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Degradation of target pollutants under simultaneous competition from coexisting compounds: Electron-beam treatment of a real hair dye wastewater

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Radiation Physics and Chemistry 2025年 236卷

作者： Bao, Qiburi Yu, Boming Li, Wangrui Yang, Miao Dong, Zhen Zhao, Long School of Chemistry Chemical Engineering and Life Sciences Wuhan University of Technology Wuhan430070 China State Key Laboratory of Advanced Electromagnetic Technology School of Electrical and Electronic Engineering Huazhong University of Science and Technology Wuhan430074 China

Water pollution resulting from the extensive production and consumption of hair dyes has been threatening human health and aquatic ecosystems globally. Gaining knowledge on the presence of compounds in real hair dye wastewater and developing efficient treatment are emerging issues. This paper studies the electron beam irradiation of a real hair dye industrial wastewater. The CODCr of the industrial wastewater was reduced by 35 % through EB irradiation at 9 kGy. Four dyestuff intermediates (phenol, 5-amino-o-cresol, 5-amino-4-chloro-o-cresol and 5-amino-6-chloro-o-cresol) were identified as the target pollutants through compositional analysis of the wastewater. The removals of target pollutants in single-component solutions reached 75.7 %–89.7 % at 9 kGy The influence of coexisting background components on the degradation of targets was investigated and the interaction between different targets was evaluated during the irradiation treatment. Compared with pure single solutions, the required doses for 50 % removal of the targets in the wastewater increased by 0.1–5.8 times. Quantitative assessment of the competing effects of non-target components and the selectivity of reactive species is performed. [rad]OH and [rad]O2− show much lower selectivity toward the targets than reducing radicals (eaq− and [rad]H). Among them, [rad]O2− exhibits the lowest selectivity toward phenol with a logf value of −0.51. The main breakdown products of the target pollutants are quinones, diphenols and carboxylic acids. © 2025 Elsevier Ltd

关键词： River pollution

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Low-potential Li2C2O4 prelithiation catalyzed by 2D MoN with dominant (002) crystal face for high-energy lithium-ion batteries

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Materials Science and engineering R: Reports 2025年 165卷

作者： Lv, Tuan Zhong, Wei He, Renjie Zhou, Feng Xiang, Jingyu Huo, Kaifu Xie, Jia State Key Laboratory of Advanced Electromagnetic Engineering and Technology School of Electrical and Electronic Engineering Huazhong University of Science and Technology Wuhan430074 China State Key Laboratory of Materials Processing and Die & Mould Technology School of Materials Science and Engineering Huazhong University of Science and Technology Wuhan430074 China School of Optical and Electronic Information Huazhong University of Science and Technology Wuhan430074 China School of Chemistry and Chemical Engineering Huazhong University of Science and Technology Wuhan430000 China

Lithium oxalate (Li2C2O4) is considered as an ideal prelithiation agent owing to its high specific capacity and cost-effectiveness. However, the high reaction energy barrier and low intrinsic conductivity lead to a lithium liberation potential higher than 4.5 V, which severely trials the tolerance of the electrolyte and electrodes and significantly compromises the battery performance. In this study, two-dimensional molybdenum nitride (MoN) with (002) dominant exposed crystal face having superior catalytic properties is engineered to promote the low-potential decomposition of Li2C2O4. With its half-filled electronic state of surface Mo atoms and ultra-high electronic conductivity, highly polarized MoN can effectively adsorb and catalyze the decomposition of Li2C2O4, thus reducing the lithium liberation reaction energy barrier by 46.8 %. As a result, the lithium liberation potential of Li2C2O4 is diminished to 3.9 V. When paired with LiFePO4 (LFP) and LiNi0.5Co0.3Mn0.2O2 (NCM) cathode, forming Graphite || LFP-L and SiOx || NCM-L full cells, the capacity increase by 5.5 % and 11 %, respectively. Additionally, prelithiation facilitates the formation of a fluorine-rich solid electrolyte interphase (SEI) on the anode, markedly improving the cycling stability of the battery. © 2025 Elsevier B.V.

