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Mild photothermal therapy-enhanced nano-ferroptosis inducer for potent treatment of advanced prostate cancer

Nano Research 2025年第4期18卷 375-387页

作者： Xiao Hu Fei Li Xin-Hang Qian Yu-Sen Zhang Shuai Ke Yun-Xia Jin Shuai Yuan Yuan-Yuan Zhang Rui Li Lei Cao Lang Rao Xian-Tao Zeng Ling-Ling Zhang Center for Evidence-Based and Translational Medicine Zhongnan Hospital of Wuhan UniversityWuhan 430071China Institute of Chemical Biology Shenzhen Bay LaboratoryShenzhen 518132China Department of Urology Zhongnan Hospital of Wuhan UniversityWuhan 430071China Hubei Collaborative Innovation Center for Advanced Organic Chemical Materials Ministry of Education Key Laboratory for the Synthesis and Application of Organic Functional Molecules&College of Chemistry and Chemical EngineeringHubei UniversityWuhan 430062China Xinjiang Key Laboratory of Solid State Physics and Devices School of Physics Science and TechnologyXinjiang UniversityUrumqi 830017China

Androgen deprivation therapy(ADT)and androgen receptor signaling inhibitors(ARSis)often have limited efficacy in patients with advanced prostate cancer(PCa)(especially AR-negative).Inducing ferroptosis in PCa cells is an attractive therapeutic *** this work,mesoporous polydopamine nanoparticles(MPDA NPs)were developed to simultaneously deliver Cu^(+)/Cu^(2+)ion pairs and glutathione peroxidase 4(GPX4)inhibitor RSL3 to tumor sites for enhanced treatment of *** prepared MPDA-Cu-RSL3@HA(MPCRH)NPs induced ferroptosis by promoting lipid peroxidation and regulating phospholipid profiles in PCa cells,and the above effects were further enhanced by mild photothermal therapy(mPTT)without damaging normal *** can promote reactive oxygen species(ROS)generation and degrade tumor extracellular matrix in vivo to promote nanodrugs intratumoral *** short,this work shows the great application potential of mPTT-enhanced nano-ferroptosis inducers in the field of PCa treatment,in order to provide a reasonable paradigm for nanodrug development and PCa treatment.

关键词： prostate cancer ferroptosis mild photothermal therapy chemodynamic therapy mesoporous polydopamine

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Electrolyte Engineering Toward High-Voltage Aqueous Energy Storage Devices

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Energy & Environmental materials 2021年第3期4卷 302-306页

作者： Jianfeng Tan Jinping Liu School of Chemistry Chemical Engineering and Life Science and State Key Laboratory of Advanced Technology for Materials Synthesis and ProcessingWuhan University of TechnologyWuhan 430070China State Center for International Cooperation on Designer Low-carbon&Environmental Materials and School of Materials Science and Engineering Zhengzhou UniversityZhengzhou 450001China

Aqueous electrochemical energy storage(EES)devices are highly safe,environmentally benign,and inexpensive,but their operating voltage and energy density must be increased if they are to efficiently power multifunctional electronics,new-energy cars as well as to be used in smart *** Minireview summarizes the key breakthroughs and progress in expanding the electrochemical stability window(ESW)of aqueous EES devices over the past five *** briefly introducing the electrode engineering ways to widen ESW,we focus on four ground-breaking electrolyte engineering strategies and classify them into two kinds from the perspective of salts and exotic solutes/*** widening degree toward ESW of these emerging electrolytes is compared and the universal fundamental mechanism relating to the interactions between limited water molecules and high-concentration salts(or large amounts of exotic solutes/solvents)is *** challenges and perspectives for high-ESW electrolytes as well as recent advances in low-cost and other metal ion(sodium,potassium,zinc,etc.)-based electrolytes for expanding ESW are also outlined.

