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SAW Resonators on 15°YX-LiNbO3/SiO2/Sapphire Substrate with Excellent Electromechanical Coupling

SAW Resonators on 15°YX-LiNbO3/SiO2/Sapphire Substrate with...

2023 Joint Conference of the European Frequency and Time Forum and IEEE International Frequency Control Symposium, EFTF/IFCS 2023

作者： Wu, Jinbo Chen, Yang Zhang, Liping Zheng, Pengcheng Yao, Hulin Fang, Xiaoli Huang, Kai Zhang, Shibin Ou, Xin Shanghai Institute of Microsystem and Information Technology The State Key Laboratory of Functional Materials for Informatics Shanghai China

ISBN: (纸本)9798350311426

In this work, the shear horizontal surface acoustic wave (SH-SAW) resonators were demonstrated on 15° YX-LiNbO3/SiO2/sapphire (LiNbO3-on-sapphire, LNOS) substrate. Compared to the reported gigahertz SAW resonators based on piezoelectric heterogeneous substrates, the fabricated resonator in this work exhibits a state-of-the-art electromechanical coupling coefficient (k2) of 42.2%, a maximum Bode-Q (Qmax) of 1457 and an excellent figure of merit (k2×Qmax) of 615. Besides, several methods for suppressing transverse modes were implemented and compared. Tilted interdigital-transducers combined with the apodization technique can suppress the transverse modes more thoroughly while maintaining decent Q values. Overall, SAW devices based on the LNOS substrate have great potential for RF filters with low insertion loss, steep skirts, and wide bandwidth. © 2023 IEEE.

关键词： electromechanical coupling coefficient LiNbO3-on-insulator RF loss sapphire Surface acoustic wave resonator transverse mode

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Multilevel optoelectronic hybrid memory based on N-doped Ge_(2)Sb_(2)Te_(5)film with low resistance drift and ultrafast speed

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Chinese Physics B 2023年第10期32卷 724-730页

作者：吴奔魏涛胡敬王瑞瑞刘倩倩程淼李宛飞凌云刘波 Suzhou Key Laboratory for Nanophotonic and Nanoelectronic Materials and Its Devices School of Materials Science and EngineeringSuzhou University of Science and TechnologySuzhou 215009China State Key Laboratory of Functional Materials for Informatics Shanghai Institute of Microsystem and Information TechnologyChinese Academy of SciencesShanghai 200050China

Multilevel phase-change memory is an attractive technology to increase storage capacity and density owing to its high-speed,scalable and non-volatile ***,the contradiction between thermal stability and operation speed is one of key factors to restrain the development of phase-change ***,N-doped Ge_(2)Sb_(2)Te_(5)-based optoelectronic hybrid memory is proposed to simultaneously implement high thermal stability and ultrafast operation *** picosecond laser is adopted to write/erase information based on reversible phase transition characteristics whereas the resistance is detected to perform information *** show that when N content is 27.4 at.%,N-doped Ge_(2)Sb_(2)Te_(5)film possesses high ten-year data retention temperature of 175℃and low resistance drift coefficient of 0.00024 at 85℃,0.00170 at 120℃,and 0.00249 at 150℃,respectively,owing to the formation of Ge–N,Sb–N,and Te–N *** SET/RESET operation speeds of the film reach 520 ps/13 *** parallel,the reversible switching cycle of the corresponding device is realized with the resistance ratio of three orders of ***-level reversible resistance states induced by various crystallization degrees are also obtained together with low resistance drift ***,the N-doped Ge_(2)Sb_(2)Te_(5)thin film is a promising phase-change material for ultrafast multilevel optoelectronic hybrid storage.