关键词： Lithium-ion batteries

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Effect of Co Content on Microstructure and Mechanical Properties of High-Entropy High-Temperature Shape Memory Alloy

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稀有金属材料与工程 2025年第1期54卷 10-16页

作者： Zhao Yanchun Jin Bo Feng Yuanfei Ma Huwen Yu Zhiqi Feng Li Liaw Peter K State Key Laboratory of Advanced Processing and Recycling of Nonferrous Metals Lanzhou University of TechnologyLanzhou 730050China Wenzhou Pump and Valve Engineering Research Institute of Lanzhou University of Technology Wenzhou 325105China Department of Materials Science and Engineering University of TennesseeKnoxville TN37996USA

(TiZrHf)_(50)Ni_(30)Cu_(20-x)Co_(x)(x=2,4,6,at%)high-entropy high-temperature shape memory alloys were fabricated by watercooled copper crucible in a magnetic levitation vacuum melting furnace,and the effects of Co content on microstructure and mechanical properties were *** results indicate that the grain size of the alloy decreases with increasing the Co *** the as-cast state,the alloy consists primarily of the B19′phase,with a trace of B2 *** fracture morphology is predominantly composed of the B19′phase,whereas the B2 phase is nearly *** the Co content or reducing the sample dimensions(d)markedly enhance the compressive strength and ductility of the *** d=2 mm,the(TiZrHf)_(50)Ni_(30)Cu_(14)Co_(6) alloy demonstrates the optimal mechanical properties,achieving a compressive strength of 2142.39±1.8 MPa and a plasticity of 17.31±0.3%.The compressive cyclic test shows that with increasing the compressive strain,the residual strain of the(TiZrHf)_(50)Ni_(30)Cu_(14)Co_(6) alloy increases while the recovery ability *** superelastic recovery capability of the alloy is continuously *** superelastic recovery rate increases from 1.36%to 2.12%,the residual strain rate rises from 1.79%to 5.52%,the elastic recovery rate ascends from 3.86%to 7.36%,while the total recovery rate declines from 74.48%to 63.20%.

关键词： high-temperature shape memory alloy high-entropy alloy microstructure mechanical property

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Polarization-encoded neural networks with simplified grating patch

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Science China(Technological Sciences) 2025年第2期68卷 269-277页

作者： Chengyan ZHONG Xiang WANG Lingfei LI Yuanchi CUI Lei XIAO Dawei SONG Junxiong GUO Wen HUANG Yufeng GUO Yu LIU College of Integrated Circuit Science and Engineering Nanjing University of Posts and TelecommunicationsNanjing 210023China National and Local Joint Engineering Laboratory of RF Integration and Micro-Assembly Technology Nanjing 210023China College of Integrated Circuits Hangzhou Global Scientific and Technological Innovation Centre Zhejiang UniversityHangzhou 310027China Nanjing Mumusili Technology Co. LTDNanjing 211100China School of Integrated Circuits Tsinghua UniversityBeijing 100084China Institute of Advanced Study School of Electronic Information and Electrical EngineeringChengdu UniversityChengdu 610106China State Key Laboratory of Electronic Thin Films and Integrated Devices School of Integrated Circuit Science and EngineeringUniversity of Electronic Science and Technology of ChinaChengdu 610054China

Optical neural networks(ONNs)offer a promising solution for high-performance,energy-efficient artificial intelligence hardware by leveraging the parallelism and speed of ***,the large-scale implementation of ONNs remains challenging due to the bulky footprint and complex control of optical *** this work,we propose and simulate a plasmonic polarized synaptic architecture that overcomes the diffraction limit and enables ultra-compact *** tuning the polarization state of incident light,the optical transmittance through each plasmonic unit can be dynamically adjusted to represent a synaptic *** plasmonic structures,with features as small as 40 nm,operate well below this limit in the visible spectrum(400-750 nm).Compared with diffraction and interference-based circuit designs,our proposed method achieves a substantial reduction in synaptic density by factors of 150000-fold and 1500-fold,***,we successfully demonstrate a proof-of-concept plasmonic ONN applied to the Canadian Institute for advanced Research—10 classes(CIFAR-10)dataset using a Visual Geometry Group network with 16 layers(VGG16)*** training for 80 epochs,the network achieves an accuracy of 93%.The polarization-tunable plasmonics paves the way towards scalable ONNs for next-generation artificial intelligence(AI)accelerators and smart sensors.

