia Huiyang Gou Kai Liu Hechang Lei School of Physics and Beijing Key Laboratory of Optoelectronic Functional Materials&MicroNano Devices Renmin University of ChinaBeijing 100872China Key Laboratory of Quantum State Construction and Manipulation(Ministry of Education) Renmin University of ChinaBeijing 100872China Department of Physics School of ScienceHebei University of Science and TechnologyShijiazhuang 050018China Center for High Pressure Science and Technology Advanced Research Beijing 100193China

We observed superconductivity in a cubic La_(3)Al single crystal that exhibits metallic behavior in the normal state without an observable structural transition and enters the superconducting state below T_(c)~6.32 *** characterization and analysis indicate that cubic La_(3)Al is a bulk type-Ⅱ BCS ***,theoretical calculations show that it can host interstitial anionic electrons located at the body center of the cubic unit cell,which confirms electron-phonon coupling as the superconducting ***,cubic La_(3)Al can be considered as a novel electride superconductor.

关键词： mechanism cubic

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Five-user quantum virtual local area network with an AlGaAs entangled photon source

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Science China(Physics,Mechanics & Astronomy) 2025年第3期68卷 61-73页

作者： Cheng Qian Hongkai Tian Xu Jing Yichen Liu Zhe Chen Huiran Luo Yuan Du Xiaodong Zheng Tangsheng Chen Yuechan Kong Hua-Lei Yin Dong Jiang Bin Niu Liangliang Lu Key Laboratory of State Manipulation and Advanced Materials in Provincial Universities School of Physical Science and TechnologyNanjing Normal UniversityNanjing210023China School of Internet Anhui UniversityHefei230039China National Key Laboratory of Solid-State Microwave Devices and Circuits Nanjing Chip Valley Industrial Technology InstituteNanjing Electronic Devices InstituteNanjing210016China Research Center for Quantum Optics and Quantum Communication School of ScienceQingdao University of TechnologyQingdao266520China Department of Physics and Beijing Key Laboratory of Opto-electronic Functional Materials and Micro-nano Devices Key Laboratory of Quantum State Construction and Manipulation(Ministry of Education)Renmin University of ChinaBeijing100872China Beijing Academy of Quantum Information Sciences Beijing100193China National Engineering Research Center of Agro-Ecological Big Data Analysis and Application Anhui UniversityHefei230601China National Laboratory of Solid-State Microstructures and School of Physics Nanjing UniversityNanjing210093China Hefei National Laboratory Hefei230088China

The promotion of quantum network applications demands the scalable connection of quantum *** is preferable to set up multiple logical networks coexisting on a single physical network infrastructure to accommodate a larger number of *** we present a quantum virtual network architecture that offers this level of scalability,without being constrained to a fixed physical-layer network relying solely on passive multiplexing *** architecture can be understood as arising from the superposition of a fully connected entanglement distribution network and port-based virtual local area network,which group multiusers by access *** terms of hardware,we leverage a semiconductor chip with a high figure-of-merit modal overlap to directly generate high-quality polarization entanglement,and a streamlined polarization analysis module,which requires only one single-photon detector for each end *** experimentally perform the BBM92 QKD protocol on the five-user quantum virtual network and demonstrate voice and image encryption on a campus area *** results may provide insights into the realization of large-scale quantum networks with integrated and cost-efficient photonic architecture.

关键词： quantum network quantum entanglement distribution integrated photonics image and voice encryption

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Edge-Mediated Magnetic Domain Rearrangement in van der Waals Magnet Fe3GaTe2

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Nano Letters 2025年第19期25卷 7885-7891页

作者： Jin, Shuaizhao Liu, Yujia Gu, Baijun Zhang, Xiangping Wang, Yiting Chen, Yichong Xia, Tianlong Huang, Boyuan Hong, Jiawang Wang, Xueyun School of Aerospace Engineering Beijing Institute of Technology Beijing100081 China Beijing Key Laboratory of Optoelectronic Functional Materials & Micro-Nano Devices Department of Physics Renmin University of China Beijing100872 China Key Laboratory of Quantum State Construction and Manipulation Ministry of Education Renmin University of China Beijing100872 China Department of Materials Science and Engineering Southern University of Science and Technology Guangdong Shenzhen518055 China