关键词： multilevel optoelectronic hybrid memory N-doped Ge_(2)Sb_(2)Te_(5)thin film low resistance drift ultrafast speed

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A self-driven photodetector based on a SnS_(2)/WS_(2) van der Waals heterojunction with an Al_(2)O_(3) capping layer

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Chinese Physics B 2023年第1期32卷 585-591页

作者：王祥骏林钰恒刘潇邓煊华贲建伟俞文杰朱德亮刘新科 College of Materials Science and Engineering Institute of Microelectronics(IME)Guangdong Research Center for Interfacial Engineering of Functional MaterialsShenzhen UniversityShenzhen 518060China State Key Laboratory of Functional Materials for Informatics Shanghai Institute of Microsystem and Information TechnologyChinese Academy of SciencesShanghai 200050China

Photodetectors based on two-dimensional(2D) materials have attracted considerable attention because of their unique properties. To further improve the performance of self-driven photodetectors based on van der Waals heterojunctions, a conductive band minimum(CBM) matched self-driven SnS_(2)/WS_(2) van der Waals heterojunction photodetector based on a SiO2/Si substrate has been designed. The device exhibits a positive current at zero voltage under 365 nm laser *** is attributed to the built-in electric field at the interface of the SnS_(2) and WS_(2) layer, which will separate and transport the photogenerated carriers, even at zero bias voltage. In addition, the Al_(2)O_(3) layer is covered by the surface of the SnS_(2)/WS_(2) photodetector to further improve the performance, because the Al_(2)O_(3) layer will introduce tensile stress on the surface of the 2D materials leading to a higher electron concentration and smaller effective mass of electrons in the films. This work provides an idea for the research of self-driven photodetectors based on a van der Waals heterogeneous junction.

关键词： SnS_(2)/WS_(2)heterogeneous junction Al_(2)O_(3)layer self-driven photodetector

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Polyphenol-mediated interfacial deposition strategy for supported manganese oxide catalysts with excellent pollutant degradation performance

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Chinese Chemical Letters 2024年第5期35卷 493-498页

作者： Dong Cheng Youyou Feng Bingxi Feng Ke Wang Guoxin Song Gen Wang Xiaoli Cheng Yonghui Deng Jing Wei The Key Laboratory of Biomedical Information Engineering of Ministry of Education State Key Lab of Transducer TechnologySchool of Life Science and TechnologyXi’an Jiaotong UniversityXi’an 710049China School of Environmental and Municipal Engineering Xi’an University of Architecture and TechnologyXi’an 710055China Department of Chemistry State Key Laboratory of Molecular Engineering of PolymersState Key Laboratory of Transducer TechnologyFudan UniversityShanghai 200433China Key Laboratory of Functional Inorganic Material Chemistry Ministry of EducationSchool of Chemistry and Materials ScienceHeilongjiang UniversityHarbin 150080China

In persulfate-based advanced oxidation process(PS-AOPs),fixing nanosized metal oxide on processable substrates is highly desirable to avoid the aggregation and loss of nanocatalysts during the practical ***,it is still challenging to develop a versatile strategy for the deposition of metal oxide nanocatalysts on various substrates with different physicochemical ***,polyphenols are utilized as a“molecular glue”and reductant to mediate the interfacial deposition of MnO_(2) nanocatalysts on different ***_(2) nanocatalysts were in-situ grown on macroscope mineral substrates(e.g.,airstone)via an interfacial redox strategy between tannic acid(TA)and oxidized KMnO4,and then employed as a fixed catalyst of peroxymonosulfate(PMS)activation for treating pharmaceutical and personal care products(PPCPs)in *** fixed MnO_(2) exhibited superior catalytic performance toward different PPCPS via a singlet oxygen(^(1)O_(2))-dominated nonradical oxidation *** in the secondary effluent of wastewater treatment plants could be effectively removed by a fixed-bed column of the fixed MnO_(2) with long term *** cycle of Mn^(4+)/Mn^(3+)and surface hydroxyl group of the fixed MnO_(2) was proved to be responsible for the activation of *** work provides a new avenue for developing fixed metal oxides for sustainable water treatment.