关键词： optical neural networks polarization dependent nanophotonic ultra-compact devices diffraction limit

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Knowledge-assisted Approach for Contactless Current Measurement in Multiconductor Systems

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IEEE Transactions on Industry Applications 2025年

作者： Ma, Chaojun Xu, Yingying Chen, Qing Jiao, Yang Qu, Zeming He, Cheng Huazhong University of Science and Technology School of Electrical and Electronic Engineering Institute of Artificial Intelligence School of Artificial Intelligence and Automation Wuhan430074 China Huazhong University of Science and Technology State Key Laboratory of Advanced Electromagnetic Technology School of Electrical and Electronic Engineering Wuhan430074 China

Current measurements of multiconductor systems are essential for smart grids, but conventional intrusive measurement approaches require power outages before deployment and maintenance and thus are expensive and may reduce system stability. Though many contactless current measurement approaches have been proposed in recent years, the challenge of easing the impact of conductor positions and decoupling current information remains. This paper proposes a novel approach that combines a cost-effective annular magnetic field (MF) sensor array with an inverse calculation technique for precise, contactless current measurements in multiconductor systems. Specifically, the MF sensor array captures the MF distribution surrounding the multiconductor systems for characterizing the coupled current information. Then, the hardware-oriented measurement task is reformulated into a computational optimization problem, where the currents and conductor positions are mathematically related to the MF distribution for decoupling. Meanwhile, an effective algorithm is tailored, where knowledge about the current and MF distribution is used to generate promising initial solutions for efficiency and effectiveness improvement. Experimental results demonstrate that the proposed approach achieves high accuracy in current measurement considering the impact of conductor positions, with error rates maintained below 1% and 2% in balanced and unbalanced cases, respectively. Additionally, an abnormal MF sensing data correction method is developed to further ensure measurement accuracy, showing resilience to sensor anomalies and maintaining a relative measurement error below 2% after correction. © 1972-2012 IEEE.

关键词： Smart power grids

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Comparative Study of Hybrid PM Assisted Synchronous Reluctance Machines with Different Configurations

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IEEE Transactions on Industry Applications 2025年

作者： Chen, Wutao Wang, Yawei Liu, Xinhua Shi, Yu Zhao, Yiru Qu, Ronghai Huazhong University of Science and Technology State Key Laboratory of Advanced Electromagnetic Engineering and Technology School of Electrical and Electronic Engineering Wuhan430074 China Investment Ltd Shanghai200050 China

In this paper, the rotor topology of hybrid permanent magnet assisted synchronous reluctance machines (HPM-SynRMs) with parallel, series and parallel-series configurations is given and the analytical models are presented. Based on the analytical models, a method for determining the initial dimensions of the rotors topology is presented. In the subsequent optimization process, a comparative analysis of the torque components, cost, external characteristics, and efficiency of the three motor configurations is conducted. The selected optimal design is compared with the reference PM machine under both overload and rated conditions. The results indicate that the HPM-SynRM achieves higher torque performance under overload conditions and slightly lower torque under rated conditions compared to the reference machine, while reducing the PM cost by 34.4%. Finally, a prototype is developed to validate the simulation results. © 1972-2012 IEEE.

关键词： Permanent magnets

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CO_(2) adsorption and activation on p-block catalyst Ga_(2)O_(3)

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Science China Materials 2025年第2期68卷 590-596页

作者： Zhizhuang Liu Xiaoxu Kuang Baowen Li Chenghua Sun Rong Tu Song Zhang Chaozhou Branch of Chemistry and Chemical Engineering Guangdong Laboratory Chaozhou 521000China School of Materials Science and Engineering Wuhan University of TechnologyWuhan 430070China Department of Chemistry and Biotechnology Swinburne University of TechnologyHawthornVictoria 3122Australia State Key Laboratory of Advanced Technology for Materials Synthesis and Processing Wuhan University of TechnologyWuhan 430070China