The emergence of van der Waals (vdW) magnets has opened new frontiers for investigation of 2-dimensional magnetism and application of spintronic memories. However, as the system approached the nanoscale, the edge effect significantly enhanced, posing critical challenges in understanding edge-mediated modifications of magnetic behavior, such as the nanoscale magnetic domain. Here, we employ magnetic force microscopy to systematically investigate edge-mediated magnetic domain rearrangement in Fe3GaTe2 flakes. By performing thermal treatment, we observed a distinct transition from labyrinthine to edge-localized stripe domains perpendicular to the flake edges. Furthermore, we reveal a competition and stabilization between size effect and edge effect by investigating thickness-dependent variation in the length of stripe domains and indicate that such an edge effect suppresses the formation of skyrmions. These findings not only elucidate the critical role of the edge effect in governing the domain morphology of vdW magnets but also provide insights for designing edge-mediated nanostructures in next-generation spintronic devices. © 2025 American Chemical Society.

关键词： Van der Waals forces

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Mild photothermal therapy-enhanced nano-ferroptosis inducer for potent treatment of advanced prostate cancer

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Nano Research 2025年第4期18卷 375-387页

作者： Xiao Hu Fei Li Xin-Hang Qian Yu-Sen Zhang Shuai Ke Yun-Xia Jin Shuai Yuan Yuan-Yuan Zhang Rui Li Lei Cao Lang Rao Xian-Tao Zeng Ling-Ling Zhang Center for Evidence-Based and Translational Medicine Zhongnan Hospital of Wuhan UniversityWuhan 430071China Institute of Chemical Biology Shenzhen Bay LaboratoryShenzhen 518132China Department of Urology Zhongnan Hospital of Wuhan UniversityWuhan 430071China Hubei Collaborative Innovation Center for Advanced Organic Chemical Materials Ministry of Education Key Laboratory for the Synthesis and Application of Organic Functional Molecules&College of Chemistry and Chemical EngineeringHubei UniversityWuhan 430062China Xinjiang Key Laboratory of Solid State Physics and Devices School of Physics Science and TechnologyXinjiang UniversityUrumqi 830017China

Androgen deprivation therapy(ADT)and androgen receptor signaling inhibitors(ARSis)often have limited efficacy in patients with advanced prostate cancer(PCa)(especially AR-negative).Inducing ferroptosis in PCa cells is an attractive therapeutic *** this work,mesoporous polydopamine nanoparticles(MPDA NPs)were developed to simultaneously deliver Cu^(+)/Cu^(2+)ion pairs and glutathione peroxidase 4(GPX4)inhibitor RSL3 to tumor sites for enhanced treatment of *** prepared MPDA-Cu-RSL3@HA(MPCRH)NPs induced ferroptosis by promoting lipid peroxidation and regulating phospholipid profiles in PCa cells,and the above effects were further enhanced by mild photothermal therapy(mPTT)without damaging normal *** can promote reactive oxygen species(ROS)generation and degrade tumor extracellular matrix in vivo to promote nanodrugs intratumoral *** short,this work shows the great application potential of mPTT-enhanced nano-ferroptosis inducers in the field of PCa treatment,in order to provide a reasonable paradigm for nanodrug development and PCa treatment.

关键词： prostate cancer ferroptosis mild photothermal therapy chemodynamic therapy mesoporous polydopamine

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Regulation of the sintering trajectory of Ho,Pr:Y_(2)O_(3) ceramics for 2.9μm mid-infrared lasers by atmospheric sintering

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Journal of advanced Ceramics 2025年第1期14卷 81-89页