关键词： aqueous energy storage systems electrolyte engineering high voltage high-energy density water electrolysis

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Enhanced Photocatalytic H_(2)-production Activity of CdS Nanoflower using Single Atom Pt and Graphene Quantum Dot as Dual Cocatalysts

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Chinese Journal of Structural Chemistry 2022年第6期41卷 6-14页

作者： Yi Yang Jinsong Wu Bei Cheng Liuyang Zhang Ahmed Abdullah Al-Ghamdi Swelm Wageh Youji Li State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Nanostructure Research Centre(NRC)Wuhan University of TechnologyWuhan 430070China Laboratory of Solar Fuel Faculty of Materials Science and ChemistryChina University of GeosciencesWuhan 430074China Department of Physics Faculty of ScienceKing Abdulaziz UniversityJeddah 21589Saudi Arabia College of Chemistry and Chemical engineering Jishou UniversityJishouHunan 416000China

Single-atom catalysts have high catalytic activity due to their unique quantum size effects and optimal atom ***,visi-ble-light-responsive photocatalysts were designed by coupling CdS with graphene quantum dots(GQDs)and platinum single atoms(PtSAs).GQDs and PtSAs were successively loaded on ultrathin CdS nanosheets through freeze-drying and in-situ photocatalytic *** synergistic effect between PtSAs and GQDs results in superior photocatalytic activity with a hydrogen production rate of 13488μmol h^(-1)g^(-1)as well as the maximum apparent quantum efficiency(AQE)of 35.5%in lactic acid aqueous solution,which is 62 times higher than that of pristine CdS(213μmol g^(-1)h^(-1)).The energy conversion efficiency is ca.13.05%.As a photosensitizer and an electron reservoir,GQDs can not only extend the light response of CdS to the visible-light region(400-800 nm),but also promotes the separation of photoinduced electron-hole ***,PtSAs,with unique electronic and geometric features,can provide more efficient proton reduction *** finding provides an effective strategy to remarkably improve the photocatalytic H_(2) production performance.

关键词： hierarchical nanostructure single-atom catalysts graphene quantum dots CdS nanosheets hydrogen production

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Effect of Cerium Sulfate on Nickel Electrocrystallization Behavior and Grain Refinement of Sedimentary Layer

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Xiyou Jinshu Cailiao Yu Gongcheng/Rare Metal materials and Engineering 2025年第5期54卷 1273-1282页

作者： Xu, Yangtao Peng, Yin Du, Haiyang Li, Yanhong Zhong, Zhiqiang State Key Laboratory of Advanced Processing and Recycling of Nonferrous Metals Lanzhou University of Technology Lanzhou730050 China School of Materials Science and Engineering Lanzhou University of Technology Lanzhou730050 China

This study investigated the effect of different concentrations of cerium sulfate Ce2(SO4)3 on the grain refinement of nickel deposition layers during the electrochemical deposition process in industrial electrolytes. The impact of different Ce2(SO4)3 concentrations on nickel electrodeposition behavior was analyzed using the linear sweep voltammetry (LSV) curve, cyclic voltammetry (CV) curve and chronoamperometry (CA) curve. The microstructure morphology and grain size of the deposition layers were analyzed using scanning electron microscopy and the preferred orientation and crystal structure were analyzed using X-ray diffraction. The results show that the addition of different concentrations of Ce2(SO4)3 to the industrial electrolyte leads to a negative shift in the starting deposition potential of nickel, an increase in cathode polarization degree, an increase in overpotential, a shortened nucleation relaxation time tm and an accelerated nucleation rate during nickel electrodeposition, resulting in grain refinement of the deposition layers. However, the addition of Ce2(SO4)3 does not modify the nucleation mechanism of nickel electrocrystallization, nor does it change the crystal structure of the nickel deposition layer, which still remains a face-centered cubic (fcc) structure. When 0.6 g/L Ce2(SO4)3 is added, the grain growth orientation is transformed from the (111) plane to a bidirectional preferred growth of the (111) and (220) planes. At this point, the grain distribution in the deposition layer is uniform, and the grains undergo obvious refinement. © 2025 Science Press. All rights reserved.