The fixation and conversion of CO_(2)frommedium-and high-temperature industrial exhaust gases arescientifically important and challenging tasks owing to theharsh conditions ***_(2)O_(3),a stable p-block compound,is surprisingly active in the thermal conversion of hot CO_(2)waste gas,but its underlying mechanism remains *** study,we investigated CO_(2)adsorption and activationacross 11 different Ga_(2)O_(3)-terminated faces using densityfunctional *** transfer and chemical bond analysesrevealed the occurrence of two distinct activation mechanismsinvolving synchronous electron gain and loss,driven by astrong synergetic effect between Ga cations and O anions onthe substrate *** Ga-O synergy enhances the CO_(2)activation efficiency compared with single active sites,with CO_(2)^(δ+) cation more readily capturing H atom than CO_(2)^(δ–).Tothe best of our knowledge,such a dual activation mechanismhas not been reported before,particularly for p-block *** findings provide new insights into the direct catalyticconversion of CO_(2)emissions and offer strategies for the rational design of industrial-grade catalysts for medium-andhigh-temperature CO_(2)tail gas conversion.

关键词： p-block catalyst gallium oxide carbon dioxide density functional theory synergetic mechanism

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Effects of Active and Reactive Power Control on Inertia in DFIG-Based Wind Turbines

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IEEE Transactions on Power Electronics 2025年

作者： Guo, Xiang Tang, Qingbo Zhu, Donghai Zhou, Yini Zou, Xudong Hu, Jiabing Kang, Yong China University of Mining and Technology School of Electrical Engineering Xuzhou221116 China Hubei Key Laboratory of Marine Electromagnetic Detection and Control Wuhan430064 China Huazhong University of Science and Technology State Key Laboratory of Advanced Electromagnetic Technology School of Electrical and Electronic Engineering Wuhan430074 China

The inertia analysis for wind turbines (WTs) typically focuses on the electromechanical timescale. Active power control (APC) and phase-locked loop (PLL) are essential considerations while reactive power control (RPC) is often deemed negligible, particularly in stiff grid. However, such assumptions may be inappropriate. Therefore, this article aims to comprehensively examine the effects of APC and RPC on the inertia for doubly fed induction generator (DFIG)-based WTs. Firstly, phase motion models are developed by incorporating various combinations of control loops, including APC, RPC, and different PLL configurations. Subsequently, the impacts of the APC and RPC on the inertia are examined in detail. The analysis reveals that the APC diminishes inertia, whereas the RPC significantly enhances the inertia. Additionally, special attention should be given to phase characteristics of the inertia transfer function, as they can substantially influence inertial performance. Furthermore, an improved frequency support method is proposed, which achieves superior frequency response without necessitating the PLL bandwidth to be adjusted to extremely low values, such as 1 Hz or lower. Finally, the analysis and the proposed method are validated through experiments. © 1986-2012 IEEE.

关键词： Wind turbines

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Mild photothermal therapy-enhanced nano-ferroptosis inducer for potent treatment of advanced prostate cancer

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Nano Research 2025年第4期18卷 375-387页

作者： Xiao Hu Fei Li Xin-Hang Qian Yu-Sen Zhang Shuai Ke Yun-Xia Jin Shuai Yuan Yuan-Yuan Zhang Rui Li Lei Cao Lang Rao Xian-Tao Zeng Ling-Ling Zhang Center for Evidence-Based and Translational Medicine Zhongnan Hospital of Wuhan UniversityWuhan 430071China Institute of Chemical Biology Shenzhen Bay LaboratoryShenzhen 518132China Department of Urology Zhongnan Hospital of Wuhan UniversityWuhan 430071China Hubei Collaborative Innovation Center for Advanced Organic Chemical Materials Ministry of Education Key Laboratory for the Synthesis and Application of Organic Functional Molecules&College of Chemistry and Chemical EngineeringHubei UniversityWuhan 430062China Xinjiang Key Laboratory of Solid State Physics and Devices School of Physics Science and TechnologyXinjiang UniversityUrumqi 830017China