作者： Qing Li Fei Liang Jun Wang Yan Ling Xue Jie Ma Peng Liu Shiyu Sun Zhan Hui Jian Zhang Changhua Zhang Lili Hu Haohai Yu Huaijin Zhang Dingyuan Tang State Key Laboratory of Crystal Materials and Institute of Crystal Materials Shandong UniversityJinan 250100China Jiangsu Key Laboratory of Advanced Laser Materials and Devices School of Physics and Electronic EngineeringJiangsu Normal UniversityXuzhou 221116China Shanghai Key Laboratory of Multidimensional Information Processing School of Communication and Electronics EngineeringEast China Normal UniversityShanghai 200241China Shanghai Branch Hefei National Laboratoryand Shanghai Research Center for Quantum SciencesShanghai 201315China Collaborative Innovation Center of Extreme Optics Shanxi UniversityTaiyuan 030006China Shanghai Institute of Optics and Fine Mechanics Chinese Academy of SciencesShanghai 201800China Shanghai Institute of Ceramics Chinese Academy of SciencesShanghai 201899China Future Technology School Shenzhen Technology UniversityShenzhen 518118China

The sintering trajectory of the Ho,Pr:Y_(2)O_(3) ceramics could be effectively adjusted by sintering in a flowing oxygen atmosphere instead of *** final-stage grain growth was significantly suppressed by the use of oxygen atmosphere presintering,resulting in smaller average grain sizes than those of samples sintered under vacuum,while the same relative density was *** hot isostatic pressing(HIP),the oxygen presintered Ho,Pr:Y_(2)O_(3) ceramics achieved excellent optical quality,with transmittance exceeding 80%at a wavelength of 680 *** codoping of Pr^(3+) as deactivating ions effectively depopulated the lower energy level 5I7 during the Ho^(3+):^(5)I_(6)→^(5)I_(7) transition,thereby making the Ho,Pr:Y_(2)O_(3) ceramics more conducive to promoting population inversion in the 2.9μm laser wavelength range.

关键词： Y_(2)O_(3) ceramics sintering trajectory Ho^(3+)/Pr^(2+) mid-infrared laser fluorescence properties

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Optical Singularities in Photonic Microstructures with Rosette Symmetries:A Unified Theoretical Scheme

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Engineering 2025年第2期45卷 59-69页

作者： Jie Yang Jiafu Wang Xinmin Fu Yueting Pan Tie Jun Cui Xuezhi Zheng Shaanxi Key Laboratory of Artificially Structured Functional Materials and Devices Xi’an 710051China Suzhou Laboratory Suzhou 215123China WaveCoRE Research Group KU LeuvenLeuven B-3001Belgium Faculty of Electronic and Information Engineering Xi’an Jiaotong UniversityXi’an 710049China Center for Advanced Quantum Studies Department of PhysicsBeijing Normal UniversityBeijing 100875China State Key Laboratory of Millimeter Wave Southeast UniversityNanjing 210096China Center for Polariton-Driven Light-Matter Interactions University of Southern DenmarkOdense 5230Denmark

Optical singularities are topological defects of electromagnetic fields;they include phase singularity in scalar fields,polarization singularity in vector fields,and three-dimensional(3D)singularities such as optical *** exploitation of photonic microstructures to generate and manipulate optical singularities has attracted wide research interest in recent years,with many photonic microstructures having been devised to this *** these designs,scattered phenomenological theories have been proposed to expound the working mechanisms behind individual *** this work,instead of focusing on a specific type of microstructure,we concentrate on the most common geometric features of these microstructures—namely,symmetries—and revisit the process of generating optical singularities in microstructures from a symmetry *** systematically employing the projection operator technique in group theory,we develop a widely applicable theoretical scheme to explore optical singularities in microstructures with rosette(i.e.,rotational and reflection)*** scheme agrees well with previously reported works and further reveals that the eigenmodes of a symmetric microstructure can support multiplexed phase singularities in different components,such as out-of-plane,radial,azimuthal,and left-and right-handed circular *** on these phase singularities,more complicated optical singularities may be synthesized,including C points,V points,L lines,Néel-and bubble-type optical skyrmions,and optical lattices,to name a *** demonstrate that the topological invariants associated with optical singularities are protected by the symmetries of the ***,based on symmetry arguments,we formulate a so-called symmetry matching condition to clarify the excitation of a specific type of optical *** work establishes a unified theoretical framework to explore optical singularities in photonic microstructures with symmetries,sheddin