关键词： Cyclic voltammetry

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Improvement of Mechanical Properties and Wall Thickness Uniformity of Hollow Ceramic Spheres by Biaxial Rotation Slurry Injection technology

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Journal of Wuhan University of technology(materials Science) 2025年第3期 619-626页

作者：王秋阳周建 LIU Guizhen WANG Lin DING Zhongjun State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of Technology National Deep Sea Center

Ceramic hollow spheres have great potential for deep-sea ***,the irregularity of the conventional molding process,among other reasons,results in low wall thickness uniformity of hollow *** solve this problem,in this work,we developed a biaxial rotation grouting process for deep-sea ceramic hollow buoyancy spheres,which improves the drawbacks of the traditional rotary grouting method that results in poor wall thickness uniformity of the hollow spheres due to its irregular rotational *** this paper,an experimental study was carried out to investigate the effects of different rotational methods,rotational speeds,rotational time,solid phase content,*** the wall thickness uniformity of ceramic hollow *** results show that the hollow floating balls prepared by the biaxial rotation method have the lowest wall thickness standard deviation (0.04) when the rotation speed is 60 rpm,the molding time is 8 min,and the solid phase content is 70 wt%.After the hydrostatic pressure test of 120 MPa,the hydrostatic compressive strength of hollow spheres prepared by the biaxial rotation method was increased by 31.67% compared with that of the traditional process.

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Permeable carbon fiber based thermoelectric film with exceptional EMI shielding performance and sensor capabilities

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Journal of advanced Ceramics 2024年第8期13卷 1119-1131页

作者： Junjie Zhu Chuan Sun Wanlin Feng Mengran Chen Peng-An Zong Chunlei Wan College of Materials Science and Engineering Nanjing Tech UniversityNanjing 211800China Nationai Innovation Institute of Defense Technology Academy of Military Sciences of the People's Liberation Army of ChinaBeijing 100089China Institute of Nuclear Physics and Chemistry Innovation Research Team for Advanced CeramicsChina Academy of Engineering PhysicsMianyang 621900China State Key Laboratory of New Ceramics and Fine Processing School of Materials Science and EngineeringTsinghua UniversityBeijing 100084China

Thermoelectric(TE)technologies offer a promising approach for directly converting skin heat into electricity for wearable *** p-type Sb2Tes and n-type BizTes as top-performing materials at room temperature,their rigid inorganic structure,with ultralow moisture permeability,poses challenges in warm and humid conditions,fostering bacterial growth and potential skin *** address this issue,we developed a cross-linked core-shell structure by electrodepositing Sb_(2)Te_(3)(Bi_(2)Te_(3))onto carbon fiber(CF).This architecture significantly improved the electrical conductivity and the Seebeck coefficient,resulting in a remarkable 300-fold increase in the power factor compared to that of pure *** CF/Sb_(2)Te_(3) and CF/Bi2Te films demonstrated optimal power factors of 450 and 121μW·m^(-1)·K^(-2),***,the fabricated films exhibited outstanding moisture permeability,over 3000 g·m^(-2)·d^(-1),exceptional electromagnetic interference shielding efficiency approaching 93 dB,and versatility as sensors for language assistance and respiratory *** attributes underline their broad applicability,emphasizing their suitability for human health protection in diverse scenarios.

关键词： thermoelectric(TE) carbon fiber(CF) Bi_(2)Te_(3) electrodeposition moisture permeability electromagnetic interference shielding

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Capacity Optimization of Hybrid Energy Storage System Based on Hysteresis Energy Management Strategy

Capacity Optimization of Hybrid Energy Storage System Based ...