Androgen deprivation therapy(ADT)and androgen receptor signaling inhibitors(ARSis)often have limited efficacy in patients with advanced prostate cancer(PCa)(especially AR-negative).Inducing ferroptosis in PCa cells is an attractive therapeutic *** this work,mesoporous polydopamine nanoparticles(MPDA NPs)were developed to simultaneously deliver Cu^(+)/Cu^(2+)ion pairs and glutathione peroxidase 4(GPX4)inhibitor RSL3 to tumor sites for enhanced treatment of *** prepared MPDA-Cu-RSL3@HA(MPCRH)NPs induced ferroptosis by promoting lipid peroxidation and regulating phospholipid profiles in PCa cells,and the above effects were further enhanced by mild photothermal therapy(mPTT)without damaging normal *** can promote reactive oxygen species(ROS)generation and degrade tumor extracellular matrix in vivo to promote nanodrugs intratumoral *** short,this work shows the great application potential of mPTT-enhanced nano-ferroptosis inducers in the field of PCa treatment,in order to provide a reasonable paradigm for nanodrug development and PCa treatment.

关键词： prostate cancer ferroptosis mild photothermal therapy chemodynamic therapy mesoporous polydopamine

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Low-input redoxomics facilitates global identification of metabolic regulators of oxidative stress in the gut

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Signal Transduction and Targeted Therapy 2025年第2期10卷 885-902页

作者： Xina Xiao Meng Hu Li Gao Huan Yuan Baochen Chong Yu Liu Rou Zhang Yanqiu Gong Dan Du Yong Zhang Hao Yang Xiaohui Liu Yan Zhang Huiyuan Zhang Heng Xu Yi Zhao Wenbo Meng Dan Xie Peng Lei Shiqian Qi Yong Peng Tao Tan Yang Yu Hongbo Hu Biao Dong Lunzhi Dai National Clinical Research Center for Geriatrics State Key Laboratory of BiotherapyWest China HospitalSichuan UniversityChengduChina Advanced Mass Spectrometry Center Research Core FacilityFrontiers Science Center for Disease-Related Molecular NetworkNHC Key Lab of Transplant Engineering and ImmunologyWest China HospitalSichuan UniversityChengduChina School of Life Sciences Tsinghua UniversityBeijingChina Department of Rheumatology and Immunology West China HospitalSichuan UniversityChengduChina The First School of Clinical Medicine Lanzhou UniversityLanzhouChina State Key Laboratory of Primate Biomedical Research Institute of Primate Translational MedicineKunming University of Science and TechnologyKunmingChina Beijing Key Laboratory of Reproductive Endocrinology and Assisted Reproductive Technology and Key Laboratory of Assisted Reproduction Ministry of EducationCenter for Reproductive MedicineDepartment of Obstetrics and GynecologyPeking University Third HospitalBeijingChina Frontiers Medical Center Tianfu Jincheng LaboratoryChengduChina

Oxidative stress plays a crucial role in organ aging and related diseases, yet the endogenous regulators involved remain largelyunknown. This work highlights the importance of metabolic homeostasis in protecting against oxidative stress in the large *** developing a low-input and user-friendly pipeline for the simultaneous profiling of five distinct cysteine (Cys) states, includingfree SH, total Cys oxidation (Sto), sulfenic acid (SOH), S-nitrosylation (SNO), and S-glutathionylation (SSG), we shed light on Cysredox modification stoichiometries and signaling with regional resolution in the aging gut of monkeys. Notably, the proteinsmodified by SOH and SSG were associated primarily with cell adhesion. In contrast, SNO-modified proteins were involved inimmunity. Interestingly, we observed that the Sto levels ranged from 0.97% to 99.88%, exhibiting two distinct peaks and increasingwith age. Crosstalk analysis revealed numerous age-related metabolites potentially involved in modulating oxidative stress and Cysmodifications. Notably, we elucidated the role of fumarate in alleviating intestinal oxidative stress in a dextran sulfate sodium (DSS)-induced colitis mouse model. Our findings showed that fumarate treatment promotes the recovery of several cell types, signalingpathways, and genes involved in oxidative stress regulation. Calorie restriction (CR) is a known strategy for alleviating oxidativestress. Two-month CR intervention led to the recovery of many antioxidative metabolites and reshaped the Cys redoxome. Thiswork decodes the complexities of redoxomics during the gut aging of non-human primates and identifies key metabolic regulatorsof oxidative stress and redox signaling.

关键词： metabolic homeostasis total cys oxidation cysteine modifications sulfenic acid gut aging redoxomics oxidative stress

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