关键词： Optical singularity Optical vortex Photonic microstructures Symmetries Group representation theory

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Charge density waves in the 2.5-dimensional quantum heterostructure

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Physical Review B 2025年第4期111卷 L041101-L041101页

作者： F. Z. Yang T. T. Zhang F. Y. Meng H. C. Lei C. Nelson Y. Q. Cai E. Vescovo A. H. Said P. M. Lozano Materials Science and Technology Division Oak Ridge National Laboratory Oak Ridge Tennessee 37831 USA Institute of Theoretical Physics Chinese Academy of Sciences Beijing 100190 China School of Physics and Beijing Key Laboratory of Opto-electronic Functional Materials & Micro-nano Devices Renmin University of China Beijing 100872 China Key Laboratory of Quantum State Construction and Manipulation (Ministry of Education) Renmin University of China Beijing 100872 China National Synchrotron Light Source II Brookhaven National Laboratory Upton New York 11973 USA Advanced Photon Source Argonne National Laboratory Lemont Illinois 60439 USA

Charge density wave (CDW) and their interplay with correlated and topological quantum states are at the forefront of condensed matter research. The 4Hb−TaS2 is a CDW ordered quantum heterostructure that is formed by alternative stacking of Mott insulating 1T-TaS2 and Ising superconducting 1H-TaS2. While the 13×13 and 3×3 CDWs have been respectively observed in the bulk 1T-TaS2 and 2H-TaS2, the CDWs and their pivotal role for unconventional superconductivity in the 4Hb−TaS2 remain unsolved. In this Letter, we reveal the two-dimensional (2D) 13×13 chiral CDW in the 1T layers and intraunit cell coupled 2D 2×2 CDW in the 1H and 1H' layers of 4Hb−TaS2. Our results establish 4Hb−TaS2 a 2.5D quantum heterostructure, where 2D quantum states emerge from 3D crystalline structure.

关键词： Charge density waves

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Photoemission evidence of a novel charge order in kagome metal FeGe

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Science China(Physics,Mechanics & Astronomy) 2025年第6期Mechanics & Astronomy) .卷 176-182页

作者： Zhisheng Zhao Tongrui Li Peng Li Xueliang Wu Jianghao Yao Ziyuan Chen Yajun Yan Shengtao Cui Zhe Sun Yichen Yang Zhicheng Jiang Zhengtai Liu Alex Louat Timur Kim Cephise Cacho Aifeng Wang Yilin Wang Dawei Shen Juan Jiang Donglai Feng Department of Physics School of Emerging Technology University of Science and Technology of China Hefei National Laboratory University of Science and Technology of China National Synchrotron Radiation Laboratory School of Nuclear Science and Technology University of Science and Technology of China Low Temperature Physics Laboratory College of Physics and Center of Quantum Materials and Devices Chongqing University State Key Laboratory of Functional Materials for Informatics Shanghai Institute of Microsystem and Information Technology (SIMIT)Chinese Academy of Sciences Shanghai Synchrotron Radiation Facility Shanghai Advanced Research Institute Chinese Academy of Sciences Diamond Light Source Ltd. Harwell Science and Innovation Campus New Cornerstone Science Laboratory University of Science and Technology of China

The kagome metal Fe Ge provides a rich platform for understanding the mechanisms behind competing orders, as it exhibits charge order(CO) emerging deep within the antiferromagnetic phase. To investigate the intrinsic origin of this behavior, we examine the evolution of the low-energy electronic structure across the phase transition in annealed Fe Ge samples using angleresolved photoemission spectroscopy. We find no evidence supporting a conventional nesting mechanism, such as Fermi surface nesting or van Hove singularities. However, we observe two notable changes in the band structure: an electron-like band around the K point and another around the A point, both shifting upward in energy when CO forms. These findings are consistent with our density-functional theory calculations, which suggest that the charge order in Fe Ge is primarily driven by magnetic energy savings due to a lattice distortion involving Ge1-dimerization. Our results provide photoemission evidence supporting this novel mechanism for CO formation in Fe Ge, in contrast to the conventional nesting-driven mechanisms.