关键词： Redox strategy Manganese oxides Fixed catalyst Peroxymonosulfate PPCPs

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Spray synthesis of rapid recovery Zno/polyaniline film ammonia sensor at room temperature

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Frontiers of materials Science 2022年第4期16卷 81-91页

作者： Yingze BAI Xin DONG Chuanyu GUO Yingming XU Bin WANG Xiaoli CHENG Key Laboratory of Functional Inorganic Material Chemistry School of Chemistry and Materials ScienceHeilongjiang UniversityHarbin 150080China State Key Laboratory of Optoelectronic Materials and Technologies Key Laboratory for Polymeric Composite and Functional MaterialsSchool of ChemistrySun Yat-sen UniversityGuangzhou 510275China

As an excellent room temperature sensing material,polyaniline(PANI)needs to be further investigated in the field of high sensitivity and sustainable gas sensors due to its long recovery time and difficulty to complete *** ZnO/PANI film with p-n heterogeneous energy levels have successfully prepared by spraying Zno nanorod synthesized by hydrothermal method on the PANI film rapidly synthesized at the gas-liquid *** presence of p-n heterogeneous energy levels enables the ZnO/PANI film to detect 0.1-100 ppm(1 ppm=10^(-6))NH_(3)at room temperature with the response value to 100 ppm NH_(3)doubled(12.96)and the recovery time shortened to 1/5(31.2s).The ability of high response and fast recovery makes the ZnO/PANI filmto be able to detect NH_(3)at room temperature *** provides a new idea for PANI to prepare sustainable room temperature sensor and promotes the development of room temperature sensor in public safety.

关键词： rapid recovery ZnO/polyaniline film ammonia sensor

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Innovations in spider silk-inspired artificial gel fibers:Methods,properties,strengthening,functionality,and challenges

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SusMat 2024年第3期4卷 104-163页

作者： Abdul Qadeer Khan Wenjin Guo Sitong Li Yutian Zhu Jie Bai Zunfeng Liu Weiqiang Zhao Xiang Zhou State Key Laboratory of Medicinal Chemical Biology Key Laboratory of Functional Polymer MaterialsTianjin Key Laboratory of Functional Polymer MaterialsSmart Sensing Interdisciplinary Science CenterCollege of ChemistryNankai UniversityTianjinChina Department of Science China Pharmaceutical UniversityNanjingChina College of Material Chemistry and Chemical EngineeringHangzhou Normal UniversityHangzhouChina Chemical Engineering College Inner Mongolia University of TechnologyHohhotChina

Spider silk,possessing exceptional combination properties,is classified as a biogel ***,it serves as a valuable origin of inspiration for the advancement of various artificial gel fiber materials with distinct *** fibers exhibit promising potential for utilization in diverse fields,including smart textiles,artificial muscle,tissue engineering,and strain ***,there are still numerous challenges in improving the performance and functionalizing applications of spider silk-inspired artificial gel ***,to gain a penetrating insight into bioinspired artificial gel fibers,this review provided a comprehensive overview encompassing three key aspects:the fundamental design concepts and implementing strategies of gel fibers,the properties and strengthening strategies of gel fibers,and the functionalities and application prospects of gel *** particular,multiple strengthening and toughening mechanisms were introduced at micro,nano,and molecular-level structures of gel ***,the existing challenges of gel fibers are *** review aims to offer significant guidance for the development and application of artificial gel fibers and inspire further research in the field of high-performance gel fibers.

关键词： artificial gel fibers biomimetic functionality spider silk strengthening

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Enhancing Low-Frequency Microwave Absorption Through Structural Polarization Modulation of MXenes

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Nano-Micro Letters 2024年第10期16卷 435-452页

作者： Bo Shan Yang Wang Xinyi Ji Yi Huang College of Light Industry Science and Engineering State Key Laboratory of Biobased Fiber Manufacturing TechnologyTianjin University of Science and TechnologyTianjin 300457People's Republic of China National Institute for Advanced Materials Tianjin Key Laboratory of Metal and Molecule Based Material ChemistryKey Laboratory of Functional Polymer MaterialsCollaborative Innovation Center of Chemical Science and Engineering(Tianjin)School of Materials Science and EngineeringNankai UniversityTianjin 300350People's Republic of China