引用

IEEE Annual Southern Power Electronics Conference (SPEC)

作者： Wenlong Yang Minwang Wang Wenchao Zhu Changjun Xie Hubei Key Laboratory of Advanced Technology for Automotive Components Wuhan University of Technology Wuhan China School of Automation Wuhan University of Technology Wuhan China State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of Technology Wuhan China

ISBN: (数字)9798350351156

ISBN: (纸本)9798350351163

This study improves the hydrogen energy module of the hydrogen-electric coupling system and proposes a hybrid hydrogen storage system structure based on Proton Exchange Membrane Electrolyzer (PEMEL), Alkaline Electrolyzer (ALKEL), and Proton Exchange Membrane Fuel Cell (PEMFC). Considering component startup and shutdown characteristics, dynamic operation, component degradation, and their impact on system reliability, a novel triple-hysteresis energy management strategy is proposed. The comprehensive optimization objectives include minimizing the Levelized Cost of Energy (LCOE), the Loss of Power Supply Probability (LPSP), and the Wind-Solar Curtailment to Load Energy Ratio (WSCLR). The optimal capacity configuration of the hybrid renewable energy system under the new energy management strategy was determined. The performance of the proposed strategy was analyzed and compared over short-term (1 year) and long-term (20 years) operations. The results indicate that the WSCLR of the ALKEL and PEMEL coupled structure is reduced by 83.3% compared to a single ALKEL system, and the LCOE and WSCLR are reduced by 2.1% and 3.5%, respectively, compared to a single PEMEL system. Compared to traditional energy management strategies, the new energy management strategy can reduce the LCOE, WSCLR, and LPSP by 2.7%, 45.0%, and 79.1%, respectively, over a 20-year long-term operation.

关键词： Protons Renewable energy sources System performance Hydrogen Lithium batteries Resource management Reliability Energy management Optimization Hysteresis

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Large linear electrostrain of acceptor-donor Co-doped ZnO films

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Journal of materials Science & technology 2022年第14期109卷 12-19页

作者： Chang Gao Yu Zhao Weili Li Yulong Qiao Zhao Wang Lu Jing Jie Sheng Wei-Dong Fei School of Materials Science and Engineering Harbin Institute of TechnologyHarbin 150001China National Key Laboratory of Science and Technology on Precision Heat Processing of Metals Harbin Institute of TechnologyHarbin 150001China Laboratory for Space Environment and Physical Science Research Center of Basic Space ScienceHarbin Institute of TechnologyHarbin 150001China State Key Laboratory of Advanced Welding and Joining Harbin Institute of TechnologyHarbin 150001China

In this paper we present the effective strategy of Fe^(3+)and Li^(+)co-doping to enhance the electrostrain of ZnO thin ***_(0.88)(Fe_(0.06)Li_(0.06))O thin film exhibits an excellent d_(33)^(*)value of 415 pm/V and large linear electrostrain of 0.68%after thermal-electric *** the X-ray diffraction and first principle calculation results have indicated that the Fe^(3+)and Li^(+)ions are inclined to adopt a preferential alignment along the edges approximately parallel to[001]direction in the zinc-oxygen tetrahedron and constitute a defect dipole(ionic pairs).It is considered that the local lattice distortion and the electric field-triggered polarization extension and rotation generated by preferential distributed Fe^(3+)-Li^(+)ionic pairs are responsible for the outstanding piezoelectric properties and large linear electrostrain.

关键词： Zno Piezoelectric Donor-acceptor ionic pairs Local lattice distortion Lead-free

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Wearable and interactive multicolored photochromic fiber display

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Light(Science & Applications) 2024年第3期13卷 454-465页