关键词： kagome metal charge order electronic structure angle-resolved photoemission spectroscopy

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Room-temperature field-tunable radiofrequency rectification in epitaxial SrIrO3 films

arXiv

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arXiv 2025年

作者： Zhou, Liang Du, Zongzheng Wang, Jinhua H. Chen, Pingbo Ye, Bicong Feng, Tao Yang, Jiahao Xiao, Zehao H. Yang, Meng Li, Junxue X. Zhang, Wenqing Lu, Hai-Zhou He, Hongtao Department of Physics Southern University of Science and Technology Shenzhen518055 China Shenzhen Institute for Quantum Science and Engineering Southern University of Science and Technology Shenzhen518055 China Shenzhen Key Laboratory of Quantum Science and Engineering Shenzhen518055 China International Quantum Academy Shenzhen518048 China Department of Materials Science and Engineering Southern University of Science and Technology Shenzhen518055 China Shenzhen Key Laboratory for Advanced Quantum Functional Materials and Devices Southern University of Science and Technology Shenzhen518055 China Guangdong Provincial Key Laboratory of Advanced Thermoelectric Materials and Device Physics Southern University of Science and Technology Shenzhen518055 China

Although significant advancements have been made in wireless technologies and portable devices, it remains a challenge for high-frequency and nanowatt-level radiofrequency rectification. In this work, we report a pronounced radiofrequency rectification up to 37 GHz in nominally centrosymmetric SrIrO3 epitaxial films, with the minimum detectable power as low as ~300 nanowatts. Strikingly, the SrIrO3 rectifier is highly field-tunable and exhibits a strong in-plane field anisotropy, thus showing a unique advantage in broad-band radiofrequency rectification. The rectification effect can persist up to at least 360 K and shows a sensitive temperature dependence including a sign inversion. By a systematic study of the nonlinear transport properties of SrIrO3, it’s further revealed that the radiofrequency rectification originates from the nonlinear Hall effect with the dominant contribution from field-induced Berry curvature dipole. Our work demonstrates the superior performance of the field-tunable SrIrO3 rectifiers, unleashing the great application potential of centrosymmetric materials in harvesting and detecting ambient electromagnetic energy. © 2025, CC BY.

关键词： Electromagnetic waves

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Magnetic control of nonreciprocal charge transport

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Physical Review B 2025年第15期111卷 155411-155411页

作者： Xu Chen Yuhao Fu Xianjie Wang Yu Sui Hong Jian Zhao L. L. Tao School of Physics Harbin Institute of Technology Harbin 150001 China Key Laboratory of Material Simulation Methods and Software of Ministry of Education College of Physics Jilin University Changchun 130012 China Heilongjiang Provincial Key Laboratory of Advanced Quantum Functional Materials and Sensor Devices Harbin 150001 China

Nonreciprocal charge transport (NCT) characterized by unequal resistances for opposite current direction enriches the fundamental physics of electron transport and is promising for potential device applications. Here, we report on a study on the magnetic control of the NCT in two-dimensional systems with different types of spin-orbit coupling (SOC). Based on the Boltzmann transport theory, we first study this effect using a general Hamiltonian model and show that the nonlinear conductivity can be efficiently tuned by the exchange field. In particular, the exchange-field orientation dependence of the nonlinear conductivity reveals significantly distinct relations for different SOCs. We further derive the analytical expressions with the weak-field approximation, which are in good accordance with numerical results. Then, we exemplify this phenomenon in the Ag2Te/Cr2O3 surface based on density functional theory calculations. We predict that the nonlinear conductivity in such a system strongly depends on the surface magnetization orientation of the Cr2O3 layer. Those findings also suggest that measuring the NCT as a function of the exchange-field orientation provides a simple electrical means to quantify the SOC type. Our results are expected to provide a valuable insight into the NCT physics and open avenues for future rectifying devices.

关键词： Spin orbit coupling

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