Two-dimensional carbon-based materials have shown promising electromagnetic wave absorption capabilities in mid-and high-frequency ranges,but face challenges in low-frequency absorption due to limited control over polarization response mecha-nisms and ambiguous resonance *** this study,we pro-pose a novel approach to enhance absorption efficiency in aligned three-dimensional(3D)MXene/CNF(cellulose nanofibers)cavities by modifying polarization properties and manipulating resonance response in the 3D MXene *** controlled polarization mechanism results in a significant shift of the main absorption region from the X-band to the S-band,leading to a remarkable reflection loss value of-47.9 dB in the low-frequency ***,our findings revealed the importance of the oriented electromagnetic coupling in influencing electromagnetic response and microwave absorption *** present study inspired us to develop a generic strategy for low-frequency tuned absorption in the absence of magnetic element participation,while orientation-induced polarization and the derived magnetic resonance coupling are the key controlling factors of the method.

关键词： Hierarchical structure MXene Microwave absorption Low-frequency

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Dimensional regulation in gigantic molybdenum blue wheels featuring{(W)Mo_(5)}motifs for enhanced proton conductivity

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Nano Research 2024年第9期17卷 8261-8268页

作者： Yu-Lun Wu Jing Du Hai-Ying Zhang Ming-Jun Hou Qiao-Yue Li Wei-Chao Chen Kui-Zhan Shao Bo Zhu Chao Qin Xin-Long Wang Zhong-Min Su Key Laboratory of Polyoxometalate and Reticular Material Chemistry of Ministry of Education Department of ChemistryNortheast Normal UniversityChangchun 130024China Hebei Key Laboratory of Organic Functional Molecules National Demonstration Center for Experimental Chemistry EducationTesting and Analysis CenterCollege of Chemistry and Materials ScienceHebei Normal UniversityShijiazhuang 050024China State Key Laboratory of Supramolecular Structure and Materials Institute of Theoretical ChemistryCollege of ChemistryJilin UniversityChangchun 130021China

Dimensional regulation in polyoxometalates is an effective strategy during the design and synthesis of polyoxometalates-based high proton conductors,but it is not available to ***,the precise regulation of dimensionality has been realized in an unprecedented gigantic molybdenum blue wheel family featuring pentagonal{(W)Mo5}motifs through optimizing the molar ratio of Mo/W,including[Gd_(2)Mo_(124)W_(14)O_(422)(H_(2)O)62]38-(0D-{Mo_(124)W_(14)},1),[Mo_(126)W_(14)O441(H_(2)O)51]^(70-)(1D-{Mo_(126)W_(14)}n,2),and[Mo_(124)W_(14)O_(430)(H_(2)O)50]60-(2D-{Mo_(124)W_(14)}n,3).Such important{(W)Mo5}structural motif brings new reactivity into gigantic Mo blue *** are different numbers and sites of{Mo2}defects in each wheel-shaped monomer in 1-3,which leads to the monomers of 2 and 3 to form 1D and 2D architectures via Mo-O-Mo covalent bonds driven by{Mo2}-mediated H_(2)O ligands substitution process,respectively,thus achieving the controllable dimensional *** expected,the proton conductivity of 3 is 10 times higher than that of 1 and 1.7 times higher than that of *** continuous proton hopping sites in 2D network are responsible for the enhanced proton conductivity with lower activation *** study highlights that this dimensional regulation approach remains great potential in preparing polyoxometalates-based high proton conductive materials.

关键词： polyoxometalate molybdenum blue wheels Mo/W mixed-addenda polyoxometalates dimensional regulation proton conduction

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In situ regulating intimately connected heterostructure by decomposition of solid solution oxides toward high-efficient water oxidation

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Rare Metals 2024年第4期43卷 1557-1569页

作者： Shao-Fei Zhang Xiao-Lu Yin Jin Wang Jian-Li Kang Tian-Tian Li Jin-Feng Sun Yong-Qiang Meng Jian-Jiang Wang Dian-Long Wang Kai-Qiang Qin Hebei Key Laboratory of Flexible Functional Materials/Hebei Key Laboratory of Material Near-Net Forming Technology School of Materials Science and EngineeringHebei University of Science and TechnologyShijiazhuang050018China Key Laboratory of Advanced Ceramics and Machining Technology/Ministry of Education School of Materials Science and EngineeringTianjin UniversityTianjin300072China Electrochemical Engine Center Department of Mechanical EngineeringPennsylvania State UniversityUniversity ParkPA16802USA