作者： Pan Li Yuwei Wang Xiaoxian He Yuyang Cui Jingyu Ouyang Ju Ouyang Zicheng He Jiayu Hu Xiaojuan Liu Hang Wei Yu Wang Xiaoling Lu Qian Ji Xinyuan Cai Li Liu Chong Hou Ning Zhou Shaowu Pan Xiangru Wang Huamin Zhou Cheng-Wei Qiu Yan-Qing Lu Guangming Tao State Key Laboratory of Material Processing and Die&Mould Technology School of Materials Science and Engineering and Wuhan National Laboratory for OptoelectronicsHuazhong University of Science and TechnologyWuhan 430074China Key Laboratory of Vascular Aging(HUST) Ministry of EducationWuhan 430030China School of Optoelectronic Science and Engineering University of Electronic Science and Technology of ChinaChengdu 611731China Department of Electrical and Computer Engineering National University of SingaporeSingapore 117583Singapore National Laboratory of Solid State Microstructures Key Laboratory of Intelligent Optical Sensing and ManipulationCollege of Engineering and Applied Sciencesand Collaborative Innovation Center of Advanced MicrostructuresNanjing UniversityNanjing 210023China School of Performing Arts Wuhan Conservatory of MusicWuhan 430060China School of Mechanical Science and Engineering Huazhong University of Science and TechnologyWuhan 430074China School of Architecture and Urban Planning Huazhong University of Science and TechnologyWuhan 430074China School of Fashion Beijing Institute of Fashion TechnologyBeijing 100029China School of Optical and Electronic Information Huazhong University of Science and TechnologyWuhan 430074China Tongji Medical College Huazhong University of Science and TechnologyWuhan 430074China State Key Laboratory for Modification of Chemical Fibers and Polymer Materials College of Materials Science and EngineeringDonghua UniversityShanghai 201620China

Endowing flexible and adaptable fiber devices with light-emitting capabilities has the potential to revolutionize the current design philosophy of intelligent,wearable interactive ***,significant challenges remain in developing fiber devices when it comes to achieving uniform and customizable light effects while utilizing lightweight ***,we introduce a mass-produced,wearable,and interactive photochromic fiber that provides uniform multicolored light *** designed independent waveguides inside the fiber to maintain total internal reflection of light as it traverses the *** impact of excessive light leakage on the overall illuminance can be reduced by utilizing the saturable absorption effect of fluorescent materials to ensure light emission uniformity along the transmission *** addition,we coupled various fluorescent composite materials inside the fiber to achieve artificially controllable spectral radiation of multiple color systems in a single *** prepared fibers on mass-produced kilometer-long using the thermal drawing *** fibers can be directly integrated into daily wearable devices or clothing in various patterns and combined with other signal input components to control and display patterns as *** work provides a new perspective and inspiration to the existing field of fiber display interaction,paving the way for future human–machine integration.

关键词： fiber interactive colored

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Mobile energy storage technologies for boosting carbon neutrality

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The Innovation 2023年第6期4卷 132-151页

作者： Chenyang Zhang Ying Yang Xuan Liu Minglei Mao Kanghua Li Qing Li Guangzu Zhang Chengliang Wang School of Integrated Circuits Wuhan National Laboratory for Optoelectronics(WNL 0)Huazhong University of Science and TechnologyWuhan 430074China State Key Laboratory of Material Processing and Die&Mould Technology School of Materials Science and EngineeringHuazhong University of Science and TechnologyWuhan 430074China Wenzhou Advanced Manufacturing Institute Huazhong University of Science and TechnologyWenzhou 325035China

Carbon neutrality calls for renewable energies,and the efficient use of renewable energies requires energy storage mediums that enable the storage of excess energy and reuse after spatiotemporal *** with traditional energy storage technologies,mobile energy storage technologies have the merits of low cost and high energy conversion efficiency,can be flexibly located,and cover a largerange from miniature to large systems and from high energy density to high power density,although most of them still face challenges or technical *** this review,we provide an overview of the opportunities and challenges of these emerging energy storagetechnologies(induding rechargeable batteries,fuel cells,and electrochemical and dielectric capacitors).Innovative materials,strategies,and technologies are ***,the future directions are *** hope this review will advance the development of mobile energy storage technologies and boost carbon neutrality.

关键词： neutral boosting energy

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