Heterogeneous interfaces produced by interdomain interactions on a nanoscale performs a crucial role in boosting the properties of an electrocatalyst toward oxygen evolution reaction(OER)***,a series of dual-phase electrodes with intimately connected heterointerfaces are prepared by in situ decomposing solid solution oxide of Ni_(x)Co_(y)Fe_(100-x-y)O,which grew on Ni foam massively via an ultrafast combustion ***,with high-reaction kinetics caused by the reduction treatment at 450℃,the less electronegative Fe and Co are more oxyphilic than Ni,which facilitated their co-exsolution and formation of CoFe_2O_4/NiO oxide with enriched oxygen *** from the nanoporous framework,heterojunction structure,and oxygen defects,the self-supporting electrodes present rapid charge/mass transmission and provide abundant active sites for *** optimized sample(R-SNCF4.5)shows low overpotentials of 226 and 324 mV at 10 and100 mA·cm^(-2),a small Tafel slope(46.7 mV·dec^(-1)),and excellent *** assembled R-SNCF4.5//Pt/C/NF electrolyzer demonstrates continuous electrolysis over 50 h at a current density of 10 mA·cm^(-2),under 1.51 *** functional theory(DFT)calculations verify that the strong electronic modulation plays a critical part in the CoFe_2O_4/NiO hybrid by lowering the energy barriers for the ratedetermining steps,and Fe sites are the most active OER sites.

关键词： Rapid combustion Decomposition of solid solution oxide Dual-phase heterostructure Oxygen evolution reaction Theoretical calculation

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Multiple-resonance thermally activated delayed emitters through multiple peripheral modulation to enable efﬁcient blue OLEDs at high doping levels

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Aggregate 2024年第5期5卷 349-357页

作者： Yuyuan Wang Zhiwei Ma Junrong Pu Danman Guo Gaoyu Li Zhu Chen Shi-Jian Su Huangjun Deng Juan Zhao Zhenguo Chi PCFM Lab GD HPPC LabGuangdong Engineering Technology Research Center for High-Performance Organic and Polymer Photoelectric Functional FilmsState Key Laboratory of Optoelectronic Material and TechnologiesSchool of ChemistrySun Yat-sen UniversityGuangzhouChina State Key Laboratory of Luminescent Materials and Devices and Institute of Polymer Optoelectronic Materials and Devices South China University of TechnologyGuangzhouChina State Key Laboratory of Optoelectronic Material and Technologies School of Materials Science and EngineeringSun Yat-sen UniversityGuangzhouChina

Organic light-emitting diodes(OLEDs)based on multiple resonance-thermallyactivated delayedﬂuorescence(MR-TADF)have the advantages of high excitonutilization and excellent color ***,the large conjugated planarity of gen-eral MR-TADF emitters makes them easily aggregate in the form ofπ–πstacking,resulting in aggregation-caused quenching(ACQ)and the formation of excimers,which reduce exciton utilization efﬁciency and color *** address these issues,large shielding units can be incorporated to prevent interchromophore interactions,whereas the majority of reported molecules are limited to blue-green light *** work proposes a strategy of incorporating steric hindrance groups atdifferent sites of the B/N core to suppress interactions between chromophore,con-tributing to blue MR-TADF emitters with high photo-luminance quantum yields(PLQYs≥95%)and narrow full width at half maximum(FWHM),and importantly,great suppression of the ACQ ***,blue OLEDs achieve high externalquantum efﬁciencies up to 34.3%and high color purity with FWHM of about 27 nmand CIE around(0.12,0.15),even at a high doping concentration of 20 wt%.

关键词： blue emission color purity multiple-resonance organic light-emitting diodes thermally activated delayedﬂuorescence

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